arXiv subjects

I. Dillmann

Publications and source records attributed to I. Dillmann.

83 records · Page 5Linked to original sources

arXiv2009

Search for long-lived isomeric states in neutron-deficient thorium isotopes

The discovery of naturally occurring long-lived isomeric states (t_1/2 > 10^8 yr) in the neutron-deficient isotopes 211,213,217,218Th [A. Marinov et al., Phys. Rev. C 76, 021303(R) (2007)] was reexamined using accelerator mass spectrometry (AMS). Because AMS does not suffer from molecular isobaric background in the detection system, it is an extremely sensitive technique. Despite our up to two orders of magnitude higher sensitivity we cannot confirm the discoveries of neutron-deficient thorium isotopes and provide upper limits for their abundances.

nucl-ex↗

arXiv2009

Determination of the stellar (n,gamma) cross section of 40Ca with accelerator mass spectrometry

The stellar (n,gamma) cross section of 40Ca at kT=25 keV has been measured with a combination of the activation technique and accelerator mass spectrometry (AMS). This combination is required when direct off-line counting of the produced activity is compromised by the long half-life and/or missing gamma-ray transitions. The neutron activations were performed at the Karlsruhe Van de Graaff accelerator using the quasistellar neutron spectrum of kT=25 keV produced by the 7Li(p,n)7Be reaction. The subsequent AMS measurements were carried out at the Vienna Environmental Research Accelerator (VERA) with a 3 MV tandem accelerator. The doubly magic 40Ca is a bottle-neck isotope in incomplete silicon burning, and its neutron capture cross section determines the amount of leakage, thus impacting on the eventual production of iron group elements. Because of its high abundance, 40Ca can also play a secondary role as "neutron poison" for the s-process. Previous determinations of this value at stellar energies were based on time-of-flight measurements. Our method uses an independent approach, and yields for the Maxwellian-averaged cross section at kT=30 keV a value of 30 keV= 5.73+/-0.34 mb.

astro-ph.SR↗

arXiv2008

Cross section measurements of $α$-induced reactions on $^{92,94}$Mo and $^{112}$Sn for $p$-process studies

The $^{92}$Mo($α,n$)$^{95}$Ru, $^{94}$Mo($α,n$)$^{97}$Ru, and $^{112}$Sn($α,γ$)$^{116}$Te cross sections were measured at the upper end of the $p$-process Gamow window between 8.2 MeV and 11.1 MeV. Our results are slightly lower than global Hauser-Feshbach calculations from the code NON-SMOKER, but still within the uncertainty of the prediction. The $^{112}$Sn($α,γ$)$^{116}$Te cross section agrees well with a recently measured thick-target cross section in the same energy range. For the $^{92,94}$Mo($α,n$) reactions the present data close to the reaction thresholds could eliminate previous uncertainties within a factor of 20, and we can present now useful comparisons to statistical model calculations with different optical potentials.

astro-ph↗

arXiv2008

Present status of the KADoNiS database

The "Karlsruhe Astrophysical Database of Nucleosynthesis in Stars" (KADoNiS) project is an online database for experimental cross sections relevant to the $s$ process and $p$ process. It is available under \http://nuclear-astrophysics.fzk.de/kadonis and consists of two parts. Part 1 is an updated sequel to the well-known Bao et al. compilations from 1987 and 2000, which is online since April 2005. An extension of this $s$-process database to $(n,p)$ and $(n,α)$ cross sections at $kT$= 30 keV, as in the first version of the Bao compilation, is planned. The second part of KADoNiS is a $p$-process library, which includes all available experimental data from $(p,γ)$, $(p,n)$, $(α,γ)$, $(α,n)$, $(α,α)$, $(n,α)$ and $(γ,n)$ reactions in or close to the respective Gamow window. Despite the great number of reactions required for a $p$-process reaction network, experimental data is still scarce and up to now restricted to stable targets. Given here is a short overview about the present status of the KADoNiS database.

astro-ph↗

arXiv2008

First measurements of the total and partial stellar cross section to the $s$-process branching-point $^{79}$Se

Although $^{79}$Se represents an important branching in the weak s process, the stellar neutron capture cross sections to this isotope have not yet been measured experimentally. In this case, experimental data is essential for evaluating the important branching in the s-process reaction path at $^{79}$Se. The total cross section of $^{78}$Se at a stellar energy of kT = 25 keV has been investigated with a combination of the activation technique and accelerator mass spectrometry (AMS), since offline decay counting is prohibitive due to the long terrestrial half life of $^{79}$Se (2.80$\pm$0.36 $\times10^5$ y) as well as the absence of suitable $γ$-ray transitions. The preliminary result for the total Maxwellian averaged cross section is $<σ>_{30 keV}$= 60.1$\pm$9.6 mbarn, significantly lower than the previous recommended value. In a second measurement, also the partial cross section to the 3.92 min-isomer was determined via $γ$-spectroscopy and yielded $<σ>_{30 keV}$(part.)= 42.0$\pm$2.0 mbarn.

astro-ph↗

arXiv2008

New Stellar $(n,γ)$ Cross Sections and The "Karlsruhe Astrophysical Database of Nucleosynthesis in Stars"

Since April 2005 a regularly updated stellar neutron cross section compilation is available online at http://nuclear-astrophysics.fzk.de/kadonis. This online-database is called the "Karlsruhe Astrophysical Database of Nucleosynthesis in Stars" project and is based on the previous Bao et al. compilation from the year 2000. The present version \textsc{KADoNiS} v0.2 (January 2007) includes recommended cross sections for 280 isotopes between $^{1}$H and $^{210}$Po and 75 semi-empirical estimates for isotopes without experimental information. Concerning stellar $(n,γ)$ cross sections of the 32 stable, proton-rich isotopes produced by the $p$ process experimental information is only available for 20 isotopes, but 9 of them have rather large uncertainties of $\geq$9%. The first part of a systematic study of stellar $(n,γ)$ cross sections of the $p$-process isotopes $^{74}$Se, $^{84}$Sr, $^{102}$Pd, $^{120}$Te, $^{130}$Ba, $^{132}$Ba, $^{156}$Dy, and $^{174}$Hf is presented. In another application \textsc{KADoNiS} v0.2 was used for an modification of a reaction library of Basel university. With this modified library $p$-process network calculations were carried out and compared to previous results.

astro-ph↗

arXiv2008

Recent Efforts in Data Compilations for Nuclear Astrophysics

Some recent efforts in compiling data for astrophysical purposes are introduced, which were discussed during a JINA-CARINA Collaboration meeting on "Nuclear Physics Data Compilation for Nucleosynthesis Modeling" held at the ECT* in Trento/ Italy from May 29th- June 3rd, 2007. The main goal of this collaboration is to develop an updated and unified nuclear reaction database for modeling a wide variety of stellar nucleosynthesis scenarios. Presently a large number of different reaction libraries (REACLIB) are used by the astrophysics community. The "JINA Reaclib Database" on http://www.nscl.msu.edu/ñero/db/ aims to merge and fit the latest experimental stellar cross sections and reaction rate data of various compilations, e.g. NACRE and its extension for Big Bang nucleosynthesis, Caughlan and Fowler, Iliadis et al., and KADoNiS. The KADoNiS (Karlsruhe Astrophysical Database of Nucleosynthesis in Stars, http://nuclear-astrophysics.fzk.de/kadonis) project is an online database for neutron capture cross sections relevant to the s process. The present version v0.2 is already included in a REACLIB file from Basel university (http://download.nucastro.org/astro/reaclib). The present status of experimental stellar $(n,γ)$ cross sections in KADoNiS is shown. A "high priority list" for measurements and evaluations for light charged-particle reactions set up by the JINA-CARINA collaboration is presented. The central web access point to submit and evaluate new data is provided by the Oak Ridge group via the http://www.nucastrodata.org homepage. "Workflow tools" aim to make the evaluation process transparent and allow users to follow the progress.

astro-ph↗

arXiv2008

KADoNiS- The Karlsruhe Astrophysical Database of Nucleosynthesis in Stars

The "Karlsruhe Astrophysical Database of Nucleosynthesis in Stars" (KADoNiS) project is an online database for experimental cross sections relevant to the s process and p process. It is available under http://nuclear-astrophysics.fzk.de/kadonis and consists of two parts. Part 1 is an updated sequel to the previous Bao et al. compilations from 1987 and 2000 for (n,$γ$) cross sections relevant to the big bang and s-process nucleosynthesis. The second part will be an experimental p-process database, which is expected to be launched in winter 2005/06. The KADoNiS project started in April 2005, and a first partial update is online since August 2005. In this paper we present a short overview of the first update of the s-process database, as well as an overview of the status of stellar (n,$γ$) cross sections of all 32 p isotopes.

astro-ph↗

arXiv2008

$p$-Process simulations with a modified reaction library

We have performed $p$-process simulations with the most recent stellar $(n,γ)$ cross sections from the "Karlsruhe Astrophysical Database of Nucleosynthesis in Stars" project (version v0.2, http://nuclear-astrophysics.fzk.de/kadonis). The simulations were carried out with a parametrized supernova type II shock front model (``$γ$ process'') of a 25 solar mass star and compared to recently published results. A decrease in the normalized overproduction factor could be attributed to lower cross sections of a significant fraction of seed nuclei located in the Bi and Pb region around the $N$=126 shell closure.

astro-ph↗

arXiv2008

Experimental (n,$γ$) cross sections of the p-process nuclei $^{74}$Se and $^{84}$Sr

The nucleosynthesis of elements beyond iron is dominated by the s and r processes. However, a small amount of stable isotopes on the proton-rich side cannot be made by neutron capture and are thought to be produced by photodisintegration reactions on existing seed nuclei in the so-called "p process". So far most of the p-process reactions are not yet accessible by experimental techniques and have to be inferred from statistical Hauser-Feshbach model calculations. The parametrization of these models has to be constrained by measurements on stable proton-rich nuclei. A series of (n,$γ$) activation measurements, related by detailed balance to the respective photodisintegrations, were carried out at the Karlsruhe Van de Graaff accelerator using the $^7$Li(p,n)$^7$Be source for simulating a Maxwellian neutron distribution of kT= 25 keV. First results for the experimental (n,$γ$) cross sections of the light p nuclei $^{74}$Se and $^{84}$Sr are reported. These experimental values were used for an extrapolation to the Maxwellian averaged cross section at 30 keV, $<σ>_{30}$, yielding 271$\pm$15 mb for $^{74}$Se, and 300$\pm$17 mb for the total capture cross section of $^{84}$Sr. The partial cross section to the isomer in $^{85}$Sr was found to be 190$\pm$10 mb.

astro-ph↗

arXiv2008

(n,$γ$) Cross Sections of Light p Nuclei -- Towards an Updated Database for the p Process

The nucleosynthesis of elements beyond iron is dominated by the s and r processes. However, a small amount of stable isotopes on the proton-rich side cannot be made by neutron capture and are thought to be produced by photodisintegration reactions on existing seed nuclei in the so-called "p process". So far most of the p-process reactions are not yet accessible by experimental techniques and have to be inferred from statistical Hauser-Feshbach model calculations. The parametrization of these models has to be constrained by measurements on stable proton-rich nuclei. A series of (n,$γ$) activation measurements on p nuclei, related by detailed balance to the respective photodisintegrations, were carried out at the Karlsruhe Van de Graaff accelerator using the $^7$Li(p,n)$^7$Be source for simulating a Maxwellian neutron distribution of kT= 25 keV. We present here preliminary results of our extended measuring program in the mass range between A=74 and A=132, including first experimental (n,$γ$) cross sections of $^{74}$Se, $^{84}$Sr, $^{120}$Te and $^{132}$Ba, and an improved value for $^{130}$Ba. In all cases we find perfect agreement with the recommended MACS predictions from the Bao et al. compilation.

astro-ph↗