arXiv subjects

I. Favero

Publications and source records attributed to I. Favero.

17 recordsLinked to original sources

arXiv2024

Optomechanical micro-rheology of complex fluids at ultra-high frequency

We present an optomechanical method for locally measuring the rheological properties of complex fluids in the ultra-high frequency range (UHF). A mechanical disk of microscale volume is used as a small-amplitude oscillating probe that monitors the fluid at rest in thermal equilibrium, while the oscillation is detected by optomechanical transduction within a sub-millisecond measurement time, thanks to an optimized signal collection. An original analytical model for fluid-structure interactions is used to extract from these measurements the rheological properties of liquids over the frequency range 100 MHz - 1 GHz. This new micro-rheology method is calibrated by measurements on liquid water, in which we observe pronounced compressibility effects above 500 MHz, but which we show remains Newtonian all over the explored range. In contrast, measurements reveal that liquid 1-decanol exhibits a non-Newtonian behavior, with a frequency-dependent viscosity associated to several relaxation frequencies in the UHF. Our data agree well with an extended Maxwell model for the viscosity of this alcohol, involving two relaxation times of 797 and 151 picoseconds, which are respectively analyzed as supramolecular and intramolecular relaxation processes. A shear elastic response of the liquid appears at the highest frequencies, compatible with the entropic elasticity of molecules as they attempt to uncurl, and whose value enables estimating the volume of a single molecule of liquid. UHF optomechanical micro-rheology demonstrates here a direct mechanical access to the fast molecular dynamics at play in a liquid, in a quantitative manner and in a short time.

cond-mat.soft↗

arXiv2018

Brillouin Scattering in Hybrid Optophononic Bragg Micropillar Resonators at 300 GHz

We introduce a monolithic Brillouin generator based on a semiconductor micropillar cavity embedding a high frequency nanoacoustic resonator operating in the hundreds of GHz range. The concept of two nested resonators allows an independent design of the ultrahigh frequency Brillouin spectrum and of the optical device. We develop an optical free-space technique to characterize spontaneous Brillouin scattering in this monolithic device and propose a measurement protocol that maximizes the Brillouin generation efficiency in the presence of optically induced thermal effects. The compact and versatile Brillouin generator studied here could be readily integrated into fibered and on-chip architectures.

physics.optics↗

arXiv2018

On-chip III-V monolithic integration of heralded single photon sources and beamsplitters

We demonstrate a monolithic III-V photonic circuit combining a heralded single photon source with a beamsplitter, at room temperature and telecom wavelength. Pulsed parametric down-conversion in an AlGaAs waveguide generates counterpropagating photons, one of which is used to herald the injection of its twin into the beamsplitter. We use this configuration to implement an integrated Hanbury-Brown and Twiss experiment, yielding a heralded second-order correlation $g^{(2)}_{\rm her}(0)=0.10 \pm 0.02$ that confirms single-photon operation. The demonstrated generation and manipulation of quantum states on a single III-V semiconductor chip opens promising avenues towards real-world applications in quantum information.

quant-ph↗

arXiv2017

Nanomechanical resonators based on adiabatic periodicity-breaking in a superlattice

We propose a novel acoustic cavity design where we confine a mechanical mode by adiabatically changing the acoustic properties of a GaAs/AlAs superlattice. By means of high resolution Raman scattering measurements, we experimentally demonstrate the presence of a confined acoustic mode at a resonance frequency around 350 GHz. We observe an excellent agreement between the experimental data and numerical simulations based on a photoelastic model. We demonstrate that the spatial profile of the confined mode can be tuned by changing the magnitude of the adiabatic deformation, leading to strong variations of its mechanical quality factor and Raman scattering cross section. The reported alternative confinement method could lead to the development of a novel generation of nanophononic and optomechanical systems.

cond-mat.mes-hall↗

arXiv2017

Optomechanical properties of GaAs/AlAs micropillar resonators operating in the 18 GHz range

Recent experiments demonstrated that GaAs-AlAs based micropillar cavities are promising systems for quantum optomechanics, allowing the simultaneous three-dimensional confinement of near-infrared photons and acoustic phonons in the 18-100 GHz range. Here, we investigate through numerical simulations the optomechanical properties of this new platform. We evidence how the Poisson's ratio and semiconductor-vacuum boundary conditions lead to very distinct features in the mechanical and optical three dimensional confinement. We find a strong dependence of the mechanical quality factor and strain distribution on the micropillar radius, in great contrast to what is predicted and observed in the optical domain. The derived optomechanical coupling constants g_0 reach ultra-large values in the 10^6 rad/s range.

cond-mat.mes-hall↗

arXiv2016

Time-Resolved Cavity Nano-Optomechanics in the 20-100 GHz range

Applications of cavity optomechanics span from gravitational wave detection to the study of quantum motion states in mesoscopic mechanical systems. The engineering of resonators supporting strongly interacting mechanical and optical modes is central to these developments. However, current technological and experimental approaches limit the accessible mechanical frequencies to a few GHz, imposing hard constraints on quantum mechanical studies. Here we demonstrate the optical control of 20-100~GHz mechanical modes confined in the three dimensions within semiconductor nano-optomechanical pillar cavities. We use a time-resolved transient optical reflectivity technique and access both the energy spectrum and dynamics of the mechanical modes at the picosecond timescale. A strong increase of the optomechanical coupling upon reducing the pillar size is observed together with unprecedent room temperature Q-frequency products above $10^{14}$. The measurements also reveal sideband generation in the optomechanical response. Such resonators can naturally integrate quantum wells and quantum dots, enabling novel applications in cavity quantum electrodynamics and high frequency nanomechanics.

physics.optics↗

arXiv2016

Quantum Communication Between Remote Mechanical Resonators

Mechanical resonators represent one of the most promising candidates to mediate the interaction between different quantum technologies, bridging the gap between efficient quantum computation and long-distance quantum communication. In this letter, we introduce a novel interferometric scheme where the interaction of a mechanical resonator with input/output quantum pulses is controlled by an independent classical drive. We design protocols for state teleportation and direct quantum state transfer, between distant mechanical resonators. The proposed device, feasible with state-of-the-art technology, can serve as building block for the implementation of long-distance quantum networks of mechanical resonators.

quant-ph↗

arXiv2016

Monolithic AlGaAs second-harmonic nanoantennas

We demonstrate monolithic aluminum gallium arsenide (AlGaAs) optical anoantennas. Using a selective oxidation technique, we fabricate such epitaxial semiconductor nanoparticles on an aluminum oxide substrate. Second harmonic generation from an AlGaAs nanocylinder of height h=400 nm and varying radius pumped with femtosecond pulses delivered at 1554-nm wavelength has been measured, revealing a peak conversion efficiency exceeding 10-5 for nanocylinders with an otpimized geometry.

physics.optics↗

arXiv2015

High frequency nano-optomechanical disk resonators in liquids

Vibrating nano- and micromechanical resonators have been the subject of research aiming at ultrasensitive mass sensors for mass spectrometry, chemical analysis and biomedical diagnosis. Unfortunately, their merits diminish dramatically in liquids due to dissipative mechanisms like viscosity and acoustic losses. A push towards faster and lighter miniaturized nanodevices would enable improved performances, provided dissipation was controlled and novel techniques were available to efficiently drive and read-out their minute displacement. Here we report on a nano-optomechanical approach to this problem using miniature semiconductor disks. These devices combine mechanical motion at high frequency above the GHz, ultra-low mass of a few picograms, and moderate dissipation in liquids. We show that high-sensitivity optical measurements allow to direct resolve their thermally driven Brownian vibrations, even in the most dissipative liquids. Thanks to this novel technique, we experimentally, numerically and analytically investigate the interaction of these resonators with arbitrary liquids. Nano-optomechanical disks emerge as probes of rheological information of unprecedented sensitivity and speed, opening applications in sensing and fundamental science.

physics.ins-det↗

arXiv2012

Cavity-enhanced optical detection of carbon nanotube Brownian motion

Optical cavities with small mode volume are well-suited to detect the vibration of sub-wavelength sized objects. Here we employ a fiber-based, high-finesse optical microcavity to detect the Brownian motion of a freely suspended carbon nanotube at room temperature under vacuum. The optical detection resolves deflections of the oscillating tube down to 50pm/Hz^1/2. A full vibrational spectrum of the carbon nanotube is obtained and confirmed by characterization of the same device in a scanning electron microscope. Our work successfully extends the principles of high-sensitivity optomechanical detection to molecular scale nanomechanical systems.

physics.optics↗

arXiv2012

Miniature GaAs disk resonators probed by a looped fiber taper for optomechanics applications

GaAs disk resonators (typical disk size 5 \mum * 200 nm in our work) are good candidates for boosting optomechanical coupling thanks to their ability to confine both optical and mechanical energy in a sub-micron interaction volume. We present results of optomechanical characterization of GaAs disks by near-field optical coupling from a tapered silica nano-waveguide. Whispering gallery modes with optical Q factor up to a few 10^5 are observed. Critical coupling, optical resonance doublet splitting and mode identification are discussed. We eventually show an optomechanical phenomenon of optical force attraction of the silica taper to the disk. This phenomenon shows that mechanical and optical degrees of freedom naturally couple at the micro-nanoscale.

physics.optics↗

arXiv2012

Damping of optomechanical disks resonators vibrating in air

We report on miniature GaAs disk optomechanical resonators vibrating in air in the radiofrequency range. The flexural modes of the disks are studied by scanning electron microscopy and optical interferometry, and correctly modeled with the elasticity theory for annular plates. The mechanical damping is systematically measured, and confronted with original analytical models for air damping. Formulas are derived that correctly reproduce both the mechanical modes and the damping behavior, and can serve as design tools for optomechanical applications in fluidic environment.

physics.optics↗

arXiv2011

Critical optical coupling between a GaAs disk and a nanowaveguide suspended on the chip

We report on an integrated GaAs disk/waveguide system. A millimeter-long waveguide is suspended and tapered on the chip over a length of 25 μm to evanescently couple to high Q optical whispering gallery modes of a GaAs disk. The critical coupling regime is obtained both by varying the disk/guide gap distance and the width of the suspended nanoscale taper. The experimental results are in good agreement with predictions from the coupled mode theory.

physics.optics↗

arXiv2009

Semiconductor ridge microcavity source of quantum light at room temperature

We experimentally demonstrate an integrated semiconductor ridge microcavity source of counterpropagating twin photons at room temperature in the telecom range. Based on parametric down conversion with a counterpropagating phase-matching, pump photons generate photon pairs with an efficiency of about 10^(-11) and a spectral linewidth of 0.3 nm for a 1mm long sample. The indistiguishability of the photons of the pair are measured via a two-photon interference experiment showing a visibility of 85%. This work opens a route towards new guided-wave semiconductor quantum devices.

quant-ph↗

arXiv2009

Fluctuating nanomechanical systems in a high finesse optical microcavity

Confining a laser field between two high reflectivity mirrors of a high-finesse cavity can increase the probability of a given cavity photon to be scattered by an atom traversing the confined photon mode. This enhanced coupling between light and atoms is successfully employed in cavity quantum electrodynamics experiments and led to a very prolific research in quantum optics. The idea of extending such experiments to sub-wavelength sized nanomechanical systems has been recently proposed in the context of optical cavity cooling. Here we present an experiment involving a single nanorod consisting of about 10^9 atoms precisely positioned to plunge into the confined mode of a miniature high finesse Fabry-Perot cavity. We show that the optical transmission of the cavity is affected not only by the static position of the nanorod but also by its vibrational fluctuation. While an imprint of the vibration dynamics is directly detected in the optical transmission, back-action of the light field is also anticipated to quench the nanorod Brownian motion. This experiment shows the first step towards optical cavity controlled dynamics of mechanical nanostructures and opens up new perspectives for sensing and manipulation of optomechanical nanosystems.

physics.optics↗

arXiv2005

Fast exciton spin relaxation in single quantum dots

Exciton spin relaxation is investigated in single epitaxially grown semiconductor quantum dots in order to test the expected spin relaxation quenching in this system. We study the polarization anisotropy of the photoluminescence signal emitted by isolated quantum dots under steady-state or pulsed non-resonant excitation. We find that the longitudinal exciton spin relaxation time is strikingly short ($\leq$100 ps) even at low temperature. This result breaks down the picture of a frozen exciton spin in quantum dots.

cond-mat.other↗

arXiv2004

Giant optical anisotropy in a single InAs quantum dot in a very dilute quantum-dot ensemble

We present the experimental evidence of giant optical anisotropy in single InAs quantum dots. Polarization-resolved photoluminescence spectroscopy reveals a linear polarization ratio with huge fluctuations, from one quantum dot to another, in sign and in magnitude with absolute values up to 82%. Systematic measurements on hundreds of quantum dots coming from two different laboratories demonstrate that the giant optical anisotropy is an intrinsic feature of dilute quantum-dot arrays.

cond-mat.other↗