arXiv subjects

Hyun-Woo Lee

Publications and source records attributed to Hyun-Woo Lee.

At least 19 recordsLinked to original sources

arXiv2026

Aharonov-Casher-induced electric quadrupole of charge-neutral particles

For charged particles, their orbital angular momentum (OAM) in solid have a direct magnetic manifestation as an orbital magnetization. For charge-neutral particles, however, the physical manifestation of the OAM in solid remains unclear. Here, we show that a charge-neutral particle carrying a magnetic moment couples to electric-field gradient through the Aharonov-Casher (AC) effect, thereby exhibiting the electric quadrupole in crystalline solids. This AC-induced electric quadrupole (AC-EQ) contains the scalar, toroidal dipole, and reduced quadrupole components, which are conjugate to the divergence, circulation, and shear of the electric field, respectively. As representative examples, we calculate the AC-EQ of magnons in two magnetic systems. In ferromagnetic pyrochlore, Dzyaloshinskii-Moriya interaction (DMI) induces a sizable AC-EQ, whereas in helical Fe langasite the AC-EQ emerges from the helical spin configuration even in the absence of DMI.

cond-mat.mes-hall↗

arXiv2026

Intra-atomic magnetic octupoles and their coupling to cluster magnetic octupoles in Chiral antiferromagnets Mn$_3$Sn

We demonstrate that Mn$_3$Sn hosts finite intra-atomic magnetic octupoles (AMOs) $\mathbf{o}$ in addition to the well-established cluster magnetic octupole (CMO) $\mathbf{O}$. In contrast to the cluster-scale CMO, the AMO is a site-localized magnetic multipole associated with the anisotropic intra-atomic spin density. Symmetry analysis shows that the CMO and AMO transform in the same representation, allowing a bilinear interaction of the form $-g\,\mathbf{O}\cdot\mathbf{o}$. Using first-principles calculations, we confirm the presence of finite AMO densities and show that the AMO transforms concomitantly with the CMO under rotations of the noncollinear magnetic structure, providing microscopic evidence for the coupling between them. We further show that the magnetic band splitting can be represented by projected AMO operators, with manifold-dependent effective octupolar exchange coefficients in realistic Mn$_3$Sn. The presence of AMOs has three important implications. First, we show that the nonrelativistic spin splitting of Mn$_3$Sn can be described in terms of projected AMO operators, with manifold-dependent effective octupolar exchange coefficients, establishing the AMO as a microscopic operator underlying the spin splitting. Second, the AMO reveals a close connection between Mn$_3$Sn and $d$-wave altermagnets from the magnetic-octupole perspective. Third, the $\mathbf{O}\cdot\mathbf{o}$ coupling suggests a new route to manipulate the CMO using AMO currents, opening a direction for controlling the multipolar order in Mn$_3$Sn.

cond-mat.mtrl-sci↗

arXiv2026

Modern Approach to Orbital Hall Effect Based on Wannier Picture of Solids

The orbital Hall effect (OHE) and its key figure of merit, the orbital Hall conductivity (OHC), are central to the emerging field of orbitronics. The OHC is conventionally computed via Kubo linear response theory, where the orbital angular momentum (OAM) operator is approximated through atom-centered projections that retain only local contributions, discarding physically important itinerant components. Here, we present a rigorous framework for the OAM operator grounded in the modern theory of orbital magnetization, formulated in a Wannier function basis. Critically, this naturally introduces a hierarchy of non-local contributions to the OAM operator. In turn, this gives rise to an additional non-Kubo contribution to the OHC of purely geometric origin, absent in all atom-centered treatments. First-principles calculations across a diverse set of materials demonstrate that this term can constitute a significant fraction of the total OHC, with its omission leading to qualitatively incorrect predictions. Our framework provides a unified and numerically tractable approach to orbital transport and improves our understanding of the OAM in solids, allowing for a more precise estimation of various orbital effects in complex materials.

cond-mat.mes-hall↗

arXiv2026

Interfacial chirality-induced magnetic-field-free switching with high energy efficiency in all-vdW heterostructures

Chirality, a central concept across many scientific disciplines, continues to inspire the discovery of novel physical phenomena. In condensed matter physics, structural chirality - defined by the absence of mirror plane symmetries - has primarily been explored in bulk materials. However, new chiral phenomena can emerge uniquely at the interface, distinct from their bulk counterparts, when a chiral material forms a heterostructure. Here, we demonstrate that all van-der-Waals (vdW) heterostructure composed of the chiral Co1/3TaS2 and the achiral vdW ferromagnet Fe3GeTe2 exhibits two distinct and unconventional spin-orbit torques originating from the interfacial chirality. These torques enable magnetic-field-free switching of perpendicular magnetization with ultralow current density ~ 10^6 A/cm^2 and minimal power dissipation < 10^15 W/m^3. Moreover, by replacing Fe3GeTe2 with a similar vdW ferromagnet, Fe3GaTe2, but of higher Curie temperature, we achieved the magnetic-field-free switching at room temperature in the Fe3GaTe2/Co1/3TaS2 vdW heterostructure. Our findings establish interfacial chirality as a powerful new handle for spintronic control, opening a new pathway to explore chirality-induced phenomena beyond the bulk symmetry constraints - and paving the way toward highly efficient, low-power spintronic devices based on all-vdW heterostructures.

cond-mat.mtrl-sci↗

arXiv2026

Intrinsic orbital Hall effect in a nonuniform electric field

Geometric analysis of electronic Bloch states offers a universal framework for understanding electronic properties, yet its role in the transport of orbital angular momentum remains unexplored. In this work, we establish an analytic connection between orbital angular momentum transport and the geometric properties of Bloch wave functions in electronic systems. Focusing on the intrinsic orbital Hall effect in the dc limit under a spatially nonuniform electric field, we show that its conductivity can be expressed in terms of universal geometric quantities, such as the orbital Berry curvature and quantum metric. This formulation provides a term-by-term correspondence with the geometric description of intrinsic charge Hall transport established in previous studies. Using a tight-binding model, we further illustrate that the higher-order orbital Hall response can exhibit enhanced sensitivity to the orientation of an anisotropic sample. Our work deepens the understanding of diverse intrinsic transverse transport phenomena and the role of quantum geometry in electronic systems.

cond-mat.mes-hall↗

arXiv2026

Comparing the orbital angular momentum and magnetic moment of magnons in the Kagome antiferromagnet with negative spin chirality

The orbital dynamics of magnons have recently drawn interest due to their potential roles in thermal and orbital transport phenomena in magnetic insulators. In this study, we investigate the orbital magnetic moment (OMM) and orbital angular momentum (OAM) of magnons in a Kagome antiferromagnet with negative vector chirality, focusing on the distinction between thermodynamic and wave-packet-based definitions. We compute the Berry curvature, the OMM, and the OAM in momentum space under an external magnetic field. Our results reveal a quantitative difference between the OMM and OAM, yet their associated Nernst coefficients exhibit similar temperature and field dependence in transport. Our results provide a quantitative comparison between the thermodynamic and wave-packet formulations of magnon orbital dynamics.

cond-mat.mes-hall↗

arXiv2026

Anatomy of the modern theory of orbital magnetism from first-principles: term-by-term analysis in the gauge-covariant formalism

We present an in-depth analysis of the orbital magnetism by means of the so-called modern theory based on the Berry phase across distinct classes of materials-d transition metals, sp metals, and transition metal dichalcogenides-highlighting the microscopic nature of band structure characteristics. We adopt a gauge-covariant formulation of the modern theory proposed in [Lopez et al. Phys. Rev. B 85, 014435 (2012)], which enables the calculation of orbital magnetism in a controlled manner in any chosen gauge of Wannier functions and gives the total contribution as a gauge-invariant measurable. This captures consistently the contributions due to the anomalous position, velocity, and orbital angular momentum of Wannier basis, as well as the contributions due to Hamiltonian such that their sum is gauge-invariant. For d transition metals, we find that the atom-centered approximation captures the majority of the total contribution given by modern theory, which we attribute to localized nature of d electrons. However, 5d metals tend to exhibit larger deviation between the two methods than 3d metals do, as 5d electrons are more delocalized than 3d electrons. On the other hand, sp metals exhibit a strong deviation between the two methods, where large kinetic energy of sp electrons is important. Finally, in 1H-MoS2, we find that the valley orbital moment far exceeds the atomic limit of d electrons due to coherent hybridization between valence and conduction bands in direct band gaps. Our work elucidates the interplay of the chemical nature of electronic orbitals and the effect of band structures in a consistent manner and highlights the role of Berry phase in orbital magnetism. The results suggest a promising direction of orbitronics beyond controlling atomic orbitals, in which the orbital magnetism can be greatly enhanced by exploiting Berry phase.

cond-mat.mes-hall↗

arXiv2026

Deterministic Néel vector switching of altermagnets via magnetic octupole torque

Altermagnets have recently emerged as promising materials for next-generation spintronic devices. For their device applications, realizing a single-domain configuration is essential but remains challenging. We theoretically consider injecting magnetic multipoles into altermagnets, which can be achieved by applying an in-plane current to an altermagnet/normal metal bilayer. We demonstrate for $d$-wave altermagnets that the torque generated by the magnetic octupole injection can achieve magnetic-field-free deterministic switching of the altermagnets' Néel vector and transform their multidomain configurations into a single domain. This method allows the switching in diverse altermagnets, thereby facilitating their device applications and fundamental studies. This work also exemplifies the usefulness of magnetic multipole currents.

cond-mat.mtrl-sci↗

arXiv2026

Enhanced transverse electron transport via disordered composite formation

Transverse electron transport in magnetic materials - manifested in effects such as the anomalous Hall and Nernst effects - holds promise for spintronic and thermoelectric applications. While recent advances have focused on enhancing such transport through topological single crystals via intrinsic mechanisms linked to Berry curvature, practical limitations remain due to their mechanical fragility and narrow material scope. Here, we demonstrate a distinct approach for transverse transport enhancement based on composite formation. Using both theoretical modeling and experiments, we show that disordered mixtures of two ferromagnetic materials can exhibit significantly stronger transverse electron deflection than either constituent alone. This enhancement originates from meandering electron pathways created by the disordered mixture of two materials and does not rely on long-range crystalline order. The identified requirements for this mechanism can be broadly satisfied across different material systems, offering a universal and tunable strategy to engineer large transverse responses in structurally robust platforms.

cond-mat.mtrl-sci↗

arXiv2025

Electrotoroidicity: New Paradigm for Transverse Electromagnetic Responses

The exploration of transverse electromagnetic responses in solids with broken spatial-inversion (I) and/or time-reversal (T) symmetries has unveiled numerous captivating phenomena, including the (anomalous) Hall effect, Faraday rotations, non-reciprocal directional dichroism, and off-diagonal linear magnetoelectricity, all within the framework of magnetotoroidicity. Here, we introduce a novel class of transverse electromagnetic responses originating from electrotoroidicity in ferro-rotational (FR) systems with preserved I and T symmetries, distinct from magnetotoroidicity. We discover a high-order off-diagonal magnetic susceptibility of FR domains and a reduced linear diagonal magnetic susceptibility at FR domain walls in doped ilmenite FeTiO3. The non-trivial "Hall-like" effect of the former corresponds to an anomalous transverse susceptibility in the presence of spontaneous electrotoroidal moments in FR materials. Our findings unveil an emergent type of transverse electromagnetic responses even in I and T symmetry-conserved conditions and illustrate new functionalities of abundant FR materials.

cond-mat.mtrl-sci↗

arXiv2025

Extrinsic Orbital Hall Effect and Orbital Relaxation in Mesoscopic Devices

Despite recent advances in orbitronics, the influence of disorder on the orbital Hall effect and orbital relaxation mechanisms remains poorly understood. In this work, we numerically investigate the role of disorder in orbital transport within mesoscopic devices using a real-space tight-binding model on a two-dimensional square lattice that hosts atomic orbitals capable of carrying atomic orbital angular momentum. By considering devices with varying geometries--square and rectangular--and systematically tuning disorder strength, we examine the disorder effect on orbital Hall current (OHC) generation, and orbital relaxation. Our results reveal a strong dependence of the OHC and orbital Hall angle on disorder strength. In square devices, we demonstrate that the orbital Hall response can be strongly enhanced by disorder and its dependence on the disorder strength indicates the dominance of skew-scattering mechanism in the diffusive regime. In rectangular geometries, the orbital current decays exponentially with increasing device width, from which the orbital relaxation length is extracted. These findings provide critical insights into disorder-driven orbital transport phenomena and lay the foundation for designing next-generation orbitronic devices.

cond-mat.mes-hall↗

arXiv2025

Magnetic octupole Hall effect in heavy transition metals

d-wave altermagnets have the magnetic octupole as their primary order parameter. A recent study [Han et al. arXiv 2409.14423 (2024)] demonstrated that magnetic octupole current can induce Néel vector dynamics. Therefore, identifying materials that can efficiently generate a magnetic octupole current is essential. In this paper, we investigate the magnetic octupole Hall effect in 4d and 5d transition metals. By employing atomic magnetic octupole operators, we calculate the magnetic octupole Hall conductivity using first-principles calculations. We also explore the microscopic origin of the magnetic octupole Hall effect and find that it results from the combined effect of orbital texture and spin-orbit coupling. Additionally, we analyze the ratio of spin Hall conductivity to magnetic octupole Hall conductivity across various materials and identify those that are optimal for observing magnetic octupole physics. We also discuss potential applications arising from the magnetic octupole Hall effect. Our work serves as a valuable reference for identifying materials suitable for studying magnetic octupole physics.

cond-mat.mtrl-sci↗

arXiv2025

Ranking dynamics in movies and music

Ranking systems are widely used to simplify and interpret complex data across diverse domains, from economic indicators and sports scores to online content popularity. While previous studies including the Zipf's law have focused on the static, aggregated properties of ranks, in recent years researchers have begun to uncover generic features in their temporal dynamics. In this work, we introduce and study a series of system-level indices that quantify the compositional changes in ranking lists over time, and also characterize the temporal ranking trajectories of individual items' ranking dynamics. We apply our method to analyze ranking dynamics of movies from the over-the-top services, including Netflix, as well as that of music items in Spotify charts. We find that newly released movies or music items influence most the system-level compositional changes of ranking lists; the highest ranks of items are strongly correlated with their lifetimes in the lists more than their first and last ranks. Our findings offer a novel lens to understand collective ranking dynamics and provide a basis for comparing fluctuation patterns across various ordered systems.

physics.soc-ph↗

arXiv2025

Local and Global Reciprocity in Orbital-Charge-Coupled Transport

The coupled transport of charge and orbital angular momentum (OAM) lies at the core of orbitronics. Here, we examine the reciprocal relation in orbital-charge-coupled transport in thin films, treating bulk and surface contributions on equal footing. We argue that the conventional definition of orbital current is ill-defiled, as it violates reciprocity due to the nonconservation of OAM. This issue is resolved by adopting the so-called \emph{proper} orbital current, which is directly linked to orbital accumulation. We establish the reciprocal relation for the \emph{global} (spatially integrated) response between orbital and charge currents, while showing that their \emph{local} (spatially resolved) responses can differ significantly. In particular, we find large surface contributions that may lead to nonreciprocity when currents are measured locally. These findings are supported by first-principles calculations on W(110) and Pt(111) thin films. In W(110), orbital-charge interconversion is strongly nonreciprocal at the layer level, despite exact reciprocity in the integrated response. Interestingly, spin-charge interconversion in W(110) remains nearly reciprocal even locally. In contrast, Pt(111) exhibits local nonreciprocity for both orbital-charge and spin-charge conversions, which we attribute to strong spin-orbit coupling. We propose that such local distinctions can be exploited to experimentally differentiate spin and orbital currents.

cond-mat.mes-hall↗

arXiv2025

Weak Ferromagnetism in Altermagnets from Alternating $g$-Tensor Anisotropy

Altermagnets are magnetic materials with antiferromagnetic spin ordering but exhibit ferromagnetic properties. Understanding the microscopic origin of the latter is a central problem. Ferromagnet-like properties such as the anomalous Hall effect are linked with weak ferromagnetism, whose microscopic origin in altermagnets remains unclear however. We show theoretically that the alternating $g$-tensor anisotropy in altermagnets can induce weak ferromagnetism even when the Dzyaloshinskii-Moriya interaction is forbidden. We demonstrate this mechanism to explain weak ferromagnetism for both collinear and noncollinear spin altermagnets. Our findings provide new insights into the origin of weak ferromagnetism and suggest orbital-based ways for manipulating magnetic configurations in altermagnets.

cond-mat.mtrl-sci↗

arXiv2025

Diverging entanglement of critical magnons in easy-axis antiferromagnets

We study the instability of antiferromagnets with easy-axis anisotropy under a magnetic field, uncovering single or even multiple phase transitions at the boundary between non-collinear and collinear spin orderings. Near the phase boundary, the entanglement between the sublattice magnons diverges due to the interplay among antiferromagnetic exchange interaction, anisotropy, and magnetic field. Furthermore, our study reveals that this magnetic criticality extends to a superradiant phase transition within cavity magnonics systems. The magnon-photon interaction results in diverging cavity photon numbers and squeezing in the ground state at the transition points between spin orderings. This investigation not only elucidates the criticality of multi-component squeezed magnons in antiferromagnets, but also proposes cavity photon measurements as a viable method for detecting magnetic phase transitions.

cond-mat.mes-hall↗

arXiv2025

Current-driven collective control of helical spin texture in van der Waals antiferromagnet

Electrical control of quantum magnetic states is essential in spintronic science. Initial studies on the ferromagnetic state control were extended to collinear antiferromagnets and, more recently, noncollinear antiferromagnets. However, electrical control mechanisms of such exotic magnetic states remain poorly understood. Here, we report the first experimental and theoretical example of the current control of helical antiferromagnets, arising from the competition between collinear antiferromagnetic exchange and interlayer Dzyaloshinskii-Moriya interaction in new van-der-Waals (vdW) material Ni1/3NbS2. Due to the intrinsic broken inversion symmetry, an in-plane current generates spin-orbit torque that, in turn, interacts directly with the helical antiferromagnetic order. Our theoretical analyses indicate that a weak ferromagnetic order coexists due to the Dzyaloshinskii-Moriya interaction, mediating the spin-orbit torque to collectively rotate the helical antiferromagnetic order. Our Ni1/3NbS2 nanodevice experiments produce current-dependent resistance change consistent with the theoretical prediction. This work widens our understanding of the electrical control of helical antiferromagnets and promotes vdW quantum magnets as interesting material platforms for electrical control.

cond-mat.mtrl-sci↗

arXiv2025

Nonlocal Electrical Detection of Reciprocal Orbital Edelstein Effect

Spin-Orbitronics leverages the spin and orbital degrees of freedom in solids for information processing. The orbital Edelstein effect and orbital Hall effect, where the charge current induces a nonequilibrium orbital angular momentum, offer a promising method to manipulate nanomagnets efficiently using light elements. Despite extensive research, understanding the Onsager reciprocity of orbital transport, fundamentally rooted in the second law of thermodynamics and time-reversal symmetry, remains elusive. In this study, we experimentally demonstrate the Onsager reciprocity of orbital transport in an orbital Edelstein system by utilizing nonlocal measurements. This method enables the precise identification of the chemical potential generated by orbital accumulation, avoiding the limitations associated with local measurements. Remarkably, we observe that the direct and inverse orbital-charge conversion processes produce identical electric voltages, confirming Onsager reciprocity in orbital transport. Additionally, we find that the orbital decay length, approximately 100 nm at room temperature, is independent of Cu thickness and decreases with lowering temperature, revealing a distinct contrast to spin transport behavior. Our findings provide valuable insights into both the reciprocity of the charge-orbital interconversion and the nonlocal correlation of orbital degree of freedom, laying the ground for orbitronics devices with long-range interconnections.

cond-mat.mes-hall↗