arXiv subjects

Iñigo Robredo

Publications and source records attributed to Iñigo Robredo.

27 records · Page 2Linked to original sources

arXiv2022

Transport signatures of Fermi arcs at twin boundaries in Weyl materials

One of the most striking signatures of Weyl fermions is their surface Fermi arcs. Less known is that Fermi arcs can also be localized at internal twin boundaries where two Weyl materials of opposite chirality meet. In this work, we derive constraints on the topology and connectivity of these "internal Fermi arcs." We show that internal Fermi arcs can exhibit transport signatures and propose two probes: quantum oscillations and a quantized chiral magnetic current. We propose merohedrally twinned B20 materials as candidates to host internal Fermi arcs, verified through both model and ab initio calculations. Our theoretical investigation sheds lights on the topological features and motivates experimental studies into the intriguing physics of internal Fermi arcs.

cond-mat.mes-hall↗

arXiv2022

Spin-momentum locking from topological quantum chemistry: applications to multifold fermions

In spin-orbit coupled crystals, symmetries can protect multifold degeneracies with large Chern numbers and Brillouin zone spanning topological surface states. In this work, we explore the extent to which the nontrivial topology of chiral multifold fermions impacts the spin texture of bulk states. To do so, we formulate a definition of spin-momentum locking in terms of reduced density matrices. Using tools from the theory of topological quantum chemistry, we show how the reduced density matrix can be determined from the knowledge of the basis orbitals and band representation forming the multifold fermion. We show how on-site spin orbit coupling, crystal field splitting, and Wyckoff position multiplicity compete to determine the spin texture of states near chiral fermions. We compute the spin texture of multifold fermions in several representative examples from space groups $P432$ (207) and $P2_13$ (198). We show that the winding number of the spin around the Fermi surface can take many different integer values, from zero all the way to $\pm 7$. Finally, we conclude by showing how to apply our theory to real materials using the example of PtGa in space group $P2_13$.

cond-mat.mes-hall↗

arXiv2021

Cubic Hall viscosity in three-dimensional topological semimetals

The nondissipative (Hall) viscosity is known to play an interesting role in two-dimensional (2D) topological states of matter, in the hydrodynamic regime of correlated materials, and in classical active fluids with broken time-reversal symmetry (TRS). However, generalizations of these effects to 3D have remained elusive. In this work, we address this question by studying the Hall viscoelastic response of 3D crystals. We show that for systems with tetrahedral symmetries, there exist new, intrinsically 3D Hall viscosity coefficients that cannot be obtained via a reduction to a quasi-2D system. To study these coefficients, we specialize to a theoretically and experimentally motivated tight-binding model for a chiral magnetic metal in (magnetic) space group [(M)SG] P2$_1$3 (No. 198.9), a nonpolar group of recent experimental interest that hosts both chiral magnets and topological semimetals (TSMs). Using the Kubo formula for viscosity, we compute two forms of the Hall viscosity, phonon and ``momentum'' (conventional) and show that for the tight-binding model we consider, both forms realize the novel cubic Hall viscosity. We conclude by discussing the implication of our results for transport in 2D magnetic metals and discuss some candidate materials in which these effects may be observed.

cond-mat.mes-hall↗

arXiv2021

Theoretical study of topological properties of ferromagnetic pyrite CoS$_2$

Since the discovery of the first topological material 15 years ago, the search for material realizations of novel topological phases has become the driving force of the field. While oftentimes we search for new materials, we forget that well established materials can also display very interesting topological properties. In this work, we revisit CoS$_2$ , a metallic ferromagnetic pyrite that has been extensively studied in the literature due to its magnetic properties. We study the topological features of its electronic band structure and identify Weyl nodes and Nodal lines, as well as a symmetry-protected 4-fold fermion close to the Fermi level. Looking at different surface cleavage planes, we observe both spin polarized Fermi arcs in the majority channel and drumhead states. These findings suggest that CoS$_2$ is a promising platform to study topological phenomena, as well as a good candidate for spintronic applications.

cond-mat.mtrl-sci↗

arXiv2021

Cubic 3D Chern photonic insulators with orientable large Chern vectors

Time Reversal Symmetry (TRS) broken topological phases provide gapless surface states protected by topology, regardless of additional internal symmetries, spin or valley degrees of freedom. Despite the numerous demonstrations of 2D topological phases, few examples of 3D topological systems with TRS breaking exist. In this article, we devise a general strategy to design 3D Chern insulating (3D CI) cubic photonic crystals in a weakly TRS broken environment with orientable and arbitrarly large Chern vectors. The designs display topologically protected chiral and unidirectional surface states with disjoint equifrequency loops. The resulting crystals present the following novel characteristics: First, by increasing the Chern number, multiple surface states channels can be supported. Second, the Chern vector can be oriented along any direction simply changing the magnetization axis, opening up larger 3D CI/3D CI interfacing possibilities as compared to 2D. Third, by lowering the TRS breaking requirements, the system is ideal for realistic photonic applications where the magnetic response is weak.

cond-mat.mes-hall↗

arXiv2020

Weyl-fermions, Fermi-arcs, and minority-spin carriers in ferromagnetic CoS2

The pyrite compound CoS2 has been intensively studied in the past due to its itinerant ferromagnetism and potential for half-metallicity, which make it a promising material for spintronic applications. However, its electronic structure remains only poorly understood. Here we use complementary bulk- and surface-sensitive angle-resolved photoelectron spectroscopy and ab-initio calculations to provide a complete picture of its band structure. We discover Weyl-cones at the Fermi-level, which presents CoS2 in a new light as a rare member of the recently discovered class of magnetic topological metals. We directly observe the topological Fermi-arc surface states that link the Weyl-nodes, which will influence the performance of CoS2 as a spin-injector by modifying its spin-polarization at interfaces. Additionally, we are for the first time able to directly observe a minority-spin bulk electron pocket in the corner of the Brillouin zone, which proves that CoS2 cannot be a true half-metal. Beyond settling the longstanding debate about half-metallicity in CoS2, our results provide a prime example of how the topology of magnetic materials can affect their use in spintronic applications.

cond-mat.mtrl-sci↗

arXiv2019

Large multi-directional spin-to-charge conversion in low symmetry semimetal MoTe$_2$ at room temperature

Efficient and versatile spin-to-charge current conversion is crucial for the development of spintronic applications, which strongly rely on the ability to electrically generate and detect spin currents. In this context, the spin Hall effect has been widely studied in heavy metals with strong spin-orbit coupling. While the high crystal symmetry in these materials limits the conversion to the orthogonal configuration, unusual configurations are expected in low symmetry transition metal dichalcogenide semimetals, which could add flexibility to the electrical injection and detection of pure spin currents. Here, we report the observation of spin-to-charge conversion in MoTe$_2$ flakes, which are stacked in graphene lateral spin valves. We detect two distinct contributions arising from the conversion of two different spin orientations. In addition to the conventional conversion where the spin polarization is orthogonal to the charge current, we also detect a conversion where the spin polarization and the charge current are parallel. Both contributions, which could arise either from bulk spin Hall effect or surface Edelstein effect, show large efficiencies comparable to the best spin Hall metals and topological insulators. Our finding enables the simultaneous conversion of spin currents with any in-plane spin polarization in one single experimental configuration.

cond-mat.mes-hall↗

arXiv2019

Spectral and optical properties of Ag$_3$Au(Se$_2$,Te$_2$) and dark matter detection

In this work we study the electronic structure of Ag${}_3$AuSe${}_2$ and Ag${}_3$AuTe${}_2$, two chiral insulators whose gap can be tuned through small changes in the lattice parameter by applying hydrostatic pressure or choosing different growth protocols. Based on first principles calculations we compute their band structure for different values of the lattice parameters and show that while Ag${}_3$AuSe${}_2$ retains its direct narrow gap at the $Γ$ point, Ag${}_3$AuTe${}_2$ can turn into a metal. Focusing on Ag${}_3$AuSe${}_2$ we derive a low energy model around $Γ$ using group theory, which we use to calculate the optical conductivity for different values of the lattice constant. We discuss our results in the context of detection of light dark matter particles, which have masses of the order of a $k$eV, and conclude that Ag${}_3$AuSe${}_2$ satisfies three important requirements for a suitable detector: small Fermi velocities, $m$eV band gap and low photon screening. Our work motivates the growth of high-quality and large samples of Ag${}_3$AuSe${}_2$ to be used as target materials in dark matter detectors.

cond-mat.mtrl-sci↗

arXiv2019

Revisiting (higher order and crystalline) topology in old models of lead telluride

In this work, we revisit the model of PbTe presented in [E. Fradkin, E. Dagotto, and D. Boyanovsky, Phys. Rev. Lett. 57, 2967 (1986)]. We show that the low energy theory of this model corresponds to a (higher-order) topological crystalline insulator in space group $Fm\bar{3}m1'$, diagnosable by symmetry indicators. We show that the gapless fermions found on antiphase domain walls are the topological boundary modes of the system, due to a nonvanishing mirror Chern number. Furthermore, we show that any symmetric completion of the model must be in this same topological phase. Finally, we comment on the relationship of this model to realistic PbTe, which has recently been predicted to have a phase which realizes same bulk symmetry indicators.

cond-mat.mes-hall↗