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Hubertus Luetkens

Publications and source records attributed to Hubertus Luetkens.

88 records · Page 5Linked to original sources

Direct evidence for the emergence of a pressure induced nodal superconducting gap in the iron-based superconductor Ba_0.65Rb_0.35Fe_2As_2

Identifying the superconducting (SC) gap structure of the iron-based high-temperature superconductors (Fe-HTS's) remains a key issue for the understanding of superconductivity in these materials. In contrast to other unconventional superconductors, in the Fe-HTS's both $d$-wave and extended s-wave pairing symmetries are close in energy, with the latter believed to be generally favored over the former. Probing the proximity between these very different SC states and identifying experimental parameters that can tune them, are of central interest. Here we report high-pressure muon spin rotation experiments on the temperature-dependent magnetic penetration depth (lambda) in the optimally doped Fe-HTS Ba_0.65Rb_0.35Fe_2As_2. At ambient pressure this material is known to be a nodeless s-wave superconductor. Upon pressure a strong decrease of (lambda) is observed, while the SC transition temperature remains nearly constant. More importantly, the low-temperature behavior of (1/lambda^{2}) changes from exponential saturation at zero pressure to a power-law with increasing pressure, providing unambiguous evidence that hydrostatic pressure promotes nodal SC gaps. Comparison to microscopic models favors a d-wave over a nodal s^{+-}-wave pairing as the origin of the nodes. Our results provide a new route of understanding the complex topology of the SC gap in Fe-HTS's.

cond-mat.supr-con↗

Spectroscopic study of the magnetic ground state of Nb$_{1-y}$Fe$_{2+y}$

We have investigated single crystals and polycrystals from the series Nb$_{1-y}$Fe$_{2+y}$, $-0.004 \leq y \leq 0.018$ by electron spin resonance, muon spin relaxation and Mössbauer spectroscopy. Our data establish that at lowest temperatures all samples exhibit bulk magnetic order. Slight Fe-excess induces low-moment ferromagnetism, consistent with bulk magnetometry ($\simeq 0.06 ~μ_B/{\rm Fe}$), Nb--rich and stoichiometric NbFe$_2$ display spin density wave order with small magnetic moment amplitudes of the order $\sim 0.001 - 0.01 ~μ_B/{\rm Fe}$. This provides microscopic evidence for a modulated magnetic state on the border of ferromagnetism in NbFe$_2$.

cond-mat.str-el↗

Short-range correlations in the magnetic ground state of Na4Ir3O8

The magnetic ground state of the hyper-kagome lattice in Na4Ir3O8 is explored via combined bulk magnetization, muon spin relaxation, and neutron scattering measurements. A short-range, frozen, state comprised of quasi-static moments develops below a characteristic temperature of T_F=6 K, revealing an inhomogeneous distribution of spins occupying the entirety of the sample volume. Quasi-static, short-range, spin correlations persist until at least 20 mK and differ substantially from the nominally dynamic response of a quantum spin liquid. Our data demonstrate that an inhomogeneous magnetic ground state arises in Na4Ir3O8 driven either by disorder inherent to the creation of the hyper-kagome lattice itself or stabilized via quantum fluctuations.

cond-mat.str-el↗

Coexistence of 3d-ferromagnetism and superconductivity in [(Li(1-x)Fex)OH](Fe(1-y)Liy)Se

Superconducting [(Li(1-x)Fex)OH](Fe(1-y)Liy)Se (x ~ 0.2, y ~ 0.08) was synthesized by hydrothermal methods and structurally characterized by single crystal X-ray diffraction. The crystal structure contains anti-PbO type (Fe(1-y)Liy)Se layers separated by layers of (Li(1-x)Fex)OH. Electrical resistivity and magnetic susceptibility measurements reveal superconductivity at 43 K. An anomaly in the diamagnetic shielding indicates ferromagnetic ordering near 10 K while superconductivity is retained. The ferromagnetism emerges from the iron atoms in the (Li(1-x)Fex)OH layer. Isothermal magnetization measurements confirm the superposition of ferromagnetic with superconducting hysteresis. The internal ferromagnetic field is larger than the lower, but smaller than the upper critical field of the superconductor, which gives evidence for a spontaneous vortex phase where both orders coexist. 57Fe-Mössbauer spectra, 7Li-NMR spectra, and muSR experiments consistently support this rare situation, especially in a bulk material where magnetism emerges from a 3d-element.

cond-mat.supr-con↗

Interplay of magnetism and superconductivity in EuFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$ single crystals probed by muon spin rotation and ${}^{57}$Fe Mössbauer spectroscopy

We present our results of a local probe study on EuFe$_{2}$(As$_{1-x}$P$_{x}$)$_{2}$ single crystals with $x$=0.13, 0.19 and 0.28 by means of muon spin rotation and ${}^{57}$Fe Mössbauer spectroscopy. We focus our discussion on the sample with $x$=0.19 viz. at the optimal substitution level, where bulk superconductivity ($T_{\text{SC}}=28$ K) sets in above static europium order ($T^{\text{Eu}}=20$K) but well below the onset of the iron antiferromagnetic (AFM) transition ($\sim$100 K). We find enhanced spin dynamics in the Fe sublattice closely above $T_{\text{SC}}$ and propose that these are related to enhanced Eu fluctuations due to the evident coupling of both sublattices observed in our experiments.

cond-mat.supr-con↗

Intrinsic paramagnetism and aggregation of manganese dopants in SrTiO$_3$

Using local-probe magnetic-characterization techniques of muon spin relaxation ($μ$SR) and electron spin resonance (ESR) we have investigated the Mn-induced magnetism of the wide-bandgap perovskite SrTiO$_3$. Our results clearly demonstrate that this diluted magnetic oxide (DMO) remains paramagnetic down to low temperatures for both doping cases, i.e., when Mn substitutes for Sr or Ti. In addition, both experimental techniques have unveiled that the distribution of individual Mn$^{2+}$ and Mn$^{4+}$ ions is nonrandom, as these ions partially aggregate into nanosized clusters.

cond-mat.str-el↗

Microscopic Coexistence of Magnetism and Superconductivity in charge compensated Ba1-xKx(Fe1-yCoy)2As2

We present a detailed investigation of the electronic phase diagram of effectively charge compensated Ba1-xKx(Fe1-yCoy)2As2 with x/2 = y. Our experimental study by means of x-ray diffraction, Mössbauer spectroscopy, muon spin relaxation and ac susceptibility measurements on polycrystalline samples is complemented by density functional electronic structure calculations. For low substitution levels of x/2 = y \< 0.13, the system displays an orthorhombically distorted and antiferromagnetically ordered ground state. The low temperature structural and magnetic order parameters are successively reduced with increasing substitution level. We observe a linear relationship between the structural and the magnetic order parameter as a function of temperature and substitution level for x/2 = y \< 0.13. At intermediate substitution levels in the range between 0.13 and 0.19, we find superconductivity with a maximum Tc of 15 K coexisting with static magnetic order on a microscopic length scale. For higher substitution levels x/2 = y \> 0.25 a tetragonal non-magnetic ground state is observed. Our DFT calculations yield a signifcant reduction of the Fe 3d density of states at the Fermi energy and a strong suppression of the ordered magnetic moment in excellent agreement with experimental results. The appearance of superconductivity within the antiferromagnetic state can by explained by the introduction of disorder due to non-magnetic impurities to a system with a constant charge carrier density. Our experimental study by means of x-ray diffraction, Mössbauer spectroscopy, muon spin relaxation and ac susceptibility measurements on polycrystalline samples is complemented by density functional electronic structure calculations.

cond-mat.supr-con↗

Ground state of bond-disordered quasi-one-dimensional spin system (CH3)2CHNH3Cu(ClxBr1-x)3 with x = 0, 0.25 and 0.3

The ground state of the quasi-one-dimensional system with bond-disorder (CH3)2CHNH3Cu(ClxBr1-x)3 with x = 0, 0.25 and 0.3 has been investigated by muSR. The Fourier spectrum of electron spin fluctuation in x =0.25 and 0.3 obtained by LF-muSR technique shows that there exists a soft-mode toward a possible phase transition to an exotic phase such as Bose-glass. In gapped system with x = 0, the Fourier spectrum is totally different from the other two, indicating the existence of the quantum critical point at a finite x between 0 and 0.25.

cond-mat.stat-mech↗

Short range magnetic order and effective suppression of superconductivity by manganese-doping in LaFe1-xMnxAsO1-yFy

We present a study of the structural and physical properties of directly hole doped LaFe1-xMnxAsO (x = 0.0-0.2) and the influence of charge compensation / electron-doping by additional F doping in LaFe0.9Mn0.1AsO1-yFy (y = 0.1-0.5). High quality polycrystalline samples were prepared using a solid state metathesis reaction. The unit cell increases upon Mn doping, but decreases again when additional F is inserted. The semiconducting character of LaFe1-xMnxAsO decreases with additional F doping. Muon spin relaxation (muSR) measurements reveal short range magnetic order in LaFe1-xMnxAsO and a suppression of magnetism by additional electron-doping with fluoride in LaFe0.9Mn0.1AsO1-yFy. Superconductivity remains absent even though the electronic preconditions are fulfilled in electron-doped LaFe0.9Mn0.1AsO1-yFy at x > 0.1, which is suggestive of effective pair breaking by Mn in this system.

cond-mat.supr-con↗

Strong Competition of Superconducting and Magnetic Order Parameters in Ba1-xNaxFe2As2

We study the interplay of magnetic and superconducting order in single crystalline hole doped Ba1-xNaxFe2As2 using muon spin relaxation. We find microscopic coexistence of magnetic order and superconductivity. In a strongly underdoped specimen the two forms of order coexist without any measurable reduction of the ordered magnetic moment by superconductivity, while in a nearly optimally doped sample the ordered magnetic moment is strongly suppressed below the superconducting transition temperature. This coupling can be well described within the framework of an effective two-band model incorporating inter- and intra-band interactions. In optimally doped Ba1-xNaxFe2As2 we observe no traces of static or dynamic magnetism and the temperature dependence of the superfluid density is consistent with two s-wave gaps without nodes.

cond-mat.supr-con↗

Structural and electronic phase diagrams of CeFeAsO1-xFx and SmFeAsO1-xFx

We have studied the structural and electronic phase diagrams of CeFeAsO1-xFx and SmFeAsO1-xFx by a detailed analysis of muon spin relaxation experiments, synchrotron X-ray diffraction, Mössbauer spectroscopy, electrical resistivity, specific heat, and magnetic susceptibility measurements (Full abstract in the main document).

cond-mat.supr-con↗

Effect of external pressure on the magnetic properties of LnFeAsO (Ln = La, Ce, Pr, Sm)

We investigate the effect of external pressure on magnetic order in undoped LnFeAsO (Ln = La, Ce, Pr, La) by using muon-spin relaxation measurements and ab-initio calculations. Both magnetic transition temperature $T_m$ and Fe magnetic moment decrease with external pressure. The effect is observed to be lanthanide dependent with the strongest response for Ln = La and the weakest for Ln = Sm. The trend is qualitatively in agreement with our DFT calculations. The same calculations allow us to assign a value of 0.68(2) $μ_B$ to the Fe moment, obtained from an accurate determination of the muon sites. Our data further show that the magnetic lanthanide order transitions do not follow the simple trend of Fe, possibly as a consequence of the different $f$-electron overlap.

cond-mat.supr-con↗

Magnetic order and transitions in the spin-web compound Cu3TeO6

The spin-web compound Cu3TeO6, belongs to an intriguing group of materials where magnetism is governed by 3d9 copper Cu2+ ions. This compound has been sparsely experimentally studied and we here present the first investigation of its local magnetic properties using muon-spin relaxation/rotation (μ+SR). Our results show a clear long-range 3D magnetic order below TN as indicated by clear zero-field (ZF) muon-precessions. At TN = 61.7 K a very sharp transition is observed in the weak transverse-field (wTF) as well as ZF data. Contrary to suggestions by susceptibility measurements and inelastic neutron scattering, we find no evidence for either static or dynamic (on the time-scale of μ+SR) spin-correlations above TN.

cond-mat.str-el↗

Negative magnetization of Li2Ni2Mo3O12 having a spin system composed of distorted honeycomb lattices and linear chains

We study themagnetism of a spin-1 substance Li2Ni2Mo3O12. The spin system consists of distorted honeycomb lattices and linear chains of Ni2+ spins. Li+ ions enter about 25% and 50% of the honeycomb and chain Ni sites, respectively, creating disorder in both spin subsystems. A magnetic phase transition occurs at Tc = 8.0 K in the zero magnetic field. In low magnetic fields, the magnetization increases rapidly below Tc, decreases below 7 K, and finally becomes negative at low temperatures. We determine the magnetic structure using neutron powder diffraction results. The honeycomb lattices and linear chains show antiferromagnetic and ferromagnetic long-range order, respectively. We investigate static and dynamic magnetic properties using the local probe technique of muon spin relaxation. We discuss the origin of the negative magnetization.

cond-mat.str-el↗

Microscopic co-existence of superconductivity and magnetism in Ba1-xKxFe2As2

It is widely believed that, in contrast to its electron doped counterparts, the hole doped compound Ba1-xKxFe2As2 exhibits a mesoscopic phase separation of magnetism and superconductivity in the underdoped region of the phase diagram. Here, we report a combined high-resolution x-ray powder diffraction and volume sensitive muon spin rotation study of underdoped Ba1-xKxFe2As2 (0 \leq x \leq 0.25) showing that this paradigm is wrong. Instead we find a microscopic coexistence of the two forms of order. A competition of magnetism and superconductivity is evident from a significant reduction of the magnetic moment and a concomitant decrease of the magneto-elastically coupled orthorhombic lattice distortion below the superconducting phase transition.

cond-mat.supr-con↗

Muon-spin rotation studies of SmFeAsO_0.85 and NdFeAsO_0.85 superconductors

Measurements of the in-plane magnetic field penetration depth λ_{ab} in Fe-based superconductors with the nominal composition SmFeAsO_0.85 (T_c\simeq52K) and NdFeAsO_0.85 (T_c\simeq51K) were carried out by means of muon-spin-rotation. The absolute values of λ_{ab} at T=0 were found to be 189(5)nm and 195(5)nm for Sm and Nd substituted samples, respectively. The analysis of the magnetic penetration depth data within the Uemura classification scheme, which considers the correlation between the superconducting transition temperature T_c and the effective Fermi temperature T_F, reveal that both families of Fe-based superconductors (with and without fluorine) falls to the same class of unconventional superconductors.

cond-mat.supr-con↗