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I. Tsekhanovich

Publications and source records attributed to I. Tsekhanovich.

13 recordsLinked to original sources

Fission mode identification in the 180Hg region: derivative analysis approach

Experimental setups commonly used to study fission properties of nuclei in the exotic neutron-deficient 180Hg region are based on the time-of-flight technique for the fission-product identification. The nuclei of interest are created via fusion reactions at excitation energies of several tens of MeV and identified with limited mass resolution. The deduced final fission-fragment mass distributions are in general structureless, which makes the identification of fission modes, along with their properties, ambiguous and author-dependent. The standard functional-analysis technique applied to the simulated limited-resolution fusion-fission data appears to provide consistent results on the number and parameters of fission modes, even in cases of strong symmetric-mode dominance, i.e. for Gaussian-like fission-fragment mass distribution shapes. The method is shown to work also on data sets with limited statistics (real experimental data with integral of a few tens of thousands of events).

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Fission of 215Fr studied with gamma spectroscopic methods

Background: Asymmetric fission is known to occur in two regions, the actinides and sub-lead, and is dependent on the fissioning system excitation energy. Experimental evidence in the sub-lead region show that this mode is surprisingly persistent with increasing energy and its origin is not fully understood. Purpose: To experimentally study the fusion-fission reaction of $^{215}$Fr at moderate excitation energy and determine previously unknown independent fission yields and other properties. Method: The compound nucleus was formed in the reaction $^{18}$O + $^{197}$Au. The prompt gamma-rays emitted during the reaction were measured with the high efficiency and high granularity $ν$-ball2 spectrometer. Independent fission yields of even-even nuclei were determined by detecting triple-gamma cascades in the fission fragments. Results: The observed yields, although dominated by a symmetric peak, show maxima for heavy fragment of $Z \approx 54-56$, which is consistent with the known results in the actinide region but unexpected for the nuclide of interest, and at the studied excitation energy. Conclusions: The mode of asymmetric fission is present even at relatively high excitation energies in the system studied. This observation matches experimental findings in the sub-lead region, contrary to the actinides, and so far there is no well-developed explanation of this phenomenon.

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Particle Identification at VAMOS++ with Machine Learning Techniques

Multi-nucleon transfer reaction between 136Xe beam and 198Pt target was performed using the VAMOS++ spectrometer at GANIL to study the structure of n-rich nuclei around N=126. Unambiguous charge state identification was obtained by combining two supervised machine learning methods, deep neural network (DNN) and positional correction using a gradient-boosting decision tree (GBDT). The new method reduced the complexity of the kinetic energy calibration and outperformed the conventional method, improving the charge state resolution by 8%

physics.ins-det

$^{178}$Hg and asymmetric fission of neutron-deficient pre-actinides

Fission at low excitation energy is an ideal playground to probe the impact of nuclear structure on nuclear dynamics. While the importance of structural effects in the nascent fragments is well-established in the (trans-)actinide region, the observation of asymmetric fission in several neutron-deficient pre-actinides can be explained by various mechanisms. To deepen our insight into that puzzle, an innovative approach based on inverse kinematics and an enhanced version of the VAMOS++ heavy-ion spectrometer was implemented at the GANIL facility, Caen. Fission of $^{178}$Hg was induced by fusion of $^{124}$Xe and $^{54}$Fe. The two fragments were detected in coincidence using VAMOS++ supplemented with a new SEcond Detection arm. For the first time in the pre-actinide region, access to the pre-neutron mass and total kinetic energy distributions, and the simultaneous isotopic identification of one the fission fragment, was achieved. The present work describes the experimental approach, and discusses the pre-neutron observables in the context of an extended asymmetric-fission island located south-west of $^{208}Pb. A comparison with different models is performed, demonstrating the importance of this "new" asymmetric-fission island for elaborating on driving effects in fission.

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Simultaneous determination of neutron-induced fission and radiative-capture cross sections from decay probabilities obtained with a surrogate reaction

Reliable neutron-induced reaction cross sections of unstable nuclei are essential for nuclear astrophysics and applications but their direct measurement is often impossible. The surrogate-reaction method is one of the most promising alternatives to access these cross sections. In this work, we successfully applied the surrogate-reaction method to infer for the first time both the neutron-induced fission and radiative-capture cross sections of 239Pu in a consistent manner from a single measurement. This was achieved by combining simultaneously-measured fission and gamma-emission probabilities for the 240Pu(4He,4He') surrogate reaction with a calculation of the angular-momentum and parity distributions populated in this reaction. While other experiments measure the probabilities for some selected gamma-ray transitions, we measure the gamma-emission probability. This enlarges the applicability of the surrogate-reaction method.

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Scission configuration of $^{239}$U from yields and kinetic information of fission fragments

The simultaneous measurement of the isotopic fission-fragment yields and fission-fragment velocities of $^{239}$U has been performed for the first time. The $^{239}$U fissioning system was produced in one-neutron transfer reactions between a $^{238}$U beam at 5.88 MeV/nucleon and a $^{9}$Be target. The combination of inverse kinematics at low energy and the use of the VAMOS++ spectrometer at the GANIL facility allows the isotopic identification of the full fission-fragment distribution and their velocity in the reference frame of the fissioning system. The proton and neutron content of the fragments at scission, their total kinetic and total excitation energy, as well as the neutron multiplicity were determined. Information from the scission point configuration is obtained from these observables and the correlation between them. The role of the octupole-deformed proton and neutron shells in the fission-fragment production is discussed.

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First investigation of the response of solar cells to heavy ions above 1 AMeV

Solar cells have been used since several decades for the detection of fission fragments at about 1 AMeV. The advantages of solar cells regarding their cost (few euros) and radiation damage resistance make them an interesting candidate for heavy ion detection and an appealing alternative to silicon detectors. A first exploratory measurement of the response of solar cells to heavy ions at energies above 1 AMeV has been performed at the GANIL facility, Caen, France. Such measurements were performed with 84Kr and 129Xe beams ranging from 7 to 13 AMeV. The energy and time response of several types of solar cells were studied. The best performance was observed for cells of 10x10 mm2, with an energy and time resolution of σ(E)/E=1.4% and 3.6 ns (FWHM), respectively. Irradiations at rates from a few hundred to 106 particles per second were also performed to investigate the behavior of the cells with increasing intensity.

physics.ins-det

First direct measurement of isotopic fission-fragment yields of $^{239}$U

A direct and complete measurement of isotopic fission-fragment yields of $^{239}$U has been performed for the first time. The $^{239}$U fissioning system was produced with an average excitation energy of 8.3 MeV in one-neutron transfer reactions between a $^{238}$U beam and a $^{9}$Be target at Coulomb barrier energies. The fission fragments were detected and isotopically identified using the VAMOS++ spectrometer at the GANIL facility. This measurement allows to directly evaluate the fission models at excitation energies of fast neutrons, relevant for next-generation nuclear reactors. The present data, in agreement with model calculations, do not support the recently reported anomaly in the fission-fragment yields of $^{239}$U and confirm the persistence of spherical shell effects in the Sn region at excitation energies exceeding the fission barrier by few MeV.

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Experimental set-up for the simultaneous measurement of fission and gamma-emission probabilities induced by transfer or inelastic-scattering reactions

Fission and gamma-emission probabilities induced by transfer or inelastic scattering reactions with light projectile nuclei are very valuable quantities for constraining the models that describe the de-excitation of heavy nuclei. We have developed an experimental set-up that allows us to simultaneously measure fission and gamma-emission probabilities. The measurement of the gamma-emission probability at excitation energies where the fission channel is open is challenging due to the intense background of gamma rays emitted by the fission fragments. We discuss the procedure to subtract such a background and the constraints that this subtraction and other experimental conditions put on the set up. We show that our set-up complies with these constraints.

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A new gas-based proton-recoil telescope for quasi-absolute neutron flux measurements between 0.2 and 2 MeV neutron energy

Absolute measurements of neutron flux are an essential prerequisite of neutron-induced cross section measurements, neutron beam lines characterization and dosimetric investigations. A new gaseous detector has been developed for measurements of 0.2 to 2 MeV neutron flux based on proton-recoil process. The detector, consisting of two segmented ionization chambers read by Micromegas technology, has beed conceived to provide quasi-absolute neutron flux measurements with an accuracy of \simeq3%. The gas pressure flexibility makes the telescope non sensitive to γ and electrons background, and therefore advantageous over semi-conductor materials as a neutron flux instrument. The adjustable gas pressure and H-sample thickness, the use of Micromegas technology and the tracking capabilities allows the detection of neutrons on a large dynamical range and down to 200 keV with a good rejection of scattered neutron events and random background

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First observation of the competing fission modes in the neutron-deficient sub-lead region

Fragment mass distributions from fission of excited compound nucleus $^{178}$Pt have been deduced from the measured fragment velocities. The $^{178}$Pt nucleus was created at the JAEA tandem facility in a complete fusion reaction $^{36}$Ar + $^{142}$Nd, at beam energies of 155, 170 and 180 MeV. The data are indicative of a mixture of the mass-asymmetric and mass-symmetric fission modes associated with higher and lower total kinetic energies of the fragments, respectively. The measured fragment yields are dominated by asymmetric mass splits, with the symmetric mode contributing at the level of $\approx1/3$. This constitutes the first observation of a multimodal fission in the sub-lead region. Most probable experimental fragment-mass split of the asymmetric mode, $A_{L}/A_{H}\approx 79/99$, is well reproduced by nuclear density functional theory using the UNEDF1-HFB and D1S potentials. The symmetric mode is associated by theory with very elongated fission fragments, which is consistent with the observed total kinetic energy/fragment mass correlation.

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Study of the 238U(d,p) surrogate reaction via the simultaneous measurement of gamma-decay and fission probabilities

We investigated the 238U(d,p) reaction as a surrogate for the n + 238U reaction. For this purpose we measured for the first time the gamma-decay and fission probabilities of 239U* simultaneously and compared them to the corresponding neutron-induced data. We present the details of the procedure to infer the decay probabilities, as well as a thorough uncertainty analysis, including parameter correlations. Calculations based on the continuum-discretized coupled-channels and distorted-wave Born approximations were used to correct our data from detected protons originating from elastic and inelastic deuteron breakup. In the region where the fission and gamma-decay probabilities compete, the corrected fission probability is in agreement with neutron-induced data, whereas the gamma-decay probability is much higher than the neutron-induced data. The performed statistical-model calculations are not able to explain these results.

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Application of the EXtrapolated Efficiency Method (EXEM) to infer the gamma-cascade detection efficiency in the actinide region

The study of transfer-induced gamma-decay probabilities is very useful for understanding the surrogate-reaction method and, more generally, for constraining statistical-model calculations. One of the main difficulties in the measurement of gamma-decay probabilities is the determination of the gamma-cascade detection efficiency. In [Nucl. Instrum. Meth. A 700, 59 (2013)] we developed the Extrapolated Efficiency Method (EXEM), a new method to measure this quantity. In this work, we have applied, for the first time, the EXEM to infer the gamma-cascade detection efficiency in the actinide region. In particular, we have considered the 238U(d,p)239U and 238U(3He,d)239Np reactions. We have performed Hauser-Feshbach calculations to interpret our results and to verify the hypothesis on which the EXEM is based. The determination of fission and gamma-decay probabilities of 239Np below the neutron separation energy allowed us to validate the EXEM.

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