arXiv subjects

Hongkun Park

Publications and source records attributed to Hongkun Park.

At least 19 recordsLinked to original sources

arXiv2026

Nanoscale magnetometry via collective many-body dynamics in diamond

Many-body dynamics constitutes a promising approach for creating correlations between quantum particles which can be used for applications in sensing and metrology. However, utilizing this potential for substantial gains in practical settings is a challenging task with only a very few applications realized to date. Here, we demonstrate an approach to nanoscale magnetic sensing enabled by strongly interacting electronic spins in a room temperature solid. By coherently controlling collective many-body dynamics of a dipolar ensemble of $\sim 10^4$ nitrogen-vacancy (NV) centres in diamond with pulsed magnetic field gradients, we demonstrate practical metrological gain up to $7.9(2)\,\mathrm{dB}$ for magnetic signal detection and $8.8(3)\,\mathrm{dB}$ for magnetic noise sensing, fully accounting for experimental overheads. Finally, we combine these methods to demonstrate a momentum-space-resolved sensing modality that enables detection of spatially correlated magnetic noise at continuously tunable length scales down to 50 nanometers. These observations open the door toward practical applications of interaction-enhanced quantum sensors for nanoscale biological imaging and material characterization.

quant-ph↗

arXiv2026

Quantum Sensors for Chemistry and Materials Science

The advancement of chemistry and materials science relies on transformative analytical tools which can overcome the sensitivity, spatial resolution, and throughput limitations of conventional techniques. This review explores the application of quantum sensors - specifically optically pumped magnetometers (OPMs) and nitrogen-vacancy (NV) centers in diamond - as robust platforms for molecular and materials analysis. We contrast the extreme magnetic sensitivity of macroscopic OPM ensembles with the atomic-scale resolution and multimodal capabilities of solid-state NV centers. We highlight their deployment in zero- to ultralow-field and nanoscale NMR spectroscopy, real-time reaction monitoring, and transient radical and pH detection. Furthermore, we discuss their integration into high-throughput chemical assays and non-destructive materials diagnostics, such as operando battery monitoring. With the ongoing commercialization of these technologies and advances in quantum-enhanced sensitivities, quantum sensors are poised to routinely address complex real-world analytical challenges.

quant-ph↗

arXiv2026

Optical signatures of antiferromagnetic correlations in a strongly interacting quantum Hall MoSe2 monolayer

Strong magnetic fields quench the kinetic energy of electrons, leading to the formation of flat energy bands, known as Landau levels (LLs). In this situation, even weak interactions can drive the emergence of various ordered phases. The simplest of such phases is a quantum Hall ferromagnet, where a spontaneous spin polarization emerges when LLs with opposite spins cross. The presence of strong electron-electron interaction at zero field changes this picture and makes the resulting states much harder to predict. Here we use magneto-optical spectroscopy to reveal quantum Hall states with unconventional correlations favouring an unpolarized state in the strongly correlated electron liquid in a MoSe2 monolayer. The oscillations of the exciton polaron energies as a function of perpendicular magnetic field and electron density demonstrate the emergence of LLs in a correlated electron liquid and density-dependent crossings between LLs of opposite valleys. On lowering the LL filling factor, where interactions within LLs are stronger, the crossings systematically broaden, indicating an increase in the Zeeman energy required to fully polarize the valley-degenerate LLs. These observations are shown to be consistent with antiferromagnetic interactions between LL electrons, favouring a ground state with zero valley polarization, and are therefore inconsistent with conventional quantum Hall ferromagnetism. This discovery demonstrates a qualitatively distinct form of quantum Hall magnetism in a strongly correlated electron liquid, establishing an anchoring point for understanding spin-unpolarized fractional and ordered states of correlated electrons driven by magnetic field.

cond-mat.mes-hall↗

arXiv2025

Dressed-state Hamiltonian engineering in a strongly interacting solid-state spin ensemble

In quantum science applications, ranging from many-body physics to quantum metrology, dipolar interactions in spin ensembles are controlled via Floquet engineering. However, this technique typically reduces the interaction strength between spins, and effectively weakens the coupling to a target sensing field, limiting the metrological sensitivity. In this work, we develop and demonstrate a method for direct tuning of the native interaction in an ensemble of nitrogen-vacancy (NV) centers in diamond. Our approach utilizes dressed-state qubit encoding under a magnetic field perpendicular to the crystal lattice orientation. This method leads to a $3.2\times$ enhancement of the dimensionless coherence parameter $JT_2$ compared to state-of-the-art Floquet engineering, and a $2.6\times$ ($8.3~$dB) enhanced sensitivity in AC magnetometry. Utilizing the extended coherence we experimentally probe spin transport at intermediate to late times. Our results provide a powerful Hamiltonian engineering tool for future studies with NV ensembles and other interacting higher-spin ($S>\frac{1}{2}$) systems.

quant-ph↗

arXiv2025

Collective many-body dynamics in a solid-state quantum sensor controlled through nanoscale magnetic gradients

Coherent collective dynamics of strongly interacting qubits are a central resource in quantum information science, with applications from quantum computing and simulation to metrology. While electronic spins interact strongly via dipolar couplings in dense solid-state ensembles, imperfections and positional disorder pose major obstacles to coherent correlated behavior, limiting their usefulness. Here, we realize collective many-body dynamics by combining time-dependent magnetic field gradients with global coherent control of dense electron spin ensembles in diamond. We control and probe the dynamics of nanometer-scale spin spirals, and, by exploiting Hamiltonian engineering that enhances the microscopic symmetry of the interactions, we observe a disorder-resilient collective spin evolution. Our results establish a pathway to interaction-enhanced quantum metrology and nanoscale imaging of materials and biological systems under ambient conditions.

quant-ph↗

arXiv2025

Wideband covariance magnetometry below the diffraction limit

We experimentally demonstrate a method for measuring correlations of wideband magnetic signals with spatial resolution below the optical diffraction limit. Our technique employs two nitrogen-vacancy (NV) centers in diamond as nanoscale magnetometers, spectrally resolved by inhomogeneous optical transitions. Using high-fidelity optical readout and long spin coherence time, we probe correlated MHz-range noise with sensitivity of 15 nT Hz$^{-1/4}$. In addition, we use this system for correlated $T_1$ relaxometry, enabling correlation measurements of GHz-range noise. Under such externally applied noise, while individual NV centers exhibit featureless relaxation, their correlation displays rich coherent and incoherent dynamics reminiscent of superradiance physics. This capability to probe high-frequency correlations provides a powerful tool for investigating a variety of condensed-matter phenomena characterized by nonlocal correlations.

quant-ph↗

arXiv2025

Signal amplification in a solid-state quantum sensor via asymmetric time-reversal of many-body dynamics

Electronic spins of nitrogen vacancy (NV) centers in diamond constitute a promising system for micro- and nano-scale magnetic sensing, due to their operation under ambient conditions, ease of placement in close proximity to sensing targets, and biological compatibility. At high densities, the electronic spins interact through dipolar coupling, which typically limits but can also potentially enhance sensing performance. Here we report the experimental demonstration of many-body signal amplification in a solid-state, room temperature quantum sensor. Our approach utilizes time-reversed two-axis-twisting interactions, engineered through dynamical control of the quantization axis and Floquet engineering in a two-dimensional ensemble of NV centers. Strikingly, we observe that the optimal amplification occurs when the backward evolution time equals twice the forward evolution time, in sharp contrast to the conventional Loschmidt echo. These observations can be understood as resulting from an underlying time-reversed mirror symmetry of the microscopic dynamics, providing key insights into signal amplification and opening the door towards entanglement-enhanced practical quantum sensing.

quant-ph↗

arXiv2024

Universal distributed blind quantum computing with solid-state qubits

Blind quantum computing (BQC) is a promising application of distributed quantum systems, where a client can perform computations on a remote server without revealing any details of the applied circuit. While the most promising realizations of quantum computers are based on various matter qubit platforms, implementing BQC on matter qubits remains an outstanding challenge. Using silicon-vacancy (SiV) centers in nanophotonic diamond cavities with an efficient optical interface, we experimentally demonstrate a universal quantum gate set consisting of single- and two-qubit blind gates over a distributed two-node network. Using these ingredients, we perform a distributed algorithm with blind operations across our two-node network, paving the way towards blind quantum computation with matter qubits in distributed, modular architectures.

quant-ph↗

arXiv2024

Optical signatures of interlayer electron coherence in a bilayer semiconductor

Emergent strongly-correlated electronic phenomena in atomically-thin transition metal dichalcogenides are an exciting frontier in condensed matter physics, with examples ranging from bilayer superconductivity~\cite{zhao2023evidence} and electronic Wigner crystals~\cite{smolenski2021signatures,zhou2021bilayer} to the ongoing quest for exciton condensation~\cite{wang2019evidence,ma2021strongly,shi2022bilayer}. Here, we experimentally investigate the properties of indirect excitons in naturally-grown MoS$_2$-homobilayer, integrated in a dual-gate device structure allowing independent control of the electron density and out-of-plane electric field. Under conditions when electron tunneling between the layers is negligible~\cite{pisoni2019absence}, upon electron doping the sample, we observe that the two excitons with opposing dipoles hybridize, displaying unusual behavior distinct from both conventional level crossing and anti-crossing. We show that these observations can be explained by static random coupling between the excitons, which increases with electron density and decreases with temperature. We argue that this phenomenon is indicative of a spatially fluctuating order parameter in the form of interlayer electron coherence, a theoretically predicted many-body state~\cite{zheng1997exchange} that has yet to be unambiguously established experimentally outside of the quantum Hall regime~\cite{sarma2008perspectives,spielman2000resonantly,kellogg2004vanishing,kellogg2002observation,spielman2001observation,fertig1989energy,shi2022bilayer}. Implications of our findings for future experiments and quantum optics applications are discussed.

cond-mat.str-el↗

arXiv2024

Dynamical Control of Excitons in Atomically Thin Semiconductors

Excitons in transition metal dichalcogenides (TMDs) have emerged as a promising platform for novel applications ranging from optoelectronic devices to quantum optics and solid state quantum simulators. While much progress has been made towards characterizing and controlling excitons in TMDs, manipulating their properties during the course of their lifetime - a key requirement for many optoelectronic device and information processing modalities - remains an outstanding challenge. Here we combine long-lived interlayer excitons in angle-aligned MoSe$_2$/WSe$_2$ heterostructures with fast electrical control to realize dynamical control schemes, in which exciton properties are not predetermined at the time of excitation but can be dynamically manipulated during their lifetime. Leveraging the out-of-plane exciton dipole moment, we use electric fields to demonstrate dynamical control over the exciton emission wavelength. Moreover, employing a patterned gate geometry, we demonstrate rapid local sample doping and toggling of the radiative decay rate through exciton-charge interactions during the exciton lifetime. Spatially mapping the exciton response reveals charge redistribution, offering a novel probe of electronic transport in twisted TMD heterostructures. Our results establish the feasibility of dynamical exciton control schemes, unlocking new directions for exciton-based information processing and optoelectronic devices, and the realization of excitonic phenomena in TMDs.

cond-mat.mes-hall↗

arXiv2024

Entanglement of Nanophotonic Quantum Memory Nodes in a Telecom Network

A key challenge in realizing practical quantum networks for long-distance quantum communication involves robust entanglement between quantum memory nodes connected via fiber optical infrastructure. Here, we demonstrate a two-node quantum network composed of multi-qubit registers based on silicon-vacancy (SiV) centers in nanophotonic diamond cavities integrated with a telecommunication (telecom) fiber network. Remote entanglement is generated via the cavity-enhanced interactions between the SiV's electron spin qubits and optical photons. Serial, heralded spin-photon entangling gate operations with time-bin qubits are used for robust entanglement of separated nodes. Long-lived nuclear spin qubits are used to provide second-long entanglement storage and integrated error detection. By integrating efficient bi-directional quantum frequency conversion of photonic communication qubits to telecom frequencies (1350 nm), we demonstrate entanglement of two nuclear spin memories through 40 km spools of low-loss fiber and a 35 km long fiber loop deployed in the Boston area urban environment, representing an enabling step towards practical quantum repeaters and large-scale quantum networks.

quant-ph↗

arXiv2024

Epitaxially defined Luttinger liquids on MoS$_2$ bicrystals

A mirror twin boundary (MTB) in a transition metal dichalcogenide (TMD) monolayer can host one-dimensional electron liquid of a topological nature with tunable interactions. Unfortunately, the electrical characterization of such boundaries has been challenging due to the paucity of samples with large enough size and high quality. Here, we report an epitaxial growth of monolayer molybdenum disulfide (MoS$_2$) bicrystals with well-isolated MTBs that are tens of micrometers long. Conductance measurements of these MTBs exhibit power-law behaviors as a function of temperature and bias voltage up to room temperature, consistent with electrons tunneling into a Luttinger liquid. Transport measurements of two distinct types of MTBs reveal the critical role of the atomic-scale defects. This study demonstrates that MTBs in TMD monolayers provide an exciting new platform for studying the interplay between electronic interactions and topology.

cond-mat.mes-hall↗

arXiv2023

Observation of an electronic microemulsion phase emerging from a quantum crystal-to-liquid transition

Strongly interacting electronic systems possess rich phase diagrams resulting from the competition between different quantum ground states. A general mechanism that relieves this frustration is the emergence of microemulsion phases, where regions of different phase self-organize across multiple length scales. The experimental characterization of these phases often poses significant challenges, as the long-range Coulomb interaction microscopically mingles the competing states. Here, we use cryogenic reflectance and magneto-optical spectroscopy to observe the signatures of the mixed state between an electronic Wigner crystal and an electron liquid in a MoSe2 monolayer. We find that the transit into this 'microemulsion' state is marked by anomalies in exciton reflectance, spin susceptibility, and Umklapp scattering, establishing it as a distinct phase of electronic matter. Our study of the two-dimensional electronic microemulsion phase elucidates the physics of novel correlated electron states with strong Coulomb interactions.

cond-mat.str-el↗

arXiv2023

Controlled Interlayer Exciton Ionization in an Electrostatic Trap in Atomically Thin Heterostructures

Atomically thin semiconductor heterostructures provide a two-dimensional (2D) device platform for creating high densities of cold, controllable excitons. Interlayer excitons (IEs), bound electrons and holes localized to separate 2D quantum well layers, have permanent out-of-plane dipole moments and long lifetimes, allowing their spatial distribution to be tuned on demand. Here, we employ electrostatic gates to trap IEs and control their density. By electrically modulating the IE Stark shift, electron-hole pair concentrations above $2\times10^{12}$ cm$^{-2}$ can be achieved. At this high IE density, we observe an exponentially increasing linewidth broadening indicative of an IE ionization transition, independent of the trap depth. This runaway threshold remains constant at low temperatures, but increases above 20 K, consistent with the quantum dissociation of a degenerate IE gas. Our demonstration of the IE ionization in a tunable electrostatic trap represents an important step towards the realization of dipolar exciton condensates in solid-state optoelectronic devices.

cond-mat.mes-hall↗

arXiv2023

Correlated Insulator and Chern Insulators in Pentalayer Rhombohedral Stacked Graphene

Rhombohedral stacked multilayer graphene is an ideal platform to search for correlated electron phenomena, due to its pair of flat bands touching at zero energy and further tunability by an electric field. Furthermore, its valley-dependent Berry phase at zero energy points to possible topological states when the pseudospin symmetry is broken by electron correlation. However, experimental explorations of these opportunities are very limited so far, due to a lack of devices with optimized layer numbers and configurations. Here we present electron transport measurements of hBN-encapsulated pentalayer graphene at down to 100 milli-Kelvin. We observed a correlated insulating state with >MOhm resistance at zero charge density and zero displacement field, where the tight-binding calculation predicts a metallic ground state. By increasing the displacement field, we observed a Chern insulator state with C = -5 and two other states with C = -3 at a low magnetic field of ~1 Tesla. At high displacement fields and charge densities, we observed isospin-polarized quarter- and half-metals. Therefore, rhombohedral-stacked pentalayer graphene is the first graphene system to exhibit two different types of Fermi-surface instabilities: driven by a pair of flat bands touching at zero energy, and by the Stoner mechanism in a single flat band. Our results demonstrate a new direction to explore intertwined electron correlation and topology phenomena in natural graphitic materials without the need of moiré superlattice engineering.

cond-mat.mes-hall↗

arXiv2023

Orbital Multiferroicity in Pentalayer Rhombohedral Graphene

Ferroic orders describe spontaneous polarization of spin, charge, and lattice degrees of freedom in materials. Materials featuring multiple ferroic orders, known as multiferroics, play important roles in multi-functional electrical and magnetic device applications. 2D materials with honeycomb lattices offer exciting opportunities to engineer unconventional multiferroicity, where the ferroic orders are driven purely by the orbital degrees of freedom but not electron spin. These include ferro-valleytricity corresponding to the electron valley and ferro-orbital-magnetism supported by quantum geometric effects. Such orbital multiferroics could offer strong valley-magnetic couplings and large responses to external fields-enabling device applications such as multiple-state memory elements, and electric control of valley and magnetic states. Here we report orbital multiferroicity in pentalayer rhombohedral graphene using low temperature magneto-transport measurements. We observed anomalous Hall signals Rxy with an exceptionally large Hall angle (tanΘH > 0.6) and orbital magnetic hysteresis at hole doping. There are four such states with different valley polarizations and orbital magnetizations, forming a valley-magnetic quartet. By sweeping the gate electric field E we observed a butterfly-shaped hysteresis of Rxy connecting the quartet. This hysteresis indicates a ferro-valleytronic order that couples to the composite field E\cdot B, but not the individual fields. Tuning E would switch each ferroic order independently, and achieve non-volatile switching of them together. Our observations demonstrate a new type of multiferroics and point to electrically tunable ultra-low power valleytronic and magnetic devices.

cond-mat.mes-hall↗

arXiv2023

An inverse-designed nanophotonic interface for excitons in atomically thin materials

Efficient nanophotonic devices are essential for applications in quantum networking, optical information processing, sensing, and nonlinear optics. Extensive research efforts have focused on integrating two-dimensional (2D) materials into photonic structures, but this integration is often limited by size and material quality. Here, we use hexagonal boron nitride (hBN), a benchmark choice for encapsulating atomically thin materials, as a waveguiding layer while simultaneously improving the optical quality of the embedded films. When combined with photonic inverse design, it becomes a complete nanophotonic platform to interface with optically active 2D materials. Grating couplers and low-loss waveguides provide optical interfacing and routing, tunable cavities provide a large exciton-photon coupling to transition metal dichalcogenides (TMD) monolayers through Purcell enhancement, and metasurfaces enable the efficient detection of TMD dark excitons. This work paves the way for advanced 2D-material nanophotonic structures for classical and quantum nonlinear optics.

physics.optics↗

arXiv2023

Telecom networking with a diamond quantum memory

Practical quantum networks require interfacing quantum memories with existing channels and systems that operate in the telecom band. Here we demonstrate low-noise, bidirectional quantum frequency conversion that enables a solid-state quantum memory to directly interface with telecom-band systems. In particular, we demonstrate conversion of visible-band single photons emitted from a silicon-vacancy (SiV) center in diamond to the telecom O-band, maintaining low noise ($g^2(0)<0.1$) and high indistinguishability ($V=89\pm8\%$). We further demonstrate the utility of this system for quantum networking by converting telecom-band time-bin pulses, sent across a lossy and noisy 50 km deployed fiber link, to the visible band and mapping their quantum states onto a diamond quantum memory with fidelity $\mathcal{F}=87\pm 2.5 \% $. These results demonstrate the viability of SiV quantum memories integrated with telecom-band systems for scalable quantum networking applications.

quant-ph↗