arXiv subjects

I. M. Pop

Publications and source records attributed to I. M. Pop.

At least 19 recordsLinked to original sources

arXiv2026

Experimental Observation of Short-Range Magnetic Correlations in Amorphous Nb$_2$O$_5$ and Ta$_2$O$_5$ Thin Films

We use muon spin rotation/relaxation/resonance ($μ$SR) to investigate the magnetic properties of niobium pentoxide (Nb$_2$O$_5$) and tantalum pentoxide (Ta$_2$O$_5$) thin films. In both oxides, we observe a magnetic response at the lowest available temperature of 2.8 K. This response appears to be structurally dependent: thermally oxidized Ta$_2$O$_5$ with low crystallinity demonstrates suppressed magnetism, while fully amorphous Ta$_2$O$_5$ demonstrates local static magnetism. In contrast, amorphous Nb$_2$O$_5$ is dominated by magnetic fluctuations and is strongly magnetically disordered compared to Ta$_2$O$_5$. Our results suggest that these fundamental differences in the magnetism of Ta and Nb oxides could explain the performance limitations in superconducting qubits and resonators.

cond-mat.other↗

arXiv2025

Spin Environment of a Superconducting Qubit in High Magnetic Fields

Superconducting qubits equipped with quantum non-demolition readout and active feedback can be used as information engines to probe and manipulate microscopic degrees of freedom, whether intentionally designed or naturally occurring in their environment. In the case of spin systems, the required magnetic field bias presents a challenge for superconductors and Josephson junctions. Here we demonstrate a granular aluminum nanojunction fluxonium qubit (gralmonium) with spectrum and coherence resilient to fields beyond one Tesla. Sweeping the field reveals a paramagnetic spin-1/2 ensemble, which is the dominant gralmonium loss mechanism when the electron spin resonance matches the qubit. We also observe a suppression of MHz range fast flux noise in magnetic field, suggesting the freezing of surface spins. Using an active state stabilization sequence, the qubit hyperpolarizes long-lived two-level systems (TLSs) in its environment, previously speculated to be spins. Surprisingly, the coupling to these TLSs is unaffected by magnetic fields, leaving the question of their origin open. The robust operation of gralmoniums in Tesla fields offers new opportunities to explore unresolved questions in spin environment dynamics and facilitates hybrid architectures linking superconducting qubits with spin systems.

quant-ph↗

arXiv2025

Kinetic inductance coupling for circuit QED with spins

In contrast to the commonly used qubit resonator transverse coupling via the $σ_{xy}$-degree of freedom, longitudinal coupling through $σ_z$ presents a tantalizing alternative: it does not hybridize the modes, eliminating Purcell decay, and it enables quantum-non-demolishing qubit readout independent of the qubit-resonator frequency detuning. Here, we demonstrate longitudinal coupling between a {Cr$_7$Ni} molecular spin qubit ensemble and the kinetic inductance of a granular aluminum superconducting microwave resonator. The inherent frequency-independence of this coupling allows for the utilization of a 7.8 GHz readout resonator to measure the full {Cr$_7$Ni} magnetization curve spanning 0-600 mT, corresponding to a spin frequency range of $f_\text{spin}=$0-15 GHz. For 2 GHz detuning from the readout resonator, we measure a $1/e$ spin relaxation time $τ=$0.38 s, limited by phonon decay to the substrate. Based on these results, we propose a path towards longitudinal coupling of single spins to a superconducting fluxonium qubit.

quant-ph↗

arXiv2023

Photon-mediated long range coupling of two Andreev level qubits

In a superconducting weak link, the supercurrent is carried by Andreev bound states (ABSs) formed by the phase-coherent reflection of electrons and their time-reversed partners. A single, highly transmissive ABS can serve as an ideal, compact two-level system, due to a potentially large energy difference to the next ABS. While the coherent manipulation of such Andreev levels qubits (ALQs) has been demonstrated, a long-range coupling between two ALQs, necessary for advanced qubit architectures, has not been achieved, yet. Here, we demonstrate a coherent remote coupling between two ALQs, mediated by a microwave photon in a novel superconducting microwave cavity coupler. The latter hosts two modes with different coupling rates to an external port. This allows us to perform fast readout of each qubit using the strongly coupled mode, while the weakly coupled mode is utilized to mediate the coupling between the qubits. When both qubits are tuned into resonance with the latter mode, we find excitation spectra with avoided-crossings, in very good agreement with the Tavis-Cummings model. Based on this model, we identify highly entangled two-qubit states for which the entanglement is mediated over a distance of six millimeters. This work establishes ALQs as compact and scalable solid-state qubits.

cond-mat.mes-hall↗

arXiv2023

Fano Interference in Microwave Resonator Measurements

Resonator measurements are a simple but powerful tool to characterize a material's microwave response. The losses of a resonant mode are quantified by its internal quality factor $Q_\mathrm{i}$, which can be extracted from the scattering coefficient in a microwave reflection or transmission measurement. Here we show that a systematic error on $Q_\mathrm{i}$ arises from Fano interference of the signal with a background path. Limited knowledge of the interfering paths in a given setup translates into a range of uncertainty for $Q_\mathrm{i}$, which increases with the coupling coefficient. We experimentally illustrate the relevance of Fano interference in typical microwave resonator measurements and the associated pitfalls encountered in extracting $Q_\mathrm{i}$. On the other hand, we also show how to characterize and utilize the Fano interference to eliminate the systematic error.

quant-ph↗

arXiv2022

Gralmonium: Granular Aluminum Nano-Junction Fluxonium Qubit

Mesoscopic Josephson junctions (JJs), consisting of overlapping superconducting electrodes separated by a nanometer thin oxide layer, provide a precious source of nonlinearity for superconducting quantum circuits and are at the heart of state-of-the-art qubits, such as the transmon and fluxonium. Here, we show that in a fluxonium qubit the role of the JJ can also be played by a lithographically defined, self-structured granular aluminum (grAl) nano-junction: a superconductor-insulator-superconductor (SIS) JJ obtained in a single layer, zero-angle evaporation. The measured spectrum of the resulting qubit, which we nickname gralmonium, is indistinguishable from the one of a standard fluxonium qubit. Remarkably, the lack of a mesoscopic parallel plate capacitor gives rise to an intrinsically large grAl nano-junction charging energy in the range of tens of $\mathrm{GHz}$, comparable to its Josephson energy $E_\mathrm{J}$. We measure average energy relaxation times of $T_1=10\,\mathrm{μs}$ and Hahn echo coherence times of $T_2^\text{echo}=9\,\mathrm{μs}$. The exponential sensitivity of the gralmonium to the $E_\text{J}$ of the grAl nano-junction provides a highly susceptible detector. Indeed, we observe spontaneous jumps of the value of $E_\text{J}$ on timescales from milliseconds to days, which offer a powerful diagnostics tool for microscopic defects in superconducting materials.

quant-ph↗

arXiv2021

Subgap kinetic inductance detector sensitive to 85-GHz radiation

We have fabricated an array of subgap kinetic inductance detectors (SKIDs) made of granular aluminum ($T_c\sim$2~K) sensitive in the 80-90 GHz frequency band and operating at 300~mK. We measure a noise equivalent power of $1.3\times10^{-16}$~W/Hz$^{0.5}$ on average and $2.6\times10^{-17}$~W/Hz$^{0.5}$ at best, for an illuminating power of 50~fW per pixel. Even though the circuit design of SKIDs is identical to that of the kinetic inductance detectors (KIDs), the SKIDs operating principle is based on their sensitivity to subgap excitations. This detection scheme is advantageous because it avoids having to lower the operating temperature proportionally to the lowest detectable frequency. The SKIDs presented here are intrinsically selecting the 80-90 GHz frequency band, well below the superconducting spectral gap of the film, at approximately 180 GHz.

physics.ins-det↗

arXiv2020

Superconducting granular aluminum resonators resilient to magnetic fields up to 1 Tesla

High kinetic inductance materials constitute a valuable resource for superconducting quantum circuits and hybrid architectures. Superconducting granular aluminum (grAl) reaches kinetic sheet inductances in the nH/$\square$ range, with proven applicability in superconducting quantum bits and microwave detectors. Here we show that the single photon internal quality factor $Q_{\mathrm{i}}$ of grAl microwave resonators exceeds $10^5$ in magnetic fields up to 1T, aligned in-plane to the grAl films. Small perpendicular magnetic fields, in the range of 0.5mT, enhance $Q_{\mathrm{i}}$ by approximately 15%, possibly due to the introduction of quasiparticle traps in the form of fluxons. Further increasing the perpendicular field deteriorates the resonators' quality factor. These results open the door for the use of high kinetic inductance grAl structures in circuit quantum electrodynamics and hybrid architectures with magnetic field requirements.

cond-mat.supr-con↗

arXiv2019

Electrodynamics of granular aluminum from superconductor to insulator: observation of collective superconducting modes

We report on a detailed study of the optical response and $T_c-ρ$ phase diagram ($T_c$ being the superconducting critical temperature and $ρ$ the normal state resistivity of the film) of granular aluminum, combining transport measurements and a high resolution optical spectroscopy technique. The $T_c-ρ$ phase diagram is discussed as resulting from an interplay between the phase stiffness, the Coulomb repulsion and the superconducting gap $Δ$. We provide a direct evidence for two different types of well resolved sub-gap absorptions, at $ω_1\simeqΔ$ and at $Δ\lesssimω_2\lesssim2Δ$ (decreasing with increasing resistivity).

cond-mat.supr-con↗

arXiv2018

Driving forbidden transitions in the fluxonium artificial atom

Atomic systems display a rich variety of quantum dynamics due to the different possible symmetries obeyed by the atoms. These symmetries result in selection rules that have been essential for the quantum control of atomic systems. Superconducting artificial atoms are mainly governed by parity symmetry. Its corresponding selection rule limits the types of quantum systems that can be built using electromagnetic circuits at their optimal coherence operation points ("sweet spots"). Here, we use third-order nonlinear coupling between the artificial atom and its readout resonator to drive transitions forbidden by the parity selection rule for linear coupling to microwave radiation. A Lambda-type system emerges from these newly accessible transitions, implemented here in the fluxonium artificial atom coupled to its "antenna" resonator. We demonstrate coherent manipulation of the fluxonium artificial atom at its sweet spot by stimulated Raman transitions. This type of transition enables the creation of new quantum operations, such as the control and readout of physically protected artificial atoms.

quant-ph↗

arXiv2018

Circuit Quantum Electrodynamics of Granular Aluminum Resonators

The introduction of crystalline defects or dopants can give rise to so-called "dirty superconductors", characterized by reduced coherence length and quasiparticle mean free path. In particular, granular superconductors such as Granular Aluminum (GrAl), consisting of remarkably uniform grains connected by Josephson contacts have attracted interest since the sixties thanks to their rich phase diagram and practical advantages, like increased critical temperature, critical field, and kinetic inductance. Here we report the measurement and modeling of circuit quantum electrodynamics properties of GrAl microwave resonators in a wide frequency range, up to the spectral superconducting gap. Interestingly, we observe self-Kerr coefficients ranging from $10^{-2}$ Hz to $10^5$ Hz, within an order of magnitude from analytic calculations based on GrAl microstructure. This amenable nonlinearity, combined with the relatively high quality factors in the $10^5$ range, open new avenues for applications in quantum information processing and kinetic inductance detectors.

cond-mat.supr-con↗

arXiv2017

Simultaneous monitoring of fluxonium qubits in a waveguide

Most quantum-error correcting codes assume that the decoherence of each physical qubit is independent of the decoherence of any other physical qubit. We can test the validity of this assumption in an experimental setup where a microwave feedline couples to multiple qubits by examining correlations between the qubits. Here, we investigate the correlations between fluxonium qubits located in a single waveguide. Despite being in a wide-bandwidth electromagnetic environment, the qubits have measured relaxation times in excess of 100 us. We use cascaded Josephson parametric amplifiers to measure the quantum jumps of two fluxonium qubits simultaneously. No correlations are observed between the relaxation times of the two fluxonium qubits, which indicates that the sources of relaxation are local to each qubit. Our architecture can easily be scaled to monitor larger numbers of qubits.

quant-ph↗

arXiv2017

Bistability in a Mesoscopic Josephson Junction Array Resonator

We present an experimental investigation of stochastic switching of a bistable Josephson junctions array resonator with a resonance frequency in the GHz range. As the device is in the regime where the anharmonicity is on the order of the linewidth, the bistability appears for a pump strength of only a few photons. We measure the dynamics of the bistability by continuously observing the jumps between the two metastable states, which occur with a rate ranging from a few Hz down to a few mHz. The switching rate strongly depends on the pump strength, readout strength and the temperature, following Kramer's law. The interplay between nonlinearity and coupling, in this little explored regime, could provide a new resource for nondemolition measurements, single photon switches or even elements for autonomous quantum error correction.

cond-mat.supr-con↗

arXiv2016

Quantization of inductively-shunted superconducting circuits

We present a method for calculating the energy levels of superconducting circuits that contain highly anharmonic, inductively-shunted modes with arbitrarily strong coupling. Our method starts by calculating the normal modes of the linearized circuit and proceeds with numerical diagonalization in this basis. As an example, we analyze the Hamiltonian of a fluxonium qubit inductively coupled to a readout resonator. While elementary, this simple example is nontrivial because it cannot be efficiently treated by the method known as "black-box quantization," numerical diagonalization in the bare harmonic oscillator basis, or perturbation theory. Calculated spectra are compared to measured spectroscopy data, demonstrating excellent quantitative agreement between theory and experiment.

quant-ph↗

arXiv2016

Planar multilayer circuit quantum electrodynamics

Experimental quantum information processing with superconducting circuits is rapidly advancing, driven by innovation in two classes of devices, one involving planar micro-fabricated (2D) resonators, and the other involving machined three-dimensional (3D) cavities. We demonstrate that circuit quantum electrodynamics can be implemented in a multilayer superconducting structure that combines 2D and 3D advantages. We employ standard micro-fabrication techniques to pattern each layer, and rely on a vacuum gap between the layers to store the electromagnetic energy. Planar qubits are lithographically defined as an aperture in a conducting boundary of the resonators. We demonstrate the aperture concept by implementing an integrated, two cavity-modes, one transmon-qubit system.

cond-mat.supr-con↗

arXiv2014

Bloch band dynamics of a Josephson junction in an inductive environment

We have measured the current-voltage characteristics of a Josephson junction with tunable Josephson energy $E_J$ embedded in an inductive environment provided by a chain of SQUIDs. Such an environment induces localization of the charge on the junction, which results in an enhancement of the zero-bias resistance of the circuit. We understand this result quantitatively in terms of the Bloch band dynamics of the localized charge. This dynamics is governed by diffusion in the lowest Bloch band of the Josephson junction as well as by Landau-Zener transitions out of the lowest band into the higher bands. In addition, the frequencies corresponding to the self-resonant modes of the SQUID array exceed the Josephson energy $E_J$ of the tunable junction, which results in a renormalization of $E_J$, and, as a consequence, of the effective bandwidth of the lowest Bloch band.

cond-mat.mes-hall↗

arXiv2014

Understanding the $μ$SR spectra of MnSi without magnetic polarons

Transverse-field muon-spin rotation ($μ$SR) experiments were performed on a single crystal sample of the non-centrosymmetric system MnSi. The observed angular dependence of the muon precession frequencies matches perfectly the one of the Mn-dipolar fields acting on the muons stopping at a 4a position of the crystallographic structure. The data provide a precise determination of the magnetic dipolar tensor. In addition, we have calculated the shape of the field distribution expected below the magnetic transition temperature $T_C$ at the 4a muon-site when no external magnetic field is applied. We show that this field distribution is consistent with the one reported by zero-field $μ$SR studies. Finally, we present ab initio calculations based on the density-functional theory which confirm the position of the muon stopping site inferred from transverse-field $μ$SR. In view of the presented evidence we conclude that the $μ$SR response of MnSi can be perfectly and fully understood without invoking a hypothetical magnetic polaron state.

cond-mat.str-el↗

arXiv2013

Planar Superconducting Whispering Gallery Mode Resonators

We introduce a microwave circuit architecture for quantum signal processing combining design principles borrowed from high-Q 3D resonators in the quantum regime and from planar structures fabricated with standard lithography. The resulting '2.5D' whispering-gallery mode resonators store 98% of their energy in vacuum. We have measured internal quality factors above 3 million at the single photon level and have used the device as a materials characterization platform to place an upper bound on the surface resistance of thin film aluminum of less than 250nOhms.

cond-mat.supr-con↗