arXiv subjects

Ian Ford

Publications and source records attributed to Ian Ford.

3 recordsLinked to original sources

arXiv2026

Generation of fully phase controlled two-photon entangled states

Control over the internal states of trapped ions makes them the ideal system to generate single and two-photon states. Coupling a single ion to an optical cavity enables efficient emission of single photons into a single spatial mode and grants control over their temporal shape, phase and frequency. Using the long coherence time of the ion's internal states and employing a scheme to protect the coherence of the ion-cavity interaction, we demonstrate the generation of a two-photon entangled state with full control over the phase. Initially, ion-photon entanglement is generated. A second photon is subsequently generated, mapping the ion's state onto the second photon. By adjusting the drive field the phase of the entangled state can be fully controlled. We implement this scheme in the most resource efficient way by utilizing a single $^{40}$Ca$^+$ ion coupled to an optical cavity and demonstrate the generation of a two-photon entangled stated with full phase control with a fidelity of up to 82\%.

quant-ph↗

arXiv2020

On Generalized Langevin Dynamics and the Modelling of Global Mean Temperature

Climate science employs a hierarchy of models, trading the tractability of simplified energy balance models (EBMs) against the detail of Global Circulation Models. Since the pioneering work of Hasselmann, stochastic EBMs have allowed treatment of climate fluctuations and noise. However, it has recently been claimed that observations motivate heavy-tailed temporal response functions in global mean temperature to perturbations. Our complementary approach exploits the correspondence between Hasselmann's EBM and the original mean-reverting stochastic model in physics, Langevin's equation of 1908. We propose mapping a model well known in statistical mechanics, the Mori-Kubo Generalised Langevin Equation (GLE) to generalise the Hasselmann EBM. If present, long range memory then simplifies the GLE to a fractional Langevin equation (FLE). We describe the corresponding EBMs that map to the GLE and FLE, briefly discuss their solutions, and relate them to Lovejoy's new Fractional Energy Balance Model.

cond-mat.stat-mech↗

arXiv2014

Investigating the significance of zero-point motion in small molecular clusters of sulphuric acid and water

The nucleation of particles from trace gases in the atmosphere is an important source of cloud condensation nuclei (CCN), and these are vital for the formation of clouds in view of the high supersaturations required for homogeneous water droplet nucleation. The methods of quantum chemistry have increasingly been employed to model nucleation due to their high accuracy and efficiency in calculating configurational energies; and nucleation rates can be obtained from the associated free energies of particle formation. However, even in such advanced approaches, it is typically assumed that the nuclei have a classical nature, which is questionable for some systems. The importance of zero-point motion (also known as quantum nuclear dynamics) in modelling small clusters of sulphuric acid and water is tested here using the path integral molecular dynamics (PIMD) method at the density functional theory (DFT) level of theory. The general effect of zero-point motion is to distort the mean structure slightly, and to promote the extent of proton transfer with respect to classical behaviour. In a particular configuration of one sulphuric acid molecule with three waters, the range of positions explored by a proton between a sulphuric acid and a water molecule at 300 K (a broad range in contrast to the confinement suggested by geometry optimisation at 0 K) is clearly affected by the inclusion of zero point motion, and similar effects are observed for other configurations.

physics.chem-ph↗