arXiv subjects

I. Dillmann

Publications and source records attributed to I. Dillmann.

At least 37 records · Page 2Linked to original sources

arXiv2023

Measurement of the Isolated Nuclear Two-Photon Decay in $^{72}\mathrm{Ge}$

The nuclear two-photon or double-gamma ($2γ$) decay is a second-order electromagnetic process whereby a nucleus in an excited state emits two gamma rays simultaneously. To be able to directly measure the $2γ$ decay rate in the low-energy regime below the electron-positron pair-creation threshold, we combined the isochronous mode of a storage ring with Schottky resonant cavities. The newly developed technique can be applied to isomers with excitation energies down to $\sim100$\,keV and half-lives as short as $\sim10$\,ms. The half-life for the $2γ$ decay of the first-excited $0^+$ state in bare $^{72}\mathrm{Ge}$ ions was determined to be $23.9\left(6\right)$\,ms, which strongly deviates from expectations.

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arXiv2023

Storage, Accumulation and Deceleration of Secondary Beams for Nuclear Astrophysics

Low-energy investigations on rare ion beams are often limited by the available intensity and purity of the ion species in focus. Here, we present the first application of a technique that combines in-flight production at relativistic energies with subsequent secondary beam storage, accumulation and finally deceleration to the energy of interest. Using the FRS and ESR facilities at GSI, this scheme was pioneered to provide a secondary beam of $^{118}$Te$^{52+}$ for the measurement of nuclear proton-capture at energies of 6 and 7 MeV/u. The technique provided stored beam intensities of about $10^6$ ions at high purity and brilliance, representing a major step towards low-energy nuclear physics studies using rare ion beams.

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arXiv2023

Decay Spectroscopy of $^{160}$Eu: Quasiparticle Configurations of Excited States and Structure of $K^π$=$4^+$ Band-heads in $^{160}$Gd

\noindent \textbf{Background:} Detailed spectroscopy of neutron-rich, heavy, deformed nuclei is of broad interest for nuclear astrophysics and nuclear structure. Nuclei in the r-process path and following freeze-out region impact the resulting r-process abundance distribution, and the structure of nuclei midshell in both proton and neutron number helps to understand the evolution of subshell gaps and large deformation in these nuclei. \noindent \textbf{Purpose:} To improve the understanding of the nuclear structure of $^{160}$Gd, specifically the $K^π$=$4^+$ bands, as well as study the $β$-decay of $^{160}$Eu into $^{160}$Gd. \noindent \textbf{Methods:} High-statistics decay spectroscopy of $^{160}$Gd resulting from the $β$-decay of $^{160}$Eu was collected using the GRIFFIN spectrometer at the TRIUMF-ISAC facility. \noindent \textbf{Results:} Two new excited states and ten new transitions were observed in $^{160}$Gd. The $β$-decaying half-lives of the low- and high-spin isomer in $^{160}$Eu were determined, and the low-spin state's half-life was measured to be $t_{1/2}=26.0(8)$~s, $\sim$16\% shorter than previous measurements. Lifetimes of the two $K^π$=$4^+$ band-heads in $^{160}$Gd were measured for the first time, as well as $γ$-$γ$ angular correlations and mixing ratios of intense transitions out of those band-heads. \noindent \textbf{Conclusions:} Lifetimes and mixing ratios suggest that the hexadecapole phonon model of the $K^π$=$4^+$ band-heads in $^{160}$Gd is preferred over a simple two-state strong mixing scenario, although further theoretical calculations are needed to fully understand these states. Additionally, the 1999.0 keV state in $^{160}$Gd heavily populated in $β$-decay is shown to have positive parity, which raises questions regarding the structure of the high-spin $β$-decaying state in $^{160}$Eu.

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arXiv2023

First Evidence of Axial Shape Asymmetry and Configuration Coexistence in $^{74}$Zn: Suggestion for a Northern Extension of the $N=40$ Island of Inversion

The excited states of $N=44$ $^{74}$Zn were investigated via $γ$-ray spectroscopy following $^{74}$Cu $β$ decay. By exploiting $γ$-$γ$ angular correlation analysis, the $2_2^+$, $3_1^+$, $0_2^+$ and $2_3^+$ states in $^{74}$Zn were firmly established. The $γ$-ray branching and $E2/M1$ mixing ratios for transitions de-exciting the $2_2^+$, $3_1^+$ and $2_3^+$ states were measured, allowing for the extraction of relative $B(E2)$ values. In particular, the $2_3^+ \to 0_2^+$ and $2_3^+ \to 4_1^+$ transitions were observed for the first time. The results show excellent agreement with new microscopic large-scale shell-model calculations, and are discussed in terms of underlying shapes, as well as the role of neutron excitations across the $N=40$ gap. Enhanced axial shape asymmetry (triaxiality) is suggested to characterize $^{74}$Zn in its ground state. Furthermore, an excited $K=0$ band with a significantly larger softness in its shape is identified. A shore of the $N=40$ ``island of inversion'' appears to manifest above $Z=26$, previously thought as its northern limit in the chart of the nuclides.

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arXiv2022

Collision-Induced Dissociation at TRIUMF's Ion Trap for Atomic and Nuclear science

The performance of high-precision mass spectrometry of radioactive isotopes can often be hindered by large amounts of contamination, including molecular species, stemming from the production of the radioactive beam. In this paper, we report on the development of Collision-Induced Dissociation (CID) as a means of background reduction for experiments at TRIUMF's Ion Trap for Atomic and Nuclear science (TITAN). This study was conducted to characterize the quality and purity of radioactive ion beams and the reduction of molecular contaminants to allow for mass measurements of radioactive isotopes to be done further from nuclear stability. This is the first demonstration of CID at an ISOL-type radioactive ion beam facility, and it is shown that molecular contamination can be reduced up to an order of magnitude.

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arXiv2022

Proton distribution radii of $^{16-24}$O: signatures of new shell closures and neutron skin

The root mean square radii of the proton density distribution in $^{16-24}$O derived from measurements of charge changing cross sections with a carbon target at $\sim$900$A$ MeV together with the matter radii portray thick neutron skin for $^{22 - 24}$O despite $^{22,24}$O being doubly magic. Imprints of the shell closures at $N$ = 14 and 16 are reflected in local minima of their proton radii that provide evidence for the tensor interaction causing them. The radii agree with it ab initio calculations employing the chiral NNLO$_{\mathrm{sat}}$ interaction, though skin thickness predictions are challenged. Shell model predictions agree well with the data.

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arXiv2022

Long-term evolution of the neutron rate at the Canfranc Underground Laboratory

We report results on the long-term variation of the neutron counting rate at the Canfranc Underground Laboratory, of importance for several low-background experiments installed there, including rare-event searches. The measurement campaign was performed employing the High Efficiency Neutron Spectrometry Array (HENSA) mounted in Hall A and lasted 412 live days. The present study is the first long-term measurement of the neutron rate with sensitivity over a wide range of neutron energies (from thermal up to 0.1 GeV and beyond) performed in any underground laboratory so far. Data on the environmental variables inside the experimental hall (radon concentration, air temperature, air pressure and humidity) were also acquired during all the measurement campaign. We have investigated for the first time the evolution of the neutron rate for different energies of the neutrons and its correlation with the ambient variables.

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arXiv2022

Horizons: Nuclear Astrophysics in the 2020s and Beyond

Nuclear Astrophysics is a field at the intersection of nuclear physics and astrophysics, which seeks to understand the nuclear engines of astronomical objects and the origin of the chemical elements. This white paper summarizes progress and status of the field, the new open questions that have emerged, and the tremendous scientific opportunities that have opened up with major advances in capabilities across an ever growing number of disciplines and subfields that need to be integrated. We take a holistic view of the field discussing the unique challenges and opportunities in nuclear astrophysics in regards to science, diversity, education, and the interdisciplinarity and breadth of the field. Clearly nuclear astrophysics is a dynamic field with a bright future that is entering a new era of discovery opportunities.

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arXiv2021

Mass measurements of $^{60-63}$Ga reduce x-ray burst model uncertainties and extend the evaluated $T=1$ isobaric multiplet mass equation

We report precision mass measurements of neutron-deficient gallium isotopes approaching the proton drip line. The measurements of $^{60-63}$Ga performed with the TITAN multiple-reflection time-of-flight mass spectrometer provide a more than threefold improvement over the current literature mass uncertainty of $^{61}$Ga and mark the first direct mass measurement of $^{60}$Ga. The improved precision of the $^{61}$Ga mass has important implications for the astrophysical rp process, as it constrains essential reaction Q-values near the $^{60}$Zn waiting point. Based on calculations with a one-zone model, we demonstrate the impact of the improved mass data on prediction uncertainties of X-ray burst models. The first-time measurement of the $^{60}$Ga ground-state mass establishes the proton-bound nature of this nuclide; thus, constraining the location of the proton drip line along this isotopic chain. Including the measured mass of $^{60}$Ga further enables us to extend the evaluated $T=1$ isobaric multiplet mass equation up to $A=60$.

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arXiv2021

Measurement of the neutron flux at the Canfranc Underground Laboratory with HENSA

We have performed a long-term measurement of the neutron flux with the High Efficiency Neutron Spectrometry Array HENSA in the Hall A of the Canfranc Underground Laboratory. The Hall A measurement campaign lasted from October 2019 to March 2021, demonstrating an excellent stability of the HENSA setup. Preliminary results on the neutron flux from this campaign are presented for the first time. In Phase 1 (113 live days) a total neutron flux of 1.66(2) $\times$10$^{-5}$ cm$^{-2}$ s$^{-1}$ is obtained. Our results are in good agreement with those from our previous shorter measurement where a reduced experimental setup was employed.

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arXiv2021

$^{145}$Ba and $^{145, 146}$La structure from lifetime measurements

The occurrence of octupole shapes in even-mass neutron-rich Ba isotopes has been well established. However, the situation with the odd-mass Ba and odd or odd-odd La nuclei around them is far from settled. In order to shed light on these less-studied isotopes, a fast-timing experiment was performed using GRIFFIN at TRIUMF-ISAC. A wealth of excited-state lifetimes in the 100~ps to few ns range have been measured in $^{144, 145, 146}$Ba and $^{145,146}$La populated in the $β^-$ and $β^--n$ decay of $^{145,146}$Cs. The results do not allow to draw firm conclusions on the possible octupole deformation of these nuclei but suggest different spin and parity assignments than previous works. This work highlights the need for more detailed study of the odd and odd-odd isotopes in this region to properly understand their structure.

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arXiv2021

Development of a Reference Database for Beta-Delayed Neutron Emission

Beta-delayed neutron emission is important for nuclear structure and astrophysics as well as for reactor applications. Significant advances in nuclear experimental techniques in the past two decades have led to a wealth of new measurements that remain to be incorporated in the databases. We report on a coordinated effort to compile and evaluate all the available beta-delayed neutron emission data. The different measurement techniques have been assessed and the data have been compared with semi-microscopic and microscopic-macroscopic models. The new microscopic database has been tested against aggregate total delayed neutron yields, time-dependent group parameters in 6-and 8-group re-presentation, and aggregate delayed neutron spectra. New recommendations of macroscopic delayed-neutron data for fissile materials of interest to applications are also presented. The new Reference Database for Beta-Delayed Neutron Emission Data is available online at: http://www-nds.iaea.org/beta-delayed-neutron/database.html.

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arXiv2021

Nuclear matter distributions in the neutron-rich carbon isotopes $^{14-17}$C from intermediate-energy proton elastic scattering in inverse kinematics

The absolute differential cross sections for small-angle proton elastic scattering off the nuclei $^{12,14-17}$C have been measured in inverse kinematics at energies near 700 MeV/u at GSI Darmstadt. The hydrogen-filled ionization chamber IKAR served simultaneously as a gas target and a detector for the recoil protons. The projectile scattering angles were measured with multi-wire tracking detectors. The radial nuclear matter density distributions and the root-mean-square nuclear matter radii were deduced from the measured cross sections using the Glauber multiple-scattering theory. A possible neutron halo structure in $^{15}$C, $^{16}$C and $^{17}$C is discussed. The obtained data show evidence for a halo structure in the $^{15}$C nucleus.

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arXiv2020

High-Precision Branching Ratio Measurement and Spin Assignment Implications for $^{62}$Ga Superallowed $β$ Decay

A high-precision branching ratio measurement for the superallowed Fermi $β^{+}$ emitter $^{62}$Ga was performed with the Gamma-Ray Infrastructure for Fundamental Investigations of Nuclei (GRIFFIN) spectrometer at the Isotope Separator and Accelerator (ISAC) radioactive ion beam facility at TRIUMF. The high efficiency of the GRIFFIN spectrometer allowed 63 $γ$-ray transitions, with intensities down to $\approx$1 part per million (ppm) per $^{62}$Ga $β^{+}$ decay, to be placed in the level scheme of the daughter nucleus $^{62}$Zn, establishing the superallowed $β$ branching ratio for $^{62}$Ga decay to be 99.8577$^{+0.0023}_{-0.0029}\%$, a factor of 4 more precise than the previous world average. For several cascades, $γ-γ$ angular correlation measurements were performed to assign spins and/or determine the mixing ratios of transitions. In particular, the spin of the 2.342 MeV excited state in the daughter nucleus $^{62}$Zn was definitively assigned as $J = 0$. This assignment resolves a discrepancy between previous measurements and has important implications for the isospin symmetry breaking correction, $δ_{C1}$, in $^{62}$Ga superallowed Fermi $β$ decay.

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arXiv2020

Absence of Low-Energy Shape Coexistence in $^{80}$Ge: The Nonobservation of a Proposed Excited 0$_2^+$ Level at 639 keV

The $^{80}$Ge structure was investigated in a high-statistics $β$-decay experiment of $^{80}$Ga using the GRIFFIN spectrometer at TRIUMF-ISAC through $γ$, $β$-$e$, $e$-$γ$ and $γ$-$γ$ spectroscopy. No evidence was found for the recently reported 0$_2^{+}$ 639-keV level suggested as evidence for low-energy shape coexistence in $^{80}$Ge. Large-scale shell model calculations performed in $^{78,80,82}$Ge place the $0^{+}_{2}$ level in $^{80}$Ge at 2\,MeV. The new experimental evidence combined with shell model predictions indicate that low-energy shape coexistence is not present in $^{80}$Ge.

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arXiv2020

Probing the Z = 6 spin-orbit shell gap with (p,2p) quasi-free scattering reactions

The evolution of the traditional nuclear magic numbers away from the valley of stability is an active field of research. Experimental efforts focus on providing key spectroscopic information that will shed light into the structure of exotic nuclei and understanding the driving mechanism behind the shell evolution. In this work, we investigate the Z = 6 spin-orbit shell gap towards the neutron dripline. To do so, we employed $^{A}$N(p,2p)$^{A-1}$C quasi-free scattering reactions to measure the proton component of the 2$^+_1$ state of $^{16,18,20}$C. The experimental findings support the notion of a moderate reduction of the proton 1p$_{1/2}$-1p$_{3/2}$ spin-orbit splitting, at variance to recent claims for a prevalent Z = 6 magic number towards the neutron dripline.

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arXiv2020

Decay Spectroscopy of $^{129}$Cd

Excited states of $^{129}$In populated following the $β$-decay of $^{129}$Cd were experimentally studied with the GRIFFIN spectrometer at the ISAC facility of TRIUMF, Canada. A 480-MeV proton beam was impinged on a uranium carbide target and $^{129}$Cd was extracted using the Ion Guide Laser Ion Source (IG-LIS). $β$- and $γ$-rays following the decay of $^{129}$Cd were detected with the GRIFFIN spectrometer comprising the plastic scintillator SCEPTAR and 16 high-purity germanium (HPGe) clover-type detectors. %, along with the $β$-particles were detected with SCEPTAR. From the $β$-$γ$-$γ$ coincidence analysis, 32 new transitions and 7 new excited states were established, expanding the previously known level scheme of $^{129}$In. The $\log ft$ values deduced from the $β$-feeding intensities suggest that some of the high-lying states were populated by the $ν0 g_{7/2} \rightarrow π0 g_{9/2}$ allowed Gamow-Teller (GT) transition, which indicates that the allowed GT transition is more dominant in the $^{129}$Cd decay than previously reported. Observation of fragmented Gamow-Teller strengths is consistent with theoretical calculations.

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arXiv2020

Neutron flux and spectrum in the Dresden Felsenkeller underground facility studied by moderated $^3$He counters

Ambient neutrons may cause significant background for underground experiments. Therefore, it is necessary to investigate their flux and energy spectrum in order to devise a proper shielding. Here, two sets of altogether ten moderated $^3$He neutron counters are used for a detailed study of the ambient neutron background in tunnel IV of the Felsenkeller facility, underground below 45 meters of rock in Dresden/Germany. One of the moderators is lined with lead and thus sensitive to neutrons of energies higher than 10 MeV. For each $^3$He counter-moderator assembly, the energy dependent neutron sensitivity was calculated with the FLUKA code. The count rates of the ten detectors were then fitted with the MAXED and GRAVEL packages. As a result, both the neutron energy spectrum from 10$^{-9}$ MeV to 300 MeV and the flux integrated over the same energy range were determined experimentally. The data show that at a given depth, both the flux and the spectrum vary significantly depending on local conditions. Energy integrated fluxes of $(0.61 \pm 0.05)$, $(1.96 \pm 0.15)$, and $(4.6 \pm 0.4) \times 10^{-4}$ cm$^{-2}$ s$^{-1}$, respectively, are measured for three sites within Felsenkeller tunnel IV which have similar muon flux but different shielding wall configurations. The integrated neutron flux data and the obtained spectra for the three sites are matched reasonably well by FLUKA Monte Carlo calculations that are based on the known muon flux and composition of the measurement room walls.

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