arXiv subjects
Publications and source records attributed to I. S. Tupitsyn.
Reply to the Comment of J.J. Alonso and J.F. Fernandez on the paper "'Hole-digging' in ensembles of tunneling molecular magnets" of I.S. Tupitsyn, P.C.E. Stamp and N.V. Prokof'ev (Phys. Rev. B 69, 132406, (2004)).
The spin coherence phenomena and the possibility of their observation in nanomagnetic insulators attract more and more attention in the last several years. Recently it has been shown that in these systems in large transverse magnetic field there can be a fairly narrow "coherence window" for phonon and nuclear spin-mediated decoherence. What kind of spin dynamics can then be expected in this window in a crystal of magnetic nanomolecules coupled to phonons, to nuclear spin bath and it to each other via dipole-dipole interactions? Studying multispin correlations, we determine the region of parameters where "coherent clusters" of collective spin excitations can appear. Although two particular systems, namely crystals of $Fe_8$-triazacyclonane and $Mn_{12}$-acetate molecules, are used in this work to illustrate the results, here we are not trying to predict an existence of collective coherent dynamics in some particular system. Instead, we discuss the way how any crystalline system of dipole-dipole coupled nanomolecules can be analyzed to decide whether this system is suitable for attempts to observe coherent dynamics. The presented analysis can be useful in the search for magnetic systems showing the spin coherence phenomena.
Comment on the paper: "Magnetization Process of Single Molecule Magnets at Low Temperatures" of J.F.Fernandez and J.J.Alonso (PRL 91, 047202 (2003)).
We discuss how the crossovers in models like spin-boson model are changed by adding the coupling of the central spin to localised modes- the latter modelled as a 'spin bath'. These modes contain most of the environmental entropy and energy at low T in solid-state systems. We find that the low T crossover between oscillator bath and spin bath dominated decoherence, occurring as one reduces the energy scale of the central spin, is characterised by very low decoherence- we show how this works out in practise in magnetic insulators. We then reconsider the standard quantum-classical crossover in the dynamics of a tunneling system, including both spin and oscillator baths. It is found that the general effect of the spin bath is to broaden the crossover in temperature between the quantum and classical activated regimes. The example of tunneling nanomagnets is used to illustrate this.
Decoherence in many solid-state systems is anomalously high, frustrating efforts to make solid-state qubits. We show that in nanomagnetic insulators in large transverse fields, there can be a fairly narrow field region in which both phonon and nuclear spin-mediated decoherence are drastically reduced. As examples we calculate decoherence rates for the $Fe$-8 nanomolecule, for $Ni$ particles, and for $Ho$ ions in $LiHo_xY_{1-z}F_4$. The reduction in the decoherence, compared to low field rates, can exceed 6 orders of magnitude. The results also give limitations on the observability of macroscopic coherence effects in magnetic systems.
The nuclear spin-mediated quantum relaxation of ensembles of tunneling magnetic molecules causes a 'hole' to appear in the distribution of internal fields in the system. The form of this hole, and its time evolution, are studied using Monte Carlo simulations. It is shown that the line-shape of the tunneling hole in a weakly polarised sample must have a Lorentzian lineshape- the short-time half-width $ξ_o$ in all experiments done so far should be $\sim E_0$, the half-width of the nuclear spin multiplet. After a time $τ_o$, the single molecule tunneling relaxation time, the hole width begins to increase rapidly. In initially polarised samples the disintegration of resonant tunneling surfaces is found to be very fast.
In a recent letter Alonso et al. (Phys. Rev. Lett. 87, 097205 (2001)) present Monte Carlo simulations for interacting dipoles. Short-time relaxation was caused by a simple noise field, acting uniformly over an "energy window" of small width (to simulate the fluctuating nuclear spin bias). However, the physics of the tunneling relaxation of an ensemble of tunneling nanomagnets or magnetic molecules (as well as of the "tunneling hole" formation) is different and here we discuss this point.
We show how the worldline quantum Monte Carlo procedure, which usually relies on an artificial time discretization, can be formulated directly in continuous time, rendering the scheme exact. For an arbitrary system with discrete Hilbert space, none of the configuration update procedures contain small parameters. We find that the most effective update strategy involves the motion of worldline discontinuities (both in space and time), i.e., the evaluation of the Green's function. Being based on local updates only, our method nevertheless allows one to work with the grand canonical ensemble and non-zero winding numbers, and to calculate any dynamic correlation function as easily as expectation values of, e.g., total energy. The principles found for the update in continuous time generalize to any continuous variables in the space of discrete virtual transitions, and in principle also make it possible to simulate continuous systems exactly.
An effective Hamiltonian, describing quantum tunneling in ferrimagnetic nanoparticles which includes interactions between the electronic spins of nanoparticle and microscopic environmental spins (like nuclear spins or paramagnetic impurities), is obtained. Two limiting cases, describing tunneling in antiferromagnetic and ferromagnetic regimes are considered, and criterion for the transition between the two regimes is found. The validity of analytic results is verified by the exact diagonalization method.
We consider here the problem of a "giant spin", with spin quantum number S>>1, interacting with a set of microscopic spins. Interactions between the microscopic spins are ignored. This model describes the low-energy properties of magnetic grains or magnetic macromolecules interacting with a surrounding spin environment, such as nuclear spins. We describe a general method for truncating the model to another one, valid at low energies, in which a two-level system interacts with the environmental spins, and higher energy terms are absorbed into a new set of couplings. This is done using an instanton technique. We then verify the accuracy of this technique, by comparing the results for the low energy effective Hamiltonian, with results derived for the original giant spin, coupled to a microscopic spin, using exact diagonalisation techniques.
We introduce an exact Monte Carlo approach to the statistics of discrete quantum systems which does not rely on the standard fragmentation of the imaginary time, or any small parameter. The method deals with discrete objects, kinks, representing virtual transitions at different moments of time. The global statistics of kinks is reproduced by explicit local procedures, the key one being based on the exact solution for the biased two-level system.
By means of exact diagonalization we study the low-energy states of seven electrons in the lowest Landau level which are confined by a cylindric external potential modelling the rest of a macroscopic system and thus controlling the filling factor $ν$. Wigner crystal is found to be the ground state for filling factors between $ ν= 1/3$ and $ ν= 1/5$ provided electrons interact via the bare Coulomb potential. Even at $ν=1/5$ the solid state has lower energy than the Laughlin's one, although the two energies are rather close. We also discuss the role of pseudopotential parameters in the lowest Landau level and demonstrate that the earlier reported gapless state, appearing when the short-range part of the interaction is suppressed, has nothing in common with the Wigner crystalization in pure Coulomb case.