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Ilya M. Eremin

Publications and source records attributed to Ilya M. Eremin.

At least 19 recordsLinked to original sources

Experimental signature of transient symmetry breaking in a cavity superconductor

Transient states of matter far from equilibrium may exhibit physical properties beyond those allowed by the equilibrium-state crystalline symmetries. We explore ultrafast and direct electronic excitations of transient states in a cavity superconductor by using time-resolved terahertz-pump terahertz-probe spectroscopy. Our results show that the strong terahertz field can transiently modify the symmetries of the electronic subsystems via the injection of a transient supercurrent, leading to high-order nonlinear dynamical responses that are not compatible with the equilibrium-state symmetries, which evidences for transient symmetry breaking on the picosecond time scale. Our study also finds that the strong coupling of the superconductor to the designed microcavities enables the sensitive detection of the nonlinear responses associated to the transient symmetry breaking.

cond-mat.supr-con↗

Nodal Orbital-Anti-Phase Superconducting State in Bilayer Nickelates

The recent discovery of high-$T_c$ superconductivity in the bilayer nickelate La$_3$Ni$_2$O$_7$ (La-327) under applied pressure and compressive strain opened a new avenue to elucidate the interplay between multiorbital intralayer and interlayer electronically driven Cooper-pairing in bilayer systems. Depending on the details of the electronic structure in the normal state, the superconducting gap in bilayer nickelates is predicted to have either bonding-antibonding $s_{\pm}$-wave symmetry, driven by dominant interlayer Cooper-pairing, or $d$-wave symmetry with substantial intralayer Cooper-pairing. Despite this general picture, the orbital structure of the superconducting gap in these multiorbital systems has been less explored. Here, we analyze the consequences of an orbital-anti-phase structure of the superconducting gap and discuss its possible experimental signatures. We demonstrate that additional pairs of nodes may appear on the $α$ and/or $β$ Fermi surface sheets due to the sign change of the superconducting gap between the involved orbitals. Apart from this additional nodal structure, which is not enforced by the symmetries of the gap function and can be probed in ARPES experiments, the orbital-anti-phase gap modifies the temperature dependence of the superfluid stiffness at low temperatures, providing a concrete experimental prediction to test its realization in bilayer nickelates and related multiorbital systems.

cond-mat.supr-con↗

Correlation-assisted spin-selective metallicity in strained and bilayer altermagnets

Altermagnets combine vanishing net magnetization with a momentum-dependent spin-split electronic structure, providing a route to spin-polarized carriers without ferromagnetism. Here, we investigate how electronic correlations, doping, uniaxial strain, and interlayer coupling control altermagnetism within a minimal Hubbard-type model for mono- and bilayer systems. Comparing Hartree--Fock theory with the rotationally invariant slave-boson (RISB) approach, we demonstrate the robustness of altermagnetic order against quasiparticle renormalization and reveal a separation between the onset of magnetic order and the loss of quasiparticle coherence at stronger coupling. In the monolayer, doping produces a pronounced particle--hole asymmetry, while its combination with uniaxial strain generates a fully spin-polarized Fermi surface close to half-filling. In the bilayer, stacking that favors ferroic alignment of the layer altermagnetic order parameters allows their momentum-dependent spin splittings to combine constructively. Weak asymmetric doping additionally induces intra-unit-cell charge order, resulting in fully spin-polarized low-energy carriers. At a bilayer filling of five electrons in four orbitals, we find a continuous paramagnet-to-altermagnet transition followed, at stronger coupling, by an evolution toward a Mott-like regime with strongly suppressed quasiparticle weight. Our results establish correlations, strain, doping, and stacking as complementary means of controlling altermagnetic metals and generating fully spin-polarized Fermi surfaces.

cond-mat.str-el↗

Density waves in low-pressure bilayer nickelates

The low-pressure phase diagram of La$_3$Ni$_2$O$_7$ provides an important reference for understanding its pressure-induced high-temperature superconductivity. While the spin-density-wave transition at $T_{\text{SDW}}\approx150$ K is increasingly well established, the origin of the second density-wave transition at $T_{\text{DW}}\approx130$ K has remained unresolved. Here, we perform unrestricted Hartree-Fock calculations to investigate the potential origin of the second transition. {Within the orthorhombic phase, the degeneracy between possible ordering wavevectors at $\boldsymbol{Q}_{Y}=(0,π)$ and at $\boldsymbol{Q}_{X}=(π,0)$ is lifted and the electronic system} develops a double-stripe spin-density wave with ordering vector $\boldsymbol{Q}_{Y}=(0,π)$. We identify that the pure double stripe spin state is unstable in La$_3$Ni$_2$O$_7$ towards a commensurate charge-density wave instability, which favors a spin-modulated double stripe order with intertwined charge and spin instabilities and establish the hierarchy of ordered states in La$_3$Ni$_2$O$_7$. We further discuss our results in the context of available experimental literature and propose further experimental tests to elucidate the origin of the SDW/DW states in this system.

cond-mat.str-el↗

Manifest charge-transfer physics in T$^\prime$-La$_2$NiO$_4$

The La$_2$NiO$_4$ compound stabilizes in nature in the so-called T structure with octahedral oxygen coordination of the Ni site. Motivated by a similarly existing polymorph for La$_2$CuO$_4$ in the cuprate system, we here study La$_2$NiO$_4$ in the T$^\prime$-structure with square-planar oxygen coordination of Ni by means of first-principles many-body theory. The hypothetical T$^\prime$-La$_2$NiO$_4$ compound turns out to be a manifest charge-transfer insulator with a cuprate-like charge gap of $\sim 1.8$ eV. Upon doping, a strong carrier asymmetry is revealed, i.e. while holes dominantly enter O$(2p)$-derived states, electrons may become itinerant majorly within effective Ni-$d_{x^2-y^2}$ states. Nearest-neighbor antiferromagnetic ordering at stoichiometry appears absent in the T$^\prime$ structure, in stark contrast to the strong antiferromagnetism in the T structure. Our theoretical study opens up new pathways for correlation physics in layered nickelates with challenging charge-transfer signatures, awaiting experimental inquiries.

cond-mat.str-el↗

Electronic theory for scanning tunneling microscopy spectra in bilayer nickelate thin films

Recent Scanning Tunneling Microscopy (STM) experiments measuring the superconducting gap features in thin films of superconducting bilayer nickelates La2PrNi2O7 at ambient pressure and compressive strain paved the way to study the Cooper-pairing models and the band-selective identification of the gap features in these systems. Here, using the realistic two-orbital bilayer model and the continuum Green's function formalism, we theoretically analyze orbital and band-selective local density of states as well as the corresponding STM spectra. We find that the multiorbital character and the spatial dependence of the Wannier functions leads to the spectra developing characteristic features depending on the position of the scanning tunneling microscope's tip. This allows for a band-resolved analysis of the superconducting coherence peaks and scattering momenta. We identify a clear path for experimental measurements to not only identify the debated incipiency of the gamma-band, but also identification of the coherence peaks' band origins via distance dependent measurements of the local density of states and its corrections through impurity scattering.

cond-mat.supr-con↗

Structural symmetry effects on the competition of density waves and superconductivity in bilayer nickelates

We investigate the interplay between spin-density-wave (SDW) order and superconductivity in the bilayer nickelate La$_3$Ni$_2$O$_7$ using the functional renormalization group~(fRG) applied to multiorbital weak-coupling models of both the ambient- and high-pressure crystal structures. As Hund's coupling increases, the leading instability evolves from superconductivity to an SDW state with ordering vector $\mathbf{Q}_1 \approx (π/2,π/2)$ (equivalently $\mathbf{Q}_Y \approx (0,π)$ in the orthorhombic $Amam$ unit cell), in agreement with experimental observations. Surprisingly, the ambient- and high-pressure structures exhibit nearly identical non-interacting susceptibilities and leading fRG instabilities, indicating that the emergence of superconductivity under pressure cannot be explained solely by changes in the low-energy electronic structure. Instead, our results identify the suppression of orthorhombicity as a key ingredient for superconductivity. As the system approaches the tetragonal limit, symmetry-related SDW fluctuations become nearly degenerate, frustrating long-range magnetic order while enhancing pairing interactions. These findings highlight lattice symmetry as a central tuning parameter of the competing ordered states in bilayer nickelates and suggest that reducing orthorhombicity through uniaxial strain could stabilize bulk superconductivity already at ambient pressure.

cond-mat.supr-con↗

Quantum dynamics of two $XX$ interacting PT-symmetric non-Hermitian qubits: enhancement of quantum annealing

Quantum information platforms enable analog quantum simulations, such as quantum annealing, offering a promising route to solving complex combinatorial optimization problems. Here, we propose a quantum information architecture based on networks of interacting parity-time (PT)-symmetric non-Hermitian qubits. While the dynamics of individual PT-symmetric qubits have been experimentally demonstrated across multiple platforms including NV centers, superconducting circuits, and trapped-ion systems yet coherent dynamics in interacting systems remain largely unexplored. To address this issue we theoretically investigate stationary and time-dependent Hamiltonians relevant to quantum annealing using a minimal model of two interacting XX-coupled PT-symmetric non-Hermitian qubits. We analyze both symmetry-preserving and symmetry-broken regimes and demonstrate that adding even tiny PT-symmetric non-Hermitian terms in the qubits Hamiltonian allows to greatly enhance the probability of reaching the ground state after annealing.

quant-ph↗

Co-operating multiorbital and nonlocal correlations in bilayer nickelate

The interplay of multiorbital physics and nonlocal self-energy effects is studied within an effective three-orbital model for the high-pressure normal state of superconducting bilayer nickelate La$_3$Ni$_2$O$_7$. The model is solved within an advanced many-body framework capturing $k$-dependent correlations beyond dynamical mean-field theory. Different low-energy scenarios subtly depend on the strength of the interorbital interaction, either placing the notorious flat $γ$ quasiparticle band in the occupied part of the spectrum, or letting it cross the Fermi level. In the latter case, intriguing spin-polaron formation due to the scattering of electrons with paramagnon excitations takes place. This leads to bound states appearing as a shadow band with incoherent low-energy spectral weight below the Fermi level. Our results uncover additional competing states that exist in bilayer nickelates and could explain the controversy of recent angle-resolved photoemission experiments.

cond-mat.str-el↗

Enhanced Superconductivity in Proximity to Peaks in Densities of States

For the BCS theory of superconductivity, the electron-phonon interaction is transformed to an attractive electron-electron interaction in the vicinity of the Fermi energy only. At the same time, its formal derivation using a unitary transformation reveals that the electrons attract one another whenever their energies do not differ more than the phonon energy $ω_\mathrm{D}$, independent of closeness to the Fermi energy. Consequently, the order parameter becomes finite even away from the Fermi level. Yet, for small interactions, its magnitude is usually small and can be safely ignored, justifying the BCS approximation. Intriguingly, we find that an accumulation of density-of-states at an energy $\varepsilon_\mathrm{peak}$ in proximity to the Fermi energy induces a significant order parameter magnitude around $\varepsilon_\mathrm{peak}$, which exceeds the one at $E_\mathrm{F}$ for moderate coupling strengths. This strong enhancement is heralded by the softening of an additional collective mode, which resembles a second phase transition. We predict measurable signatures in the thermodynamic and spectroscopic response of this unexpected phenomenon, guiding future experimental searches for it.

cond-mat.supr-con↗

Interplay of orbital-selective Mott criticality and flat-band physics in La$_3$Ni$_2$O$_6$

Superconductivity in nickelates apparently takes place in two different Ni oxidation regimes, namely either for infinite-layer-type compounds close to Ni$^{+}$, or for Ruddlesden-Popper materials close to Ni$^{2+}$. The reduced La$_3$Ni$_2$O$_6$ bilayer with a nominal Ni$^{1.5+}$ oxidation state may therefore serve as a normal-state mediator between the two known families of $3d^8$-like and $3d^9$-like superconducting nickelates. Using first-principles many-body theory, we explain its experimental 50\,meV charge gap as originating from a new type of correlated (quasi-)insulator. Flat-band electrons of Ni-$d_{z^2}$ character become localized from scattering with orbital-selective Mott-localized Ni-$d_{x^2-y^2}$ electrons, by trading in residual hopping energy for a gain in local exchange energy in a ferromagnetic Kondo-lattice scenario. Most importantly, the flat-band electrons offer another route to unconventional superconductivity in nickelates at ambient pressure.

cond-mat.str-el↗

Antiferromagnetism and spin excitations in a two-dimensional non-Hermitian Hatano-Nelson flux model

The one-dimensional Hatano-Nelson model with non-reciprocal hoppings is a prominent example of a relatively simple non-Hermitian quantum-mechanical system, which allows to study various phenomena in open quantum systems without adding extra gain and loss terms. Here we propose to use it as a building block to construct a correlated non-Hermitian Hamiltonian in two dimensions. It has the characteristic form of a flux model with clock-anticlockwise non-reciprocal hopping on each plaquette. Adding the on-site Hubbard type interaction we analyze the formation of the longe-range antiferromagnetic order and its spin excitations. Such a model is non-Hermitian, but $\mathcal{PT}$-symmetric, which leads to the existence of two regions: a region of unbroken $\mathcal{PT}$ symmetry (real-valued spectrum) and a region of broken $\mathcal{PT}$ symmetry with exceptional lines and complex-valued energy spectrum. The transition from one region to another is controlled by the value of the on-site interaction parameter and coincides with the metal-insulator transition. We also analyze the spin wave spectrum, which is characterized by two diffusive d-wave type of modes corresponding to gain and loss.

cond-mat.str-el↗

Enhanced superconductivity in the compressively strained bilayer nickelate thin films by pressure

The discovery of high temperature superconductivity in the nickelate system has stimulated enormous interest in the community of condensed matter physics. Recently, superconductivity with an onset transition temperature (Tc^onset) over 40 K was achieved in La3Ni2O7 and (La,Pr)3Ni2O7 thin films at ambient pressure due to in-plane compressive strain. This observation has sparked enormous attention because measurements on superconducting properties can be accessible with many commonly used experimental tools. On the other hand, the Tc in these thin films is much lower than that of the bulk bilayer nickelates under pressure. Here we report the enhancement of Tc^onset to over 60 K by applying hydrostatic pressure on the compressively strained superconducting bilayer nickelate thin films. The Tc^onset firstly ramps up with pressure, then it slightly drops down after reaching the maximum Tc^onset at about 61.5 K under a pressure of 9 GPa, showing a dome-like phase diagram. Hall effect measurements reveal that the dominant charge carriers are hole-like with a slight enhancement of charge carrier density with pressure in accompanying with the increase of Tc. Our theoretical results demonstrate that the enhancement of Tc arises from a cooperative amplification of magnetic fluctuations within and between the layers and increased metallicity under pressure. However, this enhancement exhibits saturation at higher pressures. These findings highlight the critical role of the interplay between interlayer and intralayer electronic correlations in bilayer nickelate superconductors and point to the potential of tuning Tc through controlled manipulation of the electronic structure and interactions.

cond-mat.supr-con↗

Superconducting gap structure and bosonic mode in La2PrNi2O7 thin films at ambient pressure

The recent discovery of high temperature superconductivity in nickelate systems has generated tremendous interests in the field of superconductivity. The core issue to understand the superconductivity mechanism is about the superconducting gap and its symmetry. By using the substrate of SrLaAlO4(00l), we have successfully synthesized the superconducting thin film of La2PrNi2O7 with Tc(onset) = 41.5 K. Superconducting tunneling spectra are successfully measured on the terraces after we expose the superconducting layer by using the tip-excavation technique. The spectrum shows a two-gap structure with Delta1=19 meV, Delta2=6-8 meV, and fittings based on the Dynes model indicate that the dominant gap should have an anisotropic s-wave structure, this allows us to put the priority in selecting the s+- among the two arguable pairing models: s+- and d-wave. Furthermore, a clear bosonic mode with energy Omega=30+-2 meV is observed, which further supports a sign reversal gap. Our results shed new light in understanding the mystery of superconductivity in bilayer nickelate superconductors.

cond-mat.supr-con↗

Low-energy perspective of interacting electrons in the normal state of superconducting bilayer nickelate

Developing a low-energy model is essential for understanding unconventional superconductivity in bilayer nickelate La$_3$Ni$_2$O$_7$. Here, we analyze distinct low-energy scenarios of the normal state by downfolding the ab-initio determined band structure and applying the mean-field regime of rotational-invariant slave-boson theory. We compare models based on the single-site two-orbital, the two-site four-orbital and a proposed minimal cluster (MC) picture. The latter builds up on three adapted orbitals located on the sites of the basic Ni-O-Ni cluster across the bilayer. Intriguing interplay between the Hund coupling $J_{\rm H}$ and the interlayer exchange $J_{\perp}$ is encountered in the multiorbital multi-site problem. While the tendency for interlayer Ni-$d_{z^2}$ singlet formation is pronounced, a complete localization remains hindered by the coupling to the Ni-$d_{x^2-y^2}$ orbitals. The correlation physics in the MC picture is peculiar with respect to the effective interorbital/site exchange.

cond-mat.str-el↗

Pressure-enhanced splitting of density wave transitions in La$_3$Ni$_2$O$_{7-δ}$

The observation of superconductivity in La$_3$Ni$_2$O$_{7-δ}$ under pressure, following the suppression of a high-temperature density wave state, has attracted considerable attention. The nature of this density wave order was not clearly identified. Here, we probe the magnetic response of the zero-pressure phase of La$_3$Ni$_2$O$_{7-δ}$ as hydrostatic pressure is applied and find that the apparent single density wave transition at zero applied pressure splits into two. The comparison of our muon-spin rotation and relaxation experiments with dipole-field numerical analysis reveals the magnetic structure's compatibility with a stripe-type arrangement of Ni moments, characterized by alternating lines of magnetic moments and nonmagnetic stripes at ambient pressure. When pressure is applied, the magnetic ordering temperature increases, while the unidentified density wave transition temperature falls. Our findings reveal that the ground state of the La$_3$Ni$_2$O$_{7-δ}$ system is characterized by the coexistence of two distinct orders -- a magnetically ordered spin density wave and a lower-temperature ordering that is most likely a charge density wave -- with a notable pressure-enhanced separation between them.

cond-mat.supr-con↗

Theory of potential impurity scattering in pressurized superconducting La$_3$Ni$_2$O$_7$

Recently discovered high-T$_c$ superconductivity in pressurized bilayer nickelate La$_3$Ni$_2$O$_7$ (La-327) is believed to be driven by the non-phononic repulsive interaction. Depending on the strength of the interlayer repulsion, the symmetry of the superconducting order parameter is expected to be either $d$-wave or sign-changing bonding-antibonding $s_{\pm}$-wave. Unfortunately, due to the need of high pressure to reach superconducting phase, conventional spectroscopic probes to validate the symmetry of the order parameter are hard to use. Here, we study the effect of the point-like non-magnetic impurities on the superconducting state of La-327 and show that $s_{\pm}$-wave and $d$-wave symmetries show a very different behavior as a function of impurity concentration, which can be studied experimentally by irradiating the La-327 samples by electrons prior applying the pressure. While $d-$wave superconducting state will be conventionally suppressed, the $s_{\pm}$-wave state shows more subtle behavior, depending on the asymmetry between bonding and antibonding subspaces. For the electronic structure, predicted to realize in La-327, the $s_{\pm}-$wave state will be robust against complete suppression and the transition temperature, $T_c$ demonstrates a transition from convex to concave behavior, indicating a crossover from $s_{\pm}$-wave to $s_{++}$-wave symmetry as a function of impurity concentration. We further analyze the sensitivity of the obtained results with respect to the potential electronic structure modification.

cond-mat.supr-con↗

Superluminal Propagation of Composite Collective Modes in Superconductor-Ferromagnet Heterostructures

Superconductor/ferromagnet/superconductor Josephson junctions are paradigmatic systems for studying the delicate interplay of superconductivity and magnetism via proximity effects as well as their composite excitations. Here, we analyse the collective modes (CM) in such a heterostructure by taking into account the interplay between the de-magnetisation field $H_{dem}$ and the field caused by the anisotropy of the ferromagnet $H_{an}$, which was previously neglected. It turns out that the spectrum of composite collective modes, $ω(k)$, has a qualitatively different form in the case of $H_{dem} H_{an}$. In the first case, the dependence $ω(k)$ has the same form as in previous studies, whereas in the second case, the spectrum looks completely different. In particular, for moderate or weak anisotropy in ferromagnet the group velocity of collective modes demonstrates inflection point where the group velocity become infinite and is superluminal. Furthermore, this point separates purely real and complex-conjugate solutions for the collective modes and is also {\it exception point}. We show that the difference of the CMs spectra can be revealed by Fiske experiment, i.\,e.\,by measuring the $I-V$ characteristics in the presence of magnetic field and voltage.

cond-mat.supr-con↗