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I. Bozovic

Publications and source records attributed to I. Bozovic.

32 records · Page 2Linked to original sources

Temporal correlations of superconductivity above the transition temperature in La$_{2-x}$Sr$_x$CuO$_4$ probed by terahertz spectroscopy

The nature of the underdoped pseudogap regime of the high-temperature superconductors has been a matter of long-term debate. On quite general grounds, one expects that due to their low superfluid densities and short correlation lengths, superconducting fluctuations will be significant for transport and thermodynamic properties in this part of the phase diagram. Although there is ample experimental evidence for such correlations, there has been disagreement about how high in temperature they may persist, their role in the phenomenology of the pseudogap, and their significance for understanding high-temperature superconductivity. In this work we use THz time-domain spectroscopy (TTDS) to probe the temporal fluctuations of superconductivity above the critical temperature (T$_c$) in La$_{2-x}$Sr$_x$CuO$_4$ thin films over a doping range that spans almost the entire superconducting dome (x = 0.09 to 0.25). Signatures of the fluctuations persist in the conductivity in a comparatively narrow temperature range, at most 16 K above Tc. Our measurements show that superconducting correlations do not make an appreciable contribution to the charge transport anomalies of the pseudogap in LSCO at temperatures well above T$_c$.

cond-mat.supr-con↗

On the possibility of fast vortices in the cuprates: A vortex plasma model analysis of THz conductivity and diamagnetism in La$_{2-x}$Sr$_{x}$CuO$_4$

We present measurements of the fluctuation superconductivity in an underdoped thin film of La$_{1.905}$Sr$_{0.095}$CuO$_4$ using time-domain THz spectroscopy. We compare our results with measurements of diamagnetism in a similarly doped crystal of La$_{2-x}$Sr$_x$CuO$_4$. We show through a vortex-plasma model that if the fluctuation diamagnetism solely originates in vortices, then they must necessarily exhibit an anomalously large vortex diffusion constant, which is more than two orders of magnitude larger than the Bardeen-Stephen estimate. This points to either the extremely unusual properties of vortices in the under-doped d-wave cuprates or a contribution to the diamagnetic response that is not superconducting in origin.

cond-mat.supr-con↗

Photoinduced melting of superconductivity in the high-Tc superconductor La2-xSrxCuO4 probed by time-resolved optical and THz techniques

Dynamics of depletion and recovery of superconducting state in La2-xSrxCuO_4 thin films is investigated utilizing optical pump-probe and optical pump - THz probe techniques as a function of temperature and excitation fluence. The absorbed energy density required to suppress superconductivity is found to be about 8 times higher than the thermodynamically determined condensation energy density and nearly temperature independent between 4 and 25 K. These findings indicate that during the time when superconducting state suppression takes place (~0.7 ps), a large part (nearly 90%) of the energy is transferred to the phonons with energy lower than twice the maximum value of of the SC gap and only 10% is spent on Cooper pair breaking.

cond-mat.supr-con↗

Superconducting transition at 38 K in insulating-overdoped La2CuO4-La1.64Sr0.36CuO4 superlattices: Evidence for interface electronic redistribution from resonant soft x-ray scattering

We use resonant soft x-ray scattering (RSXS) to quantify the hole distribution in a superlattice of insulating La2CuO4 (LCO) and overdoped La_{2-x}Sr_{x}CuO4 (LSCO). Despite its non-superconducting constituents, this structure is superconducting with T_{c}=38 K. We found that the conducting holes redistribute electronically from LSCO to the LCO layers. The LCO layers were found to be optimally doped, suggesting they are the main drivers of superconductivity. Our results demonstrate the utility of RSXS for separating electronic from structural effects at oxide interfaces.

cond-mat.str-el↗

High-temperature interface superconductivity between metallic and insulating cuprates

High-temperature superconductivity confined to nanometer-size interfaces has been a long standing goal because of potential applications^{1,2} and the opportunity to study quantum phenomena in reduced dimensions^{3,4}. However, this is a challenging target: in conventional metals the high electron density restricts interface effects such as carrier depletion/accumulation to a region much narrower than the coherence length, the scale necessary for superconductivity to occur. In contrast, in copper oxides the carrier density is low while the critical temperature (T_c) is high and the coherence length very short; so, this provides a breakthrough opportunity but at a price: the interface must be atomically perfect. Here we report on superconductivity in bilayers consisting of an insulator (La_2CuO_4) and a metal (La_{1.55}Sr_{0.45}CuO_{4}), neither of which is superconducting in isolation. However, in bilayers T_c is either ~15 K or ~30 K, depending on the layering sequence. This highly robust phenomenon is confined within 2-3 nm from the interface. If such a bilayer is exposed to ozone, T_c exceeds 50 K and this enhanced superconductivity is also shown to originate from the interface layer about 1-2 unit cell thick. Enhancement of T_c in bilayer systems was observed previously^5 but the essential role of the interface was not recognized at the time. Our results demonstrate that engineering artificial heterostructures provides a novel, unconventional way to fabricate stable, quasi two-dimensional high T_c phases and to significantly enhance superconducting properties in known or new superconductors.

cond-mat.supr-con↗

Surface Structure Analysis of Atomically Smooth BaBiO$_3$ Films

Using low energy Time-of-Flight Scattering and Recoil Spectroscopy (TOF-SARS) and Mass Spectroscopy of Recoiled Ions (MSRI) we analyze the surface structure of an atomically smooth BaBiO$_3$ film grown by molecular beam epitaxy. We demonstrate high sensitivity of the TOF-SARS and MSRI spectra to slight changes in the orientation of the ion scattering plane with respect to the crystallographic axes. The observed angle dependence allows us to clearly identify the termination layer as BiO$_2$. Our data also indicate that angle-resolved MSRI data can be used for high resolution studies of surface structure of complex oxide thin films.

cond-mat.other↗

A Structural Probe of the Doped Holes in Cuprate Superconductors

An unresolved issue concerning cuprate superconductors is whether the distribution of carriers in the CuO(2) plane is uniform or inhomogeneous. Because the carriers comprise a small fraction of the total charge density and may be rapidly fluctuating, modulations are difficult to detect directly. Here we demonstrate that in anomalous x-ray scattering at the oxygen K edge of the cuprates, the contribution of carriers to the scattering amplitude is selectively magnified 82 times. This enhances diffraction from the doped holes by more than 10^3, permitting direct structural analysis of the superconducting ground state. Scattering from thin films of La(2)CuO(4+x) (Tc = 39 K) at T=(50 +/- 5) K on the reciprocal space intervals (0,0,0.21) -> (0,0,1.21) and (0,0,0.6) -> (0.3,0,0.6) show a rounding of the carrier density near the substrate suggestive of a depletion zone or similar effect. The structure factor for off-specular scattering was less than 3x10-7 e, suggesting an absence of in-plane hole ordering in this material.

cond-mat.supr-con↗

Nonlinear I-V, High Flux-Flow Velocity Instability and Evidence for Quantum Fluctuations in BSCCO Superconducting Films

The large flux-flow velocity behavior of the high temperature superconductor BSCCO in the mixed state is studied by measurement of the current-voltage characteristic as a function of temperature and magnetic field direction. We find strong evidence for vortex-antivortex pairs that are excited by quantum fluctuations and contribute to the dissipation when dissociated by a large current.

cond-mat.supr-con↗

Optical dichroism in nanotubes

Utilizing the line-group symmetry of single-wall nanotubes, we have assigned their electron-energy bands by the symmetry-based quantum numbers. The selection rules for optical absorption are presented in terms of these quantum numbers. Different interband transitions become allowed as the polarization of incident light is varied, and we predict a substantial optical dichroism. We propose how to observe this effect in experiments on a single nanotube, and how it can be used to control quantum transport in nanotubes to obtain information about the structure.

cond-mat.soft↗

Low Temperature AC Conductivity in BSCCO (2212)

We report measurements of anamolously large dissipative conductivities in BiSrCaCuO(2212) at low temperatures. We have measured the complex conductivity of BSCCO thin films at 100-600 GHz as a function of doping from the underdoped to the overdoped state. At low temperatures there exists a residual dissipative conductivity which scales with the T=0 superfluid density as the doping is varied. This residual dissipative conductivity is larger than the possible contribution from a thermal population of quasiparticles at the d-wave gap nodes.

cond-mat.supr-con↗

Vanishing of phase coherence in underdoped Bi_2Sr_2CaCu_2O_8+d

Coherent time-domain spectroscopy is used to measure the screening and dissipation of high-frequency electromagnetic fields in a set of underdoped Bi_2Sr_2CaCu_2O_8+d thin films. The measurements provide direct evidence for a phase-fluctuation driven transition from the superconductor to normal state, with dynamics described well by the Berezinskii-Kosterlitz-Thouless theory of vortex-pair unbinding.

cond-mat.supr-con↗

Photoemission Evidence for a Remnant Fermi Surface and d-Wave-Like Dispersion in Insulating Ca2CuO2Cl2

An angle resolved photoemission study on Ca2CuO2Cl2, a parent compound of high Tc superconductors is reported. Analysis of the electron occupation probability, n(k) from the spectra shows a steep drop in spectral intensity across a contour that is close to the Fermi surface predicted by the band calculation. This analysis reveals a Fermi surface remnant even though Ca2CuO2Cl2 is a Mott insulator. The lowest energy peak exhibits a dispersion with approximately the |cos(kxa)-cos(kya)| form along this remnant Fermi surface. Together with the data from Dy doped Bi2Sr2CaCu2O(8 + delta) these results suggest that this d-wave like dispersion of the insulator is the underlying reason for the pseudo gap in the underdoped regime.

cond-mat.supr-con↗

Anomalous superconducting state gap size versus Tc behavior in underdoped Bi_2Sr_2Ca_1-xDy_xCu_2O_8+d

We report angle-resolved photoemission spectroscopy measurements of the excitation gap in underdoped superconducting thin films of Bi_2Sr_2Ca_{1-x}Dy_xCu_2O_{8+d}. As Tc is reduced by a factor of 2 by underdoping, the superconducting state gap Δdoes not fall proportionally, but instead stays constant or increases slightly, in violation of the BCS mean-field theory result. The different doping dependences of Δand kT_c indicate that they represent different energy scales. The measurements also show that Δis highly anisotropic and consistent with a d_{x^2-y^2} order parameter, as in previous studies of samples with higher dopings. However, in these underdoped samples, the anisotropic gap persists well above T_c. The existence of a normal state gap is related to the failure of Δto scale with T_c in theoretical models that predict pairing without phase coherence above T_c.

cond-mat.supr-con↗

Transmission Electron Study of Heteroepitaxial Growth in the BiSrCaCuO System

Films of Bi$\rm _2$Sr$\rm _2$CaCu$\rm _2$O$\rm _8$ and Bi$\rm _2$Sr$\rm _2$CuO$\rm _6$ have been grown using Atomic-Layer-by-Layer Molecular Beam Epitaxy (ALL-MBE) on lattice-matched substrates. These materials have been combined with layers of closely-related metastable compounds like Bi$\rm _2$Sr$\rm _2$Ca$\rm _7$Cu$\rm _8$O$\rm _{20}$ (2278) and rare-earth-doped compounds like Bi$\rm _2$Sr$\rm _2$Dy$\rm _x$Ca$\rm _{1-x}$Cu$\rm _2$O$\rm _8$ (Dy:2212) to form heterostructures with unique superconducting properties, including superconductor/insulator multilayers and tunnel junctions. Transmission electron microscopy (TEM) has been used to study the morphology and microstructure of these heterostructures. These TEM studies shed light on the physical properties of the films, and give insight into the growth mode of highly anisotropic solids like Bi$\rm _2$Sr$\rm _2$CaCu$\rm _2$O$\rm _8$.

cond-mat↗