arXiv subjects

I. A. Shelykh

Publications and source records attributed to I. A. Shelykh.

At least 55 records · Page 3Linked to original sources

arXiv2021

Theory of nonlinear excitonic response of hybrid organic perovskites in the regime of strong light-matter coupling

We present a quantitative study of the nonlinear optical response of layered perovskites placed inside planar photonic microcavities in the regime of strong light matter coupling, when excitonic and photonic modes hybridize and give rise to cavity polaritons. Two sources of nonlinearity are specified, the saturation of the excitonic transition with increase of the optical pump and Coulomb interaction between the excitons. It is demonstrated, that peculiar form of the interaction potential, specific to multilayer structure of organic perovskites, is responsible for substantial increase of the exciton binding energy and Rabi splitting with respect to conventional semiconductor systems. This results in dominant contribution of the Rabi splitting quench effect in the nonlinear optical response. Moreover, due to the tightly bound character of excitons, the density of Mott transition is essentially higher, allowing to reach extremely large polariton blueshifts of about 50 meV, which is order of magnitude higher than in conventional semiconductors.

cond-mat.mes-hall↗

arXiv2021

Bound photonic pairs in 2D waveguide quantum electrodynamics

We theoretically predict the formation of two-photon bound states in a two-dimensional waveguide network hosting a lattice of two-level atoms. The properties of these bound pairs and the exclusive domains of the parameter space where they emerge due to the interplay between the on-site photon blockade and peculiar shape of polariton dispersion resulting from the long-range radiative couplings between the qubits are investigated in detail. In addition, we analyze the effect of the finite-size system on localization characteristics of these excitations.

quant-ph↗

arXiv2021

Machine learning of phase transitions in nonlinear polariton lattices

Polaritonic lattices offer a unique testbed for studying nonlinear driven-dissipative physics. They show qualitative changes of a steady state as a function of system parameters, which resemble non-equilibrium phase transitions. Unlike their equilibrium counterparts, these transitions cannot be characterised by conventional statistical physics methods. Here, we study a lattice of square-arranged polariton condensates with nearest-neighbour coupling, and simulate the polarisation (pseudo-spin) dynamics of the polariton lattice, observing regions with distinct steady-state polarisation patterns. We classify these patterns using machine learning methods and determine the boundaries separating different regions. First, we use unsupervised data mining techniques to sketch the boundaries of phase transitions. We then apply learning by confusion, a neural network-based method for learning labels in the dataset, and extract the polaritonic phase diagram. Our work takes a step towards AI-enabled studies of polaritonic systems.

cond-mat.mes-hall↗

arXiv2021

Tunable strongly interacting dipolar excitons in hybrid perovskites

We study theoretically the excitonic nonlinearity in hybrid organic-inorganic Ruddlesden-Popper perovskite thin films. The composite layered structure of these materials allows for flexible modulation of their excitonic response between the limiting cases of single atomic layer and wide quasi-two-dimensional quantum well. In particular, we demonstrate that transverse electric field leads to the spatial separation of charge carriers within the inorganic layer, giving rise to strongly interacting excitons possessing built-in dipole moment. Combined with exciton binding energy of the order of hundreds of meVs, this makes hybrid perovskites an optimal platform for tailoring of nonlinear optical response at reduced dimensionality.

cond-mat.mes-hall↗

arXiv2021

Dissipative Josephson vortices in annular polariton fluids

We consider two concentric rings formed by bosonic condensates of exciton-polaritons. A circular superfluid flow of polaritons in one of the rings can be manipulated by acting upon the second annular polariton condensate. The complex coupling between the rings with different topological charges triggers nucleation of stable Josephson vortices (JVs) which are revealed as topological defects of the angular dependence of the relative phase between rings. Being dependent on the coupling strength, the structure of the JV governs the difference of the mean angular momenta of the inner and the outer rings. At the vanishing coupling the condensates rotate independently demonstrating no correlations of their winding numbers. At the moderate coupling, the interaction between two condensates tends to equalize their mean angular momenta despite of the mismatch of the winding numbers demonstrating the phenomenology of a drag effect. Above the critical coupling strength the synchronous rotation is established via the phase slip events.

cond-mat.quant-gas↗

arXiv2021

Valley polarization of trions in monolayer MoSe$_2$ interfaced with bismuth iron garnet

Interfacing atomically thin van der Waals semiconductors with magnetic substrates enables additional control on their intrinsic valley degree of freedom and provides a promising platform for the development of novel valleytronic devices for information processing and storage. Here we study circularly polarized photoluminescence in heterostructures of monolayer MoSe$_2$ and thin films of ferrimagnetic bismuth iron garnet. We observe strong emission from charged excitons with negative valley polarization, which switches sign with increasing temperature, and demonstrate contrasting response to left and right circularly polarized excitation, associated with finite out-of-plane magnetization in the substrate. We propose a theoretical model accounting for magnetization-induced imbalance of charge carriers in the two valleys of MoSe$_2$, as well as for valley-switching scattering from B to A excitons and fast formation of trions with extended valley relaxation times, which shows excellent agreement with the experimental data. Our results provide new insights into valley physics in 2D semiconductors interfaced with magnetic substrates.

cond-mat.mes-hall↗

arXiv2021

All optical resonant magnetization switching in $\text{CrI}_3$ monolayers

Efficient control of a magnetization without an application of the external magnetic fields is the ultimate goal of spintronics. We demonstrate, that in monolayers of $\text{CrI}_3$, magnetization can be switched all optically, by application of the resonant pulses of circularly polarized light. This happens because of the efficient coupling of the lattice magnetization with bright excitonic transition. $\text{CrI}_3$ is thus perspective functional material with high potential for applications in the domains of spintronics and ultra-fast magnetic memory.

cond-mat.mes-hall↗

arXiv2021

Anomalous Exciton Hall Effect

It is well known that electrically neutral excitons can still be affected by crossed electric and magnetic fields that make them move in a direction perpendicular to both fields. We show that a similar effect appears in the absence of external electric fields, in the case of scattering of an exciton flow by charged impurities in the presence of the external magnetic field. As a result, the exciton flow changes the direction of its propagation that may be described in terms of the Hall conductivity for excitons. We develop a theory of this effect, which we refer to as the anomalous exciton Hall effect, to distinguish it from the exciton Hall effect that arises due to the valley selective exciton transport in transition metal dichalcogenides. According to our estimations, the effect is relatively weak for optically active or bright excitons in conventional GaAs quantum wells, but it becomes significant for optically inactive or dark excitons, because of the difference of the lifetimes. This makes the proposed effect a convenient tool for spatial separation of dark and bright excitons.

cond-mat.mes-hall↗

arXiv2020

Two-dimensional chiral waveguide quantum electrodynamics: long range qubit correlations and flat-band dark polaritons

We consider a two-dimensional extension of the 1D waveguide quantum electrodynamics and investigate the nature of linear excitations in two-dimensional arrays of qubits coupled to networks of chiral waveguides. We show that the combined effects of chirality and long-range photon mediated qubit-qubit interactions lead to the emergence of the two-dimensional flat bands in the polaritonic spectrum, corresponding to slow strongly correlated light.

quant-ph↗

arXiv2020

Dynamics of spin polarization in tilted polariton rings

We have observed the effect of pseudo magnetic field originating from the polaritonic analog of spin-orbit coupling (TE$-$TM splitting) on a polariton condensate in a ring-shaped microcavity. The effect gives rise to a stable four-leaf pattern around the ring as seen from the linear polarization measurements of the condensate photoluminescence. This pattern is found to originate from the interplay of the cavity potential, energy relaxation, and TE-TM splitting in the ring. Our observations are compared to the dissipative one-dimensional spinor Gross-Pitaevskii equation with the TE-TM splitting energy which shows good qualitative agreement.

cond-mat.quant-gas↗

arXiv2020

Optical analogue of Dresselhaus spin-orbit interaction in photonic graphene

The concept of gauge fields plays a significant role in many areas of physics from particle physics and cosmology to condensed matter systems, where gauge potentials are a natural consequence of electromagnetic fields acting on charged particles and are of central importance in topological states of matter. Here, we report on the experimental realization of a synthetic non-Abelian gauge field for photons in a honeycomb microcavity lattice. We show that the effective magnetic field associated with TE-TM splitting has the symmetry of Dresselhaus spin-orbit interaction around Dirac points in the dispersion, and can be regarded as an SU(2) gauge field. The symmetry of the field is revealed in the optical spin Hall effect (OSHE), where under resonant excitation of the Dirac points precession of the photon pseudospin around the field direction leads to the formation of two spin domains. Furthermore, we observe that the Dresselhaus field changes its sign in the same Dirac valley on switching from s to p bands in good agreement with the tight binding modelling. Our work demonstrating a non-Abelian gauge field for light on the microscale paves the way towards manipulation of photons via spin on a chip.

cond-mat.mes-hall↗

arXiv2020

Tunable optical nonlinearity for TMD polaritons dressed by a Fermi sea

We study a system of a transition metal dichalcogenide (TMD) monolayer placed in an optical resonator, where strong light-matter coupling between excitons and photons is achieved. We present quantitative theory of the nonlinear optical response for exciton-polaritons for the case of doped TMD monolayer, and analyze in detail two sources of nonlinearity. The first nonlinear response contribution stems from the Coulomb exchange interaction between excitons. The second contribution comes from the reduction of Rabi splitting that originates from phase space filling at increased exciton concentration and the composite nature of excitons. We demonstrate that both nonlinear contributions are enhanced in the presence of free electrons. As free electron concentration can be routinely controlled by an externally applied gate voltage, this opens a way of electrical tuning of the nonlinear optical response.

cond-mat.mes-hall↗

arXiv2020

Atomic frustrated impurity states in Weyl metals

We theoretically analyze the effect of the inversion symmetry breaking on the structure of the impurity molecular states in Weyl metals. We show that for the case of a highly noncentrosymmetric Weyl metallic host, the standard picture of the alternating bonding and antibonding orbitals breaks down, and a qualitatively different frustrated atomic state emerges. This is a consequence of the pseudogap closing and related delicate Fano interplay between intra- and inter-impurity scattering channels.

cond-mat.str-el↗

arXiv2020

Majorana molecules and their spectral fingerprints

We introduce the concept of a Majorana molecule, a topological bound state appearing in the geometry of a double quantum dot (QD) structure flanking a topological superconducting nanowire. We demonstrate that, if the Majorana bound states (MBSs) at opposite edges are probed nonlocally in a two probe experiment, the spectral density of the system reveals the so-called half-bowtie profiles, while Andreev bound states (ABSs) become resolved into bonding and antibonding molecular configurations. We reveal that this effect is due to the Fano interference between pseudospin superconducting pairing channels and propose that it can be catched by a pseudospin resolved Scanning Tunneling Microscope (STM)-tip.

cond-mat.mes-hall↗

arXiv2020

Spin-valley dynamics in alloy-based transition metal dichalcogenide heterobilayers

Van der Waals heterobilayers based on 2D transition metal dichalcogenides have been recently shown to support robust and long-lived valley polarization for potential valleytronic applications. However, the role of the band structure and alignment of the constituent layers in the underlying dynamics remains largely unexplored. Here we study spin--valley relaxation dynamics in heterobilayers with different band structures engineered via the use of alloyed monolayer semiconductors. Through a combination of time-resolved Kerr rotation spectroscopic measurements and theoretical modelling for Mo$_{1-x}$W$_{x}$Se$_2$/WSe$_2$ samples with different chemical compositions and stacking angles, we uncover the roles of interlayer exciton recombination and charge carrier spin depolarization in the overall valley dynamics. Our results provide insights into the microscopic spin--valley polarization mechanisms in van der Waals heterostructures for the development of future 2D valleytronic devices.

cond-mat.mes-hall↗

arXiv2020

Propagative oscillations in co-directional polariton waveguide couplers

We report on novel exciton-polariton routing devices created to study and purposely guide light-matter particles in their condensate phase. In a co-directional coupling device, two waveguides are connected by a partially etched section which facilitates tunable coupling of the adjacent channels. This evanescent coupling of the two macroscopic wavefunctions in each waveguide reveals itself in real space oscillations of the condensate. This Josephson-like oscillation has only been observed in coupled polariton traps so far. Here, we report on a similar coupling behavior in a controllable, propagative waveguide-based design. By controlling the gap width, channel length or the propagation energy, the exit port of the polariton flow can be chosen. This co-directional polariton device is a passive and scalable coupler element that can serve in compact, next generation logic architectures.

cond-mat.mes-hall↗

arXiv2020

Floquet engineering of the Luttinger Hamiltonian

Within the Floquet theory of periodically driven quantum systems, we developed the theory of light-induced modification of electronic states in semiconductor materials described by the Luttinger Hamiltonian (the electronic term $Γ_8$). Particularly, exact solutions of the Floquet problem are found for the band edge in the cases of linearly and circularly polarized irradiation. It is shown that the irradiation changes electron effective masses near the band edge, induces anisotropy of the electron dispersion and splits the bands. It is demonstrated that the light-induced band splitting strongly depends on the light polarization. Namely, the circularly polarized light acts similarly to a stationary magnetic field and lifts the spin degeneracy of electron branches, whereas a linearly polarized light does not affect the spin degeneracy and only splits the bands in the center of the Brillouin zone. The present theory can be applied to describe electronic properties of various semiconductor structures irradiated by an electromagnetic field in the broad frequency range.

cond-mat.mes-hall↗

arXiv2020

Interaction induced hybridization of Majorana zero-modes in a coupled quantum-dot hybrid-nanowire system

We study the low-energy transport properties of a hybrid device composed by a native quantum dot coupled to both ends of a topological superconducting nanowire section hosting Majorana zero-modes. The account of the coupling between the dot and the farthest Majorana zero-mode allows to introduce the topological quality factor, characterizing the level of topological protection in the system. We demonstrate that Coulomb interaction between the dot and the topological superconducting section leads to the onset of the additional overlap of the wavefunctions describing the Majorana zero-modes, leading to the formation of trivial Andreev bound states even for spatially well-separated Majoranas. This leads to the spoiling of the quality factor and introduces a constraint for the braiding process required to perform topological quantum computing operations.

cond-mat.mes-hall↗