arXiv subjects

Huan Zhao

Publications and source records attributed to Huan Zhao.

At least 55 records · Page 3Linked to original sources

arXiv2025

Enabling Continuous THz Band Coverage via Precise Electron Beam Tailoring in Free-electron Lasers

High-power, continuously tunable narrowband terahertz (THz) sources are essential for advancing nonlinear optics, THz-driven material dynamics, and ultrafast spectroscopy. Conventional techniques typically impose a trade-off between pulse energy and frequency tunability. Here, we introduce a novel free-electron laser approach that overcomes these limitations by pre-modulating a relativistic electron beam with a frequency-beating laser pulse and leveraging bunch compression along with collective effects to enhance microbunching. Experimental results demonstrate that this technique generates narrowband THz emission with continuous frequency tunability from 7.8 to 30.8THz, achieving pulse energies up to 385μJ while maintaining spectral bandwidths between 7.7% and 14.7%. Moreover, the method exhibits exceptional robustness and scalability, highlighting its unique ability to bridge the long-standing THz gap and offering a promising solution for diverse cutting-edge scientific applications.

physics.acc-ph↗

arXiv2025

Defect Engineering in Large-Scale CVD-Grown Hexagonal Boron Nitride: Formation, Spectroscopy, and Spin Relaxation Dynamics

Recently, numerous techniques have been reported for generating optically active defects in exfoliated hexagonal boron nitride (hBN), which hold transformative potential for quantum photonic devices. However, achieving on-demand generation of desirable defect types in scalable hBN films remains a significant challenge. Here, we demonstrate that formation of negative boron vacancy defects, VB-, in suspended, large-area CVD-grown hBN is strongly dependent on the type of bombarding particles (ions, neutrons, and electrons) and irradiation conditions. In contrast to suspended hBN, defect formation in substrate-supported hBN is more complex due to the uncontrollable generation of secondary particles from the substrate, and the outcome strongly depends on the thickness of the hBN. We identify different defect types by correlating spectroscopic and optically detected magnetic resonance features, distinguishing boron vacancies (formed by light ions and neutrons) from other optically active defects emitting at 650 nm assigned to anti-site nitrogen vacancy (NBVN) and reveal the presence of additional dark paramagnetic defects that influence spin-lattice relaxation time (T1) and zero-field splitting parameters, all of which strongly depend on the defect density. These results underscore the potential for precisely engineered defect formation in large-scale CVD-grown hBN, paving the way for the scalable fabrication of quantum photonic devices.

cond-mat.mtrl-sci↗

arXiv2025

Electric Field-Induced Formation of a 2D Adatom Gas on Cryogenic Li Surfaces

Intense electrostatic fields, such as those able to break bonds and cause field-ion emission, can fundamentally alter the behaviour of atoms at and on the surface. Using density functional theory (DFT) calculations on the Li (110) surface under high electrostatic fields, we identify a critical field strength at which surface atoms occupying a kink site become thermodynamically unstable against adatom formation. This mechanism leads to the formation of a highly concentrated two-dimensional (2D) adatom gas on the surface. Moreover, the applied field reverses the stability of preferred adsorption sites, enabling barrierless diffusion of lithium atoms even well below the threshold required for field evaporation. The here identified mechanisms offer a unified explanation for experimental observations in atom probe tomography and for understanding high electric field phenomena in systems such as battery interfaces and electrochemical environments.

cond-mat.mtrl-sci↗

arXiv2025

Leveraging Surgical Activity Grammar for Primary Intention Prediction in Laparoscopy Procedures

Surgical procedures are inherently complex and dynamic, with intricate dependencies and various execution paths. Accurate identification of the intentions behind critical actions, referred to as Primary Intentions (PIs), is crucial to understanding and planning the procedure. This paper presents a novel framework that advances PI recognition in instructional videos by combining top-down grammatical structure with bottom-up visual cues. The grammatical structure is based on a rich corpus of surgical procedures, offering a hierarchical perspective on surgical activities. A grammar parser, utilizing the surgical activity grammar, processes visual data obtained from laparoscopic images through surgical action detectors, ensuring a more precise interpretation of the visual information. Experimental results on the benchmark dataset demonstrate that our method outperforms existing surgical activity detectors that rely solely on visual features. Our research provides a promising foundation for developing advanced robotic surgical systems with enhanced planning and automation capabilities.

cs.RO↗

arXiv2024

Coordinated Power Smoothing Control for Wind Storage Integrated System with Physics-informed Deep Reinforcement Learning

The Wind Storage Integrated System with Power Smoothing Control (PSC) has emerged as a promising solution to ensure both efficient and reliable wind energy generation. However, existing PSC strategies overlook the intricate interplay and distinct control frequencies between batteries and wind turbines, and lack consideration of wake effect and battery degradation cost. In this paper, a novel coordinated control framework with hierarchical levels is devised to address these challenges effectively, which integrates the wake model and battery degradation model. In addition, after reformulating the problem as a Markov decision process, the multi-agent reinforcement learning method is introduced to overcome the bi-level characteristic of the problem. Moreover, a Physics-informed Neural Network-assisted Multi-agent Deep Deterministic Policy Gradient (PAMA-DDPG) algorithm is proposed to incorporate the power fluctuation differential equation and expedite the learning process. The effectiveness of the proposed methodology is evaluated through simulations conducted in four distinct scenarios using WindFarmSimulator (WFSim). The results demonstrate that the proposed algorithm facilitates approximately an 11% increase in total profit and a 19% decrease in power fluctuation compared to the traditional methods, thereby addressing the dual objectives of economic efficiency and grid-connected energy reliability.

eess.SY↗

arXiv2024

Hard-Synth: Synthesizing Diverse Hard Samples for ASR using Zero-Shot TTS and LLM

Text-to-speech (TTS) models have been widely adopted to enhance automatic speech recognition (ASR) systems using text-only corpora, thereby reducing the cost of labeling real speech data. Existing research primarily utilizes additional text data and predefined speech styles supported by TTS models. In this paper, we propose Hard-Synth, a novel ASR data augmentation method that leverages large language models (LLMs) and advanced zero-shot TTS. Our approach employs LLMs to generate diverse in-domain text through rewriting, without relying on additional text data. Rather than using predefined speech styles, we introduce a hard prompt selection method with zero-shot TTS to clone speech styles that the ASR model finds challenging to recognize. Experiments demonstrate that Hard-Synth significantly enhances the Conformer model, achieving relative word error rate (WER) reductions of 6.5\%/4.4\% on LibriSpeech dev/test-other subsets. Additionally, we show that Hard-Synth is data-efficient and capable of reducing bias in ASR.

cs.CL↗

arXiv2024

Legal Evalutions and Challenges of Large Language Models

In this paper, we review legal testing methods based on Large Language Models (LLMs), using the OPENAI o1 model as a case study to evaluate the performance of large models in applying legal provisions. We compare current state-of-the-art LLMs, including open-source, closed-source, and legal-specific models trained specifically for the legal domain. Systematic tests are conducted on English and Chinese legal cases, and the results are analyzed in depth. Through systematic testing of legal cases from common law systems and China, this paper explores the strengths and weaknesses of LLMs in understanding and applying legal texts, reasoning through legal issues, and predicting judgments. The experimental results highlight both the potential and limitations of LLMs in legal applications, particularly in terms of challenges related to the interpretation of legal language and the accuracy of legal reasoning. Finally, the paper provides a comprehensive analysis of the advantages and disadvantages of various types of models, offering valuable insights and references for the future application of AI in the legal field.

cs.CL↗

arXiv2024

Survey on Large Language Model-Enhanced Reinforcement Learning: Concept, Taxonomy, and Methods

With extensive pre-trained knowledge and high-level general capabilities, large language models (LLMs) emerge as a promising avenue to augment reinforcement learning (RL) in aspects such as multi-task learning, sample efficiency, and high-level task planning. In this survey, we provide a comprehensive review of the existing literature in LLM-enhanced RL and summarize its characteristics compared to conventional RL methods, aiming to clarify the research scope and directions for future studies. Utilizing the classical agent-environment interaction paradigm, we propose a structured taxonomy to systematically categorize LLMs' functionalities in RL, including four roles: information processor, reward designer, decision-maker, and generator. For each role, we summarize the methodologies, analyze the specific RL challenges that are mitigated, and provide insights into future directions. Lastly, a comparative analysis of each role, potential applications, prospective opportunities, and challenges of the LLM-enhanced RL are discussed. By proposing this taxonomy, we aim to provide a framework for researchers to effectively leverage LLMs in the RL field, potentially accelerating RL applications in complex applications such as robotics, autonomous driving, and energy systems.

cs.LG↗

arXiv2024

Low-Dimensional Solid-State Single-Photon Emitters

Solid-state single-photon emitters (SPEs) are attracting significant attention as fundamental components in quantum computing, communication, and sensing. Low-dimensional materials-based SPEs (LD-SPEs) have drawn particular interest due to their high photon extraction efficiency, ease of integration with photonic circuits, and strong coupling with external fields. The accessible surfaces of LD materials allow for deterministic control over quantum light emission, while enhanced quantum confinement and light-matter interactions improve photon emissive properties. This review examines recent progress in LDSPEs across four key materials: zero-dimensional (0D) semiconductor quantum dots, one-dimensional (1D) nanotubes, two-dimensional (2D) materials, including hexagonal boron nitride (hBN) and transition metal dichalcogenides (TMDCs). We explore their structural and photophysical properties, along with techniques such as spectral tuning and cavity coupling that enhance SPE performance. Finally, we address future challenges and suggest strategies for optimizing LD-SPEs for practical quantum applications.

physics.optics↗

arXiv2024

Nanoscale magnetic ordering dynamics in a high Curie temperature ferromagnet

Thermally driven transitions between ferromagnetic and paramagnetic phases are characterized by critical behavior with divergent susceptibilities, long-range correlations, and spin dynamics that can span kHz to GHz scales as the material approaches the critical temperature $\mathrm{T_c}$, but it has proven technically challenging to probe the relevant length and time scales with most conventional measurement techniques. In this study, we employ scanning nitrogen-vacancy center based magnetometry and relaxometry to reveal the critical behavior of a high-$\mathrm{T_c}$ ferromagnetic oxide near its Curie temperature. Cluster analysis of the measured temperature-dependent nanoscale magnetic textures points to a 3D universality class with a correlation length that diverges near $\mathrm{T_c}$. Meanwhile, the temperature-dependent spin dynamics, measured through all optical relaxometry suggest that the phase transition is in the XY universality class. Our results capture both static and dynamic aspects of critical behavior, providing insights into universal properties that govern phase transitions in magnetic materials.

cond-mat.mtrl-sci↗

arXiv2024

Telecom-wavelength Single-photon Emitters in Multi-layer InSe

The development of robust and efficient single photon emitters (SPEs) at telecom wavelengths is critical for advancements in quantum information science. Two-dimensional (2D) materials have recently emerged as promising sources for SPEs, owing to their high photon extraction efficiency, facile coupling to external fields, and seamless integration into photonic circuits. In this study, we demonstrate the creation of SPEs emitting in the 1000 to 1550 nm near-infrared range by coupling 2D indium selenide (InSe) with strain-inducing nanopillar arrays. The emission wavelength exhibits a strong dependence on the number of layers. Hanbury Brown and Twiss experiments conducted at 10 K reveal clear photon antibunching, confirming the single-photon nature of the emissions. Density-functional-theory calculations and scanning-tunneling-microscopy analyses provide insights into the electronic structures and defect states, elucidating the origins of the SPEs. Our findings highlight the potential of multilayer 2D metal monochalcogenides for creating SPEs across a broad spectral range, paving the way for their integration into quantum communication technologies.

physics.optics↗

arXiv2024

Large Language Model Should Understand Pinyin for Chinese ASR Error Correction

Large language models can enhance automatic speech recognition systems through generative error correction. In this paper, we propose Pinyin-enhanced GEC, which leverages Pinyi, the phonetic representation of Mandarin Chinese, as supplementary information to improve Chinese ASR error correction. Our approach only utilizes synthetic errors for training and employs the one-best hypothesis during inference. Additionally, we introduce a multitask training approach involving conversion tasks between Pinyin and text to align their feature spaces. Experiments on the Aishell-1 and the Common Voice datasets demonstrate that our approach consistently outperforms GEC with text-only input. More importantly, we provide intuitive explanations for the effectiveness of PY-GEC and multitask training from two aspects: 1) increased attention weight on Pinyin features; and 2) aligned feature space between Pinyin and text hidden states.

cs.CL↗

arXiv2024

A Versatile Graph Learning Approach through LLM-based Agent

Designing versatile graph learning approaches is important, considering the diverse graphs and tasks existing in real-world applications. Existing methods have attempted to achieve this target through automated machine learning techniques, pre-training and fine-tuning strategies, and large language models. However, these methods are not versatile enough for graph learning, as they work on either limited types of graphs or a single task. In this paper, we propose to explore versatile graph learning approaches with LLM-based agents, and the key insight is customizing the graph learning procedures for diverse graphs and tasks. To achieve this, we develop several LLM-based agents, equipped with diverse profiles, tools, functions and human experience. They collaborate to configure each procedure with task and data-specific settings step by step towards versatile solutions, and the proposed method is dubbed GL-Agent. By evaluating on diverse tasks and graphs, the correct results of the agent and its comparable performance showcase the versatility of the proposed method, especially in complex scenarios.The low resource cost and the potential to use open-source LLMs highlight the efficiency of GL-Agent.

cs.LG↗

arXiv2024

ElecBench: a Power Dispatch Evaluation Benchmark for Large Language Models

In response to the urgent demand for grid stability and the complex challenges posed by renewable energy integration and electricity market dynamics, the power sector increasingly seeks innovative technological solutions. In this context, large language models (LLMs) have become a key technology to improve efficiency and promote intelligent progress in the power sector with their excellent natural language processing, logical reasoning, and generalization capabilities. Despite their potential, the absence of a performance evaluation benchmark for LLM in the power sector has limited the effective application of these technologies. Addressing this gap, our study introduces "ElecBench", an evaluation benchmark of LLMs within the power sector. ElecBench aims to overcome the shortcomings of existing evaluation benchmarks by providing comprehensive coverage of sector-specific scenarios, deepening the testing of professional knowledge, and enhancing decision-making precision. The framework categorizes scenarios into general knowledge and professional business, further divided into six core performance metrics: factuality, logicality, stability, security, fairness, and expressiveness, and is subdivided into 24 sub-metrics, offering profound insights into the capabilities and limitations of LLM applications in the power sector. To ensure transparency, we have made the complete test set public, evaluating the performance of eight LLMs across various scenarios and metrics. ElecBench aspires to serve as the standard benchmark for LLM applications in the power sector, supporting continuous updates of scenarios, metrics, and models to drive technological progress and application.

cs.AI↗

arXiv2024

GAIA -- A Large Language Model for Advanced Power Dispatch

Power dispatch is essential for providing stable, cost-effective, and eco-friendly electricity to society. However, traditional methods falter as power systems grow in scale and complexity, struggling with multitasking, swift problem-solving, and human-machine collaboration. This paper introduces GAIA, the pioneering Large Language Model (LLM) tailored for power dispatch tasks. We have developed a novel dataset construction technique that harnesses a range of data sources to fine-tune GAIA for optimal performance in this domain. This approach streamlines LLM training, allowing for the seamless integration of multidimensional data in power system management. Additionally, we have crafted specialized prompt strategies to boost GAIA's input-output efficiency in dispatch scenarios. When evaluated on the ElecBench benchmark, GAIA surpasses the baseline model LLaMA2 on multiple metrics. In practical applications, GAIA has demonstrated its ability to enhance decision-making processes, improve operational efficiency, and facilitate better human-machine interactions in power dispatch operations. This paper expands the application of LLMs to power dispatch and validates their practical utility, paving the way for future innovations in this field.

eess.SY↗

arXiv2024

WenetSpeech4TTS: A 12,800-hour Mandarin TTS Corpus for Large Speech Generation Model Benchmark

With the development of large text-to-speech (TTS) models and scale-up of the training data, state-of-the-art TTS systems have achieved impressive performance. In this paper, we present WenetSpeech4TTS, a multi-domain Mandarin corpus derived from the open-sourced WenetSpeech dataset. Tailored for the text-to-speech tasks, we refined WenetSpeech by adjusting segment boundaries, enhancing the audio quality, and eliminating speaker mixing within each segment. Following a more accurate transcription process and quality-based data filtering process, the obtained WenetSpeech4TTS corpus contains $12,800$ hours of paired audio-text data. Furthermore, we have created subsets of varying sizes, categorized by segment quality scores to allow for TTS model training and fine-tuning. VALL-E and NaturalSpeech 2 systems are trained and fine-tuned on these subsets to validate the usability of WenetSpeech4TTS, establishing baselines on benchmark for fair comparison of TTS systems. The corpus and corresponding benchmarks are publicly available on huggingface.

eess.AS↗

arXiv2024

Self-supervised Graph Neural Network for Mechanical CAD Retrieval

CAD (Computer-Aided Design) plays a crucial role in mechanical industry, where large numbers of similar-shaped CAD parts are often created. Efficiently reusing these parts is key to reducing design and production costs for enterprises. Retrieval systems are vital for achieving CAD reuse, but the complex shapes of CAD models are difficult to accurately describe using text or keywords, making traditional retrieval methods ineffective. While existing representation learning approaches have been developed for CAD, manually labeling similar samples in these methods is expensive. Additionally, CAD models' unique parameterized data structure presents challenges for applying existing 3D shape representation learning techniques directly. In this work, we propose GC-CAD, a self-supervised contrastive graph neural network-based method for mechanical CAD retrieval that directly models parameterized CAD raw files. GC-CAD consists of two key modules: structure-aware representation learning and contrastive graph learning framework. The method leverages graph neural networks to extract both geometric and topological information from CAD models, generating feature representations. We then introduce a simple yet effective contrastive graph learning framework approach, enabling the model to train without manual labels and generate retrieval-ready representations. Experimental results on four datasets including human evaluation demonstrate that the proposed method achieves significant accuracy improvements and up to 100 times efficiency improvement over the baseline methods.

cs.IR↗

arXiv2024

Towards establishing best practice in the analysis of hydrogen and deuterium by atom probe tomography

As hydrogen is touted as a key player in the decarbonization of modern society, it is critical to enable quantitative H analysis at high spatial resolution, if possible at the atomic scale. Indeed, H has a known deleterious impact on the mechanical properties (strength, ductility, toughness) of most materials that can hinder their use as part of the infrastructure of a hydrogen-based economy. Enabling H mapping, including local hydrogen concentration analyses at specific microstructural features, is essential for understanding the multiple ways that H affect the properties of materials, including for instance embrittlement mechanisms and their synergies, but also spatial mapping and quantification of hydrogen isotopes is essential to accurately predict tritium inventory of future fusion power plants, ensuring their safe and efficient operation for example. Atom probe tomography (APT) has the intrinsic capabilities for detecting hydrogen (H), and deuterium (D), and in principle the capacity for performing quantitative mapping of H within a material's microstructure. Yet the accuracy and precision of H analysis by APT remain affected by the influence of residual hydrogen from the ultra-high vacuum chamber that can obscure the signal of H from within the material, along with a complex field evaporation behavior. The present article reports the essence of discussions at a focused workshop held at the Max-Planck Institute for Sustainable Materials in April 2024. The workshop was organized to pave the way to establishing best practices in reporting APT data for the analysis of H. We first summarize the key aspects of the intricacies of H analysis by APT and propose a path for better reporting of the relevant data to support interpretation of APT-based H analysis in materials.

cond-mat.mtrl-sci↗