Topological Nodal-Line Fermions in the Non-Centrosymmetric Superconductor Compound PbTaSe2
We report the identification of a Topological Nodal-Line Semimetal state in PbTaSe2.
cond-mat.mes-hall↗
arXiv subjects
Horng-Tay Jeng
Publications and source records attributed to Horng-Tay Jeng.
Two distinct topological phases in the mixed valence compound YbB6 and its differences from SmB6
We discuss the evolution of topological states and their orbital textures in the mixed valence compounds SmB6 and YbB6 within the framework of the generalized gradient approximation plus onsite Coulomb interaction (GGA+U) scheme for a wide range of values of U. In SmB6, the topological Kondo insulator (TKI) gap is found to be insensitive to the value of U, but in sharp contrast, Kondo physics in isostructural YbB6 displays a surprising sensitivity to U. In particular, as U is increased in YbB6, the correlated TKI state in the weak-coupling regime transforms into a d-p-type topological insulator phase with a band inversion between Yb-5d and B-2p orbitals in the intermediate coupling range, without closing the insulating energy gap throughout this process. Our theoretical predictions related to the TKI and non-TKI phases in SmB6 and YbB6 are in substantial accord with recent angle-resolved photoemission spectroscopy (ARPES) experiments.
cond-mat.mtrl-sci↗
Unconventional transformation of spin Dirac phase across a topological quantum phase transition
The topology of a topological material can be encoded in its surface states. These surface states can only be removed by a bulk topological quantum phase transition into a trivial phase. Here we use photoemission spectroscopy to image the formation of protected surface states in a topological insulator as we chemically tune the system through a topological transition. Surprisingly, we discover an exotic spin-momentum locked, gapped surface state in the trivial phase that shares many important properties with the actual topological surface state in anticipation of the change of topology. Using a spin-resolved measurement, we show that apart from a surface band-gap these states develop spin textures similar to the topological surface states well-before the transition. Our results offer a general paradigm for understanding how surface states in topological phases arise and are suggestive for future realizing Weyl arcs, condensed matter supersymmetry and other fascinating phenomena in the vicinity of topological quantum criticality.
cond-mat.mes-hall↗
Observation of Fermi Arc Surface States in a Topological Metal: A New Type of 2D Electron Gas beyond Z2 Topological Insulators
In a topological insulator, it is the electrons on the surface or edge that carry the signature of topology. Recently, a novel topological state has been proposed in metals or semimetals (gapless) whose band-structure is similar to that of a three-dimensional analog of graphene. However, to this date the signature of its topology remains an open question. We report the experimental discovery of a pair of polarized Fermi arc surface state modes in the form of a new type of two-dimensional polarized electron gas on the surfaces of Dirac semimetals. These Fermi arc surface states (FASS) are observed to connect across an even number of bulk band gapless nodes and found to have their spin uniquely locked to their momentum. We show that these states are distinctly different from the topological surface states (TSS) seen in all known topological insulators. Our observed exotic two-dimensional states not only uncover the novel topology of gapless Dirac metals (such as sodium tribismuth Na$_3$Bi) but also opens new research frontiers for the utilization of topological Fermi arc electron gases for a wide range of fundamental physics and spintronic studies.
cond-mat.mes-hall↗
Ultraquantum magnetoresistance in single-crystalline $β$-Ag$_2$Se
In the history of condensed matter physics, reinvestigation of a well-studied material with enhanced quality sometimes led to important scientific discoveries. A well-known example is the discovery of fractional quantum Hall effect in high quality GaAs/AlGaAs heterojunctions. Here we report the first single crystal growth and magnetoresistance (MR) measurements of the silver chalcogenide $β$-Ag$_2$Se (Naumannite), a compound has been known for the unusual, linear-field-dependent MR in its polycrystalline form for over a decade. With the quantum limit (QL) as low as 3 Tesla, a moderate field produced by a superconductor magnet available in many laboratories can easily drive the electrons in Ag$_2$Se to an unprecedented state. We observed significant negative longitudinal MR beyond the QL, which was understood as a `charge-pumping' effect between the novel fermions with opposite chiralities. Characterization of the single-crystalline Ag$_2$Se and the fabrication of electric devices working above the QL, will represent a new direction for the study of these exotic electrons.
cond-mat.str-el↗
Non-Kondo-like Electronic Structure in the Correlated Rare-Earth Hexaboride YbB$_6$
We present angle-resolved photoemission studies on the rare-earth hexaboride YbB$_6$, which has recently been predicted to be a topological Kondo insulator. Our data do not agree with the prediction and instead show that YbB$_6$ exhibits a novel topological insulator state in the absence of a Kondo mechanism. We find that the Fermi level electronic structure of YbB$_6$ has three 2D Dirac cone like surface states enclosing the Kramers' points, while the f-orbital which would be relevant for the Kondo mechanism is $\sim1$ eV below the Fermi level. Our first-principles calculation shows that the topological state which we observe in YbB$_6$ is due to an inversion between Yb $d$ and B $p$ bands. These experimental and theoretical results provide a new approach for realizing novel correlated topological insulator states in rare-earth materials.
cond-mat.str-el↗
Surface Versus Bulk Dirac States Tuning in a Three-Dimensional Topological Dirac Semimetal
Recently, crystalline-symmetry-protected three-dimensional (3D) bulk Dirac semimetal phase has been experimentally identified in a stoichiometric high-mobility compound, Cd3As2. The Dirac state observed in Cd3As2 has been attributed to originate mostly from the bulk state while calculations show that the bulk and surface states overlap over the entire Dirac dispersion energy range. In this study, we unambiguously reveal doping induced evolution of the ground state of surface and bulk electron dynamics in a 3D Dirac semimetal. We develop a systematic technique to isolate the surface and bulk states in Cd3As2, by simultaneously utilizing angle-resolved photoemission spectroscopy (ARPES) and in-situ surface deposition. Our experimental results provide a method for tuning the chemical potential as well as to observe surface states degenerate with bulk states, which will be useful for future applications of 3D Dirac semimetal.
cond-mat.mes-hall↗
Nanoscale interplay of strain and doping in a high-temperature superconductor
The highest temperature superconductors are electronically inhomogeneous at the nanoscale, suggesting the existence of a local variable which could be harnessed to enhance the superconducting pairing. Here we report the relationship between local doping and local strain in the cuprate superconductor Bi$_2$Sr$_2$CaCu$_2$O$_{8+x}$. We use scanning tunneling microscopy to discover that the crucial oxygen dopants are periodically distributed, in correlation with local strain. Our picoscale investigation of the intra-unit-cell positions of all oxygen dopants provides essential structural input for a complete microscopic theory.
cond-mat.str-el↗
Observation of Quantum-Tunneling Modulated Spin Texture in Ultrathin Topological Insulator Bi2Se3 Films
Understanding the spin-texture behavior of boundary modes in ultrathin topological insulator films is critically essential for the design and fabrication of functional nano-devices. Here by using spin-resolved photoemission spectroscopy with p-polarized light in topological insulator Bi2Se3 thin films, we report tunneling-dependent evolution of spin configuration in topological insulator thin films across the metal-to-insulator transition. We observe strongly binding energy- and wavevector-dependent spin polarization for the topological surface electrons in the ultra-thin gapped-Dirac-cone limit. The polarization decreases significantly with enhanced tunneling realized systematically in thin insulating films, whereas magnitude of the polarization saturates to the bulk limit faster at larger wavevectors in thicker metallic films. We present a theoretical model which captures this delicate relationship between quantum tunneling and Fermi surface spin polarization. Our high-resolution spin-based spectroscopic results suggest that the polarization current can be tuned to zero in thin insulating films forming the basis for a future spin-switch nano-device.
cond-mat.mes-hall↗
Spin correlated electronic state on the surface of a spin-orbit Mott system (Layered Iridates)
Novel phases of two dimensional electron systems resulting from new surface or interface modified electronic structures have generated significant interest in material science. We utilize photoemission spectroscopy to show that the near-surface electronic structure of a bulk insulating iridate Sr$_3$Ir$_2$O$_7$ lying near metal-Mott insulator transition exhibit weak metallicity signified by finite electronic spectral weight at the Fermi level. The surface electrons exhibit a unique spin structure resulting from an interplay of spin-orbit, Coulomb interaction and surface quantum magnetism, distinct from a topological insulator state. Our results suggest the experimental realization of a novel quasi two dimensional interacting electron surface ground state, opening the door for exotic quantum entanglement and transport phenomena in iridate-based oxide devices.
cond-mat.str-el↗
Direct observation of the transition from indirect to direct bandgap in atomically thin epitaxial MoSe2
Quantum systems in confined geometries are host to novel physical phenomena. Examples include quantum Hall systems in semiconductors and Dirac electrons in graphene. Interest in such systems has also been intensified by the recent discovery of a large enhancement in photoluminescence quantum efficiency and a potential route to valleytronics in atomically thin layers of transition metal dichalcogenides, MX2 (M = Mo, W; X = S, Se, Te), which are closely related to the indirect to direct bandgap transition in monolayers. Here, we report the first direct observation of the transition from indirect to direct bandgap in monolayer samples by using angle resolved photoemission spectroscopy on high-quality thin films of MoSe2 with variable thickness, grown by molecular beam epitaxy. The band structure measured experimentally indicates a stronger tendency of monolayer MoSe2 towards a direct bandgap, as well as a larger gap size, than theoretically predicted. Moreover, our finding of a significant spin-splitting of 180 meV at the valence band maximum of a monolayer MoSe2 film could expand its possible application to spintronic devices.
cond-mat.mtrl-sci↗
Surface electronic structure of the topological Kondo insulator candidate correlated electron system SmB6
The Kondo insulator SmB6 has long been known to exhibit low temperature transport anomalies whose origin is of great interest. Here we uniquely access the surface electronic structure of the anomalous transport regime by combining state-of-the-art laser- and synchrotron-based angle-resolved photoemission techniques. We observe clear in-gap states (up to 4 meV), whose temperature dependence is contingent upon the Kondo gap formation. In addition, our observed in-gap Fermi surface oddness tied with the Kramers' points topology, their coexistence with the two-dimensional transport anomaly in the Kondo hybridization regime, as well as their robustness against thermal recycling, taken together, collectively provide by-far the strongest evidence for protected surface metallicity with a Fermi surface whose topology is consistent with the theoretically predicted topological surface Fermi surface (TSS). Our observations of systematic surface electronic structure provide the fundamental electronic parameters for the anomalous Kondo ground state of the correlated electron material SmB6.
cond-mat.str-el↗
Imaging the evolution of metallic states in a spin-orbit interaction driven correlated iridate
The Ruddlesden-Popper (RP) series of iridates (Srn+1IrnO3n+1) have been the subject of much recent attention due to the anticipation of emergent physics arising from the cooperative action of spin-orbit (SO) driven band splitting and Coulomb interactions[1-3]. However an ongoing debate over the role of correlations in the formation of the charge gap and a lack of understanding of the effects of doping on the low energy electronic structure have hindered experimental progress in realizing many of the predicted states[4-8] including possible high-Tc superconductivity[7,9]. Using scanning tunneling spectroscopy we map out the spatially resolved density of states in the n=2 RP member, Sr3Ir2O7 (Ir327). We show that the Ir327 parent compound, argued to exist only as a weakly correlated band insulator in fact possesses a substantial ~130meV charge excitation gap driven by an interplay between structure, SO coupling and correlations. A critical component in distinguishing the intrinsic electronic character within the inhomogeneous textured electronic structure is our identification of the signature of missing apical oxygen defects, which play a critical role in many of the layered oxides. Our measurements combined with insights from calculations reveal how apical oxygen vacancies transfer spectral weight from higher energies to the gap energies thereby revealing a path toward obtaining metallic electronic states from the parent-insulating states in the iridates.
cond-mat.mtrl-sci↗
Gated Silicene as a tunable source of nearly 100% spin-polarized electrons
Silicene is a one-atom-thick 2D crystal of silicon with a hexagonal lattice structure that is related to that of graphene but with atomic bonds that are buckled rather than flat. This buckling confers advantages on silicene over graphene, because it should, in principle, generate both a band gap and polarized spin-states that can be controlled with a perpendicular electric field. Here we use first-principles calculations to show that field-gated silicene possesses two gapped Dirac cones exhibiting nearly 100% spin-polarization, situated at the corners of the Brillouin zone. Using this fact, we propose a design for a silicene-based spin-filter that should enable the spin-polarization of an output current to be switched electrically, without switching external magnetic fields. Our quantum transport calculations indicate that the proposed designs will be highly efficient (nearly 100% spin polarization) and robust against weak disorder and edge imperfections. We also propose a Y-shaped spin/valley separator that produces spin-polarized current at two output terminals with opposite spins.
cond-mat.mtrl-sci↗
Hedgehog Spin-texture and Berry's Phase tuning in a Magnetic Topological Insulator
Understanding and control of spin degrees of freedom on the surfaces of topological materials are key to future applications as well as for realizing novel physics such as the axion electrodynamics associated with time-reversal (TR) symmetry breaking on the surface. We experimentally demonstrate magnetically induced spin reorientation phenomena simultaneous with a Dirac-metal to gapped-insulator transition on the surfaces of manganese-doped Bi2Se3 thin films. The resulting electronic groundstate exhibits unique hedgehog-like spin textures at low energies, which directly demonstrate the mechanics of TR symmetry breaking on the surface. We further show that an insulating gap induced by quantum tunnelling between surfaces exhibits spin texture modulation at low energies but respects TR invariance. These spin phenomena and the control of their Fermi surface geometrical phase first demonstrated in our experiments pave the way for the future realization of many predicted exotic magnetic phenomena of topological origin.
cond-mat.mes-hall↗
Quantized magnetic moment at the edge of a single-walled carbon nanotube
We investigate many-body effects near the edge of a single-walled carbon nanotube and find it turns magnetic with quantized edge moment solely depends on the chiral vector, i.e. the topology of the carbon nanotube. The distribution of the edge moment reveals an approximate supersymmetry even in a realistic model. Our findings demonstrate crucial importance of the interplay between the electronic correlation and the edge morphology. The edge moment provides an excellent candidate for nanomagnet farbrication which has potential applications in biological and chemical detections, and in spintronics.
cond-mat.mes-hall↗
Ferromagnetism in armchair graphene nanoribbon
Due to the weak spin-orbit interaction and the peculiar relativistic dispersion in graphene, there are exciting proposals to build spin qubits in graphene nanoribbons with armchair boundaries. However, the mutual interactions between electrons are neglected in most studies so far and thus motivate us to investigate the role of electronic correlations in armchair graphene nanoribbon by both analytical and numerical methods. Here we show that the inclusion of mutual repulsions leads to drastic changes and the ground state turns ferromagnetic in a range of carrier concentrations. Our findings highlight the crucial importance of the electron-electron interaction and its subtle interplay with boundary topology in graphene nanoribbons. Furthermore, since the ferromagnetic properties sensitively depends on the carrier concentration, it can be manipulated at ease by electric gates. The resultant ferromagnetic state with metallic conductivity is not only surprising from an academic viewpoint, but also has potential applications in spintronics at nanoscale.
cond-mat.mes-hall↗