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Hsin-Ying Chiu

Publications and source records attributed to Hsin-Ying Chiu.

9 recordsLinked to original sources

Exceptional and Anisotropic Transport Properties of Photocarriers in Black Phosphorus

We show that black phosphorus has room-temperature charge mobilities on the order of 10$^4$ cm$^2$V$^{-1}$s$^{-1}$, which are about one order of magnitude larger than silicon. We also demonstrate strong anisotropic transport in black phosphorus, where the mobilities along the armchair direction are about one order of magnitude larger than zigzag direction. A photocarrier lifetime as long as 100 ps is also determined. These results illustrate that black phosphorus is a promising candidate for future electronic and optoelectronic applications.

cond-mat.mtrl-sci

Graphene Side Gate Engineering

Various mesoscopic devices exploit electrostatic side gates for their operation. In this paper, we investigate how voltage-biasing of graphene side gates modulates the electrical transport characteristics of graphene channel. We explore myriads of typical side gated devices such as symmetric dual side gates and asymmetric single side gate biasing, in monolayer and bilayer graphene. The side gates modulate the electrostatic doping in the graphene channel whose effect is reflected in transport measurement. This modulation efficiency is systematically characterized for all our devices and agrees well with the modeling presented.

cond-mat.mes-hall

Third harmonic generation in graphene and few-layer graphite films

We observe optical third harmonic generation from graphene and few-layer graphite flakes produced by exfoliation. The emission scales with the cube of the intensity of the incident near-infrared femtosecond pulses and has a wavelength that is one-third of the incident wavelength, both consistent with third harmonic generation. We extract an effective third-order susceptibility for graphene that is on the order of 1e-16 square meter per square volt, which is comparable to that for materials that are resonantly excited, but larger than for materials that are transparent at the fundamental and third harmonic wavelengths. By measuring a set of flakes with different numbers of atomic layers, we find that the emission scales with the square of the number of atomic layers, which suggests that the susceptibility of graphene is independent of layer number, at least for a few layers.

cond-mat.mes-hall

Ultrafast and spatially resolved studies of charge carriers in atomically-thin molybdenum disulfide

Atomically-thin molybdenum disulfide is emerging as a new nanomaterial with potential applications in the fields of electronic and photonics. Charge carrier dynamics plays an essential role in determining its electronic and optical properties. We report spatially and temporally resolved pump-probe studies of charge carriers in atomically-thin molybdenum disulfide samples fabricated by mechanical exfoliation. Carriers are injected by interband absorption of a 390-nm pump pulse and detected by measuring differential reflection of a time-delayed and spatially-scanned probe pulse that is tuned to an exciton transition. Several parameters on charge carrier dynamics are deduced, including carrier lifetime, diffusion coefficient, diffusion length, and mobility.

cond-mat.mes-hall

Optical pump-probe studies of carrier dynamics in few-layer MoS2

Femtosecond optical pump-probe technique is used to study charge carrier dynamics in few-layer MoS2 samples fabricated by mechanical exfoliation. An ultrafast pump pulse excites carriers and differential reflection of a probe pulse tuned to an excitonic resonance is detected. We find that the spectrum of the differential reflection signal is similar to the derivative of the resonance. The decay time of the signal is in the range of 150 to 400 ps, increasing with the probe wavelength. With a fixed probe wavelength, the signal magnitude is proportional to the pump fluence, while the decay time is independent of it.

cond-mat.mes-hall

Thermal infrared emission reveals the Dirac point movement in biased graphene

Graphene is a 2-dimensional material with high carrier mobility and thermal conductivity, suitable for high-speed electronics. Conduction and valence bands touch at the Dirac point. The absorptivity of single-layer graphene is 2.3%, nearly independent of wavelength. Here we investigate the thermal radiation from biased graphene transistors. We find that the emission spectrum of single-layer graphene follows that of a grey body with constant emissivity (1.6 \pm 0.8)%. Most importantly, we can extract the temperature distribution in the ambipolar graphene channel, as confirmed by Stokes/anti-Stokes measurements. The biased graphene exhibits a temperature maximum whose location can be controlled by the gate voltage. We show that this peak in temperature reveals the spatial location of the minimum in carrier density, i.e. the Dirac point.

cond-mat.mes-hall

100 GHz Transistors from Wafer Scale Epitaxial Graphene

High-performance graphene field-effect transistors have been fabricated on epitaxial graphene synthesized on a two-inch SiC wafer, achieving a cutoff frequency of 100 GHz for a gate length of 240 nm. The high-frequency performance of these epitaxial graphene transistors not only shows the highest speed for any graphene devices up to date, but it also exceeds that of Si MOSFETs at the same gate length. The result confirms the high potential of graphene for advanced electronics applications, marking an important milestone for carbon electronics.

cond-mat.mtrl-sci

Dual Gate Graphene FETs with fT of 50 GHz

A dual-gate graphene field-effect transistors is presented, which shows improved RF performance by reducing the access resistance using electrostatic doping. With a carrier mobility of 2700 cm2/Vs, a cutoff frequency of 50 GHz is demonstrated in a 350-nm gate length device. This fT value is the highest frequency reported to date for any graphene transistor, and it also exceeds that of Si MOSFETs at the same gate length, illustrating the potential of graphene for RF applications.

cond-mat.mes-hall

Utilization of a Buffered Dielectric to Achieve High Field-Effect Carrier Mobility in Graphene Transistors

We utilize an organic polymer buffer layer between graphene and conventional gate dielectrics in top-gated graphene transistors. Unlike other insulators, this dielectric stack does not significantly degrade carrier mobility, allowing for high field-effect mobilities to be retained in top-gate operation. This is demonstrated in both two-point and four-point analysis, and in the high-frequency operation of a graphene transistor. Temperature dependence of the carrier mobility suggests that phonons are the dominant scatterers in these devices.

cond-mat.mtrl-sci