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I. Aharonovich

Publications and source records attributed to I. Aharonovich.

At least 19 recordsLinked to original sources
arXiv2025

Coherent all-optical control of the germanium vacancy in diamond

The germanium vacancy in diamond (GeV) is a promising candidate for color center based quantum networking. Yet, like for other group-IV vacancy defects in diamond, achieving fast, high-fidelity qubit operations using traditional magnetic resonance techniques is experimentally challenging due to a weak magnetic dipole and susceptibility to thermally induced decoherence. Here, we perform all-optical control of the GeV and realize Rabi frequencies exceeding $\sim 20$~MHz. We do so by driving the two $Λ$-systems of the GeV simultaneously and apply this to probe the spin coherence ($T_2^*=224\pm14$~ns, $T_2^{\rm H}=11.9\pm0.3$~$μ$s). Our control scheme is applicable to other color centers and particularly, other group-IV defects for which, the scheme may be optimized to improve all-optical control in these systems.

cond-mat.mes-hall↗
arXiv2023

Exploring methods for creation of Boron-vacancies in hexagonal Boron Nitride exfoliated from bulk crystal

Boron vacancies (VB${^-}$) in hexagonal boron-nitride (hBN) have sparked great interest in recent years, due to their electronic spin properties. Since hBN can be readily integrated into devices where it interfaces a huge variety of other 2D materials, boron vacancies may serve as a precise sensor which can be deployed at very close proximity to many important materials systems. Boron vacancy defects may be produced by a number of existing methods, the use of which may depend on the final application. Any method should reproducibly generate defects with controlled density and desired pattern. To date, however, detailed studies of such methods are missing. In this paper we study various techniques, focused ion beam (FIB), electron irradiation and ion implantation, for the preparation of hBN flakes from bulk crystals, and relevant post-processing treatments to create VB${^-}$s as a function of flake thickness and defect concentrations. We find that flake thickness plays an important role when optimising implantation parameters, while careful sample cleaning proved important to achieve best results.

physics.app-ph↗
arXiv2023

Dual-band coupling between nanoscale polaritons and vibrational and electronic excitations in molecules

Strong coupling (SC) between light and matter excitations such as excitons and molecular vibrations bear intriguing potential for controlling chemical reactivity, conductivity or photoluminescence. So far, SC has been typically achieved either between mid-infrared (mid-IR) light and molecular vibrations or between visible light and excitons. Achieving SC simultaneously in both frequency bands may open unexplored pathways for manipulating material properties. Here, we introduce a polaritonic nanoresonator (formed by h-BN layers placed on Al ribbons) hosting surface plasmon polaritons (SPPs) at visible frequencies and phonon polaritons (PhPs) at mid-IR frequencies, which simultaneously couple to excitons and atomic vibration in an adjacent molecular layer (CoPc). Employing near-field optical nanoscopy, we first demonstrate the co-localization of strongly confined near-fields at both visible and mid-IR frequencies. After covering the nanoresonator structure with a layer of CoPc molecules, we observe clear mode splittings in both frequency ranges by far-field transmission spectroscopy, unambiguously revealing simultaneous SPP-exciton and PhP-vibron coupling. Dual-band SC may be exploited for manipulating the coupling between excitons and molecular vibrations in future optoelectronics, nanophotonics, and quantum information applications.

physics.optics↗
arXiv2021

Quantum microscopy with van der Waals heterostructures

Quantum microscopes based on solid-state spin quantum sensors have recently emerged as powerful tools for probing material properties and physical processes in regimes not accessible to classical sensors, especially on the nanoscale. Such microscopes have already found utility in a variety of problems, from imaging magnetism and charge transport in nanoscale devices, to mapping remanent magnetic fields from ancient rocks and biological organisms. However, applications of quantum microscopes have so far relied on sensors hosted in a rigid, three-dimensional crystal, typically diamond, which limits their ability to closely interact with the sample under study. Here we demonstrate a versatile and robust quantum microscope using quantum sensors embedded within a thin layer of a van der Waals (vdW) material, hexagonal boron nitride (hBN). To showcase the capabilities of this platform, we assemble several active vdW heterostructures, with an hBN layer acting as the quantum sensor. We demonstrate time-resolved, simultaneous temperature and magnetic imaging near the Curie temperature of a vdW ferromagnet as well as apply this unique microscope to map out charge currents and Joule heating in graphene. By enabling intimate proximity between sensor and sample, potentially down to a single atomic layer, the hBN quantum sensor represents a paradigm shift for nanoscale quantum sensing and microscopy. Moreover, given the ubiquitous use of hBN in modern materials and condensed matter physics research, we expect our technique to find rapid and broad adoption in these fields, further motivated by the prospect of performing in-situ chemical analysis and noise spectroscopy using advanced quantum sensing protocols.

cond-mat.mes-hall↗
arXiv2019

A solid state single photon source with Fourier Transform limited lines at room temperature

Solid state single photon sources with Fourier Transform (FT) limited lines are among the most crucial constituents of photonic quantum technologies and have been accordingly the focus of intensive research over the last several decades. However, so far, solid state systems have only exhibited FT limited lines at cryogenic temperatures due to strong interactions with the thermal bath of lattice phonons. In this work, we report a solid state source that exhibits FT limited lines measured in photo luminescence excitation (sub 100 MHz linewidths) from 3K-300K. The studied source is a color center in the two-dimensional hexagonal boron nitride and we propose that the center's decoupling from phonons is a fundamental consequence of material's low dimensionality. While the center's luminescence lines exhibit spectral diffusion, we identify the likely source of the dffusion and propose to mitigate it via dynamic spectral tuning. The discovery of FT-limited lines at room temperature, which once the spectral diffusion is controlled, will also yield FT-limited emission. Our work motivates a significant advance towards room temperature photonic quantum technologies and a new research direction in the remarkable fundamental properties of two-dimensional materials.

cond-mat.mes-hall↗
arXiv2019

Acoustically modulated optical emission of hexagonal boron nitride layers

We investigate the effect of surface acoustic waves on the atomic-like optical emission from defect centers in hexagonal boron nitride layers deposited on the surface of a LiNbO$_3$ substrate. The dynamic strain field of the surface acoustic waves modulates the emission lines resulting in intensity variations as large as 50% and oscillations of the emission energy with an amplitude of almost 1 meV. From a systematic study of the dependence of the modulation on the acoustic wave power, we determine a hydrostatic deformation potential for defect centers in this two-dimensional material of about 40 meV/%. Furthermore, we show that the dynamic piezoelectric field of the acoustic wave could contribute to the stabilization of the optical properties of these centers. Our results show that surface acoustic waves are a powerful tool to modulate and control the electronic states of two-dimensional materials.

cond-mat.mes-hall↗
arXiv2018

Electron Paramagnetic Resonance signature of point defects in neutron irradiated hexagonal Boron Nitride

Hexagonal boron nitride (h-BN) is an attractive van der Waals material for studying fluorescent defects due to its large bandgap. In this work, we demonstrate enhanced pink color due to neutron irradiation and perform electron paramagnetic resonance (EPR) measurements. The new point defects are tentatively assigned to doubly- occupied nitrogen vacancies with (S = 1) and a zero-field splitting (D = 1.2 GHz). These defects are associated with a broad visible optical absorption band and near infrared photoluminescence band centered at ~ 490 nm and 820 nm, respectively. The EPR signal intensities are strongly affected by thermal treatments in temperature range between 600 to 800°C, where also the irradiation - induced pink color is lost. Our results are important for understanding of point defects in h-BN and their deployment for quantum and integrated photonic applications.

cond-mat.mtrl-sci↗
arXiv2017

Narrowband quantum emitters over large spectral range with Fourier-limited linewidth in hexagonal boron nitride

Single defect centers in layered hexagonal boron nitride (hBN) are promising candidates as single photon sources for quantum optics and nanophotonics applications. However, until today spectral instability hinders many applications. Here, we perform resonant excitation measurements and observe Fourier-Transform limited (FL) linewidths down to $\approx 50$ MHz. We investigate optical properties of more than 600 quantum emitters (QE) in hBN. The QEs exhibit narrow zero-phonon lines (ZPL) distributed over a spectral range from 580 nm to 800 nm and with dipole-like emission with high polarization contrast. The emission frequencies can be divided into four main regions indicating distinct families or crystallographic structures of the QEs, in accord with ab-initio calculations. Finally, the emitters withstand transfer to a foreign photonic platform - namely a silver mirror, which makes them compatible with photonic devices such as optical resonators and paves the way to quantum photonics applications including quantum commmunications and quantum repeaters.

cond-mat.mes-hall↗
arXiv2017

Single crystal diamond membranes for nanoelectronics

Single crystal, nanoscale diamond membranes are highly sought after for a variety of applications including nanophotonics, nanoelectronics and quantum information science. However, so far, the availability of conductive diamond membranes remained an unreachable goal. In this work we present a complete nanofabrication methodology for engineering high aspect ratio, electrically active single crystal diamond membranes. The membranes have large lateral directions, exceeding 500x500 um2 and are only several hundreds of nanometers thick. We further realize vertical single crystal p-n junctions, made from the diamond membranes that exhibit onset voltages of ~ 10V and a current of several mA. Moreover, we deterministically introduce optically active color centers into the membranes, and demonstrate for the first time a single crystal nanoscale diamond LED. The robust and scalable approach to engineer the electrically active single crystal diamond membranes, offers new pathways for advanced nanophotonics, nanoelectronics and optomechanics devices employing diamond.

physics.app-ph↗
arXiv2016

An upper limit on the lateral vacancy diffusion length in diamond

Ion implantation is widely used to modify the structural, electrical and optical properties of materials. By appropriate masking, this technique can be used to define nano- and micro-structures. However, depending on the type of mask used, experiments have shown that vacancy-related substrate modification can be inferred tens of microns away from the edge of the mask used to define the implanted region. This could be due to fast diffusion of vacancies from the implanted area during annealing or to a geometric effect related to ion scattering around the mask edges. For quantum and single-atom devices, stray ion damage can be deleterious and must be minimized. In order to profile the distribution of implantation-induced damage, we have used the nitrogen-vacancy colour centre as a sensitive marker for vacancy concentration and distribution following MeV He ion implantation into diamond and annealing. Results show that helium atoms implanted through a mask clamped to the diamond surface are scattered underneath the mask to distances in the range of tens of micrometers from the mask edge. Implantation through a lithographically defined and deposited mask, with no spacing between the mask and the substrate, significantly reduces the scattering to <5 m but does not eliminate it. These scattering distances are much larger than the theoretically estimated vacancy diffusion distance of 260 nm under similar conditions. This paper shows that diffusion, upon annealing, of vacancies created by ion implantation in diamond is limited and the appearance of vacancies many tens of micrometers from the edge of the mask is due to scattering effects.

cond-mat.mtrl-sci↗
arXiv2015

Photoluminescence from voids created by femtosecond laser pulses inside cubic-BN

Photoluminescence (PL) from femtosecond laser modified regions inside cubic-boron nitride (c-BN) was measured under UV and visible light excitation. Bright PL at the red spectral range was observed, with a typical excited state lifetime of $\sim 4$~ns. Sharp emission lines are consistent with PL of intrinsic vibronic defects linked to the nitrogen vacancy formation (via Frenkel pair) observed earlier in high energy electron irradiated and ion-implanted c-BN. These, formerly known as the radiation centers, RC1, RC2, and RC3 have been identified at the locus of the voids formed by single fs-laser pulse. The method is promising to engineer color centers in c-BN for photonic applications.

cond-mat.mes-hall↗
arXiv2013

Lorentz Invariant Berry Phase for a Perturbed Relativistic Four Dimensional Harmonic Oscillator

We show the existence of Lorentz invariant Berry phases generated, in the Stueckleberg-Horwitz-Piron manifestly covariant quantum theory (SHP), by a perturbed four dimensional harmonic oscillator. These phases are associated with a fractional perturbation of the azimuthal symmetry of the oscillator. They are computed numerically by using time independent perturbation theory and the definition of the Berry phase generalized to the framework of SHP relativistic quantum theory.

math-ph↗
arXiv2013

On Chip Manipulation of Single Photons from a Diamond Defect

Operating reconfigurable quantum circuits with single photon sources is a key goal of photonic quantum information science and technology. We use an integrated waveguide device comprising of directional couplers and a reconfigurable thermal phase controller to manipulate single photons emitted from a chromium related colour centre in diamond. Observation of both a wave-like interference pattern and particle-like sub-Poissionian autocorrelation functions demonstrates coherent manipulation of single photons emitted from the chromium related centre and verifies wave particle duality.

quant-ph↗
arXiv2013

Neutrinos and $v<c$

The Stueckelberg formulation of a manifestly covariant relativistic classical and quantum mechanics is briefly reviewed and it is shown that in this framework a simple (semiclassical) model exists for the description of neutrino oscillations. The model is shown to be consistent with the field equations and the Lorentz force (developed here without and with spin by canonical methods) for Glashow-Salam-Weinberg type non-Abelian fields interacting with the leptons. We discuss a possible fundamental mechanism, in the context of a relativistic theory of spin for (first quantized) quantum mechanical systems, for CP violation. The model also predicts a possibly small "pull back", i.e., early arrival of a neutrino beam, for which the neutrino motion is almost everywhere within the light cone, a result which may emerge from future long baseline experiments designed to investigate neutrino transit times with significantly higher accuracy than presently available.

physics.gen-ph↗
arXiv2011

Radiation-reaction in classical offshell electrodynamics: I. The above mass-shell case

Offshell electrodynamics based on a manifestly covariant off-shell relativistic dynamics of Stueckelberg, Horwitz and Piron, is five-dimensional. In this paper, we study the problem of radiation reaction of a particle in motion in this framework. In particular, the case of above-mass-shell is studied in detail, where the renormalization of the Lorentz force leads to a system of non-linear differential equations for 3 Lorentz scalars. The system is then solved numerically, where it is shown that the mass-shell deviation scalar $\ve$ either smoothly falls down to 0 (this result provides a mechanism for the mass stability of the off-shell theory), or strongly diverges under more extreme conditions. In both cases, no runaway motion is observed. Stability analysis indicates that the system seems to have chaotic behavior in the divergent case. It is also shown that, although a motion under which the mass-shell deviation $\ve$ is constant but not-zero, is indeed possible, but, it is unstable, and eventually it either decays to 0 or diverges.

math-ph↗
arXiv2011

On the Green-Functions of the classical offshell electrodynamics under the manifestly covariant relativistic dynamics of Stueckelberg

In previous paper derivations of the Green function have been given for 5D off-shell electrodynamics in the framework of the manifestly covariant relativistic dynamics of Stueckelberg (with invariant evolution parameter $τ$). In this paper, we reconcile these derivations resulting in different explicit forms, and relate our results to the conventional fundamental solutions of linear 5D wave equations published in the mathematical literature. We give physical arguments for the choice of the Green function retarded in the fifth variable $τ$.

math-ph↗
arXiv2011

Wide range electrical tunability of single photon emission from chromium-based colour centres in diamond

We demonstrate electrical control of the single photon emission spectrum from chromium-based colour centres implanted in monolithic diamond. Under an external electric field the tunability range is typically three orders of magnitude larger than the radiative linewidth and at least one order of magnitude larger than the observed linewidth. The electric and magnetic field dependence of luminescence gives indications on the inherent symmetry and we propose Cr-X or X-Cr-Y type noncentrosymmetric atomic configurations as most probable candidates for these centres.

cond-mat.mes-hall↗