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I. A. Tolstukhin

Publications and source records attributed to I. A. Tolstukhin.

12 recordsLinked to original sources

Detailed Study of the $^{59}$Cu(p,$α)^{56}$Ni Reaction and Constraints on Its Astrophysical Reaction Rate

The $^{59}$Cu$(p,α)^{56}$Ni reaction plays an important role in explosive astrophysical scenarios such as Type I X-ray bursts and the $νp$-process in neutrino-driven winds following a core-collapse supernova, where it regulates the flow of nucleosynthesis through the NiCu cycle and the synthesis of heavier nuclei. We present a direct measurement of the $^{59}\mathrm{Cu}(p,α)^{56}\mathrm{Ni}$ excitation function from 2.43--5.88~MeV in the center-of-mass frame, performed in inverse kinematics with the high-efficiency MUSIC active-target detector at FRIB. The angle- and energy-integrated cross sections extend direct measurements to lower energies than previously reported and remove the angular-integration model dependence of earlier work. To extrapolate the rate to astrophysical energies, we constrain the statistical-model description through a systematic optimization of the DEM-3 $α$-optical model potential geometry, and quantify the model-selection uncertainty with a Bayesian model averaging analysis over 96 TALYS combinations. The resulting stellar rate carries a temperature-dependent uncertainty factor of 1.26--1.63 over $T_9 = 0.2$--10 and is systematically lower than the REACLIB evaluation, remaining below the competing $(p,γ)$ rate for $T_9 \lesssim 3.94$. These results substantially weaken the inferred NiCu cycle strength and establish the $^{59}$Cu$(p,γ)^{60}$Zn rate as the dominant remaining uncertainty.

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Direct Measurement of the $^{59}$Cu$(p,α)^{56}$Ni Excitation Function to Constrain the Ni--Cu Cycle Strength and Its Impact on Explosive Nucleosynthesis

A new direct measurement of the 59Cu(p,a)56Ni excitation function from 2.43-5.88 MeV in the center-of-mass was performed in inverse kinematics using the high-efficiency MUSIC active-target detector at FRIB. This reaction plays a critical role in constraining the strength of the NiCu cycle in different explosive astrophysical scenarios such as Type I X-ray bursts and the nu-p process in neutrino-driven winds after a core-collapse supernova. The newly derived stellar rate is systematically lower than previous estimates, suppressing NiCu cycle recycling in X-ray bursts to below 3% and enhancing nu-p process efficiency throughout the relevant temperature range, potentially extending its effective operation to temperatures as high as T9 = 3.94 (+0.99/-0.85).

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Valence $1s-0d$ proton vacancy of the $^{32}$Si ground state

The $^{32}$Si($^3$He,$d$)$^{33}$P reaction was studied in inverse kinematics at 6.3~MeV/$u$. States in $^{33}$P corresponding to the proton $1s-0d$ single-particle orbitals were identified up to $\sim$4.5 MeV in excitation energy. The ($^{3}$He,$d$) spectroscopic factors were determined from Distorted Wave Born Approximation calculations. When combined with complementary neutron-adding data, the $1s-0d$ proton vacancies in the $^{32}$Si ground state were extracted. In conjunction with a re-analysis of data from previous single-particle measurements, the trends in proton and neutron vacancy were explored across the $^{28,30,32,34}$Si isotopes. Both proton and neutron vacancy data show gradual changes in their occupancies. The proton $1s_{1/2}$ orbitals in $^{32}$Si and $^{34}$Si are both consistent with being empty. The ground-state nucleon distributions are described by shell-model calculations constrained to the $1s-0d$ model space.

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Quenching of single-particle strength inferred from nucleon-removal transfer reactions on $^{15}$C

The difference in the proton and neutron separation energies ($ΔS$) of the weakly bound $^{15}$C ground state is -19.86 MeV, an extreme value. Data from intermediate-energy heavy-ion induced (HI-induced) knockout reactions on nuclei spanning $-20\lesssimΔS\lesssim+20$ MeV, suggest that the degree to which single-particle strength is quenched, $R\mathrm{_{s}}$, has a negative correlation with $ΔS$, decreasing from unity around $-20$~MeV to around 0.2 at $+20$~MeV. For the $^{15}$C ground state ($R_s=0.96(4)$ in HI-induced knockout), contrasting results have recently been obtained via the neutron-adding transfer reaction, which reveal a value of $R_s=0.64(15)$, similar to the value observed at modest $ΔS$ and more extreme values of $ΔS$ with reaction probes other than HI knockout. In order to explore the any potential differences between $adding$ and $removing$ processes in transfer reactions at extreme $ΔS$, single-neutron removal transfer reactions on $^{15}$C were performed at 7.1MeV/u in inverse kinematics. The removal of a valence neutron in 2$s_{1/2}$ orbit using both ($p$,$d$) and ($d$,$t$) reactions shows consistent quenching factors and agrees with those from the neutron-adding reaction. The present results, which can be compared with neutron knockout reaction, suggest that correlations, represented by the quenching factor, show limited dependence on neutron-proton asymmetry under the most extreme asymmetry conditions so far achieved in transfer reactions.

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First measurement of 87Rb(α, xn) cross sections at weak r-process energies in supernova ν-driven ejecta to investigate elemental abundances in low-metallicity stars

Observed abundances of Z ~ 40 elements in metal-poor stars vary from star to star, indicating that the rapid and slow neutron capture processes may not contribute alone to the synthesis of elements beyond iron. The weak r-process was proposed to produce Z ~ 40 elements in a subset of old stars. Thought to occur in the ν-driven ejecta of a core-collapse supernova, (α, xn) reactions would drive the nuclear flow toward heavier masses at T = 2-5 GK. However, current comparisons between modelled and observed yields do not bring satisfactory insights into the stellar environment, mainly due to the uncertainties of the nuclear physics inputs where the dispersion in a given reaction rate often exceeds one order of magnitude. Involved rates are calculated with the statistical model where the choice of an α-optical-model potential (αOMP) leads to such a poor precision. The first experiment on 87Rb(α, xn) reactions at weak r-process energies is reported here. Total inclusive cross sections were assessed at Ec.m. = 8.1 - 13 MeV (3.7 - 7.6 GK) with the active target MUlti-Sampling Ionization Chamber (MUSIC). With a N = 50 seed nucleus, the measured values agree with statistical model estimates using the αOMP Atomki-V2. A re-evaluated reaction rate was incorporated into new nucleosynthesis calculations, focusing on ν-driven ejecta conditions known to be sensitive to this specific rate. These conditions were found to fail to reproduce the lighter-heavy element abundances in metal-poor stars.

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Meaurement of spin vs. TKE of $^{144}$Ba produced in spontaneous fission of $^{252}$Cf

We measure the average spin of $^{144}$Ba, a common fragment produced in $^{252}$Cf(sf), as a function of the total kinetic energy (TKE). We combined for the first time a twin Frisch-gridded ionization chamber with a world-class $γ$-ray spectrometer that was designed to measure high-multiplicity $γ$-ray events, Gammasphere. The chamber, loaded with a $^{252}$Cf(sf) source, provides a fission trigger, the TKE of the fragments, the approximate fragment masses, and the polar angle of the fission axis. Gammasphere provides the total $γ$-ray yield, fragment identification through the tagging of decay $γ$ rays, and the feeding of rotational bands in the fragments. We determine the dependence of the average spin of $^{144}$Ba on the fragments' TKE by correlating the fragment properties with the distribution of discrete levels that are fed. We find that the average spin only changes by about $0.5$ $\hbar$ across the TKE range of 158-203 MeV. The virtual independence of the spin on TKE suggests that spin is not solely generated through the statistical excitation of rotational modes, and more complex mechanisms are required.

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Evolution of the nuclear spin-orbit splitting explored via the $^{32}$Si($d$,$p$)$^{33}$Si reaction using SOLARIS

The spin-orbit splitting between neutron 1$p$ orbitals at $^{33}$Si has been deduced using the single-neutron-adding ($d$,$p$) reaction in inverse kinematics with a beam of $^{32}$Si, a long-lived radioisotope. Reaction products were analyzed by the newly implemented SOLARIS spectrometer at the reaccelerated-beam facility at the National Superconducting Cyclotron Laboratory. The measurements show reasonable agreement with shell-model calculations that incorporate modern cross-shell interactions, but they contradict the prediction of proton density depletion based on relativistic mean-field theory. The evolution of the neutron 1$p$-shell orbitals is systematically studied using the present and existing data in the isotonic chains of $N=17$, 19, and 21. In each case, a smooth decrease in the separation of the $1p_{3/2}$-$1p_{1/2}$ orbitals is seen as the respective $p$-orbitals approach zero binding, suggesting that the finite nuclear potential strongly influences the evolution of nuclear structure in this region.

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Direct cross-section measurement of the weak r-process 88Sr(α,n)91Zr reaction in ν-driven winds of core collapse supernovae

About half of the heavy elements beyond iron are known to be produced by the rapid neutron capture process, known as r-process. However, the astrophysical site producing the r-process is still uncertain. Chemical abundances observed in several cosmic sites indicate that different mechanisms should be at play. For instance, the abundances around silver measured in a subset of metal-poor stars indicate the presence of a weak r-process. This process may be active in neutrino-driven winds of core collapse supernovae where ($α$,n) reactions dominate the synthesis of Z ~ 40 elements in the expelled materials. Scarcely measured, the rates of ($α$,n) reactions are determined from statistical Hauser-Feshbach calculations with $α$-optical-model potentials, which are still poorly constrained. The uncertainties of the ($α$,n) reaction rates therefore make a significant contribution to the uncertainties of the abundances determined from stellar modeling. In this work, the $^{88}$Sr($α$,n)$^{91}$Zr reaction which impacts the weak r-process abundances has been probed at astrophysics energy for the first time; directly measuring the total cross sections at astrophysical energies of 8.37 - 13.09 MeV in the center of mass (3.8 - 7.5 GK). Two measurements were performed at ATLAS with the electrically-segmented ionization chamber MUSIC, in inverse kinematics, while following the active target technique. The cross sections of this $α$-induced reaction on $^{88}$Sr, located at the shell closure N = 50, have been found to be lower than expected, by a factor of 3, despite recent statistical calculations validated by measurements on neighboring nuclei. This result encourages more experimental investigations of ($α$,n) reactions, at N = 50 and towards the neutron-rich side, to further test the predictive power and reliability of such calculations.

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Direct Determination of Fission-Barrier Heights Using Light-Ion Transfer in Inverse Kinematics

We demonstrate a new technique for obtaining fission data for nuclei away from $β$-stability. These types of data are pertinent to the astrophysical \textit{r-}process, crucial to a complete understanding of the origin of the heavy elements, and for developing a predictive model of fission. These data are also important considerations for terrestrial applications related to power generation and safeguarding. Experimentally, such data are scarce due to the difficulties in producing the actinide targets of interest. The solenoidal-spectrometer technique, commonly used to study nucleon-transfer reactions in inverse kinematics, has been applied to the case of transfer-induced fission as a means to deduce the fission-barrier height, among other variables. The fission-barrier height of $^{239}$U has been determined via the $^{238}$U($d$,$pf$) reaction in inverse kinematics, the results of which are consistent with existing neutron-induced fission data indicating the validity of the technique.

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Probing the quadrupole transition strength of 15C via deuteron inelastic scattering

Deuteron elastic scattering from 15C and inelastic scattering reactions to the first excited state of 15C were studied using a radioactive beam of 15C in inverse kinematics. The scattered deuterons were measured using HELIOS. The elastic scattering differential cross sections were analyzed using the optical model. A matter deformation length δd = 1.04(11) fm has been extracted from the differential cross sections of inelastic scattering to the first excited state. The ratio of neutron and proton matrix elements Mn/Mp = 3.6(4) has been determined from this quadrupole transition. Neutron effective charges and core-polarization parameters of 15C were determined and discussed. Results from ab-initio no-core configuration interaction calculations were also compared with the experimental observations. This result supports a moderate core decoupling effect of the valence neutron in 15C similarly to its isotone 17O, in line with the interpretation of other neutron-rich carbon isotopes.

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Study of the Isomeric State in $^{16}$N Using the $^{16}$N$^{g,m}$($d$,$^3$He) Reaction

The isomeric state of $^{16}$N was studied using the $^{16}$N$^{g,m}$($d$,$^3$He)~proton-removal reactions at \mbox{11.8~MeV/$u$} in inverse kinematics. The $^{16}$N beam, of which 24% was in the isomeric state, was produced using the ATLAS in-fight facility and delivered to the HELIOS spectrometer, which was used to analyze the $^{3}$He ions from the ($d$,$^{3}$He) reactions. The simultaneous measurement of reactions on both the ground and isomeric states, reduced the systematic uncertainties from the experiment and in the analysis. A direct and reliable comparison of the relative spectroscopic factors was made based on a Distorted-Wave Born Approximation approach. The experimental results suggest that the isomeric state of $^{16}$N is an excited neutron-halo state. The results can be understood through calculations using a Woods-Saxon potential model, which captures the effects of weak-binding.

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Quenching of Single-Particle Strength in A=15 Nuclei

Absolute cross sections for the addition of $s$- and $d$-wave neutrons to $^{14}$C and $^{14}$N have been determined simultaneously via the ($d$,$p$) reaction at 10 MeV/u. The difference between the neutron and proton separation energies, $ΔS$, is around $-20$ MeV for the $^{14}$C$+$$n$ system and $+8$ MeV for $^{14}$N$+$$n$. The population of the $1s_{1/2}$ and $0d_{5/2}$ orbitals for both systems is reduced by a factor of approximately 0.5 compared to the independent single-particle model, or about 0.6 when compared to the shell model. This finding strongly contrasts with results deduced from intermediate-energy knockout reactions between similar nuclei on targets of $^{9}$Be and $^{12}$C. The simultaneous technique used removes many systematic uncertainties.

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