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I. Babushkin

Publications and source records attributed to I. Babushkin.

At least 19 recordsLinked to original sources

Isotopic variations and Zeeman-like splitting in the spectra of nonlinear photonic meta-atoms

We study photonic meta-atoms, a unique class of composite solitary wave, supported in nonlinear waveguides. We establish an analogy to one-dimensional soft-core atoms, allowing to describe the complex dynamics via concepts from atomic physics. Higher-order dispersive effects cause specific spectral resonances characteristic for the eigenspectrum of a meta-atom. We demonstrate that subtle changes in this level spectrum causes frequency shifts of the resonances. These shifts consist of isotopic and isomeric contributions that can be distinguished in terms of a simple model. We further demonstrate a generic mechanism that causes a Zeeman-like splitting of resonance lines.

physics.optics

Universal properties of locally generated terahertz waveforms from polarization-controlled two- and multi-color ionizing fields

The polarization states of terahertz (THz) radiation generated in a photo-ionized gas driven by strong two- or multi-frequency fields with locally controlled polarization are studied. We reveal a universal property of the resulting THz waveforms: the ellipticity of their polarization state increases linearly with the frequency. This ``linear chirp of ellipticity'' makes plasma-based THz generation unique among other THz sources. However, it also puts some constraints on the polarization properties of the generated THz radiation. We derive a general expression for the THz ellipticity and demonstrate how the polarization states of the generated THz waveforms can be manipulated and controlled by the polarization of the pump pulses.

physics.optics

All-optical attoclock for imaging tunnelling wavepackets

Recent experiments on measuring time-delays during tunnelling of cold atoms through an optically created potential barrier are reinvigorating the controversial debate regarding possible time-delays during light-induced tunnelling of an electron from an atom. Compelling theoretical and experimental arguments have been put forward to advocate opposite views, confirming or refuting the existence of finite tunnelling time delays. Yet, such a delay, whether present or not, is but a single quantity characterizing the tunnelling wavepacket; the underlying dynamics are richer. Here we propose to augment photo-electron detection in laser-induced tunnelling with detection of light emitted by the tunnelling electron -- the so-called Brunel radiation. Using a combination of single-color and two-color driving fields, we identify the all-optical signatures of the re-shaping of the tunnelling wavepacket as it emerges from the tunnelling barrier and moves away from the core. This reshaping includes not only an effective time-delay but also time-reversal asymmetry of the ionization process, which we describe theoretically and observe experimentally. We show how both delay and reshaping are mapped on the polarization properties of the Brunel radiation, with different harmonics behaving as different hands of a clock moving at different speeds. The all-optical detection paves the way to time-resolving optical tunnelling in condensed matter systems, e.g. tunnelling across bandgaps in solids, on the attosecond time-scale.

physics.optics

Two-color soliton meta-atoms and molecules

We present a detailed overview of the physics of two-color soliton molecules in nonlinear waveguides, i.e. bound states of localized optical pulses which are held together due to an incoherent interaction mechanism. The mutual confinement, or trapping, of the subpulses, which leads to a stable propagation of the pulse compound, is enabled by the nonlinear Kerr effect. Special attention is paid to the description of the binding mechanism in terms of attractive potential wells, induced by the refractive index changes of the subpulses, exerted on one another through cross-phase modulation. Specifically, we discuss nonlinear-photonics meta atoms, given by pulse compounds consisting of a strong trapping pulse and a weak trapped pulse, for which trapped states of low intensity are determined by a Schrödinger-type eigenproblem. We discuss the rich dynamical behavior of such meta-atoms, demonstrating that an increase of the group-velocity mismatch of both subpulses leads to an ionization-like trapping-to-escape transition. We further demonstrate that if both constituent pulses are of similar amplitude, molecule-like bound-states are formed. We show that z-periodic amplitude variations permit a coupling of these pulse compound to dispersive waves, resulting in the resonant emission of Kushi-comb-like multi-frequency radiation.

physics.optics

Soliton compression and supercontinuum spectra in nonlinear diamond photonics

We numerically explore synthetic crystal diamond for realizing novel light sources in ranges which are up to now difficult to achieve with other materials, such as sub-10-fs pulse durations and challenging spectral ranges. We assess the performance of on-chip diamond waveguides for controlling light generation by means of nonlinear soliton dynamics. Tailoring the cross-section of such diamond waveguides allows to design dispersion profiles with custom zero-dispersion points and anomalous dispersion ranges exceeding an octave. Various propagation dynamics, including supercontinuum generation by soliton fission, can be realized in diamond photonics. In stark contrast to usual silica-based optical fibers, where such processes occur on the scale of meters, in diamond millimeter-scale propagation distances are sufficient. Unperturbed soliton-dynamics prior to soliton fission allow to identify a pulse self-compression scenario that promises record-breaking compression factors on chip-size propagation lengths.

physics.optics

Two-color pulse compounds in waveguides with a zero-nonlinearity point

We study incoherently coupled two-frequency pulse compounds in waveguides with single zero-dispersion and zero-nonlinearity points. In such waveguides, supported by a negative nonlinearity, soliton dynamics can be obtained even in domains of normal dispersion. We demonstrate trapping of weak pulses by solitary-wave wells, forming nonlinear-photonics meta-atoms, and molecule-like bound-states of pulses. We study the impact of Raman effect on these pulse compounds, finding that, depending on the precise subpulse configuration, they decelerate, accelerate, or are completely unaffected. Our results extend the range of systems in which two-frequency pulse compounds can be expected to exist and demonstrate further unique and unexpected behavior.

physics.optics

Resonant Kushi-comb-like multi-frequency radiation of oscillating two-color soliton molecules

Nonlinear waveguides with two distinct domains of anomalous dispersion can support the formation of molecule-like two-color pulse compounds. They consist of two tightly bound subpulses with frequency loci separated by a vast frequency gap. Perturbing such a two-color pulse compound triggers periodic amplitude and width variations, reminiscent of molecular vibrations. With increasing strength of perturbation, the dynamics of the pulse compound changes from harmonic to nonlinear oscillations. The periodic amplitude variations enable coupling of the pulse compound to dispersive waves, resulting in the resonant emission of multi-frequency radiation. We demonstrate that the location of the resonances can be precisely predicted by phase-matching conditions. If the pulse compound consists of a pair of identical subpulses, inherent symmetries lead to degeneracies in the resonance spectrum. Weak perturbations lift existing degeneracies and cause a splitting of the resonance lines into multiple lines. Strong perturbations result in more complex emission spectra, characterized by well separated spectral bands caused by resonant Cherenkov radiation and additional four-wave mixing processes.

nlin.PS

Terahertz pulse generation by two-color laser fields with circular polarization

We study the influence of the polarization states of femtosecond two-color pulses ionizing gases on the emitted terahertz radiation. A local-current model and plane-wave evaluations justify the previously-reported impact on the THz energy yield and an (almost) linearly-polarized THz field when using circularly-polarized laser harmonics. For such pump pulses, the THz yield is independent on the relative phase between the two colors. When the pump pulses have same helicity, the increase in the THz yield is associated to longer ionization sequences and higher electron transverse momenta acquired in the driving field. Reversely, for two color pulses with opposite helicity, the dramatic loss of THz power comes from destructive interferences driven by the highly symmetric response of the photocurrents lined up on the third harmonic of the fundamental pulse. While our experiments confirm an increased THz yield for circularly polarized pumps of same helicity, surprisingly, the emitted THz radiation is not linearly-polarized. This effect is explained by means of comprehensive 3D numerical simulations highlighting the role of the spatial alignment and non-collinear propagation of the two colors.

physics.optics

Coherently controlled generation of single-cycle terahertz pulses from thin layer of nonlinear medium with low-frequency resonances

We propose a novel scheme to generate single-cycle terahertz (THz) pulses via reflection of an optical femtosecond pulse train from a thin layer of nonlinear resonant medium. Our method is based on a coherent control of low-frequency oscillations and free induction decay in the medium. The specific single-cycle shape of generated THz pulses requires a plane wavefront and detection in the near field. Our theoretical results pave the way to a new, simple and high-efficiency way to generate single-cycle waveshape-tunable terahertz pulses.

physics.optics

Self-induced transparency mode-locking in a Ti:sapphire laser with an intracavity rubidium cell

In a Ti:Sa laser with an absorbing with Rb vapor cell stable self-starting passive mode-locking is demonstrated. We show that the mode-locking appears due to self-induced transparency (SIT) in the Rb cell, that is, the pulse in the Rb cell is a 2pi SIT pulse. For the best of our knowledge, in these experiments we present the first time demonstration of SIT mode-locking in laser systems, which was discussed only theoretical before.

physics.optics

Passive and hybrid mode locking in multi-section terahertz quantum cascade lasers

It is believed that passive mode locking is virtually impossible in quantum cascade lasers (QCLs) because of too fast carrier relaxation time. Here, we revisit this possibility and theoretically show that stable mode locking and pulse durations in the few cycle regime at terahertz (THz) frequencies are possible in suitably engineered bound-to-continuum QCLs. We achieve this by utilizing a multi-section cavity geometry with alternating gain and absorber sections. The critical ingredients are the very strong coupling of the absorber to both field and environment as well as a fast absorber carrier recovery dynamics. Under these conditions, even if the gain relaxation time is several times faster than the cavity round trip time, generation of few-cycle pulses is feasible. We investigate three different approaches for ultrashort pulse generation via THz quantum cascade lasers, namely passive, hybrid and colliding pulse mode locking.

physics.optics

Terahertz and higher-order Brunel harmonics: from tunnel to multiphoton ionization regime in tailored fields

Brunel radiation appears as a result of a two-step process of photo-ionization and subsequent acceleration of electron, without the need of electron recollision. We show that for generation of Brunel harmonics at all frequencies the subcycle ionization dynamics is of critical importance. Namely, such harmonics disappear at low pump intensities when the ionization dynamics depends only on the slow envelope (so called multiphoton ionization regime) and not on the instantaneous field. Nevertheless, if the pump pulse contains incommensurate frequencies, Brunel mechanism does generate new frequencies even in the multiphoton ionization regime.

physics.plasm-ph

Spectral dynamics of THz pulses generated by two-color laser filaments in air: The role of Kerr nonlinearities and pump wavelength

We theoretically and numerically study the influence of both instantaneous and Raman-delayed Kerr nonlinearities as well as a long-wavelength pump in the terahertz (THz) emissions produced by two-color femtosecond filaments in air. Although the Raman-delayed nonlinearity induced by air molecules weakens THz generation, four-wave mixing is found to impact the THz spectra accumulated upon propagation via self-, cross-phase modulations and self-steepening. Besides, using the local current theory, we show that the scaling of laser-to-THz conversion efficiency with the fundamental laser wavelength strongly depends on the relative phase between the two colors, the pulse duration and shape, rendering a universal scaling law impossible. Scaling laws in powers of the pump wavelength may only provide a rough estimate of the increase in the THz yield. We confront these results with comprehensive numerical simulations of strongly focused pulses and of filaments propagating over meter-range distances.

physics.optics

Generation of unipolar pulses in a circular Raman-active medium excited by few-cycle optical pulses

We study theoretically a new possibility of unipolar pulses generation in Raman-active medium excited by a series of few-cycle optical pulses. We consider the case when the Raman-active particles are uniformly distributed along the circle, and demonstrate a possibility to obtain a unipolar rectangular video pulses with an arbitrarily long duration, ranging from a minimum value equal to the natural period of the low frequency vibrations in the Raman-active medium.

physics.optics

Self-starting stable coherent mode-locking in a two-section laser

Coherent mode-locking (CML) uses self-induced transparency (SIT) soliton formation to achieve, in contrast to conventional schemes based on absorption saturation, the pulse durations below the limit allowed by the gain line width. Despite of the great promise it is difficult to realize it experimentally because a complicated setup is required. In all previous theoretical considerations CML is believed to be non-self-starting. In this article we show that if the cavity length is selected properly, a very stable (CML) regime can be realized in an elementary two-section ring-cavity geometry, and this regime is self-developing from the non-lasing state. The stability of the pulsed regime is the result of a dynamical stabilization mechanism arising due to finite-cavity-size effects.

physics.optics

Self-induced transparency mode-locking, and area theorem

Self-induced transparency mode-locking (or coherent mode-locking, CML) which is based on intracavity self-induced transparency soliton dynamics, allows potentially to achieve nearly single cycle intracavity pulse durations, much below the phase relaxation time $T_2$ in a laser, which, despite of great promise, has not yet been realized experimentally. We develop a diagram technique which allows to predict the main features of CML regimes in a generic two-section laser. We show that CML can arise directly at the first laser threshold if the phase relaxation time is large enough. Furthermore, CML regimes can be unconditionally stable. We also predict the existence of ``super-CML regimes``, with a pulse coupled to several Rabi oscillations in the nonlinear medium.

physics.optics

Boosting terahertz generation in laser-field ionized gases using a sawtooth wave shape

Broadband ultrashort terahertz (THz) pulses can be produced using plasma generation in a noble gas ionized by femtosecond two-color pulses. Here we demonstrate that, by using multiple-frequency laser pulses, one can obtain a waveform which optimizes the free electron trajectories in such a way that they reach the highest velocity at the electric field extrema. This allows to increase the THz conversion efficiency to the percent level, an unprecedented performance for THz generation in gases. Besides the analytical study of THz generation using a local current model, we perform comprehensive 3D simulations accounting for propagation effects which confirm this prediction. Our results show that THz conversion via tunnel ionization can be greatly improved with well-designed multicolor pulses.

physics.optics

The fundamental solution of the unidirectional pulse propagation equation

The fundamental solution of a variant of the three-dimensional wave equation known as "unidirectional pulse propagation equation" (UPPE) and its paraxial approximation is obtained. It is shown that the fundamental solution can be presented as a projection of a fundamental solution of the wave equation to some functional subspace. We discuss the degree of equivalence of the UPPE and the wave equation in this respect. In particular, we show that the UPPE, in contrast to the common belief, describes wave propagation in both longitudinal and temporal directions, and, thereby, its fundamental solution possesses a non-causal character.

math-ph