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Iliya Esin

Publications and source records attributed to Iliya Esin.

17 recordsLinked to original sources

Self-organized Floquet band geometry in cavity-driven quantum materials

Floquet engineering has emerged as a powerful route to dynamically control band structure and topology in quantum materials, but most implementations rely on externally imposed laser fields that are power intensive, difficult to integrate into devices, and weakly coupled to the electronic system. We propose and analyze an alternative paradigm in which a self-generated cavity field Floquet-dresses the electronic bands and produces a geometric Hall response in an electrically driven cavity material system. We consider a semiconductor layer embedded in a cavity and coupled to external leads and a bath of acoustic phonons, where dc pumping leads to the buildup of a coherent intracavity field through light-matter coupling. We determine the resulting nonequilibrium steady state self-consistently and show that, above threshold, the coupled system settles into a stable time-periodic limit cycle with a field amplitude set by the cavity quality factor and dissipation. This emergent periodic field Floquet-dresses the electronic bands and modifies the anomalous Hall response of a material with broken time-reversal symmetry. We demonstrate that the resulting Hall conductivity can be directly probed via in-plane dc transport measurements. Our work establishes a route to self organized Floquet band reconstruction and geometric transport without external laser illumination, highlighting cavity driven steady states as a platform for electrically controlled nonequilibrium phases.

cond-mat.mes-hall

Light-induced trion-exciton competition revealed by ultrafast photoemission

Strong Coulomb interactions in low-dimensional quantum materials give rise to emergent bound states such as excitons and trions. Trions are conventionally secondary excitations, requiring both optical excitation and charge doping. In quasi-one-dimensional Ta$_2$NiS$_5$, however, an exceptionally large binding energy exceeding the single-particle band gap stabilizes an equilibrium trion gas under surface doping alone. Here, using time- and angle-resolved photoemission spectroscopy, we show that trions can also be generated purely optically, without external charge. Following photoexcitation of pristine Ta$_2$NiS$_5$ we observe a bright, momentum-localized, in-gap feature with a slow, fluence-dependent relaxation. Rate-equation modeling identifies it as a mixed population of trions and excitons, with the trions formed via an unconventional single-particle pathway that requires no photoexcited hole. The trion-exciton composition is controlled by pump fluence, with trions dominating the late-time relaxation. In surface doped samples, the same model with unchanged rates reproduces the full dynamics, linking the light-induced trions to their equilibrium counterparts through pump-induced dissociation and recapture. These results establish trARPES as a direct probe of charged quasiparticles far from equilibrium and open routes to optical control of neutral and charged excitations in correlated materials.

cond-mat.str-el

Time-hidden magnetic order in a multi-orbital Mott insulator

Photo-excited quantum materials can be driven into thermally inaccessible metastable states that exhibit structural, charge, spin, topological and superconducting orders. Metastable states typically emerge on timescales set by the intrinsic electronic and phononic energy scales, ranging from femtoseconds to picoseconds, and can persist for weeks. Therefore, studies have primarily focused on ultrafast or quasi-static limits, leaving the intermediate time window less explored. Here we reveal a metastable state with broken glide-plane symmetry in photo-doped Ca$_2$RuO$_4$ using time-resolved optical second-harmonic generation and birefringence measurements. We find that the metastable state appears long after intralayer antiferromagnetic order has melted and photo-carriers have recombined. Its properties are distinct from all known states in the equilibrium phase diagram and are consistent with intralayer ferromagnetic order. Furthermore, model Hamiltonian calculations reveal that a non-thermal trajectory to this state can be accessed via photo-doping. Our results expand the search space for out-of-equilibrium electronic matter to metastable states emerging at intermediate timescales.

cond-mat.str-el

Quantum geometry and bounds on dissipation in slowly driven quantum systems

We show that energy dissipation in slowly-driven, Markovian quantum systems at low temperature is linked to the geometry of the driving protocol through the quantum (or Fubini-Study) metric. Utilizing these findings, we establish lower bounds on dissipation rates in two-tone protocols, such as those employed for topological frequency conversion. Notably, in appropriate limits these bounds are only determined by the topology of the protocol and an effective quality factor of the system-bath coupling. Our results bridge topological and geometric phenomena with energy dissipation in open quantum systems, and further provide design principles for optimal driving protocols.

quant-ph

Topological frequency conversion in rhombohedral multilayer graphene

We show that rhombohedral multilayer graphene supports topological frequency conversion, whereby a fraction of electrons transfer energy between two monochromatic light sources at a quantized rate. The pristine nature and gate tunability of these materials, along with a Berry curvature that directly couples to electric fields, make them ideal platforms for the experimental realization of topological frequency conversion. Among the rhombohedral family, we find that Bernal bilayer graphene appears most promising for THz-scale applications due to lower dissipation. We discuss strategies to circumvent cancellations between the two valleys of graphene and to minimize dissipative losses using commensurate frequencies, thus opening a potential pathway for net amplification.

cond-mat.mes-hall

Evidence of Floquet electronic steady states in graphene under continuous-wave mid-infrared irradiation

Light-induced phenomena in materials can exhibit exotic behavior that extends beyond equilibrium properties, offering new avenues for understanding and controlling electronic phases. So far, non-equilibrium phenomena in solids have been predominantly explored using femtosecond laser pulses, which generate transient, ultra-fast dynamics. Here, we investigate the steady non-equilibrium regime in graphene induced by a continuous-wave (CW) mid-infrared laser. Our transport measurements reveal signatures of a long-lived Floquet phase, where a non-equilibrium electronic population is stabilized by the interplay between coherent photoexcitation and incoherent phonon cooling. The observation of non-equilibrium steady states using CW lasers opens a new regime for low-temperature Floquet phenomena, paving the way toward Floquet engineering of steady-state phases of matter.

cond-mat.mes-hall

Quantized Acoustoelectric Floquet Effect in Quantum Nanowires

External coherent fields can drive quantum materials into non-equilibrium states, revealing exotic properties that are unattainable under equilibrium conditions -- an approach known as ``Floquet engineering.'' While optical lasers have commonly been used as the driving fields, recent advancements have introduced nontraditional sources, such as coherent phonon drives. Building on this progress, we demonstrate that driving a metallic quantum nanowire with a coherent wave of terahertz phonons can induce an electronic steady state characterized by a persistent quantized current along the wire. The quantization of the current is achieved due to the coupling of electrons to the nanowire's vibrational modes, providing the low-temperature heat bath and energy relaxation mechanisms. Our findings underscore the potential of using non-optical drives, such as coherent phonon sources, to induce non-equilibrium phenomena in materials. Furthermore, our approach suggests a new method for the high-precision detection of coherent phonon oscillations via transport measurements.

cond-mat.mes-hall

Hyperbolic phonon-polariton electroluminescence in graphene-hBN van der Waals heterostructures

Phonon-polaritons are electromagnetic waves resulting from the coherent coupling of photons with optical phonons in polar dielectrics. Due to their exceptional ability to confine electric fields to deep subwavelength scales with low loss, they are uniquely poised to enable a suite of applications beyond the reach of conventional photonics, such as sub-diffraction imaging and near-field energy transfer. The conventional approach to exciting phonon-polaritons through optical methods, however, necessitates costly mid-infrared and terahertz coherent light sources along with near-field scanning probes, and generally leads to low excitation efficiency due to the substantial momentum mismatch between phonon-polaritons and free-space photons. Here, we demonstrate that under proper conditions, phonon-polaritons can be excited all-electrically by flowing charge carriers. Specifically, in hexagonal boron nitride (hBN)/graphene heterostructures, by electrically driving charge carriers in ultra-high-mobility graphene out of equilibrium, we observe bright electroluminescence of hBN's hyperbolic phonon-polaritons (HPhPs) at mid-IR frequencies. The HPhP electroluminescence shows a temperature and carrier density dependence distinct from black-body or super-Planckian thermal emission. Moreover, the carrier density dependence of HPhP electroluminescence spectra reveals that HPhP electroluminescence can arise from both inter-band transition and intra-band Cherenkov radiation of charge carriers in graphene. The HPhP electroluminescence offers fundamentally new avenues for realizing electrically-pumped, tunable mid-IR and THz phonon-polariton lasers, and efficient cooling of electronic devices.

cond-mat.mes-hall

Optical Control of Slow Topological Electrons in Moiré Systems

Floquet moiré materials possess optically-induced flat-electron bands with steady-states sensitive to drive parameters. Within this regime, we show that strong interaction screening and phonon bath coupling can overcome enhanced drive-induced heating. In twisted bilayer graphene (TBG) irradiated by a terahertz-frequency continuous circularly polarized laser, the extremely slow electronic states enable the drive to control the steady state occupation of high-Berry curvature electronic states. In particular, above a critical field amplitude, high-Berry-curvature states exhibit a slow regime where they decouple from acoustic phonons, allowing the drive to control the anomalous Hall response. Our work shows that the laser-induced control of topological and transport physics in Floquet TBG are measurable using experimentally available probes.

cond-mat.mes-hall

Generating coherent phonon waves in narrow-band materials: a twisted bilayer graphene phaser

Twisted bilayer graphene (TBG) exhibits extremely low Fermi velocities for electrons, with the speed of sound surpassing the Fermi velocity. This regime enables the use of TBG for amplifying vibrational waves of the lattice through stimulated emission, following the same principles of operation of free-electron lasers. Our work proposes a lasing mechanism relying on the slow-electron bands to produce a coherent beam of acoustic phonons. We propose a device based on undulated electrons in TBG, which we dub the phaser. The device generates phonon beams in a terahertz (THz) frequency range, which can then be used to produce THz electromagnetic radiation. The ability to generate coherent phonons in solids breaks new ground in controlling quantum memories, probing quantum states, realizing non-equilibrium phases of matter, and designing new types of THz optical devices.

cond-mat.mes-hall

Universal transport in periodically driven systems without long-lived quasiparticles

An intriguing regime of universal charge transport at high entropy density has been proposed for periodically driven interacting one-dimensional systems with Bloch bands separated by a large single-particle band gap. For weak interactions, a simple picture based on well-defined Floquet quasiparticles suggests that the system should host a quasisteady state current that depends only on the populations of the system's Floquet-Bloch bands and their associated quasienergy winding numbers. Here we show that such topological transport persists into the strongly interacting regime where the single-particle lifetime becomes shorter than the drive period. Analytically, we show that the value of the current is insensitive to interaction-induced band renormalizations and lifetime broadening when certain conditions are met by the system's non-equilibrium distribution function. We show that these conditions correspond to a quasisteady state. We support these predictions through numerical simulation of a system of strongly interacting fermions in a periodically-modulated chain of Sachdev-Ye-Kitaev dots. Our work establishes universal transport at high entropy density as a robust far from equilibrium topological phenomenon, which can be readily realized with cold atoms in optical lattices.

cond-mat.quant-gas

Electronic Floquet Liquid Crystals

"Floquet engineering" - designing band structures "on-demand" through the application of coherent time-periodic drives - has recently emerged as a powerful tool for creating new topological and anomalous phases of matter. In this manuscript, we show that the same principle can be applied to create non-equilibrium correlated states with spontaneously broken symmetry in a lightly doped semiconductor. The periodic drive provides means for obtaining large electronic densities of states necessary for the broken symmetry phase. The phase transition occurs in the steady-state of the system achieved due to interplay between the coherent external drive, electron-electron interactions, and dissipative processes arising from the coupling to phonons and the electromagnetic environment. We obtain the phase diagram of the system using numerical calculations that match predictions obtained from a phenomenological treatment and discuss the conditions on the system and the external drive under which spontaneous symmetry breaking occurs. Our results imply that Floquet engineering of the density of states provides a new route for generating and controlling correlated states of electrons with external fields.

cond-mat.str-el

Detection of quantum interference without interference

Quantum interference is typically detected through the dependence of the interference signal on certain parameters (path length, Aharonov-Bohm flux, etc.), which can be varied in a controlled manner. The destruction of interference by a which-path measurement is a paradigmatic manifestation of quantum effects. Here we report on a novel measurement protocol that realizes two objectives: (i) certifying that a measured signal is the result of interference avoiding the need to vary parameters of the underlying interferometer, and (ii) certifying that the interference signal at hand is of quantum nature. In particular, it yields a null outcome in the case of classical interference. Our protocol comprises measurements of cross-correlations between the readings of which-path weakly coupled detectors positioned at the respective interferometer's arms and the current in one of the interferometer's drains. We discuss its implementation with an experimentally available platform: an electronic Mach-Zehnder interferometer (MZI) coupled electrostatically to "detectors" (quantum point contacts).

cond-mat.mes-hall

Floquet metal to insulator phase transitions in semiconductor nanowires

We study steady-states of semiconductor nanowires subjected to strong resonant time-periodic drives. The steady-states arise from the balance between electron-phonon scattering, electron-hole recombination via photo-emission, and Auger scattering processes. We show that tuning the strength of the driving field drives a transition between an electron-hole metal (EHM) phase and a Floquet insulator (FI) phase. We study the critical point controlling this transition. The EHM-to-FI transition can be observed by monitoring the presence of peaks in the density-density response function which are associated with the Fermi momentum of the EHM phase, and are absent in the FI phase. Our results may help guide future studies towards inducing novel non-equilibrium phases of matter by periodic driving.

cond-mat.mes-hall

Steady states and edge state transport in topological Floquet-Bloch systems

We study the open system dynamics and steady states of two dimensional Floquet topological insulators: systems in which a topological Floquet-Bloch spectrum is induced by an external periodic drive. We solve for the bulk and edge state carrier distributions, taking into account energy and momentum relaxation through radiative recombination and electron-phonon interactions, as well as coupling to an external lead. We show that the resulting steady state resembles a topological insulator in the Floquet basis. The particle distribution in the Floquet edge modes exhibits a sharp feature akin to the Fermi level in equilibrium systems, while the bulk hosts a small density of excitations. We discuss two-terminal transport and describe the regimes where edge-state transport can be observed. Our results show that signatures of the non-trivial topology persist in the non-equilibrium steady state.

cond-mat.mes-hall

How to extract weak values from a mesoscopic electronic system

Weak value (WV) protocols may lead to extreme expectation values that are larger than the corresponding orthodox expectation values. Recent works have proposed to implement this concept in nano-scale electronic systems. Here we address the issue of how one calibrates the setup in question, maximizes the measurement's sensitivity, and extracts distinctly large WVs. Our concrete setup consists of two Mach-Zehnder interferometers (MZIs): the "system" and the "detector". Such setups have already been implemented in experiment.

cond-mat.mes-hall

Crossover between strong and weak measurement in interacting many-body systems

Measurements with variable system-detector interaction strength, ranging from weak to strong, have been recently reported in a number of electronic nanosystems. In several such instances many-body effects play a significant role. Here we consider the weak--to--strong crossover for a setup consisting of an electronic Mach-Zehnder interferometer, where a second interferometer is employed as a detector. In the context of a conditional which-path protocol, we define a generalized conditional value (GCV), and determine its full crossover between the regimes of weak and strong (projective) measurement. We find that the GCV has an oscillatory dependence on the system-detector interaction strength. These oscillations are a genuine many-body effect, and can be experimentally observed through the voltage dependence of cross current correlations.

cond-mat.mes-hall