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Honglin Du

Publications and source records attributed to Honglin Du.

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A Unified Framework for Structure-Aware Clustering and Heterogeneous Causal Graph Learning

In complex multivariate systems, interactions among variables are defined by dependency structures, often encoded as directed acyclic graphs ($\text{DAGs}$). However, dependency structures can vary across subjects, and ignoring this structural heterogeneity introduces bias and obscures subpopulation-specific dependencies. To address this, we propose Directed Acyclic Graph-based Dependency Clustering via Alternating Direction Method of Multipliers (DAG-DC-ADMM), a unified framework built upon Structural Equation Modeling (SEM) that jointly learns cluster assignments and cluster-specific dependency structures. We encode acyclicity via a smooth constraint and integrate a groupwise truncated Lasso fusion penalty (gTLP) to cluster subjects based on their structural similarity. This yields a nonconvex optimization problem that incorporates sparsity, acyclicity, and structural consensus constraints. We address the nonconvexity by using the augmented Lagrangian method and solve it with an adapted version of the Alternating Direction Method of Multipliers (ADMM) for difference-of-convex programs. For certain graph structures, such as upper triangular adjacency matrices, our algorithm is guaranteed to converge to a Karush-Kuhn-Tucker (KKT) point. Experiments demonstrate that our method recovers cluster-specific causal dependency structures with a high true positive rate and a low false discovery rate. This capability enables the robust discovery of heterogeneous dependencies across subjects where the subpopulation label is unknown.

stat.ML

Observation of the Orbital Rashba-Edelstein Magnetoresistance

We report the observation of magnetoresistance (MR) originating from the orbital angular momentum transport (OAM) in a Permalloy (Py) / oxidized Cu (Cu*) heterostructure: the orbital Rashba-Edelstein magnetoresistance. The angular dependence of the MR depends on the relative angle between the induced OAM and the magnetization in a similar fashion as the spin Hall magnetoresistance (SMR). Despite the absence of elements with large spin-orbit coupling, we find a sizable MR ratio, which is in contrast to the conventional SMR which requires heavy elements. By varying the thickness of the Cu* layer, we confirm that the interface is responsible for the MR, suggesting that the orbital Rashba-Edelstein effect is responsible for the generation of the OAM. Through Py thickness-dependence studies, we find that the effective values for the spin diffusion and spin dephasing lengths of Py are significantly larger than the values measured in Py / Pt bilayers, approximately by the factor of 2 and 4, respectively. This implies that another mechanism beyond the conventional spin-based scenario is responsible for the MR observed in Py / Cu* structures originated in a sizeable transport of OAM. Our findings not only unambiguously demonstrate the current-induced torque without using any heavy element via the OAM channel but also provide an important clue towards the microscopic understanding of the role that OAM transport can play for magnetization dynamics.

cond-mat.mtrl-sci

Discovery of Two-Dimensional Multiferroicity in van der Waals CuCrP2S6 Layers

Multiferroic materials are potential to be applied in novel magnetoelectric devices, for example, high-density non-volatile storage. Last decades, research on multiferroic materials was focused on three-dimensional (3D) materials. However, 3D materials suffer from the dangling bonds and quantum tunneling in the nano-scale thin films. Two-dimensional (2D) materials might provide an elegant solution to these problems, and thus are highly on demand. Using first-principles calculations, we predict ferromagnetism and driven ferroelectricity in the monolayer and even a few-layers of CuCrP2S6. Although the total energy of the ferroelectric phase of monolayer is higher than that of the antiferroelectric phase, the ferroelectric phases can be realized by applying a large electric field. Besides the degrees of freedoms in the common multiferroic materials, the valley degree of freedom is also polarized according to our calculations. The spins, electric dipoles and valleys are coupled with each other as shown in the computational results. In experiment, we observe the out-of-plane ferroelectricity in a few-layer CuCrP2S6 (approximately 13 nm thick) at room temperature. 2D ferromagnetism of few-layers is inferred from magnetic hysteresis loops of the massively stacked nanosheets at 10 K. The experimental observations support our calculation very well. Our findings may provide a series of 2D materials for further device applications.

cond-mat.mtrl-sci

Tunable giant exchange bias in single-phase rare earth-transition metal intermetallics YMn12-xFex with highly homogenous inter-sublattice exchange coupling

In this paper, we have found a family of intermetallic compounds YMn12-xFex (x = 6.6-8.8) showing a bulk form of tunable giant exchange bias effect which arises from global interactions among ferromagnetic (FM) and antiferromagnetic (AFM) sublattices but not the interfacial exchange coupling or inhomogeneous magnetic clusters. A giant exchange bias with a loop shift up to 6.1 kOe has been observed in YMn4.4Fe7.6 compound with the strongest competing magnetic interactions. In a narrow temperature range, the exchange bias field shows a sudden switching off whereas the coercivity shows a sudden switching on with increasing temperature. This unique feature indicates that the inter-sublattice exchange coupling is highly homogenous, which can be perfectly interperated by our theoretical calculations.

cond-mat.str-el

Wide temperature span of entropy change in first-order metamagnetic MnCo1-xFexSi

The crystal structure and magnetic properties of MnCoxFe1-xSi (x=0-0.5) compounds were investigated. With increasing Fe content, the unit cell changes anisotropically and the magnetic property evolves gradually: Curie temperature decreases continuously, the first-order metamagnetic transition from a low-temperature helical antiferromagnetic state to a high-temperature ferromagnetic state disappears gradually and then a spin-glass-like state and another antiferromagnetic state emerge in the low temperature region. The Curie transition leads to a moderate conventional entropy change. The metamagnetic transition not only yields a larger negative magnetocaloric effect at lower applied fields than in MnCoSi but also produces a very large temperature span (103 K for H=5 T) of delta S(T), which results in a large refrigerant capacity. These phenomena were explained in terms of crystal structure change and magnetoelastic coupling mechanism. The low-cost MnCo1-xFexSi compounds are promising candidates for near room temperature magnetic refrigeration applications because of the large isothermal entropy change and the wide working temperature span.

cond-mat.mtrl-sci