arXiv subjects

Ilja Gerhardt

Publications and source records attributed to Ilja Gerhardt.

At least 37 records · Page 2Linked to original sources

arXiv2015

Faraday Filtering on the Cs-D$_1$-Line for Quantum Hybrid Systems

Narrow-band filtering of light is widely used in optical spectroscopy. Atomic filters, which rely on the Faraday effect, allow for GHz-wide transmission spectra, which are intrinsically matched to an atomic transition. We present an experimental realization and a theoretical study of a Faraday anomalous dispersion optical filter (FADOF) based on cesium and its D$_1$-line-transition ($6^2S_{1/2}\rightarrow6^2P_{1/2}$) around 894nm. We also present the prospects and visions for combining this filter with the single photon emission of a single quantum dot (QD), which matches with the atomic transition.

physics.atom-ph↗

arXiv2015

Single Molecule DNA Detection with an Atomic Vapor Notch Filter

The detection of single molecules has facilitated many advances in life- and material-sciences. Commonly, it founds on the fluorescence detection of single molecules, which are for example attached to the structures under study. For fluorescence microscopy and sensing the crucial parameters are the collection and detection efficiency, such that photons can be discriminated with low background from a labeled sample. Here we show a scheme for filtering the excitation light in the optical detection of single stranded labeled DNA molecules. We use the narrow-band filtering properties of a hot atomic vapor to filter the excitation light from the emitted fluorescence of a single emitter. The choice of atomic sodium allows for the use of fluorescent dyes, which are common in life-science. This scheme enables efficient photon detection, and a statistical analysis proves an enhancement of the optical signal of more than 15% in a confocal and in a wide-field configuration.

physics.optics↗

arXiv2015

Observation of Topological Structures in Photonic Quantum Walks

Phases of matter with non-trivial topological order are predicted to exhibit a variety of exotic phenomena, such as the existence robust localized bound states in 1D systems, and edge states in 2D systems, which are expected to display spin-helicity, immunity to back-scattering, and weak anti-localization. In this Letter, we present an experimental observation of topological structures generated via the controlled implementation of two consecutive non-commuting rotations in photonic discrete-time quantum walks. The second rotation introduces valley-like Dirac points in the system, allowing to create the non-trivial topological pattern. By choosing specific values for the rotations, it is possible to coherently drive the system between topological sectors characterized by different topological invariants. We probe the full topological landscape, demonstrating the emergence of localized bound states hosted at the topological boundaries, and the existence of extremely localized or delocalized non-Gaussian quantum states. Our results pave the way for the study of valley-based electronics and applications of topological mechanisms in robust optical-device engineering.

quant-ph↗

arXiv2014

Modification of the Absorption Cross Section in the Optical Near-field

The optical interaction of light and matter is modeled as an oscillating dipole in a plane wave. We analyze absorption, scattering and extinction for this system by the energy flow, which is depicted by streamlines of the Poynting vector. Depending on the dissipative damping of the oscillator, the streamlines end up in the dipole. Based on a graphical investigation of the streamlines, this represents the absorption cross section, and forms a far-field absorption aperture. In the near-field of the oscillator, a modification of the aperture is observed. This scheme can be adapted to a single dipolar emitter, interacting with a light field. In the case of the absorption by a single atom, where the oscillator has a circular dipole characteristics, we model the energy flow and derive the apertures.

physics.optics↗

arXiv2014

Better Randomness with Single Photons

Randomness is one of the most important resources in modern information science, since encryption founds upon the trust in random numbers. Since it is impossible to prove if an existing random bit string is truly random, it is relevant that they be generated in a trust worthy process. This requires specialized hardware for random numbers, for example a die or a tossed coin. But when all input parameters are known, their outcome might still be predicted. A quantum mechanical superposition allows for provably true random bit generation. In the past decade many quantum random number generators (QRNGs) were realized. A photonic implementation is described as a photon which impinges on a beam splitter, but such a protocol is rarely realized with non-classical light or anti-bunched single photons. Instead, laser sources or light emitting diodes are used. Here we analyze the difference in generating a true random bit string with a laser and with anti-bunched light. We show that a single photon source provides more randomness than even a brighter laser. This gain of usable entropy proves the advantages of true single photons versus coherent input states of light in an experimental implementation. The underlying advantage can be adapted to microscopy and sensing.

quant-ph↗

arXiv2014

Coherent control of single spins in silicon carbide at room temperature

Spins in solids are cornerstone elements of quantum spintronics. Leading contenders such as defects in diamond, or individual phosphorous dopants in silicon have shown spectacular progress but either miss established nanotechnology or an efficient spin-photon interface. Silicon carbide (SiC) combines the strength of both systems: It has a large bandgap with deep defects and benefits from mature fabrication techniques. Here we report the characterization of photoluminescence and optical spin polarization from single silicon vacancies in SiC, and demonstrate that single spins can be addressed at room temperature. We show coherent control of a single defect spin and find long spin coherence time under ambient conditions. Our study provides evidence that SiC is a promising system for atomic-scale spintronics and quantum technology.

cond-mat.mes-hall↗

arXiv2014

Microscopic diamond Solid-Immersion-Lenses fabricated around single defect ceneters by focussed ion beam milling

Recent efforts to define microscopic solid-immersion-lenses (SIL) by focused ion beam milling into diamond substrates that are registered to a preselected single photon emitter are summarized. We show how we determine the position of a single emitter with at least 100 nm lateral and 500 nm axial accuracy, and how the milling procedure is optimized. The characteristics of a single emitter, a Nitrogen Vacancy (NV) center in diamond, are measured before and after producing the SIL and compared with each other. A count rate of 1.0 million counts per second is achieved with a $[111]$ oriented NV center.

physics.optics↗

arXiv2013

A universal setup for active control of a single-photon detector

The influence of bright light on a single-photon detector has been described in a number of recent publications. The impact on quantum key distribution (QKD) is important, and several hacking experiments have been tailored to fully control single-photon detectors. Special attention has been given to avoid introducing further errors into a QKD system. We describe the design and technical details of an apparatus which allows to attack a quantum-cryptographic connection. This device is capable of controlling free-space and fiber-based systems and of minimizing unwanted clicks in the system. With different control diagrams, we are able to achieve a different level of control. The control was initially targeted to the systems using BB84 protocol, with polarization encoding and basis switching using beamsplitters, but could be extended to other types of systems. We further outline how to characterize the quality of active control of single-photon detectors.

quant-ph↗

arXiv2012

Homomorphic Payment Addresses and the Pay-to-Contract Protocol

We propose an electronic payment protocol for typical customer-merchant relations which does not require a trusted (signed) payment descriptor to be sent from the merchant to the customer. Instead, the destination "account" number for the payment is solely created on the customer side. This eliminates the need for any encrypted or authenticated communication in the protocol and is secure even if the merchant's online infrastructure is compromised. Moreover, the payment transaction itself serves as a timestamped receipt for the customer. It proves what has been paid for and who received the funds, again without relying on any merchant signatures. In particular, funds and receipt are exchanged in a single atomic action. The asymmetric nature of the customer-merchant relation is crucial. The protocol is specifically designed with bitcoin in mind as the underlying payment system. Thereby, it has the useful benefit that all transactions are public. However, the only essential requirement on the payment system is that "accounts" are arbitrary user-created keypairs of a cryptosystem whose keypairs enjoy a homomorphic property. All ElGamal-type cryptosystems have this feature. For use with bitcoin we propose the design of a deterministic bitcoin wallet whose addresses can be indexed by clear text strings.

cs.CR↗

arXiv2012

Excitation and emission spectra of rubidium in rare-gas thin-films

To understand the optical properties of atoms in solid state matrices, the absorption, excitation and emission spectra of rubidium doped thin-films of argon, krypton and xenon were investigated in detail. A two-dimensional spectral analysis extends earlier reports on the excitation and emission properties of rubidium in rare-gas hosts. We found that the doped crystals of krypton and xenon exhibit a simple absorption-emission relation, whereas rubidium in argon showed more complicated spectral structures. Our sample preparation employed in the present work yielded different results for the Ar crystal, but our peak positions were consistent with the prediction based on the linear extrapolation of Xe and Kr data. We also observed a bleaching behavior in rubidium excitation spectra, which suggests a population transfer from one to another spectral feature due to hole-burning. The observed optical response implies that rubidium in rare-gas thin-films is detectable with extremely high sensitivity, possibly down to a single atom level, in low concentration samples.

physics.atom-ph↗

arXiv2012

Full-field implementation of a perfect eavesdropper on a quantum cryptography system

Quantum key distribution (QKD) allows two remote parties to grow a shared secret key. Its security is founded on the principles of quantum mechanics, but in reality it significantly relies on the physical implementation. Technological imperfections of QKD systems have been previously explored, but no attack on an established QKD connection has been realized so far. Here we show the first full-field implementation of a complete attack on a running QKD connection. An installed eavesdropper obtains the entire 'secret' key, while none of the parameters monitored by the legitimate parties indicate a security breach. This confirms that non-idealities in physical implementations of QKD can be fully practically exploitable, and must be given increased scrutiny if quantum cryptography is to become highly secure.

quant-ph↗

arXiv2011

Experimentally faking the violation of Bell's inequalities

Entanglement witnesses such as Bell inequalities are frequently used to prove the non-classicality of a light source and its suitability for further tasks. By demonstrating Bell inequality violations using classical light in common experimental arrangements, we highlight why strict locality and efficiency conditions are not optional, particularly in security-related scenarios.

quant-ph↗

arXiv2011

Detection of Single Molecules Illuminated by a Light-Emitting Diode

Optical detection and spectroscopy of single molecules has become an indispensable tool in biological imaging and sensing. Its success is based on fluorescence of organic dye molecules under carefully engineered laser illumination. In this paper we demonstrate optical detection of single molecules on a wide-field microscope with an illumination based on a commercially available, green light-emitting diode. The results are directly compared with laser illumination in the same experimental configuration. The setup and the limiting factors, such as light transfer to the sample, spectral filtering and the resulting signal-to-noise ratio are discussed. A theoretical and an experimental approach to estimate these parameters are presented. The results can be adapted to other single emitter and illumination schemes.

physics.chem-ph↗

arXiv2010

Coherent Nonlinear Single Molecule Microscopy

We investigate a nonlinear localization microscopy method based on Rabi oscillations of single emitters. We demonstrate the fundamental working principle of this new technique using a cryogenic far-field experiment in which subwavelength features smaller than $λ$/10 are obtained. Using Monte Carlo simulations, we show the superior localization accuracy of this method under realistic conditions and a potential for higher acquisition speed or a lower number of required photons as compared to conventional linear schemes. The method can be adapted to other emitters than molecules and allows for the localization of several emitters at different distances to a single measurement pixel.

quant-ph↗

arXiv2009

Control and imaging of single-molecule spectral dynamics using a nano-electrode

We study the influence of a scanning nano-electrode on fluorescence excitation spectra of single terrylene molecules embedded in thin p-terphenyl films at cryogenic temperatures. We show that applied voltages less than 10 V can result in reversible Stark shifts of up to 100 times and linewidth increase greater than 10 times the natural linewidth. We discuss the potential of our experimental scheme for direct imaging of individual two-level systems (TLS) in the nanometer vicinity of single molecules.

physics.chem-ph↗

arXiv2008

Daylight operation of a free space, entanglement-based quantum key distribution system

Many quantum key distribution (QKD) implementations using a free space transmission path are restricted to operation at night time in order to distinguish the signal photons used for a secure key establishment from background light. Here, we present a lean entanglement-based QKD system overcoming that imitation. By implementing spectral, spatial and temporal filtering techniques, we were able to establish a secure key continuously over several days under varying light and weather conditions.

quant-ph↗

arXiv2008

Coherent State Preparation and Observation of Rabi Oscillations in a Single Molecule

We report on the excitation of single molecules via narrow zero-phonon transitions using short laser pulses. By monitoring the Stokes-shifted fluorescence, we studied the excited state population as a function of the delay time, laser intensity, and frequency detuning. A pi-pulse excitation was demonstrated with merely 500 photons, and 5 Rabi cycles were achieved at higher excitation powers. Our findings are in good agreement with theoretical calculations and provide a first step toward coherent manipulation of the electronic states of single molecules with few photons.

quant-ph↗

arXiv2008

Exploring the limits of single emitter detection in fluorescence and extinction

We present an experimental comparison and a theoretical analysis of the signal-to-noise ratios in fluorescence and extinction spectroscopy of a single emitter. We show that extinction measurements can be advantageous if the emitter is weakly excited. Furthermore, we discuss the potential of this method for the detection and spectroscopy of weakly emitting systems such as rare earth ions.

quant-ph↗