arXiv subjects

Immo Söllner

Publications and source records attributed to Immo Söllner.

15 recordsLinked to original sources

arXiv2020

Narrow optical linewidths and spin pumping on charge-tunable, close-to-surface self-assembled quantum dots in an ultra-thin diode

We demonstrate full charge control, narrow optical linewidths, and optical spin pumping on single self-assembled InGaAs quantum dots embedded in a $162.5\,\text{nm}$ thin diode structure. The quantum dots are just $88\,\text{nm}$ from the top GaAs surface. We design and realize a p-i-n-i-n diode that allows single-electron charging of the quantum dots at close-to-zero applied bias. In operation, the current flow through the device is extremely small resulting in low noise. In resonance fluorescence, we measure optical linewidths below $2\,μ\text{eV}$, just a factor of two above the transform limit. Clear optical spin pumping is observed in a magnetic field of $0.5\,\text{T}$ in the Faraday geometry. We present this design as ideal for securing the advantages of self-assembled quantum dots -- highly coherent single photon generation, ultra-fast optical spin manipulation -- in the thin diodes required in quantum nano-photonics and nano-phononics applications.

cond-mat.mes-hall↗

arXiv2018

A gated quantum dot far in the strong-coupling regime of cavity-QED at optical frequencies

The strong-coupling regime of cavity-quantum-electrodynamics (cQED) represents light-matter interaction at the fully quantum level. Adding a single photon shifts the resonance frequencies, a profound nonlinearity. cQED is a test-bed of quantum optics and the basis of photon-photon and atom-atom entangling gates. At microwave frequencies, success in cQED has had a transformative effect. At optical frequencies, the gates are potentially much faster and the photons can propagate over long distances and be easily detected, ideal features for quantum networks. Following pioneering work on single atoms, solid-state implementations are important for developing practicable quantum technology. Here, we embed a semiconductor quantum dot in a microcavity. The microcavity has a $\mathcal{Q}$-factor close to $10^{6}$ and contains a charge-tunable quantum dot with close-to-transform-limited optical linewidth. The exciton-photon coupling rate $g$ exceeds both the photon decay rate $κ$ and exciton decay rate $γ$ by a large margin ($g/γ=14$, $g/κ=5.3$); the cooperativity is $C=2g^{2}/(γκ)=150$, the $β$-factor 99.7%. We observe pronounced vacuum Rabi oscillations in the time-domain, photon blockade at a one-photon resonance, and highly bunched photon statistics at a two-photon resonance. We use the change in photon statistics as a sensitive spectral probe of transitions between the first and second rungs of the Jaynes-Cummings ladder. All experiments can be described quantitatively with the Jaynes-Cummings model despite the complexity of the solid-state environment. We propose this system as a platform to develop optical-cQED for quantum technology, for instance a photon-photon entangling gate.

quant-ph↗

arXiv2018

Coherent optical control of a quantum-dot spin-qubit in a waveguide-based spin-photon interface

Waveguide-based spin-photon interfaces on the GaAs platform have emerged as a promising system for a variety of quantum information applications directly integrated into planar photonic circuits. The coherent control of spin states in a quantum dot can be achieved by applying circularly polarized laser pulses that may be coupled into the planar waveguide vertically through radiation modes. However, proper control of the laser polarization is challenging since the polarization is modified through the transformation from the far field to the exact position of the quantum dot in the nanostructure. Here we demonstrate polarization-controlled excitation of a quantum-dot electron spin and use that to perform coherent control in a Ramsey interferometry experiment. The Ramsey interference reveals a pure dephasing time of $ 2.2\pm0.1 $ ns, which is comparable to the values so far only obtained in bulk media. We analyze the experimental limitations in spin initialization fidelity and Ramsey contrast and identify the underlying mechanisms.

quant-ph↗

arXiv2018

Excitons in InGaAs Quantum Dots without Electron Wetting Layer States

The Stranski-Krastanov (SK) growth-mode facilitates the self-assembly of quantum dots (QDs) using lattice-mismatched semiconductors, for instance InAs and GaAs. SK QDs are defect-free and can be embedded in heterostructures and nano-engineered devices. InAs QDs are excellent photon emitters: QD-excitons, electron-hole bound pairs, are exploited as emitters of high quality single photons for quantum communication. One significant drawback of the SK-mode is the wetting layer (WL). The WL results in a continuum rather close in energy to the QD-confined-states. The WL-states lead to unwanted scattering and dephasing processes of QD-excitons. Here, we report that a slight modification to the SK-growth-protocol of InAs on GaAs -- we add a monolayer of AlAs following InAs QD formation -- results in a radical change to the QD-excitons. Extensive characterisation demonstrates that this additional layer eliminates the WL-continuum for electrons enabling the creation of highly charged excitons where up to six electrons occupy the same QD. Single QDs grown with this protocol exhibit optical linewidths matching those of the very best SK QDs making them an attractive alternative to standard InGaAs QDs.

cond-mat.mes-hall↗

arXiv2018

Quantum optics with near lifetime-limited quantum-dot transitions in a nanophotonic waveguide

Establishing a highly efficient photon-emitter interface where the intrinsic linewidth broadening is limited solely by spontaneous emission is a key step in quantum optics. It opens a pathway to coherent light-matter interaction for, e.g., the generation of highly indistinguishable photons, few-photon optical nonlinearities, and photon-emitter quantum gates. However, residual broadening mechanisms are ubiquitous and need to be combated. For solid-state emitters charge and nuclear spin noise is of importance and the influence of photonic nanostructures on the broadening has not been clarified. We present near lifetime-limited linewidths for quantum dots embedded in nanophotonic waveguides through a resonant transmission experiment. It is found that the scattering of single photons from the quantum dot can be obtained with an extinction of $66 \pm 4 \%$, which is limited by the coupling of the quantum dot to the nanostructure rather than the linewidth broadening. This is obtained by embedding the quantum dot in an electrically-contacted nanophotonic membrane. A clear pathway to obtaining even larger single-photon extinction is laid out, i.e., the approach enables a fully deterministic and coherent photon-emitter interface in the solid state that is operated at optical frequencies.

quant-ph↗

arXiv2017

Indistinguishable and efficient single photons from a quantum dot in a planar nanobeam waveguide

We demonstrate a high-purity source of indistinguishable single photons using a quantum dot embedded in a nanophotonic waveguide. The source features a near-unity internal coupling efficiency and the collected photons are efficiently coupled off-chip by implementing a taper that adiabatically couples the photons to an optical fiber. By quasi-resonant excitation of the quantum dot, we measure a single-photon purity larger than 99.4% and a photon indistinguishability of up to 94+-1% by using p-shell excitation combined with spectral filtering to reduce photon jitter. A temperature-dependent study allows pinpointing the residual decoherence processes notably the effect of phonon broadening. Strict resonant excitation is implemented as well as another mean of suppressing photon jitter, and the additional complexity of suppressing the excitation laser source is addressed. The study opens a clear pathway towards the long-standing goal of a fully deterministic source of indistinguishable photons, which is integrated on a planar photonic chip.

quant-ph↗

arXiv2017

Spin-photon interface and spin-controlled photon switching in a nanobeam waveguide

Access to the electron spin is at the heart of many protocols for integrated and distributed quantum-information processing [1-4]. For instance, interfacing the spin-state of an electron and a photon can be utilized to perform quantum gates between photons [2,5] or to entangle remote spin states [6-9]. Ultimately, a quantum network of entangled spins constitutes a new paradigm in quantum optics [1]. Towards this goal, an integrated spin-photon interface would be a major leap forward. Here we demonstrate an efficient and optically programmable interface between the spin of an electron in a quantum dot and photons in a nanophotonic waveguide. The spin can be deterministically prepared with a fidelity of 96\%. Subsequently the system is used to implement a "single-spin photonic switch", where the spin state of the electron directs the flow of photons through the waveguide. The spin-photon interface may enable on-chip photon-photon gates [2], single-photon transistors [10], and efficient photonic cluster state generation [11].

quant-ph↗

arXiv2017

Numerical modelling of the coupling efficiency of single quantum emitters in photonic-crystal waveguides

Planar photonic nanostructures have recently attracted a great deal of attention for quantum optics applications. In this article, we carry out full 3D numerical simulations to fully account for all radiation channels and thereby quantify the coupling efficiency of a quantum emitter embedded in a photonic-crystal waveguide. We utilize mixed boundary conditions by combining active Dirichlet boundary conditions for the guided mode and perfectly-matched layers for the radiation modes. In this way, the leakage from the quantum emitter to the surrounding environment can be determined and the spectral and spatial dependence of the coupling to the radiation modes can be quantified. The spatial maps of the coupling efficiency, the $β$-factor, reveal that even for moderately slow light, near-unity $β$ is achievable that is remarkably robust to the position of the emitter in the waveguide. Our results show that photonic-crystal waveguides constitute a suitable platform to achieve deterministic interfacing of a single photon and a single quantum emitter, which has a range of applications for photonic quantum technology.

quant-ph↗

arXiv2017

Deterministic enhancement of coherent photon generation from a nitrogen-vacancy center in ultrapure diamond

The nitrogen-vacancy (NV) center in diamond has an optically addressable, highly coherent spin. However, an NV center even in high quality single-crystalline material is a very poor source of single photons: extraction out of the high-index diamond is inefficient, the emission of coherent photons represents just a few per cent of the total emission, and the decay time is large. In principle, all three problems can be addressed with a resonant microcavity. In practice, it has proved difficult to implement this concept: photonic engineering hinges on nano-fabrication yet it is notoriously difficult to process diamond without degrading the NV centers. We present here a microcavity scheme which uses minimally processed diamond, thereby preserving the high quality of the starting material, and a tunable microcavity platform. We demonstrate a clear change in the lifetime for multiple individual NV centers on tuning both the cavity frequency and anti-node position, a Purcell effect. The overall Purcell factor $F_{\rm P}=2.0$ translates to a Purcell factor for the zero phonon line (ZPL) of $F_{\rm P}^{\rm ZPL}\sim30$ and an increase in the ZPL emission probability from $\sim 3 \%$ to $\sim 46 \%$. By making a step-change in the NV's optical properties in a deterministic way, these results pave the way for much enhanced spin-photon and spin-spin entanglement rates.

quant-ph↗

arXiv2016

Engineering chiral light--matter interaction in photonic crystal waveguides with slow light

We design photonic crystal waveguides with efficient chiral light--matter interfaces that can be integrated with solid-state quantum emitters. By using glide-plane-symmetric waveguides, we show that chiral light-matter interaction can exist even in the presence of slow light with slow-down factors of up to $100$ and therefore the light--matter interaction exhibits both strong Purcell enhancement and chirality. This allows for near-unity directional $β$-factors for a range of emitter positions and frequencies. Additionally, we design an efficient mode adapter to couple light from a standard nanobeam waveguide to the glide-plane symmetric photonic crystal waveguide. Our work sets the stage for performing future experiments on a solid-state platform.

physics.optics↗

arXiv2016

Deterministic Single-Phonon Source Triggered by a Single Photon

We propose a scheme that enables the deterministic generation of single phonons at GHz frequencies triggered by single photons in the near infrared. This process is mediated by a quantum dot embedded on-chip in an opto-mechanical circuit, which allows for the simultaneous control of the relevant photonic and phononic frequencies. We devise new opto-mechanical circuit elements that constitute the necessary building blocks for the proposed scheme and are readily implementable within the current state-of-the-art of nano-fabrication. This will open new avenues for implementing quantum functionalities based on phonons as an on-chip quantum bus.

quant-ph↗

arXiv2015

Deterministic photon-emitter coupling in chiral photonic circuits

The ability to engineer photon emission and photon scattering is at the heart of modern photonics applications ranging from light harvesting, through novel compact light sources, to quantum-information processing based on single photons. Nanophotonic waveguides are particularly well suited for such applications since they confine photon propagation to a 1D geometry thereby increasing the interaction between light and matter. Adding chiral functionalities to nanophotonic waveguides lead to new opportunities enabling integrated and robust quantum-photonic devices or the observation of novel topological photonic states. In a regular waveguide, a quantum emitter radiates photons in either of two directions, and photon emission and absorption are reverse processes. This symmetry is violated in nanophotonic structures where a non-transversal local electric field implies that both photon emission and scattering may become directional. Here we experimentally demonstrate that the internal state of a quantum emitter determines the chirality of single-photon emission in a specially engineered photonic-crystal waveguide. Single-photon emission into the waveguide with a directionality of more than 90\% is observed under conditions where practically all emitted photons are coupled to the waveguide. Such deterministic and highly directional photon emission enables on-chip optical diodes, circulators operating at the single-photon level, and deterministic quantum gates. Based on our experimental demonstration, we propose an experimentally achievable and fully scalable deterministic photon-photon CNOT gate, which so far has been missing in photonic quantum-information processing where most gates are probabilistic.

quant-ph↗

arXiv2012

Nonuniversal intensity correlations in 2D Anderson localizing random medium

Complex dielectric media often appear opaque because light traveling through them is scattered multiple times. Although the light scattering is a random process, different paths through the medium can be correlated encoding information about the medium. Here, we present spectroscopic measurements of nonuniversal intensity correlations that emerge when embedding quantum emitters inside a disordered photonic crystal that is found to Anderson-localize light. The emitters probe in-situ the microscopic details of the medium, and imprint such near-field properties onto the far-field correlations. Our findings provide new ways of enhancing light-matter interaction for quantum electrodynamics and energy harvesting, and may find applications in subwavelength diffuse-wave spectroscopy for biophotonics.

physics.optics↗

arXiv2011

Testing Born's Rule in Quantum Mechanics for Three Mutually Exclusive Events

We present a new experimental approach using a three-path interferometer and find a tighter empirical upper bound on possible violations of Born's Rule. A deviation from Born's rule would result in multi-order interference. Among the potential systematic errors that could lead to an apparent violation we specifically study the nonlinear response of our detectors and present ways to calibrate this error in order to obtain an even better bound.

quant-ph↗

arXiv2008

Testing Born's Rule in Quantum Mechanics with a Triple Slit Experiment

In Mod. Phys. Lett. A 9, 3119 (1994), one of us (R.D.S) investigated a formulation of quantum mechanics as a generalized measure theory. Quantum mechanics computes probabilities from the absolute squares of complex amplitudes, and the resulting interference violates the (Kolmogorov) sum rule expressing the additivity of probabilities of mutually exclusive events. However, there is a higher order sum rule that quantum mechanics does obey, involving the probabilities of three mutually exclusive possibilities. We could imagine a yet more general theory by assuming that it violates the next higher sum rule. In this paper, we report results from an ongoing experiment that sets out to test the validity of this second sum rule by measuring the interference patterns produced by three slits and all the possible combinations of those slits being open or closed. We use attenuated laser light combined with single photon counting to confirm the particle character of the measured light.

quant-ph↗