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Hongxia Zhang

Publications and source records attributed to Hongxia Zhang.

At least 19 recordsLinked to original sources

Vacancy Order and Physical Properties of a Ternary Compound Fe0.68Pd0.80Te with an {\alpha}-Fe1+xTe-Type Structure

We report the identification and characterization of a new compound Fe0.68Pd0.80Te with an {\alpha}-Fe1+xTe prototype structure. Different from the Fe-square net and minor occupancy of interstitial Fe-sites in Fe1+xTe, Fe0.68Pd0.80Te is featured by a Pdsquare net and near 68% occupancy of the corresponding interstitial Fe-sites. Furthermore, noncontact atomic force microscopy and X-ray diffraction provide evidence for the existence of a 3*3*3 Pd-vacancy order in this layered material. A spin-glass ground state below Tg 40 K is identified via magnetic characterization. Electrical transport measurements show that Fe0.68Pd0.80Te is a semiconductor with a very small band gap below 10 meV. It has weak negative magnetoresistance and holelike charge carriers below room temperature. Our results demonstrate its potentials for further exploring various quantum phenomena.

cond-mat.mtrl-sci

Noncollinear antiferromagnetic structure and physical properties of CrRhAs with distorted kagome lattice

CrRhAs was theoretically proposed to be a kagome metal with unusual magnetic ground states; however, little is known about its magnetic structure and physical properties experimentally. Here, we present an experimental investigation of CrRhAs with ZrNiAl-type structure and a distorted Cr kagome lattice. CrRhAs is an antiferromagnet with TN = 149 K. Powder neutron diffraction analysis reveals a noncollinear antiferromagnetic structure with propagation vector k = (1/3, 1/3, 1/2), which features a ferromagnetic second nearest neighbor coupling in the kagome plane that is different from the prediction in previous density functional theory calculations. Furthermore, CrRhAs exhibits anomalous electrical transport properties which are possibly related to multiband effects and strong spin fluctuations. For the temperature-dependent longitudinal resistivity \r{ho}xx, it is semiconductinglike above TN and becomes metallic below TN . The Hall coefficients exhibit two sign changes near 70 and 300 K. Combined with the results of heat capacity measurements, a large Kadowaki-Woods ratio {\alpha} = 33.9 {\mu}{\Omega} cm mol2 K2/J2 is obtained. The above results suggest CrRhAs is a strongly correlated kagome metal with multiband and noncollinear magnetic structure features.

cond-mat.str-el

Tilting Objects via Recollements and $p$-Cycles on Weighted Projective Lines

In this paper, we provide a new method for constructing tilting objects in a triangulated category via recollements. The $p$-cycle approach to exceptional curve processes significant advantages in constructing recollements and ladders, due to the existence of reduction/insertion functors. In order to construct tilting objects in the stable category of vector bundles over a weighted projective line, we give explicit expressions for line bundles and extension bundles due to the $p$-cycles constuctions. Furthermore, we provide an essential proof for tilting cuboic object and tilting objects consisting of Auslander bundles. Moreover, we construct certain new tilting objects in the stable category of vector bundles over a weighted projective line.

math.RT

Design and construction of the multiplexing cold neutron spectrometer BOYA with double-column Rowland focusing analyzers

Developing neutron spectrometers with higher counting efficiency has been an essential pursuit in neutron instrumentation. In this work, we present BOYA, a multiplexing cold neutron spectrometers designed and implemented at the China Advanced Research Reactor. Equipped with 34 angular analyzing channels spanning 119{\deg}, each containing 5 inelastic channels and 1 diffraction channel, BOYA enhances the measurement efficiency by two orders of magnitude over a traditional triple-axis spectrometer. To optimize both intensity and energy resolution, innovative double-column Rowland focusing analyzers have been developed. By filling the crystal gaps in the traditional Rowland focusing geometry, our design enhances the neutron beam coverage without introducing appreciable double-scattering. Our commissioning results on vanadium and MnWO4 have confirmed the success of the design, establishing BOYA as a successful multiplexing instrument for neutron spectroscopy.

physics.ins-det

Structural and magnetic characterization of CeTa$_7$O$_{19}$ and YbTa$_7$O$_{19}$ with two-dimensional pseudospin-1/2 triangular lattice

Triangular lattice antiferromagnets are prototypes for frustrated magnetism and may potentially realize novel quantum magnetic states such as a quantum spin liquid ground state. A recent work suggests NdTa$_7$O$_{19}$ with rare-earth triangular lattice is a quantum spin liquid candidate and highlights the large family of rare-earth heptatantalates as a framework for quantum magnetism investigation. In this paper, we report the structural and magnetic characterization of CeTa$_7$O$_{19}$ and YbTa$_7$O$_{19}$. Both compounds are isostructural to NdTa$_7$O$_{19}$ with no detectable structural disorder. For CeTa$_7$O$_{19}$, the crystal field energy levels and parameters are determined by inelastic neutron scattering measurements. Based on the crystal field result, the magnetic susceptibility data could be well fitted and explained, which reveals that CeTa$_7$O$_{19}$ is a highly anisotropic Ising triangular-lattice antiferromagnet ($g_z$/$g_{xy}$$\sim$3) with very weak exchange interaction (J$\sim$0.22~K). For YbTa$_7$O$_{19}$, millimeter sized single crystals could be grown. The anisotropic magnetization and electron spin resonance data show that YbTa$_7$O$_{19}$ has a contrasting in-plane magnetic anisotropy with $g_z$/$g_{xy}$$\sim$0.67 similar as that of YbMgGaO$_4$. The above results indicate that CeTa$_7$O$_{19}$ and YbTa$_7$O$_{19}$ with pseudospin-1/2 ground states might either be quantum spin liquid candidate materials or find applications in adiabatic demagnetization refrigeration due to the weak exchange interaction.

cond-mat.str-el

FePd2Te2: An Anisotropic Two-Dimensional Ferromagnet with One-Dimensional Fe Chains

Two-dimensional (2D) magnets have attracted significant attentions in recent years due to their importance in the research on both fundamental physics and spintronic applications. Here, we report the discovery of a new ternary compound FePd2Te2. It features a layered quasi-2D crystal structure with one-dimensional Fe zigzag chains extending along the b-axis in the cleavage plane. Single crystals of FePd2Te2 with centimeter-size could be grown. Density functional theory calculations, mechanical exfoliation and atomic force microscopy on these crystals reveal that they are 2D materialsthat can be thinned down to 5 nm. Magnetic characterization shows that FePd2Te2 is an easy-plane ferromagnet with Tc 183 K and strong in-plane uniaxial magnetic anisotropy. Magnetoresistance and anomalous Hall effect demonstrate that ferromagnetism could maintain in FePd2Te2 flakes with large coercivity. A crystal twinning effect is observed by scanning tunneling microscopy which makes the Fe chains right-angle bent in the cleavage plane and creates an intriguing spin texture. Our results show that FePd2Te2 is a correlated anisotropic 2D magnets that may attract multidisciplinary research interests.

cond-mat.mtrl-sci

Magnetic properties of van der Waals layered single crystals DyOBr and SmOCl

Two-dimensional van der Waals single crystals DyOBr and SmOCl have been grown by flux method and their anisotropic magnetic properties are reported. DyOBr orders antiferromagnetically at T$_{N}$=9.5 K with magnetic moments lying along $a$-axis, similar as DyOCl. Its magnetic susceptibility shows an anomaly at T$^{*}$=30 K possibly due to the crystal field effect. Furthermore a 1/3 magnetization plateau is clearly observed under H$\parallel$a and H$\parallel$[110], which might be a field-induced spin-flop phase or some exotic quantum magnetic state. On the other hand, isostructural SmOCl undergoes an antiferromagnetic transition at T$_{N}$=7.1 K and exhibits a contrasting Ising-like perpendicular $c$-axis magnetic anisotropy, which could be well explained by our crystal field calculations. Both DyOBr and SmOCl are insulators with band gap of $\sim$5 eV, our results suggest they are promising in building van der Waals heterostructures and applications in multifunctional devices.

cond-mat.mtrl-sci

Number of full exceptional collections modulo spherical twists for elliptic orbifolds

This paper calculates the number of full exceptional collections modulo an action of a group as the set generated by spherical twists for an abelian category of coherent sheaves on an orbifold projective line with a zero orbifold Euler characteristic. This is done by a recursive formula naturally generalizing the one for the Dynkin case by Deligne whose categorical interpretation is due to Obaid-Nauman-Shammakh-Fakieh-Ringel and an abelian category of coherent sheaves on an orbifold projective line with a positive orbifold Euler characteristic is due to Otani-Shiraishi-Takahashi.

math.AG

Geometric model for weighted projective lines of type $(p,q)$

We give a geometric model for the category of coherent sheaves over the weighted projective line of type $(p,q)$ in terms of an annulus with marked points on its boundary. We establish a bijection between indecomposable sheaves over the weighted projective line and certain homotopy classes of oriented curves in the annulus, and prove that the dimension of extension group between indecomposable sheaves equals to the positive intersection number between the corresponding curves. By using the geometric model, we provide a combinatorial description for the titling graph of tilting bundles, which is composed by quadrilaterals (or degenerated to a line). Moreover, we obtain that the automorphism group of the coherent sheaf category is isomorphic to the mapping class group of the marked annulus, and show the compatibility of their actions on the tilting graph of coherent sheaves and on the triangulation of the geometric model respectively. A geometric description of the perpendicular category with respect to an exceptional sheaf is presented at the end of the paper.

math.RT

FeGe1-xSbx:a series of novel kagome metals with noncollinear antiferromagnetism

Kagome metals are important for exploring emergent phenomena due to the interplay between band topology and electron correlation.Motivated by the recent discovery of charge density wave in a kagome lattice antiferromagnetic FeGe,we investigate the impact of Sb doping on the structural,charge and magnetic order of FeGe.The charge density wave is rapidly suppressed by Sb doping(~1.5%) and the antiferromagnetic ordering temperature gradually shifts to 280K for FeGe0.7Sb0.3.For FeGe1-xSbx with x>0.1,crystal structures with slightly distorted Fe kagome lattice are formed.Their magnetic anisotropy has significant change,temperature driven spin-reorientation and field-induced spin-flop transition are identified from magnetization measurement.Interestingly,neutron diffraction reveals noncollinear antiferromagnetic structures widely exist below TN for all sample with x>0.1.This noncollinear magnetic orders could possibly be unconventional and resulted from onsite repulsion and filling condition of kagome flat band,as predicted by a recent theoretical work.

cond-mat.str-el

Multiple magnetic transitions and complex magnetic structures in Fe$_2$SiSe$_4$ with the sawtooth lattice

The sawtooth lattice shares some structural similarities with the kagome lattice and may attract renewed research interest. Here, we report a comprehensive study on the physical properties of Fe$_2$SiSe$_4$, an unexplored member in the olivine chalcogenides with the sawtooth lattice of Fe. Our results show that Fe$_2$SiSe$_4$ is a magnetic semiconductor with band gap of 0.66~eV. It first undergoes an antiferromagnetic transition at T$_{m1}$=110~K, then an ferrimagnetic-like one at T$_{m2}$=50~K and finally a magnetic transition at T$_{m3}$=25~K which is likely driven by the thermal populations of spin-orbit manifold on the Fe site. Neutron diffraction analysis reveals a non-collinear antiferromagnetic structure with propagation vector $\mathbf{q_1}$=(0,0,0) at T$_{m2}$<T<T$_{m1}$. Interestingly, below T$_{m2}$, an additional antiferromagnetic structure with $\mathbf{q_2}$=(0,0.5,0) appears and Fe$_2$SiSe$_4$ exhibits a complex double-$\mathbf{q}$ magnetic structure which has never been observed in sawtooth olivines. Density functional theory calculations suggest this complex noncollinear magnetic structure may originate from the competing antiferromagnetic interactions for both intra- and inter-chain in the sawtooth lattice. Furthermore, band structural calculations show that Fe$_2$SiSe$_4$ has quasi-flat band features near the valence and conduction bands. Based on the above results, we propose Fe$_2$SiSe$_4$ as a new material platform to condensed matter researches.

cond-mat.mtrl-sci

Topological Hall Effect Driven by Short-Range Magnetic Orders in EuZn$_2$As$_2$

Short-range (SR) magnetic orders such as magnetic glass orders or fluctuations in a quantum system usually host exotic states or critical behaviors. As the long-range (LR) magnetic orders, SR magnetic orders can also break time-reversal symmetry and drive the non-zero Berry curvature leading to novel transport properties. In this work, we report that in EuZn$_2$As$_2$ compound, besides the LR A-type antiferromagnetic (AF) order, the SR magnetic order is observed in a wide temperature region. The magnetization measurements and electron spin resonance (ESR) measurements reveal the ferromagnetic (FM) correlations for this SR magnetic order which results in an obvious anomalous Hall effect above the AF transition. Moreover the ESR results reveal that this FM SR order coexists with LR AF order exhibiting anisotropic magnetic correlations below the AF transition. The interactions of LR and SR magnetism evolving with temperature and field can host non-zero spin charility and berry curvature leading the additional topological Hall contribution even in a centrosymmetric simple AF system. Our results indicate that EuZn$_2$As$_2$ is a fertile platform to investigate exotic magnetic and electronic states.

cond-mat.str-el

Anisotropic magnetic properties and tunable conductivity in two-dimensional layered NaCrX2 (X=Te,Se,S) single crystals

Monolayer NaCrX2 (X=Te,Se,S) were theoretically proposed to be two-dimensional intrinsic ferromagnetic semiconductors while their physical properties have not been thoroughly investigated in bulk single crystals. We report the single-crystal growth, structural, magnetic and electronic transport properties of NaCr(Te1-xSex)2 (0 6 x 6 1) and NaCrS2. For NaCr(Te1-xSex)2, the strong perpendicular magnetic anisotropy of NaCrTe2 can be gradually tuned to be a nearly isotropic one by Se-doping. Meanwhile, a systematic change in the conductivity with increasing x is observed, displaying a doping-induced metal-insulator-like transition. Under magnetic field larger than 30 koe, both NaCrTe2 and NaCrSe2 can be polarized to a ferromagnetic state. While for NaCrS2, robust antiferromagnetism is observed up to 70 kOe and two field-induced metamagnetic transitions are identified along H||ab. These intriguing properties together with the potential to be exfoliated down to few-layer thickness make NaCrX2 (X=Te,Se,S) promising for exploring spintronic applications.

cond-mat.mtrl-sci

Exchange field enhanced upper critical field of the superconductivity in compressed antiferromagnetic EuTe2

We report high pressure studies on the C-type antiferromagnetic semiconductor EuTe2 up to 36.0 GPa. A structural transition from the I4/mcm to C2/m space group is identified at ~16 GPa. Superconductivity is discovered above ~5 GPa in both the I4/mcm and C2/m space groups. In the low-pressure phase (< 16 GPa), the antiferromagnetic transition temperature is enhanced with increasing pressure due to the enhanced magnetic exchange interactions. Magnetoresistance measurements indicate an interplay between the local moments of Eu2+ and the conduction electrons of Te 5p orbits. The upper critical field of the superconductivity is well above the Pauli limit. Across the structural transition to the high-pressure phase (> 16 GPa), EuTe2 becomes nonmagnetic and the superconducting transition temperature evolves smoothly with the upper critical field below the Pauli limit. Therefore, the high upper critical field of EuTe2 in the low-pressure phase is due to the exchange field compensation effect of the Eu magnetic order and the superconductivity in both structures may arise in the framework of the BCS theory.

cond-mat.supr-con

Antiferromagnetic structure and magnetic properties of Dy2O2Te: An isostructural analog of the rare-earth superconductors R2O2Bi

The rare-earth compounds R2O2Bi (R=Tb, Dy, Er, Lu, Y) are newly discovered superconductors in the vicinity of a rare-earth magnetic long-range order. In this work, we determine the magnetic order of the parent compound Dy2O2Te by neutron scattering as the A-type antiferromagnetic structure below the N\'eel temperature TN=9.7K. The large staggered magnetic moment 9.4(1) {\mu}B per Dy at T=3.5K lies in the basal ab plane. In a magnetic field, anomalous magnetic properties including the bifurcation between zero-field- and field-cooling magnetization, a butterfly-shaped magnetic hysteresis, and slow magnetic relaxation emerge, which are related to the field-induced metamagnetic transitions in Dy2O2Te. Our experimental findings could stimulate further research on the relation between antiferromagnetism and superconductivity in these rare-earth compounds.

cond-mat.supr-con

DyOCl: a rare-earth based two-dimensional van der Waals material with strong magnetic anisotropy

Comparing with the widely known transitional metal based van der Waals (vdW) materials, rare-earth based ones are rarely explored in the research of intrinsic two-dimensional (2D) magnetism. In this work, we report the physical properties of DyOCl, a rare-earth based vdW magnetic insulator with direct band gap of $\sim 5.72~eV$. The magnetic order of bulk DyOCl is determined by neutron scattering as the $A$-type antiferromagnetic structure below the N\'{e}el temperature $T_N=10~$K. The large magnetic moment near 10.1 $ \mu_{B} $/Dy lies parallel to the $a$-axis with strong uniaxial magnetic anisotropy. At $2~K$, a moderate magnetic field ($\sim 2~T$) applied along the easy axis generates spin-flip transitions and polarizes DyOCl to a ferromagnetic state. Density functional theory calculations reveal an extremely large magnetic anisotropy energy ($-5850~\mu eV/Dy$) for DyOCl, indicating the great potentials to realize magnetism in 2D limit. Furthermore, the mechanical exfoliation of bulk DyOCl single crystals down to seven layers is demonstrated. Our findings suggest DyOCl is a promising material playground to investigate 2D $f$-electron magnetism and spintronic applications at the nanoscale.

cond-mat.mtrl-sci

Equivariant approach to weighted projective curves

We investigate group actions on the category of coherent sheaves over weighted projective lines. We show that the equivariant category with respect to certain finite group action is equivalent to the category of coherent sheaves over a weighted projective curve, where the genus of the underlying smooth projective curve and the weight data are given by explicit formulas. Moreover, we obtain a trichotomy result for all such equivariant relations. This equivariant approach provides an effective way to investigate smooth projective curves via weighted projective lines. As an application, we give a description for the category of coherent sheaves over a hyperelliptic curve of arbitrary genus. Links to smooth projective curves of genus 2 and also to Arnold's exceptional unimodal singularities are also established.

math.RT

Extreme Suppression of Antiferromagnetic Order and Critical Scaling in a Two-Dimensional Random Quantum Magnet

Sr$_2$CuTeO$_6$ is a square-lattice Néel antiferromagnet with superexchange between first-neighbor $S=1/2$ Cu spins mediated by plaquette centered Te ions. Substituting Te by W, the affected impurity plaquettes have predominantly second-neighbor interactions, thus causing local magnetic frustration. Here we report a study of Sr$_2$CuTe$_{1-x}$W$_x$O$_6$ using neutron diffraction and $μ$SR techniques, showing that the Néel order vanishes already at $x = 0.025 \pm 0.005$. We explain this extreme order suppression using a two-dimensional Heisenberg spin model, demonstrating that a W-type impurity induces a deformation of the order parameter that decays with distance as $1/r^2$ at temperature $T=0$. The associated logarithmic singularity leads to loss of order for any $x>0$. Order for small $x>0$ and $T>0$ is induced by weak interplane couplings. In the nonmagnetic phase of Sr$_2$CuTe$_{1-x}$W$_x$O$_6$, the $μ$SR relaxation rate exhibits quantum critical scaling with a large dynamic exponent, $z \approx 3$, consistent with a random-singlet state.

cond-mat.str-el