arXiv subjects

I. Chiorescu

Publications and source records attributed to I. Chiorescu.

At least 37 records · Page 2Linked to original sources

arXiv2010

Magnetic strong coupling in a spin-photon system and transition to classical regime

We study the energy level structure of the Tavis-Cumming model applied to an ensemble of independent magnetic spins $s=1/2$ coupled to a variable number of photons. Rabi splittings are calculated and their distribution is analyzed as a functin of photon number $n_{\rm max}$ and spin system size $N$. A sharp transition in the distribution of the Rabi frequency is found at $n_{\rm max}\approx N$. The width of the Rabi frequency spectrum diverges as $\sqrt{N}$ at this point. For increased number of photons $n_{\rm max}>N$, the Rabi frequencies converge to a value proportional to $\sqrt{n_{\rm max}}$. This behavior is interpreted as analogous to the classical spin resonance mechanism where the photon is treated as a classical field and one resonance peak is expected. We also present experimental data demonstrating cooperative, magnetic strong coupling between a spin system and photons, measured at room temperature. This points towards quantum computing implementation with magnetic spins, using cavity quantum-electrodynamics techniques.

cond-mat.mes-hall↗

arXiv2010

Measurement of the nonlinear Meissner effect in superconducting Nb films using a resonant microwave cavity: A probe of unconventional pairing symmetries

We report observation of the nonlinear Meissner effect (NLME) in Nb films by measuring the resonance frequency of a planar superconducting cavity as a function of the magnitude and the orientation of a parallel magnetic field. Use of low power rf probing in films thinner than the London penetration depth, significantly increases the field for the vortex penetration onset and enables NLME detection under true equilibrium conditions. The data agree very well with calculations based on the Usadel equations. We propose to use NLME angular spectroscopy to probe unconventional pairing symmetries in superconductors.

cond-mat.supr-con↗

arXiv2009

Coherent spin rotation in the presence of a phonon-bottleneck effect

A characteristic of spin reversal in the presence of phonon-bottleneck is the deviation of the magnetization cycle from a reversible function into an opened hysterezis cycle. In recent experiments on molecular magnets (e.g. V$_{15}$ and Ru$_2$), the zero-field level repulsion was sufficiently large to ensure an otherwise adiabatic passage through zero-field and the magnetization curves can be described by using only a phonon-bottleneck model. Here, we generalize the phonon-bottleneck model into a model able to blend the non-adiabatic dynamics of spins with the presence of a non-equilibrium phonon bath. In this simple phenomenological model, Bloch equations are written in the eigenbasis of the effective spin Hamiltonian, considered to be a two-level system at low temperatures. The relaxation term is given by the phonon-bottleneck mechanism. To the expense of calculus time, the method can be generalized to multi-level systems, where the notion of Bloch sphere does not apply but the density matrix formalism is still applicable.

cond-mat.mes-hall↗

arXiv2009

Entrapment of magnetic micro-crystals for on-chip electron spin resonance studies

On-chip Electron Spin Resonance (ESR) of magnetic molecules requires the ability to precisely position nanosized samples in antinodes of the electro-magnetic field for maximal magnetic interaction. A method is developed to entrap micro-crystals containing spins in a well defined location on a substrate's surface. Traditional cavity ESR measurements are then performed on a mesoscopic crystal at 34 GHz. Polycrystalline diluted Cr$^{5+}$ spins were entrapped as well and measured while approaching the lower limit of the ESR sensitivity. This method suggests the feasibility of on-chip ESR measurements at dilution refrigerator temperatures by enabling the positioning of samples atop an on-chip superconducting cavity.

cond-mat.mes-hall↗

arXiv2009

Multiphoton coherent manipulation in large-spin qubits

Large spin Mn2+ ions (S=5/2) diluted in a non-magnetic MgO matrix of high crystalline symmetry are used to realize a six level system that can be operated by means of multi-photon coherent Rabi oscillations. This spin system has a very small anisotropy which can be tuned in-situ to reversibly transform the system between harmonic and non-harmonic level configurations. Decoherence effects are strongly suppressed as a result of the quasi-isotropic electron interaction with the crystal field and with the 55Mn nuclear spins. These results suggest new ways of manipulating, reading and resetting spin quantum states which can be applied to encode a qubit across several quantum levels.

cond-mat.mes-hall↗

arXiv2007

Coherent manipulation of electron spins up to ambient temperatures in Cr$^{5+}$(S=1/2) doped K$_3$NbO$_8$

We report coherent spin manipulation on Cr$^{5+}$ (\emph{S} = 1/2, \emph{I} = 0) doped K$_3$NbO$_8$, which constitutes a dilute two-level model relevant for use as a spin qubit. Rabi oscillations are observed for the first time in a spin system based on transition metal oxides up to room temperature. At liquid helium temperature the phase coherence relaxation time \emph{$T_2$} reaches $\sim 10$ $μ$s and, with a Rabi frequency of 20 MHz, yields a single qubit figure of merit \emph{$Q_M$} of about 500. This shows that a diluted ensemble of Cr$^{5+}$ (\emph{S} = 1/2) doped K$_3$NbO$_8$ is a potential candidate for solid-state quantum information processing.

cond-mat.mes-hall↗

arXiv2006

Phonon-bottleneck enhanced magnetic hysteresis in a molecular paddle wheel complex of Ru$_2^{5+}$

The ruthenium based molecular magnet [Ru$_2$(D(3,5-Cl$_2$Ph)F)$_4$Cl(0.5H$_2$O)$\cdotp$C$_6$H$_{14}$] (hereafter Ru$_2$) behaves as a two-level system at sufficiently low temperatures. The authors performed spin detection by means of single-crystal measurements and obtained magnetic hysteresis loops around zero bias as a function of field sweeping rate. Compared to other molecular systems, Ru$_2$ presents an enhanced irreversibility as shown by ``valleys'' of negative differential susceptibility in the hysteresis curves. Simulations based on phonon bottleneck model are in good qualitative agreement and suggest an abrupt spin reversal combined with insufficient thermal coupling between sample and cryostat phonon bath.

cond-mat.mes-hall↗

arXiv2005

Dephasing of a superconducting qubit induced by photon noise

We have studied the dephasing of a superconducting flux-qubit coupled to a DC-SQUID based oscillator. By varying the bias conditions of both circuits we were able to tune their effective coupling strength. This allowed us to measure the effect of such a controllable and well-characterized environment on the qubit coherence. We can quantitatively account for our data with a simple model in which thermal fluctuations of the photon number in the oscillator are the limiting factor. In particular, we observe a strong reduction of the dephasing rate whenever the coupling is tuned to zero. At the optimal point we find a large spin-echo decay time of $4 μs$.

cond-mat.mes-hall↗

arXiv2005

Dephasing of a flux-qubit coupled to a harmonic oscillator

Decoherence in superconducting qubits is known to arise because of a variety of environmental degrees of freedom. In this article, we focus on the influence of thermal fluctuations in a weakly damped circuit resonance coupled to the qubit. Because of the coupling, the qubit frequency is shifted by an amount $n δν_0$ if the resonator contains $n$ energy quanta. Thermal fluctuations induce temporal variations $n(t)$ and thus dephasing. We give an approximate formula for the qubit dephasing time as a function of $δν_0$. We discuss the specific case of a flux-qubit coupled to the plasma mode of its DC-SQUID detector. We first derive a plasma mode-qubit interaction hamiltonian which, in addition to the usual Jaynes-Cummings term, has a coupling term quadratic in the oscillator variables coming from the flux-dependence of the SQUID Josephson inductance. Our model predicts that $δν_0$ cancels in certain non-trivial bias conditions for which dephasing due to thermal fluctuations should be suppressed.

cond-mat.mes-hall↗

arXiv2005

Asymmetry and decoherence in a double-layer persistent-current qubit

Superconducting circuits fabricated using the widely used shadow evaporation technique can contain unintended junctions which change their quantum dynamics. We discuss a superconducting flux qubit design that exploits the symmetries of a circuit to protect the qubit from unwanted coupling to the noisy environment, in which the unintended junctions can spoil the quantum coherence. We present a theoretical model based on a recently developed circuit theory for superconducting qubits and calculate relaxation and decoherence times that can be compared with existing experiments. Furthermore, the coupling of the qubit to a circuit resonance (plasmon mode) is explained in terms of the asymmetry of the circuit. Finally, possibilities for prolonging the relaxation and decoherence times of the studied superconducting qubit are proposed on the basis of the obtained results.

cond-mat.supr-con↗

arXiv2004

Relaxation and Dephasing in a Flux-qubit

We report detailed measurements of the relaxation and dephasing time in a flux-qubit measured by a switching DC SQUID. We studied their dependence on the two important circuit bias parameters: the externally applied magnetic flux and the bias current through the SQUID in two samples. We demonstrate two complementary strategies to protect the qubit from these decoherence sources. One consists in biasing the qubit so that its resonance frequency is stationary with respect to the control parameters ({\it optimal point}) ; the second consists in {\it decoupling} the qubit from current noise by chosing a proper bias current through the SQUID. At the decoupled optimal point, we measured long spin-echo decay times of up to $4 μs$.

cond-mat.mes-hall↗

arXiv2004

Coherent dynamics of a flux qubit coupled to a harmonic oscillator

In the emerging field of quantum computation and quantum information, superconducting devices are promising candidates for the implementation of solid-state quantum bits or qubits. Single-qubit operations, direct coupling between two qubits, and the realization of a quantum gate have been reported. However, complex manipulation of entangled states - such as the coupling of a two-level system to a quantum harmonic oscillator, as demonstrated in ion/atom-trap experiments or cavity quantum electrodynamics - has yet to be achieved for superconducting devices. Here we demonstrate entanglement between a superconducting flux qubit (a two-level system) and a superconducting quantum interference device (SQUID). The latter provides the measurement system for detecting the quantum states; it is also an effective inductance that, in parallel with an external shunt capacitance, acts as a harmonic oscillator. We achieve generation and control of the entangled state by performing microwave spectroscopy and detecting the resultant Rabi oscillations of the coupled system.

cond-mat.mes-hall↗

arXiv2004

Detection of a persistent-current qubit by resonant activation

We present the implementation of a new scheme to detect the quantum state of a persistent-current qubit. It relies on the dependency of the measuring Superconducting Quantum Interference Device (SQUID) plasma frequency on the qubit state, which we detect by resonant activation. With a measurement pulse of only 5ns, we observed Rabi oscillations with high visibility (65%).

cond-mat.mes-hall↗

arXiv2003

Coherent Quantum Dynamics of a Superconducting Flux Qubit

We have observed coherent time evolution between two quantum states of a superconducting flux qubit comprising three Josephson junctions in a loop. The superposition of the two states carrying opposite macroscopic persistent currents is manipulated by resonant microwave pulses. Readout by means of switching-event measurement with an attached superconducting quantum interference device revealed quantum-state oscillations with high fidelity. Under strong microwave driving it was possible to induce hundreds of coherent oscillations. Pulsed operations on this first sample yielded a relaxation time of 900 nanoseconds and a free-induction dephasing time of 20 nanoseconds. These results are promising for future solid-state quantum computing.

cond-mat.mes-hall↗

arXiv2002

Adiabatic Landau-Zener-Stückelberg transition with or without dissipation in low spin molecular system V15

The spin one half molecular system V15 shows no barrier against spin reversal. This makes possible direct phonon activation between the two levels. By tuning the field sweeping rate and the thermal coupling between sample and thermal reservoir we have control over the phonon-bottleneck phenomena previously reported in this system. We demonstrate adiabatic motion of molecule spins in time dependent magnetic fields and with different thermal coupling to the cryostat bath. We also discuss the origin of the zero-field tunneling splitting for a half-integer spin.

cond-mat.mes-hall↗

arXiv2002

The V15 molecule, a multi-spin two-level system: adiabatic LZS transition with or without dissipation and Kramers theorem

The so-called V15 molecule is formed of 15 spins 1/2 antiferromagnetically coupled. The resultant spin is equal to 1/2. Contrary to what is expected at first sight, this half-integer spin is gapped. We show that this is a consequence of the multi-spin character of the molecule. Time reversal symmetry (Kramers theorem) is preserved due to the existence of a groundstate degeneracy larger than 2. Magnetization experiments have been performed at different temperatures, sweeping-field rates and couplings with the cryostat. Their interpretation in terms of the Landau-Zener-Stuckelberg model gives evidence for adiabatic LZS spin reversal with and without dissipation.

cond-mat.mes-hall↗

arXiv2000

Phonon-assisted tunneling in the quantum regime of Mn12-ac

Longitudinal or transverse magnetic fields applied on a crystal of Mn12-ac allows to observe independent tunnel transitions between m=-S+p and m=S-n-p (n=6-10, p=0-2 in longitudinal field and n=p=0 in transverse field). We observe a smooth transition (in longitudinal) from coherent ground-state to thermally activated tunneling. Furthermore two ground-state relaxation regimes showing a crossover between quantum spin relaxation far from equilibrium and near equilibrium, when the environment destroys multimolecule correlations. Finally, we stress that the complete Hamiltonian of Mn12 should contain odd spin operators of low order.

cond-mat.mes-hall↗

arXiv2000

Mesoscopic Spin Tunneling in Molecular Crystals

The phenomenon of Quantum Tunneling of Mesoscopic Spins is reviewed in the light of the behavior of the archetype of these systems: the molecular complex Mn12-ac. Most observations can be understood in the framework of the reduced Hilbert space dimension 2S+1=21. Due to the large spin S=10, the energy barrier preventing spin rotation is large, and as a consequence, quantum relaxation is very slow. The application of a magnetic field of a few Tesla below 1 K allows to observe tunneling (i) between the states m=-10 and m=10-n with n=8 to 11 if the field is longitudinal, or (ii) between the two ground-states m~-10 and m~10 if the field is transverse. The crossover temperature between ground-state and thermally assisted tunneling in a longitudinal field extrapolates in zero field at ~1.7 K. The observation of square root relaxation at short-times/low-temperatures and of exponential relaxation at long-times/high-temperatures, as observed previously above 1.5 K, confirms the important role of the spin bath dynamics which is out of equilibrium in the first regime and at equilibrium in the second one. In a second part of this paper a new molecule, so-called V15, with resultant spin S=1/2 is investigated. Contrary to high spin molecules, the energy barrier of low spin molecules is small or null, and the splitting between the symmetrical and anti-symmetrical states is sufficiently large to allow spin-phonon transitions during spin rotation. In low spin molecules the coupling to the environment is quite different from the one found in large spin molecules in low fields.

cond-mat.mes-hall↗