arXiv subjects

I. M. Bradaric

Publications and source records attributed to I. M. Bradaric.

4 recordsLinked to original sources

arXiv2008

Hidden Orbital Liquid State Within Ferromagnetically Ordered Metallic SrRuO3

We have experimentally found related anomalies in electrical resistivity, dc and ac magnetic susceptibility, appearing deeply within ferromagnetically ordered state in SrRuO3. Lack of Jahn-Teller distortion in this regime rules out conventional orbital order, forcing one to describe these in terms of an orbital liquid ground state coexisting with ferromagnetic spin order. We suggest that weak spin-orbit coupling in such an unusual state underpins the observed anomalies.

cond-mat.str-el↗

arXiv2008

Charge transfer mechanism and Tc(x) dependence in Y0.8(Ca)0.2Ba2Cu3O6+x

We propose a model for charge transfer mechanism in Y0.8(Ca)0.2Ba2Cu3O6+x to count hole doping of CuO2 planes and x dependence of critical transition temperature T_c. It is assumed the total number of doped holes in the planes is sum of holes that are introduced through two separate channels: substitution of Y3+ by Ca2+ and from CuO chains that are longer than a minimal (critical) length l_min needed for charge transfer to take place. The T_c(x) dependence is obtained by combining calculated x dependence of doping, p(x), and universal T_c versus p relation. Although calculated T_c(x) dependences for l_min=3 and l_min=4 both remarkably correlate to the experimental T_c(x), we argue that the value l_min=4 gives a reasonable overall agreement.

cond-mat.supr-con↗

arXiv2001

The magnetic behavior of Li2MO3 (M=Mn, Ru and Ir) and Li2(Mn1-xRux)O3

The present study summerizes magnetic and Mossbauer measurements on ceramic Li2MO3 M= Mn, Ru and Ir and the mixed Li2(Mn1-xRux)O3 materials, which show many of the features reflecting to antiferromagnetic ordering or to existence of paramagnetic states. Li2IrO3 and Li2RuO3 are paramagnetic down to 5 K. Li2(Mn1-xRux)O3 compounds are antiferromagnetically ordered at TN = 48 K for x=0. TN decreases as the Ru content increases and, for x=0.8, TN =34 K.

cond-mat.mtrl-sci↗

arXiv2001

Metal-to-insulator transition and magnetic ordering in CaRu_{1-x}Cu_xO_3

CaRuO_3 is perovskite with an orthorhombic distortion and is believed to be close to magnetic ordering. Magnetic studies of single crystal and polycrystalline CaRu_{1-x}Cu_xO_3 (0\le x \le 15 at.%Cu) reveal that spin-glass-like transition develops for x\le 7 at.%Cu and obtained value for effective magnetic moment p_{eff}=3.55 mu_B for x=5 at.% Cu, single crystal, indicates presence of Ru^{5+}. At higher Cu concentrations more complex magnetic behaviors are observed. Electrical resistivity measured on polycrystalline samples shows metal-to-insulator transition (MIT) at 51 K for only 2 at.% Cu. Charge compensation, which is assumed to be present upon Cu^{2+/3+} substitution, induces appearance of Ru^{5+} and/or creation of oxygen vacancies in crystal structure. Since the observed changes in physical properties are completely attributable to the charge compensation, they cannot be related to behaviors of pure compound where no such mechanism is present. This study provides the criterion for "good" chemical probes for studying Ru-based perovskites.

cond-mat.str-el↗