arXiv subjects

Hyun-Woo Lee

Publications and source records attributed to Hyun-Woo Lee.

At least 55 records · Page 3Linked to original sources

arXiv2022

Chiral anomaly in noncentrosymmetric systems induced by spin-orbit coupling

The chiral anomaly may be realized in condensed matter systems with pairs of Weyl points. Here we show that the chiral anomaly can be realized in diverse noncentrosymmetric systems even without Weyl point pairs when spin-orbit coupling induces nonzero Berry curvature flux through Fermi surfaces. This motivates the condensed matter chiral anomaly to be interpreted as a Fermi surface property rather than a Weyl point property. The spin-orbit-coupling-induced anomaly reproduces the well-known charge transport properties of the chiral anomaly such as the negative longitudinal magnetoresistance and the planar Hall effect in Weyl semimetals. Since it is of spin-orbit coupling origin, it also affects the spin transport and gives rise to anomaly-induced longitudinal spin currents and the magnetic spin Hall effect, which are absent in conventional Weyl semimetals.

cond-mat.mes-hall↗

arXiv2022

In-plane optical phonon modes of current-carrying graphene

In this work, we study the in-plane optical phonon modes of current-carrying single-layer graphene whose coupling to the $π$ electron gas is strong. Such modes are expected to undergo a frequency shift compared to the non-current-carrying state due to the non-equilibrium occupation of the Dirac cone electronic eigen-states with the flowing $π$ electron gas. Large electron-phonon coupling (EPC) can be identified by an abrupt change in the slope of the phonon mode dispersion known as the Kohn anomaly, which mainly occurs for (i) the in-plane longitudinal/transverse optical (LO/TO) modes at the Brillouin zone (BZ) center ($Γ$ point), and (ii) the TO modes at the BZ corners ($K$ points). We show that the breaking of the rotational symmetry by the DC current results in different frequency shifts to the $Γ$-TO and $Γ$-LO modes. More specifically, the DC current breaks the TO-LO mode degeneracy at the $Γ$ point which ideally would be manifested as the splitting of the Raman G peak.

cond-mat.mes-hall↗

arXiv2022

Long-Range Orbital Magnetoelectric Torque in Ferromagnets

While it is often assumed that the orbital response is suppressed and short-ranged due to strong crystal field potential and orbital quenching, we show that the orbital magnetoelectric response can be remarkably long-ranged in ferromagnets. In a bilayer consisting of a nonmagnet and a ferromagnet, spin injection from the interface results in spin accumulation and torque in the ferromagnet, which rapidly oscillate and decay by spin dephasing. In contrast, we find that even when an external electric field is applied only on the nonmagnet, we find substantially long-ranged orbital magnetoelectric response in the FM, which can go far beyond the spin dephasing length. This unusual feature is attributed to nearly degenerate orbital characters imposed by the crystal symmetry, which form hotspots for the intrinsic orbital response. Because only the states near the hotspots contribute dominantly, the induced orbital angular momentum does not exhibit destructive interference among states with different momentum as in the case of the spin dephasing. This gives rise to a distinct type of orbital torque on the magnetization, increasing with the thickness of the ferromagnet. Such behavior may serve as critical long-sought evidence of orbital transport to be directly tested in experiments. Our findings open the possibility of using long-range orbital magnetoelectric effect in orbitronic device applications.

cond-mat.mes-hall↗

arXiv2022

Orbital Dynamics in Centrosymmetric Systems

Orbital dynamics in time-reversal-symmetric centrosymmetric systems is examined theoretically. Contrary to common belief, we demonstrate that many aspects of orbital dynamics are qualitatively different from spin dynamics because the algebraic properties of the orbital and spin angular momentum operators are different. This difference generates interesting orbital responses, which do not have spin counterparts. For instance, the orbital angular momentum expectation values may oscillate even without breaking neither the time-reversal nor the inversion symmetry. Our quantum Boltzmann approach reproduces the previous result on the orbital Hall effect and reveals additional orbital dynamics phenomena, whose detection schemes are discussed briefly. Our work will be useful for the experimental differentiation of the orbital dynamics from the spin dynamics.

cond-mat.mes-hall↗

arXiv2021

Observation of the orbital Hall effect in a light metal Ti

The orbital angular momentum is a core ingredient of orbital magnetism, spin Hall effect, giant Rashba spin splitting, orbital Edelstein effect, and spin-orbit torque. However, its experimental detection is tricky. In particular, direct detection of the orbital Hall effect remains elusive despite its importance for electrical control of magnetic nanodevices. Here we report the direct observation of the orbital Hall effect in a light metal Ti. The Kerr rotation by the accumulated orbital magnetic moment is measured at Ti surfaces, whose result agrees with theoretical calculations semiquantitatively and is supported by the orbital torque measurement in Ti-based magnetic heterostructures. The results confirm the electron orbital angular momentum as an essential dynamic degree of freedom, which may provide a novel mechanism for the electric control of magnetism. The results may also deepen the understanding of spin, valley, phonon, and magnon dynamics coupled with orbital dynamics.

cond-mat.mes-hall↗

arXiv2021

Orbitronics: Orbital Currents in Solids

In solids, electronic Bloch states are formed by atomic orbitals. While it is natural to expect that orbital composition and information about Bloch states can be manipulated and transported, in analogy to the spin degree of freedom extensively studied in past decades, it has been assumed that orbital quenching by the crystal field prevents significant dynamics of orbital degrees of freedom. However, recent studies reveal that an orbital current, given by the flow of electrons with a finite orbital angular momentum, can be electrically generated and transported in wide classes of materials despite the effect of orbital quenching in the ground state. Orbital currents also play a fundamental role in the mechanisms of other transport phenomena such as spin Hall effect and valley Hall effect. Most importantly, it has been proposed that orbital currents can be used to induce magnetization dynamics, which is one of the most pivotal and explored aspects of magnetism. Here, we give an overview of recent progress and the current status of research on orbital currents. We review proposed physical mechanisms for generating orbital currents and discuss candidate materials where orbital currents are manifest. We review recent experiments on orbital current generation and transport and discuss various experimental methods to quantify this elusive object at the heart of $orbitronics$ $-$ an area which exploits the orbital degree of freedom as an information carrier in solid-state devices.

cond-mat.mes-hall↗

arXiv2021

Spin-orbit Torque Switching in an All-Van der Waals Heterostructure

Current-induced control of magnetization in ferromagnets using spin-orbit torque (SOT) has drawn attention as a new mechanism for fast and energy efficient magnetic memory devices. Energy-efficient spintronic devices require a spin-current source with a large SOT efficiency ($ξ$) and electrical conductivity ($σ$), and an efficient spin injection across a transparent interface. Herein, we use single crystals of the van der Waals (vdW) topological semimetal WTe$_2$ and vdW ferromagnet Fe$_3$GeTe$_2$ to satisfy the requirements in their all-vdW-heterostructure with an atomically sharp interface. The results exhibit values of $ξ{\approx}4.6$ and $σ{\approx}2.25{\times}10^5 Ω^{-1} m^{-1}$ for WTe$_2$. Moreover, we obtain the significantly reduced switching current density of $3.90{\times}10^6 A/cm^2$ at 150 K, which is an order of magnitude smaller than those of conventional heavy-metal/ ferromagnet thin films. These findings highlight that engineering vdW-type topological materials and magnets offers a promising route to energy-efficient magnetization control in SOT-based spintronics.

cond-mat.mes-hall↗

arXiv2021

Spin-memory loss induced by bulk spin-orbit coupling at ferromagnet/heavy-metal interfaces

A spin current through a ferromagnet/heavy-metal interface may shrink due to the spin-flip at the interface, resulting in the spin-memory loss. Here we propose a mechanism of the spin-memory loss. In contrast to other mechanisms based on interfacial spin-orbit coupling, our mechanism is based on the bulk spin-orbit coupling in a heavy-metal. We demonstrate that the bulk spin-orbit coupling induces the entanglement between the spin and orbital degrees of freedom and this spin-orbital entanglement can give rise to sizable spin-flip at the interface even when the interfacial spin-orbit coupling is weak. Our mechanism emphasizes crucial roles of the atomic orbital degree of freedom and induces the strong spin-memory loss near band crossing points between bands of different orbital characters.

cond-mat.mes-hall↗

arXiv2021

Universality in Phyllotaxis: a Mechanical Theory

One of humanity's earliest mathematical inquiries might have involved the geometric patterns in plants. The arrangement of leaves on a branch, seeds in a sunflower, and spines on a cactus exhibit repeated spirals, which appear with an intriguing regularity providing a simple demonstration of mathematically complex patterns. Surprisingly, the numbers of these spirals are pairs of Fibonacci numbers consecutive in the series 1, 2, 3, 5, 8, 13, 21, 34, 55... obeying a simple rule 1+2=3, 2+3=5, 5+8=13 and so on. This article describes how physics helps to clarify the origin of this fascinating behavior by linking it to the properties of deformable lattices growing and undergoing structural rearrangements under stress.

nlin.PS↗

arXiv2020

Orbital Rashba effect in surface oxidized Cu film

Recent experimental observation of unexpectedly large current-induced spin-orbit torque in surface oxidized Cu on top of a ferromagnet suggested a possible role of the orbital Rashba effect (ORE). With this motivation, we investigate the ORE from first principles by considering an oxygen monolayer on top of a Cu(111) film. We show that surface oxidization of Cu film leads to gigantic enhancement of the ORE for states near the Fermi surface. The resulting chiral orbital texture in the momentum space is exceptionally strong, reaching $\sim 0.5\hbar$ in magnitude. We find that resonant hybridization between O $p$-states and Cu $d$-states is responsible for the emergence of the ORE. We demonstrate that application of an external electric field generates huge orbital Hall current, which is an order of magnitude larger than the spin Hall current found in heavy metals. This implies that "orbital torque" mechanism may be significant in surface oxidized Cu/ferromagnet structures. It also encourages experimental verification of the orbital texture in surface oxidized Cu through optical measurements such as angle-resolved photoemission spectroscopy.

cond-mat.mes-hall↗

arXiv2020

Theory of Current-Induced Angular Momentum Transfer Dynamics in Spin-Orbit Coupled Systems

Motivated by the importance of understanding competing mechanisms to current-induced spin-orbit torque in complex magnets, we develop a unified theory of current-induced spin-orbital coupled dynamics. The theory describes angular momentum transfer between different degrees of freedom in solids, e.g., the electron orbital and spin, the crystal lattice, and the magnetic order parameter. Based on the continuity equations for the spin and orbital angular momenta, we derive equations of motion that relate spin and orbital current fluxes and torques describing the transfer of angular momentum between different degrees of freedom. We then propose a classification scheme for the mechanisms of the current-induced torque in magnetic bilayers. Based on our first-principles implementation, we apply our formalism to two different magnetic bilayers, Fe/W(110) and Ni/W(110), which are chosen such that the orbital and spin Hall effects in W have opposite sign and the resulting spin- and orbital-mediated torques can compete with each other. We find that while the spin torque arising from the spin Hall effect of W is the dominant mechanism of the current-induced torque in Fe/W(110), the dominant mechanism in Ni/W(110) is the orbital torque originating in the orbital Hall effect of W. It leads to negative and positive effective spin Hall angles, respectively, which can be directly identified in experiments. This clearly demonstrates that our formalism is ideal for studying the angular momentum transfer dynamics in spin-orbit coupled systems as it goes beyond the "spin current picture" by naturally incorporating the spin and orbital degrees of freedom on an equal footing. Our calculations reveal that, in addition to the spin and orbital torque, other contributions such as the interfacial torque and self-induced anomalous torque within the ferromagnet are not negligible in both material systems.

cond-mat.mes-hall↗

arXiv2020

Non-trivial charge-to-spin conversion in ferromagnetic metal/Cu/Al2O3 by orbital transport

Efficient spin/charge interconversion is desired to develop innovative spin-based devices. So far, the interconversion has been performed by using heavy atomic elements, strong spin-orbit interaction of which realizes the interconversion through the spin Hall effect and the Edelstein effect. We demonstrate highly efficient charge-to-spin conversion in a ferromagnetic metal/Cu/Al2O3 trilayers, which do not contain any heavy element. The resulting spin torque efficiency is higher than those of conventional spin Hall and Rashba systems consisting of heavy elements such as Pt and Bi. Our experimental results qualitatively deviate from typical behaviors arising from spin transport. However, they are surprisingly consistent with the behaviors arising from the orbital transport. Our results thus demonstrate a new direction for efficient charge-to-spin conversion through the orbital transport.

cond-mat.mes-hall↗

arXiv2020

Numerical Computation of Spin-Transfer Torques for Antiferromagnetic Domain walls

We numerically compute current-induced spin-transfer torques for antiferromagnetic domain walls, based on a linear response theory in a tight-binding model. We find that, unlike for ferromagnetic domain wall motion, the contribution of adiabatic spin torque to antiferromagnetic domain wall motion is negligible, consistent with previous theories. As a result, the non-adiabatic spin-transfer torque is a main driving torque for antiferromagnetic domain wall motion. Moreover, the non-adiabatic spin-transfer torque for narrower antiferromagnetic domain walls increases more rapidly than that for ferromagnetic domain walls, which is attributed to the enhanced spin mistracking process for antiferromagnetic domain walls.

cond-mat.mes-hall↗

arXiv2019

Orbital Torque: Torque Generation by Orbital Current Injection

We propose a mechanism of torque generation by injection of an orbital current, which we call $\textit{orbital torque}$. In a magnetic bilayer consisting of a nonmagnet (NM) and a ferromagnet (FM), we consider a situation where the spin-orbit coupling (SOC) is present only in the FM. Although the SOC is absent in the NM, the orbital Hall effect can arise in the NM. When the resulting orbital Hall current is injected to the FM, the SOC of the FM converts the orbital angular momentum into spin, which exerts torque to the magnetization of the FM. Remarkably, even for small SOC strength comparable to that of $3d$ FMs, the orbital torque can be comparable to the spin torque induced by the spin Hall effect of the NM with strong SOC. This provides a way to experimentally probe the OHE and opens a new venue to achieving spin-torque devices based on light elements that exhibit gigantic orbital response. Experimental implications are discussed.

cond-mat.mes-hall↗

arXiv2019

Strain-engineering of Berry curvature dipole and valley magnetization in monolayer MoS$_2$

The Berry curvature dipole is a physical quantity that is expected to allow various quantum geometrical phenomena in a range of solid-state systems. Monolayer transition metal dichalcogenides provide an exceptional platform to modulate and investigate the Berry curvature dipole through strain. Here we theoretically demonstrate and experimentally verify for monolayer MoS$_\rm{2}$ the generation of valley orbital magnetization as a response to an in-plane electric field due to the Berry curvature dipole. The measured valley orbital magnetization shows excellent agreement with the calculated Berry curvature dipole which can be controlled by the magnitude and direction of strain. Our results show that the Berry curvature dipole acts as an effective magnetic field in current-carrying systems, providing a novel route to generate magnetization.

cond-mat.mes-hall↗

arXiv2019

Enhanced perpendicular magnetocrystalline anisotropy energy in an artificial magnetic material with bulk spin-momentum coupling

We systematically investigate the perpendicular magnetocrystalline anisotropy (MCA) in Co$-$Pt/Pd-based multilayers. Our magnetic measurement data shows that the asymmetric Co/Pd/Pt multilayer has a significantly larger perpendicular magnetic anisotropy (PMA) energy compared to the symmetric Co/Pt and Co/Pd multilayer samples. We further support this experiment by first principles calculations on the CoPt$_2$, CoPd$_2$, and CoPtPd, which are composite bulk materials that consist of three atomic layers in a unit cell, Pt/Co/Pt, Pd/Co/Pd, Pt/Co/Pd, respectively. By estimating the contribution of bulk spin-momentum coupling to the MCA energy, we show that the CoPtPd multilayer with the symmetry breaking has a significantly larger perpendicular magnetic anisotropy (PMA) energy than the other multilayers that are otherwise similar but lack the symmetry breaking. This observation thus provides an evidence of the PMA enhancement due to the structural inversion symmetry breaking and highlights the asymmetric CoPtPd as the first artificial magnetic material with bulk spin-momentum coupling, which opens a new pathway toward the design of materials with strong PMA.

cond-mat.mtrl-sci↗

arXiv2019

Unidirectional Magnon-Driven Domain Wall Motion Due to the Interfacial Dzyaloshinskii-Moriya Interaction

We demonstrate a unidirectional motion of a quasiparticle without an explicit symmetry breaking along the space-time coordinate of the particle motion. This counterintuitive behavior originates from a combined action of two intrinsic asymmetries in the other two directions. We realize this idea with the magnon-driven motion of a magnetic domain wall in thin films with interfacial asymmetry. Contrary to previous studies, the domain wall moves along the same direction regardless of the magnon-flow direction. Our general symmetry analysis and numerical simulation reveal that the odd order contributions from the interfacial asymmetry is unidirectional, which is dominant over bidirectional contributions in the realistic regime. We develop a simple analytic theory on the unidirectional motion, which provides an insightful description of this counterintuitive phenomenon.

cond-mat.mes-hall↗

arXiv2018

Spin-orbit-stable type-II nodal line band crossing in n-doped monolayer MoX2 (X=S,Se,Te)

1H-phase monolayer transition-metal dichalcogenides have spin-split electronic band structures near the K(K') point due to strong spin-orbit coupling and intrinsic inversion symmetry breaking. In case of the monolayer MoX2 (X=S, Se, Te), the spin-split conduction bands cross near the K(K') point. We show that the band crossing occurs not only along the high symmetry directions, but also along arbitrary directions due to a mirror reflection symmetry of the monolayer. As a result, n-doped monolayer MoX2 is a two-dimensional type-II nodal-line material.

cond-mat.mtrl-sci↗