arXiv subjects

Ian Stevenson

Publications and source records attributed to Ian Stevenson.

18 recordsLinked to original sources

arXiv2026

Electrostriction in a Bose-Einstein Condensate of Dipolar Molecules

The recent creation of a Bose-Einstein condensate (BEC) of dipolar molecules has opened a new frontier for many-body quantum systems in which dipolar interactions can drive novel self-organization phenomena. Here, we observe electrostriction in a molecular BEC, an elliptical deformation driven by anisotropic dipolar interactions. We use double microwave dressing, involving $\sigma$- and $\pi$-polarized fields, to control non-axially symmetric dipolar interactions. We compare the experimental observations of electrostriction to a model based on an extended Gross-Pitaevskii equation and find excellent agreement in the regime of weak to moderate interactions. Using electrostriction, we demonstrate that the molecular BEC can be torqued by dynamically changing the orientation of the elliptical $\sigma$ microwave field. This provides a route to setting molecular quantum gases into rotation, opening opportunities to probe vorticity, superfluidity, and supersolidity in strongly dipolar matter.

cond-mat.quant-gas↗

arXiv2026

Mapping the parameter space of double microwave shielding

Double microwave shielding employs $\sigma^{+}$- and $\pi$-polarized microwave fields, tuned close to the lowest rotational transition, to engineer a long-range repulsive barrier between polar molecules. By preventing molecules from reaching the short range, this technique suppresses detrimental two-body losses and recently enabled the realization of molecular Bose-Einstein condensates and self-bound droplets. Yet, the optimal operating regimes of the shielding mechanism remain largely unexplored. Here, by leveraging the underlying universality of the scattering problem, we systematically map the four-dimensional microwave parameter space-spanned by the detunings and intensities of the two fields-to identify configurations that maximize both shielding efficiency and interaction tunability. We define optimal operating regimes as configurations that are strictly free of field-linked bound states while sufficiently suppressing two-body losses to exceed typical lifetimes of ultracold samples. In these regimes, we evaluate the elastic-to-inelastic collision ratios required for efficient evaporative cooling and explore the accessible tuning range of the effective dipolar interactions. Finally, to identify the best platforms for future quantum simulation experiments, we conduct a global survey of candidate molecular species under realistic field constraints. We identify heavy, strongly dipolar molecules as the most promising candidates, demonstrating that they can achieve extreme loss suppression-reaching two-body loss rates as low as $10^{-18}$ cm$^{3}$/s-alongside robust interaction tunability using only moderate field strengths.

cond-mat.quant-gas↗

arXiv2025

Strongly dipolar molecular Bose-Einstein condensates: From few- to many-body physics

Recent advances in molecular cooling have enabled the realization of strongly dipolar Bose--Einstein condensates (BECs) of molecules, and BECs of many different molecular species may become experimentally accessible in the near future. Here, we explore the unique properties of such BECs and the new insights they may offer into dipolar quantum fluids and many-body physics. We explore which parameter regimes can realistically be achieved using currently available experimental techniques, discuss how to implement these techniques, and outline which molecular species are particularly well suited to explore exotic new states of matter. We further determine how state-of-the-art beyond mean-field theories, originally developed for weakly dipolar magnetic gases, can be pushed to their limits and beyond, and what other long-standing questions in the field of dipolar physics may realistically come within reach using molecular systems.

cond-mat.quant-gas↗

arXiv2025

Observation of Self-Bound Droplets of Ultracold Dipolar Molecules

Ultracold gases of dipolar molecules have long been envisioned as a platform for the realization of novel quantum phases. Recent advances in collisional shielding, protecting molecules from inelastic losses, have enabled the creation of degenerate Fermi gases and, more recently, Bose-Einstein condensation of dipolar molecules. However, the observation of quantum phases in ultracold molecular gases that are driven by dipole-dipole interactions has so far remained elusive. In this work, we report the formation of self-bound droplets and droplet arrays in an ultracold gas of strongly dipolar sodium-cesium molecules. Starting from a molecular Bose-Einstein condensate (BEC), microwave dressing fields are used to induce dipole-dipole interactions with controllable strength and anisotropy. By varying the speed at which interactions are induced, covering a dynamic range of four orders of magnitude, we prepare droplets under equilibrium and non-equilibrium conditions, observing a transition from robust one-dimensional (1D) arrays to fluctuating two-dimensional (2D) structures. The droplets exhibit densities up to 100 times higher than the initial BEC, reaching the strongly interacting regime, and suggesting the possibility of a quantum-liquid or crystalline state. This work establishes ultracold molecules as a system for the exploration of strongly dipolar quantum matter and opens the door to the realization of self-organized crystal phases and dipolar spin liquids in optical lattices.

cond-mat.quant-gas↗

arXiv2025

Extreme Loss Suppression and Wide Tunability of Dipolar Interactions in an Ultracold Molecular Gas

Ultracold dipolar molecules hold great promise for the creation of novel quantum states of matter, but the realization of long-lived molecular bulk samples with strong dipole-dipole interactions has remained elusive. Here, we realize a collisionally stable gas of ultracold ground state molecules with a lifetime of several seconds. Utilizing double microwave dressing, we achieve an extreme suppression of inelastic two- and three-body losses by factors of more than 10,000 and 1,000, respectively. We find that losses remain suppressed across a wide range of dipole-dipole interactions, allowing the continuous tuning of the dipolar length from 0 to 1 um $\sim$ 20,000 $a_0$. Combined with the recent realization of Bose-Einstein condensation of dipolar molecules, our findings open the door to the exploration of strongly dipolar quantum liquids.

cond-mat.quant-gas↗

arXiv2025

Double Microwave Shielding

We develop double microwave shielding, which has recently enabled evaporative cooling to the first Bose-Einstein condensate of polar molecules [Bigagli et al., Nature 631, 289 (2024)]. Two microwave fields of different frequency and polarization are employed to effectively shield polar molecules from inelastic collisions and three-body recombination. Here, we describe in detail the theory of double microwave shielding. We demonstrate that double microwave shielding effectively suppresses two- and three-body losses. Simultaneously, dipolar interactions and the scattering length can be flexibly tuned, enabling comprehensive control over interactions in ultracold gases of polar molecules. We show that this approach works universally for a wide range of molecules. This opens the door to studying many-body physics with strongly interacting dipolar quantum matter.

cond-mat.quant-gas↗

arXiv2024

Three-Body Recombination of Ultracold Microwave-Shielded Polar Molecules

A combined experimental and theoretical study is carried out on the three-body recombination process in a gas of microwave-shielded polar molecules. For ground-state polar molecules dressed with a strong microwave field, field-linked bound states can appear in the intermolecular potential. We model three-body recombination into such bound states using classical trajectory calculations. Our results show that recombination can explain the enhanced loss rates observed at small microwave detunings in trapped samples of bosonic NaCs [Bigagli, $\textit{et al.}$, Nat. Phys. $\textbf{19}$ 1579-1584 (2023)]. Specifically, our calculations reproduce the experimentally measured three-body loss rates across a wide range of microwave Rabi couplings, detunings, and temperatures. This work suggests that for bosonic shielded molecular systems in which the two-body loss is sufficiently suppressed and a field-linked bound state is present, the dominant loss process will be three-body recombination.

cond-mat.quant-gas↗

arXiv2024

Dressed-State Spectroscopy and Magic Trapping of Microwave-Shielded NaCs Molecules

We report on the optical polarizability of microwave-shielded ultracold NaCs molecules in an optical dipole trap. While dressing a pair of rotational states with a microwave field, we observe a marked dependence of the optical polarizability on the intensity and detuning of the dressing field. To precisely characterize differential energy shifts between dressed rotational states, we establish dressed-state spectroscopy. For strong dressing fields, we find that a magic rotational transition can be engineered and demonstrate its insensitivity to laser intensity fluctuations. The results of this work have direct relevance for evaporative cooling and the recent demonstration of molecular Bose-Einstein condensates [Bigagli, et al., Nature (2024)] and may open a door to precision microwave spectroscopy in interacting many-body systems of microwave-shielded molecules.

cond-mat.quant-gas↗

arXiv2023

Observation of Bose-Einstein Condensation of Dipolar Molecules

Ensembles of particles governed by quantum mechanical laws exhibit fascinating emergent behavior. Atomic quantum gases, liquid helium, and electrons in quantum materials all show distinct properties due to their composition and interactions. Quantum degenerate samples of bosonic dipolar molecules promise the realization of novel phases of matter with tunable dipolar interactions and new avenues for quantum simulation and quantum computation. However, rapid losses, even when reduced through collisional shielding techniques, have so far prevented cooling to a Bose-Einstein condensate (BEC). In this work, we report on the realization of a BEC of dipolar molecules. By strongly suppressing two- and three-body losses via enhanced collisional shielding, we evaporatively cool sodium-cesium (NaCs) molecules to quantum degeneracy. The BEC reveals itself via a bimodal distribution and a phase-space-density exceeding one. BECs with a condensate fraction of 60(10) % and a temperature of 6(2) nK are created and found to be stable with a lifetime close to 2 seconds. This work opens the door to the exploration of dipolar quantum matter in regimes that have been inaccessible so far, promising the creation of exotic dipolar droplets, self-organized crystal phases, and dipolar spin liquids in optical lattices.

cond-mat.quant-gas↗

arXiv2023

A planar cloverleaf antenna for the creation of circularly polarized microwave fields

We report on the design and characterization of a compact microwave antenna for atomic and molecular physics experiments. The antenna is comprised of four loop antennas arranged in cloverleaf shape, allowing for precise adjustment of polarization by tuning the relative phase of the loops. We optimize the antenna for left-circularly polarized microwaves at 3.5 GHz and characterize its performance using ultracold NaCs molecules as a precise quantum sensor. Observing an unusually high Rabi frequency of $2\pi \times 46$ MHz, we extract an electric field amplitude of 33(2) V/cm at 22 mm distance from the antenna. The polarization ellipticity is 2.3(4) degrees, corresponding to a 24 dB suppression of right-circular polarization. The cloverleaf antenna is planar and provides large optical access, making it highly suitable for quantum control of atoms and molecules, and potentially other quantum systems that operate in the microwave regime.

physics.atom-ph↗

arXiv2023

Collisionally Stable Gas of Bosonic Dipolar Ground State Molecules

Stable ultracold ensembles of dipolar molecules hold great promise for many-body quantum physics, but high inelastic loss rates have been a long-standing challenge. Recently, it was shown that gases of fermionic molecules can be effectively stabilized through external fields. However, many quantum applications will benefit from molecular ensembles with bosonic statistics. Here, we stabilize a bosonic gas of strongly dipolar NaCs molecules against inelastic losses via microwave shielding, decreasing losses by more than a factor of 200 and reaching lifetimes on the scale of 1 second. We also measure high elastic scattering rates, a result of strong dipolar interactions, and observe the anisotropic nature of dipolar collisions. Finally, we demonstrate evaporative cooling of a bosonic molecular gas to a temperature of 36(5) nK, increasing its phase-space density by a factor of 20. This work is a critical step towards the creation of a Bose-Einstein condensate of dipolar molecules.

cond-mat.quant-gas↗

arXiv2023

Efficient Pathway to NaCs Ground State Molecules

We present a study of two-photon pathways for the transfer of NaCs molecules to their rovibrational ground state. Starting from NaCs Feshbach molecules, we perform bound-bound excited state spectroscopy in the wavelength range from 900~nm to 940~nm, covering more than 30 vibrational states of the $c \, ^3\Sigma^+$, $b \, ^3\Pi$, and $B \, ^1\Pi$ electronic states. Analyzing the rotational substructure, we identify the highly mixed $c \, ^3\Sigma^+_1 \, |v=22 \rangle \sim b \, ^3\Pi_1 \, | v=54\rangle$ state as an efficient bridge for stimulated Raman adiabatic passage (STIRAP). We demonstrate transfer into the NaCs ground state with an efficiency of up to 88(4)\%. Highly efficient transfer is critical for the realization of many-body quantum phases of strongly dipolar NaCs molecules and high fidelity detection of single molecules, for example, in spin physics experiments in optical lattices and quantum information experiments in optical tweezer arrays.

physics.atom-ph↗

arXiv2022

Jet-Loaded Cold Atomic Beam Source for Strontium

We report on the design and characterization of a cold atom source for strontium (Sr) based on a two-dimensional magneto-optical trap (MOT) that is directly loaded from the atom jet of a dispenser. We characterize the atom flux of the source by measuring the loading rate of a three-dimensional MOT. We find loading rates of up to $10^{8}$ atoms per second. The setup is compact, easy to construct, and has low power consumption. It addresses the long standing challenge of reducing the complexity of cold beam sources for Sr, which is relevant for optical atomic clocks and quantum simulation and computing devices based on ultracold Sr.

physics.atom-ph↗

arXiv2022

Ultracold Gas of Dipolar NaCs Ground State Molecules

We report on the creation of bosonic NaCs molecules in their absolute rovibrational ground state via stimulated Raman adiabatic passage. We create ultracold gases with up to 22,000 dipolar NaCs molecules at a temperature of 300(50) nK and a peak density of $1.0(4) \times 10^{12}$ cm$^{-3}$. We demonstrate comprehensive quantum state control by preparing the molecules in a specific electronic, vibrational, rotational, and hyperfine state. Employing the tunability and strength of the permanent electric dipole moment of NaCs, we induce dipole moments of up to 2.6 D. Dipolar systems of NaCs molecules are uniquely suited to explore strongly interacting phases in dipolar quantum matter.

cond-mat.quant-gas↗

arXiv2022

A High Phase-Space Density Gas of NaCs Feshbach Molecules

We report on the creation of ultracold gases of bosonic Feshbach molecules of NaCs. The molecules are associated from overlapping gases of Na and Cs using a Feshbach resonance at 864.12(5) G. We characterize the Feshbach resonance using bound state spectroscopy, in conjunction with a coupled-channel calculation. By varying the temperature and atom numbers of the initial atomic mixtures, we demonstrate the association of NaCs gases over a wide dynamic range of molecule numbers and temperatures, reaching 70 nK for our coldest systems and a phase-space density near 0.1. This is an important stepping-stone for the creation of degenerate gases of strongly dipolar NaCs molecules in their absolute ground state.

cond-mat.quant-gas↗

arXiv2021

Overlapping Bose-Einstein Condensates of $^{23}$Na and $^{133}$Cs

We report on the creation of dual-species Bose-Einstein condensates (BECs) of $^{23}$Na atoms and $^{133}$Cs atoms. We demonstrate sympathetic cooling of Cs with Na in a magnetic quadrupole trap and a crossed optical dipole trap, leading to Na BECs with $8 \times 10^5$ atoms and Cs BECs with $3.5 \times 10^4$ atoms. Investigating cross-thermalization and lifetimes of the mixture, we find that the Na and Cs BECs are miscible and overlapping, interacting with a moderate interspecies scattering length of $18(4)\,a_0$ at $23\,$G and $29(4)\,a_0$ at $894\,$G and coexisting for tens of seconds. Overlapping condensates of Na and Cs offer new possibilities for many-body physics with ultracold bosonic mixtures and constitute an ideal starting point for the creation of ultracold ensembles of NaCs ground state molecules.

cond-mat.quant-gas↗

arXiv2020

Compact Two-Dimensional Magneto-Optical Trap for Ultracold Atom Setups

We report on the design, implementation, and performance of a compact two-dimensional magneto-optical trap (2D MOT) for cesium. In a small-volume vacuum chamber, the setup uses cesium dispensers in close proximity to the trapping region of the 2D MOT and operates at low vapor pressures in the $10^{-9}$ torr range. We achieve a cold atom flux of $4 \times 10^8$ atoms/s that is comparable to the performance of more complex atomic sources. The setup is simple to construct and can be adapted to a broad range of atomic species.

physics.atom-ph↗

arXiv2017

Genetic fitting techniques for precision ultracold spectroscopy

We present development of a genetic algorithm for fitting potential energy curves of diatomic molecules to experimental data. Our approach does not involve any functional form for fitting, which makes it a general fitting procedure. In particular, it takes in a guess potential, perhaps from an $ab \ initio$ calculation, along with experimental measurements of vibrational binding energies, rotational constants, and their experimental uncertainties. The fitting procedure is able to modify the guess potential until it converges to better than 1% uncertainty, as measured by $\barχ^2$. We present the details of this technique along with a comparison of potentials calculated by our genetic algorithm and the state of the art fitting techniques based on inverted perturbation approach for the $X \ ^1Σ^+$ and $C \ ^1Σ^+$ potentials of lithium-rubidium.

physics.chem-ph↗