arXiv subjects

Huanqian Loh

Publications and source records attributed to Huanqian Loh.

At least 19 recordsLinked to original sources

arXiv2025

Statistical Localization in a Rydberg Simulator of $U(1)$ Lattice Gauge Theory

Lattice gauge theories (LGTs) provide a framework for describing dynamical systems ranging from nuclei to materials. LGTs that host concatenated conservation laws can exhibit Hilbert space fragmentation, where each subspace may be labeled by a conserved quantity with nonlocal operator support. It is expected that nonlocal conservation laws will not impede thermalization locally. However, this expectation has recently been challenged by the notion of statistical localization, wherein particular motifs of microscopic configurations may remain frozen in time due to strong Hilbert space fragmentation. Here, we report the first experimental signatures of statistically-localized behavior. We realize a novel constrained LGT model using a facilitated Rydberg atom array, where atoms mediate the dynamics of electric charge clusters whose nonlocal pattern of net charges remains invariant. By experimentally reconstructing observables sampled from a temporal ensemble, we probe the spatial distribution of each conserved quantity. We find that as a result of strong Hilbert space fragmentation, the expectation values of all conserved quantities remain locally distributed in typical quantum states, even though they are described by nonlocal string-like operators. Our work opens the door to high-energy explorations of cluster dynamics and low-energy studies of strong zero modes that persist in infinite-temperature topological systems.

quant-ph↗

arXiv2024

Observation of quantum thermalization restricted to Hilbert space fragments

Quantum thermalization occurs in a broad class of systems from elementary particles to complex materials. Out-of-equilibrium quantum systems have long been understood to either thermalize or retain memory of their initial states, but not both. Here we achieve the first coexistence of thermalization and memory in a quantum system, where we use both Rydberg blockade and facilitation in an atom array to engineer a fragmentation of the Hilbert space into exponentially many disjointed subspaces. We find that the kinetically constrained system yields quantum many-body scars arising from the $\mathbb{Z}_{2k}$ class of initial states, which generalizes beyond the $\mathbb{Z}_{2}$ scars previously reported in other quantum systems. When bringing multiple long-range interactions into resonance, we observe quantum thermalization restricted to Hilbert space fragments, where the thermalized system retains characteristics of the initial configuration. Intriguingly, states belonging to different subspaces do not thermalize with each other even when they have the same energy. Our work challenges established ideas of quantum thermalization while experimentally resolving the longstanding tension between thermalization and memory. These results may be applied to control entanglement dynamics in quantum processors and quantum sensors.

quant-ph↗

arXiv2023

Floquet-Tailored Rydberg Interactions

The Rydberg blockade is a key ingredient for entangling atoms in arrays. However, it requires atoms to be spaced well within the blockade radius, which limits the range of local quantum gates. Here we break this constraint using Floquet frequency modulation, with which we demonstrate Rydberg-blockade entanglement beyond the traditional blockade radius and show how the enlarged entanglement range improves qubit connectivity in a neutral atom array. Further, we find that the coherence of entangled states can be extended under Floquet frequency modulation. Finally, we realize Rydberg anti-blockade states for two sodium Rydberg atoms within the blockade radius. Such Rydberg anti-blockade states for atoms at close range enables the robust preparation of strongly-interacting, long-lived Rydberg states, yet their steady-state population cannot be achieved with only the conventional static drive. Our work transforms between the paradigmatic regimes of Rydberg blockade versus anti-blockade and paves the way for realizing more connected, coherent, and tunable neutral atom quantum processors with a single approach.

quant-ph↗

arXiv2023

Proposal for Observing Yang-Lee Criticality in Rydberg Atomic Arrays

Yang-Lee edge singularities (YLES) are the edges of the partition function zeros of an interacting spin model in the space of complex control parameters. They play an important role in understanding non-Hermitian phase transitions in many-body physics, as well as characterizing the corresponding nonunitary criticality. Even though such partition function zeroes have been measured in dynamical experiments where time acts as the imaginary control field, experimentally demonstrating such YLES criticality with a physical imaginary field has remained elusive due to the difficulty of physically realizing non-Hermitian many-body models. We provide a protocol for observing the YLES by detecting kinked dynamical magnetization responses due to broken PT symmetry, thus enabling the physical probing of nonunitary phase transitions in nonequilibrium settings. In particular, scaling analyses based on our nonunitary time evolution circuit with matrix product states accurately recover the exponents uniquely associated with the corresponding nonunitary CFT. We provide an explicit proposal for observing YLES criticality in Floquet quenched Rydberg atomic arrays with laser-induced loss, which paves the way towards a universal platform for simulating non-Hermitian many-body dynamical phenomena.

quant-ph↗

arXiv2022

Parallel assembly of arbitrary defect-free atom arrays with a multi-tweezer algorithm

Defect-free atom arrays are an important precursor for quantum information processing and quantum simulation. Yet, large-scale defect-free atom arrays can be challenging to realize, due to the losses encountered when rearranging stochastically loaded atoms to achieve a desired target array. Here, we demonstrate a novel parallel rearrangement algorithm that uses multiple mobile tweezers to independently sort and compress atom arrays in a way that naturally avoids atom collisions. With a high degree of parallelism, our algorithm offers a reduced move complexity compared to both single-tweezer algorithms and existing multi-tweezer algorithms. We further determine the optimal degree of parallelism to be a balance between an algorithmic speedup and multi-tweezer inhomogeneity effects. The defect-free probability for a 225-atom array is demonstrated to be as high as 33(1)% in a room temperature setup after multiple cycles of rearrangement. The algorithm presented here can be implemented for any target array geometry with an underlying periodic structure.

physics.atom-ph↗

arXiv2022

2022 Roadmap for Materials for Quantum Technologies

Quantum technologies are poised to move the foundational principles of quantum physics to the forefront of applications. This roadmap identifies some of the key challenges and provides insights on materials innovations underlying a range of exciting quantum technology frontiers. Over the past decades, hardware platforms enabling different quantum technologies have reached varying levels of maturity. This has allowed for first proof-of-principle demonstrations of quantum supremacy, for example quantum computers surpassing their classical counterparts, quantum communication with reliable security guaranteed by laws of quantum mechanics, and quantum sensors uniting the advantages of high sensitivity, high spatial resolution, and small footprints. In all cases, however, advancing these technologies to the next level of applications in relevant environments requires further development and innovations in the underlying materials. From a wealth of hardware platforms, we select representative and promising material systems in currently investigated quantum technologies. These include both the inherent quantum bit systems as well as materials playing supportive or enabling roles, and cover trapped ions, neutral atom arrays, rare earth ion systems, donors in silicon, color centers and defects in wide-band gap materials, two-dimensional materials and superconducting materials for single-photon detectors. Advancing these materials frontiers will require innovations from a diverse community of scientific expertise, and hence this roadmap will be of interest to a broad spectrum of disciplines.

quant-ph↗

arXiv2021

D1 magic wavelength tweezers for scaling atom arrays

D1 magic wavelengths have been predicted for the alkali atoms but are not yet observed to date. We experimentally confirm a D1 magic wavelength that is predicted to lie at 615.87 nm for $^{23}$Na, which we then use to trap and image individual atoms with 80.0(6)% efficiency and without having to modulate the trapping and imaging light intensities. We further demonstrate that the mean loading efficiency remains as high as 74.2(7)% for a 1D array of eight atoms. Leveraging on the absence of trap intensity modulation and lower trap depths afforded by the D1 light, we achieve an order-of-magnitude reduction on the tweezer laser power requirements and a corresponding increase in the scalability of atom arrays. The methods reported here are applicable to all the alkalis, including those that are attractive candidates for dipolar molecule assembly, Rydberg dressing, or are fermionic in nature.

physics.atom-ph↗

arXiv2020

A universal graph description for one-dimensional exchange models

We demonstrate that a large class of one-dimensional quantum and classical exchange models can be described by the same type of graphs, namely Cayley graphs of the permutation group. Their well-studied spectral properties allow us to derive crucial information about those models of fundamental importance in both classical and quantum physics, and to completely characterize their algebraic structure. Notably, we prove that the spectral gap can be obtained in polynomial computational time, which has strong implications in the context of adiabatic quantum computing with quantum spin-chains. This quantity also characterizes the rate to stationarity of some important classical random processes such as interchange and exclusion processes. Reciprocally, we use results derived from the celebrated Bethe ansatz to obtain original mathematical results about these graphs in the unweighted case. We also discuss extensions of this unifying framework to other systems, such as asymmetric exclusion processes -- a paradigmatic model in non-equilibrium physics, or the more exotic non-Hermitian quantum systems.

cond-mat.stat-mech↗

arXiv2020

Graph-theory treatment of one-dimensional strongly repulsive fermions

One-dimensional atomic mixtures of fermions can effectively realize spin chains and thus constitute a clean and controllable platform to study quantum magnetism. Such strongly correlated quantum systems are also of sustained interest to quantum simulation and quantum computation due to their computational complexity. In this article, we exploit spectral graph theory to completely characterize the symmetry properties of one-dimensional fermionic mixtures in the strong interaction limit. We also develop a powerful method to obtain the so-called Tan contacts associated with certain symmetry classes. In particular, compared to brute force diagonalization that is already virtually impossible for a moderate number of fermions, our analysis enables us to make unprecedented efficient predictions about the energy gap of complex spin mixtures. Our theoretical results are not only of direct experimental interest, but also provide important guidance for the design of adiabatic control protocols in strongly correlated fermion mixtures.

quant-ph↗

arXiv2020

Resonant dipolar collisions of ultracold molecules induced by microwave dressing

We demonstrate microwave dressing on ultracold, fermionic ${}^{23}$Na${}^{40}$K ground-state molecules and observe resonant dipolar collisions with cross sections exceeding three times the $s$-wave unitarity limit. The origin of these collisions is the resonant alignment of the approaching molecules' dipoles along the intermolecular axis, which leads to strong attraction. We explain our observations with a conceptually simple two-state picture based on the Condon approximation. Furthermore, we perform coupled-channels calculations that agree well with the experimentally observed collision rates. While collisions are observed here as laser-induced loss, microwave dressing on chemically stable molecules trapped in box potentials may enable the creation of strongly interacting dipolar gases of molecules.

cond-mat.quant-gas↗

arXiv2016

Second-Scale Nuclear Spin Coherence Time of Trapped Ultracold $^{23}$Na$^{40}$K Molecules

Coherence, the stability of the relative phase between quantum states, lies at the heart of quantum mechanics. Applications such as precision measurement, interferometry, and quantum computation are enabled by physical systems that have quantum states with robust coherence. With the creation of molecular ensembles at sub-$μ$K temperatures, diatomic molecules have become a novel system under full quantum control. Here, we report on the observation of stable coherence between a pair of nuclear spin states of ultracold fermionic NaK molecules in the singlet rovibrational ground state. Employing microwave fields, we perform Ramsey spectroscopy and observe coherence times on the scale of one second. This work opens the door for the exploration of single molecules as a versatile quantum memory. Switchable long-range interactions between dipolar molecules can further enable two-qubit gates, allowing quantum storage and processing in the same physical system. Within the observed coherence time, $10^4$ one- and two-qubit gate operations will be feasible.

cond-mat.quant-gas↗

arXiv2016

Coherent Microwave Control of Ultracold $^{23}$Na$^{40}$K Molecules

We demonstrate coherent microwave control of rotational and hyperfine states of trapped, ultracold, and chemically stable $^{23}$Na$^{40}$K molecules. Starting with all molecules in the absolute rovibrational and hyperfine ground state, we study rotational transitions in combined magnetic and electric fields and explain the rich hyperfine structure. Following the transfer of the entire molecular ensemble into a single hyperfine level of the first rotationally excited state, $J{=}1$, we observe collisional lifetimes of more than $3\, \rm s$, comparable to those in the rovibrational ground state, $J{=}0$. Long-lived ensembles and full quantum state control are prerequisites for the use of ultracold molecules in quantum simulation, precision measurements and quantum information processing.

cond-mat.quant-gas↗

arXiv2015

A quantum parametric oscillator with trapped ions

A system of harmonic oscillators coupled via nonlinear interaction is a fundamental model in many branches of physics, from biophysics to electronics and condensed matter physics. In quantum optics, weak nonlinear interaction between light modes has enabled, for example, the preparation of squeezed states of light and generation of entangled photon pairs. While strong nonlinear interaction between the modes has been realized in circuit QED systems, achieving significant interaction strength on the level of single quanta in other physical systems remains a challenge. Here we experimentally demonstrate such interaction that is equivalent to photon up- and down-conversion using normal modes of motion in a system of two Yb ions. The nonlinearity is induced by the intrinsic anharmonicity of the Coulomb interaction between the ions and can be used to simulate fully quantum operation of a degenerate optical parametric oscillator. We exploit this interaction to directly measure the parity and Wigner functions of ion motional states. The nonlinear coupling, combined with near perfect control of internal and motional states of trapped ions, can be applied to quantum computing, quantum thermodynamics, and even shed some light on the quantum information aspects of Hawking radiation.

quant-ph↗

arXiv2014

Zeeman-Splitting-Assisted Quantum Logic Spectroscopy of Trapped Ions

We present a quantum logic scheme to detect atomic and molecular ions in different states of angular momentum based on their magnetic $g$-factors. The state-dependent magnetic $g$-factors mean that electronic, rotational or hyperfine states may be distinguished by their Zeeman splittings in a given magnetic field. Driving motional sidebands of a chosen Zeeman splitting enables reading out the corresponding state of angular momentum with an auxillary logic ion. As a proof-of-principle demonstration, we show that we can detect the ground electronic state of a ${^{174}}$Yb$^+$ ion using ${^{171}}$Yb$^+$ as the logic ion. Further, we can distinguish between the ${^{174}}$Yb$^+$ ion being in its ground electronic state versus the metastable ${^{2}}D_{3/2}$ state. We discuss the suitability of this scheme for the detection of rotational states in molecular ions.

physics.atom-ph↗

arXiv2014

Microwave control of trapped-ion motion assisted by a running optical lattice

We experimentally demonstrate microwave control of the motional state of a trapped ion placed in a state-dependent potential generated by a running optical lattice. Both the optical lattice depth and the running lattice frequency provide tunability of the spin-motion coupling strength. The spin-motional coupling is exploited to demonstrate sideband cooling of a Yb171 ion to the ground state of motion.

quant-ph↗

arXiv2014

State-specific detection of trapped HfF$^+$ by photodissociation

We use (1+1$'$) resonance-enhanced multiphoton photodissociation (REMPD) to detect the population in individual rovibronic states of trapped HfF$^+$ with a single-shot absolute efficiency of 18%, which is over 200 times better than that obtained with fluorescence detection. The first photon excites a specific rotational level to an intermediate vibronic band at 35,000-36,500 cm$^{-1}$, and the second photon, at 37,594 cm$^{-1}$ (266 nm), dissociates HfF$^+$ into Hf$^+$ and F. Mass-resolved time-of-flight ion detection then yields the number of state-selectively dissociated ions. Using this method, we observe rotational-state heating of trapped HfF$^+$ ions from collisions with neutral Ar atoms. Furthermore, we measure the lifetime of the $^3Δ_1$ $v=0,\, J=1$ state to be 2.1(2) s. This state will be used for a search for a permanent electric dipole moment of the electron.

physics.atom-ph↗

arXiv2013

Precision Spectroscopy of Polarized Molecules in an Ion Trap

Polar molecules are desirable systems for quantum simulations and cold chemistry. Molecular ions are easily trapped, but a bias electric field applied to polarize them tends to accelerate them out of the trap. We present a general solution to this issue by rotating the bias field slowly enough for the molecular polarization axis to follow but rapidly enough for the ions to stay trapped. We demonstrate Ramsey spectroscopy between Stark-Zeeman sublevels in 180Hf19F+ with a coherence time of 100 ms. Frequency shifts arising from well-controlled topological (Berry) phases are used to determine magnetic g-factors. The rotating-bias-field technique may enable using trapped polar molecules for precision measurement and quantum information science, including the search for an electron electric dipole moment.

physics.atom-ph↗

arXiv2012

REMPI Spectroscopy of HfF

The spectrum of electronic states at 30000--33000 cm$^{-1}$ in hafnium fluoride has been studied using (1+1) resonance-enhanced multi-photon ionization (REMPI) and (1+1$'$) REMPI. Six $Ω' = 3/2$ and ten $Π_{1/2}$ vibronic bands have been characterized. We report the molecular constants for these bands and estimate the electronic energies of the excited states using a correction derived from the observed isotope shifts. When either of two closely spaced $Π_{1/2}$ electronic states is used as an intermediate state to access autoionizing Rydberg levels, qualitatively distinct autoionization spectra are observed. The intermediate state-specificity of the autoionization spectra bodes well for the possibility of using a selected $Π_{1/2}$ state as an intermediate state to create ionic HfF$^+$ in various selected quantum states, an important requirement for our electron electric dipole moment (eEDM) search in HfF$^+$.

physics.chem-ph↗