arXiv subjects

I. V. Doronin

Publications and source records attributed to I. V. Doronin.

8 recordsLinked to original sources

arXiv2025

Resonant pump intensity dependence of luminescence achieved via Floquet engineering

We discover an unexpected behavior in a hybrid system composed of cavity strongly coupled to molecules and subjected to high intensity coherent pumping. We show that if the frequency of the pumping wave is close to polariton transitions in the hybrid system, non monotone dependence of fluorescence and scattering amplitudes on pump intensity with a narrow resonance-like response occurs. We demonstrate that this phenomenon occurs due to hybridization of lower and upper polaritons with substantially different excitation numbers caused by the pumping affecting polariton states of the system. This occurs when the Rabi interaction with coherent field is comparable to the field-matter coupling constant which in turn needs to be sufficient for the manifestation of strong coupling. This non-monotonic dependence of the fluorescence and scattering amplitudes on pump rate intensity pave the way for creation of nonlinear optical devices.

quant-ph↗

arXiv2023

Transition from inhomogeneous to homogeneous broadening at a lasing prethreshold

The emission linewidth in active medium emerges due to homogeneous and inhomogeneous broadening. We demonstrate that in lasers with inhomogeneous broadening there is a critical pump rate, above which the special mode forms. This mode consists of locked-in oscillations of cavity mode and of the active particles with different transition frequencies. Below the critical value of the pump rate, the radiation spectrum of the laser has a Gaussian profile, provided that inhomogeneous broadening is dominant. Above the critical value of pump rate, the special mode mostly determines the laser radiation spectrum. As the result, the spectrum attains Lorentz shape characteristic for homogeneous broadening. We demonstrate that the formation of the special mode precedes lasing and that the critical pump rate plays the role of lasing prethreshold. We obtain expressions for the threshold and generation frequency of single-mode laser where both homogeneous and inhomogeneous broadening are present.

physics.optics↗

arXiv2023

Influence of correlations in active medium on pump-induced exceptional points and strong coupling

Exceptional points show great prospects for applications such as imaging, sensing and designing lasers. Recently, systems with amplifying active medium exhibiting pump-induced exceptional points have attracted much attention due to possibility of controlling strong coupling between light and matter with the aid of pumping. In such structures, the interaction of active molecules with external degrees of freedom, such as phonons or impurities, leads to the destruction of the correlation between polarizations of different molecules. We study the effect of the correlations decay on a system behavior near pump-induced exceptional point. We show that strong coupling persists and eigenvectors together with eigenfrequencies coalesce at a negative value of population inversion, regardless of correlation decay magnitude. Thus, we show that exceptional points are robust to correlation decay, which is crucial for designing systems with exceptional points.

quant-ph↗

arXiv2020

Quantum theory of Rayleigh scattering

We develop a quantum theory of atomic Rayleigh scattering. Scattering is considered as a relaxation of incident photons from a selected mode of free space to the reservoir of the other free space modes. Additional excitations of the reservoir states which appear are treated as scattered light. We show that an entangled state of the excited atom and the incident photon is formed during the scattering. Due to entanglement, a photon is never completely absorbed by the atom. We show that even if the selected mode frequency is incommensurable with any atomic transition frequency, the scattered light spectrum has a maximum at the frequency of the selected mode. The linewidth of scattered light is much smaller than that of the spontaneous emission of a single atom, therefore, the process can be considered as elastic. The developed theory does not use the phenomenological concept of virtual level.

quant-ph↗

arXiv2020

Exceptional points as lasing pre-thresholds in open-cavity lasers

The genesis of lasing, as an evolution of the laser hybrid eigenstates comprised of electromagnetic modes and atomic polarization, is considered. It is shown that the start of coherent generation at the laser threshold is preceded by the formation of a special hybrid state at the lasing pre-threshold. This special state is characterized by an enhanced coupling among excited atoms and electromagnetic modes. This leads to an increase in the rate of stimulated emission in the special state and, ultimately, to lasing. At the lasing pre-threshold, the transformation of hybrid eigenstates has the features of an exceptional point (EP) observed in non-Hermitian systems. The special state is formed when eigenfrequencies of two hybrid states coalesce or come close to each other. Below the pre-threshold, lifetimes of all hybrid states grow with increasing pump rate. When the pump rate crosses the pre-threshold, resonance trapping occurs with the lifetime of the special state continuing to increase while the lifetimes of all other eigenstates begin to decrease. Consequently, the latter eigenstates do not participate in the lasing. Thus, above the pre-threshold, a laser transitions into the single-mode regime.

physics.optics↗

arXiv2019

Self-formation of coherent emission in a cavity-free system

It is commonly accepted that a collection of pumped atoms without a resonator, which provides feedback, cannot lase. We show that intermodal coupling via active atoms pulls the frequencies of the free-space modes towards the transition frequency of the atoms. Although at a low pump rate mode phases randomly fluctuate, phase realizations at which interference of pulled modes is constructive emerge. This results in an increase of stimulated emission into such realizations and makes their lifetime longer. Thus, mode pulling provides positive feedback. When the pump rate exceeds a certain threshold, the lifetime of one of the realizations diverges, and radiation becomes coherent.

physics.optics↗

arXiv2018

Photon statistics of amplified spontaneous emission

Developments in quantum technologies lead to new applications that require radiation sources with specific photon statistics. A widely used Poissonian statistics are easily produced by lasers; however, some applications require super- or sub-Poissonian statistics. Statistical properties of a light source are characterized by the second-order coherence function g^(2)(0). This function distinguishes stimulated radiation of lasers with g^(2)(0)=1 from light of other sources. For example, g^(2)(0)=2 for black-body radiation, and g^(2)(0)=0 for single-photon emission. One of the applications requiring super-Poissonian statistics (g^(2)(0)>1) is ghost imaging with thermal light. Ghost imaging also requires light with a narrow linewidth and high intensity. Currently, rather expensive and inefficient light sources are used for this purpose. In the last year, a superluminescent diode based on amplified spontaneous emission (ASE) has been considered as a new light source for ghost imaging. Even though ASE has been widely studied, its photon statistics has not been settled - there are neither reliable theoretical estimates of the second-order coherence function nor unambiguous experimental data. Our computer simulation clearly establishes that coherence properties of light produced by ASE are similar to that of a thermal source with g^(2)(0)=2 independent of pump power. This result manifests the fundamental difference between ASE and laser radiation.

physics.optics↗

arXiv2017

Inversion of a two-level atom by quantum superoscillations

We show that a two-level atom with a high transition frequency ω_SO can be inverted via non-radiative interaction with a cluster of excited low-frequency two-level atoms or quantum oscillators whose transition frequencies are smaller than ω_SO. This phenomenon occurs due to the Förster resonant energy transfer arising during a train of quantum superoscillation of low-frequency two-level atoms. The suggested model could explain the mechanism of biophoton emission.

physics.optics↗