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Indranil Paul

Publications and source records attributed to Indranil Paul.

At least 19 recordsLinked to original sources

Revealing the nature of the charge density wave order of ErTe$_3$ via Raman scattering under anisotropic strain

The nature of the charge density wave (CDW) order of the rare-earth tritelluride ErTe3 is investigated by Raman scattering under anisotropic strain. The CDW state of ErTe3 is unconventional since it is accompanied by an unusual mirror symmetry breaking, whose origin remains to be understood. Studying the polarization-resolved Raman spectrum of the CDW amplitude mode as a function of strain and temperature, we find that the mirror symmetry breakings of the CDW state are not independent, arguing against the recently proposed ferro-axial multi-component CDW order. Instead, we show that a single component CDW order parameter with an ordering wavevector tilted away from the principle crystallographic axis can reproduce the observed mirror symmetry breakings and their manifestation in the Raman spectra.

cond-mat.str-el

Pseudogap-induced change in the nature of the Lifshitz transition in the two-dimensional Hubbard model

We study the behavior of the density of states and the $B_{1g}$ nematic susceptibility extracted from Raman response data across the doping-driven Lifshitz transition comparing the weak and strong interaction cases. Our results were obtained using cluster dynamical mean field theory for the two-dimensional Hubbard model. In the weakly correlated Fermi liquid regime, both quantities are approximately symmetric around the Lifshitz transition doping $p_{LT}$. In the strongly correlated regime, the low-doping pseudogap leads to an asymmetric, discontinuous evolution when the Fermi surface changes from hole-like to electron-like at $p_{LT}$. The Lifshitz transition thus changes character because it is tied to the pseudogap-Fermi-liquid transition. These results are consistent with available observations and should foster further experimental investigations.

cond-mat.str-el

Destructive Interference induced constraints in Floquet systems

We introduce the paradigm of destructive many-body interference between quantum trajectories as a means to systematically generate prethermal kinetically constrained dynamics in Floquet systems driven at special frequencies. Depending on the processes that are suppressed by interference, the constraint may or may not be associated with an emergent global conservation; the latter kind having no mechanism of generation in time-independent settings. As an example, we construct an one-dimensional interacting spin model exhibiting strong Hilbert space fragmentation with and without dipole moment conservation, depending on the drive frequency. By probing the spatiotemporal profile of the out-of-time-ordered correlator, we show that this model, in particular, has initial states in which quantum information can be spatially localized - a useful feature in the field of quantum technologies. Our paradigm unifies various types of Hilbert space fragmentation that can be realized in driven systems.

cond-mat.str-el

Antisymmetric Raman response

We develop the theory of antisymmetric Raman response, defined as the difference between the Raman signals of two scattering geometries related by an exchange of mutually perpendicular incoming and the outgoing photon polarizations. Such responses, finite in orthorhombic or lower symmetry systems, are related to cross-susceptibilities of two Raman operators and are characterized by the absence of intraband terms. This is in contrast to standard Raman responses which measure auto-susceptibilities where both intra- and interband processes contribute. We illustrate the theory with examples from the charge density wave rare-earth tritellurides and the excitonic insulator Ta$_2$NiSe$_5$. Our theory establishes antisymmetric Raman response as a unique tool to probe microscopic features such as interband energy scales and to detect reflection symmetry breaking.

cond-mat.str-el

Signatures of fragmentation for periodically driven fermions

We study the possible signatures of prethermal strong Hilbert space fragmentation (HSF) for one-dimensional (1D) fermions subjected to a periodic drive. We extend the results of Phys. Rev. Lett. 130, 120401 (2023) to show the possibility of such fragmentation for a large class of experimentally relevant drive protocols. Moreover, we demonstrate the persistence of HSF when the fermion chain is taken away from half-filling. Both these analysis indicate the robustness of the fragmentation phenomenon reported earlier. We also provide an alternate derivation of the Floquet Hamiltonian of the driven chain which yields insight into the generic nested commutator structure of its higher order terms. Finally, we study the density-density out-of-time-correlators (OTOC) of the driven chain both away and near the special drive frequencies at which its first order Floquet Hamiltonian exhibits fragmentation. We show that these OTOCs, for a chain with open boundary condition, exhibit a distinct periodic unscrambling of information at special drive frequencies; such unscrambling can therefore serve as a marker of prethermal HSF. We provide an approximate analytic explanation of the role of HSF behind such periodic unscrambling and discuss experiments which can detect signatures of strong HSF in such driven chains.

cond-mat.str-el

Hilbert space fragmentation imposed real spectrum of non-Hermitian systems

We show that constraints imposed by strong Hilbert space fragmentation (HSF) along with the presence of certain global symmetries can ensure the reality of eigenspectra of non-Hermitian quantum systems; such a reality cannot be guaranteed by global symmetries alone. We demonstrate this insight for two interacting finite chains, namely the fermionic Nelson-Hatano and the Su-Schrieffer-Heeger models, none of which has a $\mathcal{PT}$ symmetry. We show analytically that strong HSF and real spectrum are both consequences of the same dynamical constraints in the limit of large interaction, provided the systems have sufficient global symmetries. We also show that a local equal-time correlation function can detect the many-body exceptional point at a finite critical interaction strength above which the eigenspectrum is real.

cond-mat.str-el

Prethermal fragmentation in a periodically driven Fermionic chain

We study a Fermionic chain with nearest-neighbor hopping and density-density interactions, where the nearest-neighbor interaction term is driven periodically. We show that such a driven chain exhibits prethermal strong Hilbert space fragmentation (HSF) in the high drive amplitude regime at specific drive frequencies $\omega_m^{\ast}$. This constitutes the first realization of HSF for out-of-equilibrium systems. We obtain analytic expressions of $\omega_m^{\ast}$ using a Floquet perturbation theory and provide exact numerical computation of entanglement entropy, equal-time correlation functions, and the density autocorrelation of Fermions for finite chains. All of these quantities indicate clear signatures of strong HSF. We study the fate of the HSF as one tunes away from $\omega_m^{\ast}$ and discuss the extent of the prethermal regime as a function of the drive amplitude.

cond-mat.str-el

Exceptional van Hove Singularities in Pseudogapped Metals

Motivated by the pseudogap state of the cuprates, we introduce the concept of an "exceptional" van Hove singularity that appears when strong electron-electron interaction splits an otherwise simply connected Fermi surface into multiply connected pieces. The singularity describes the touching of two pieces of the split Fermi surface. We show that this singularity is proximate to a second order van Hove singularity, which can be accessed by tuning a dispersion parameter. We argue that, in a wide class of cuprates, the end-point of the pseudogap is accessed only by triggering the exceptional van Hove singularity. The resulting Lifshitz transition is characterized by enhanced specific heat and nematic susceptibility, as seen in experiments.

cond-mat.str-el

Detection of squeezed phonons in pump-probe spectroscopy

Robust engineering of phonon squeezed states in optically excited solids has emerged as a promising tool to control and manipulate their properties. However, in contrast to quantum optical systems, detection of phonon squeezing is subtle and elusive, and an important question is what constitutes an unambiguous signature of it. The state of the art involves observing oscillations at twice the phonon frequency in time resolved measurements of the out of equilibrium phonon fluctuation. Using Keldysh formalism we show that such a signal is a necessary but not a sufficient signature of a squeezed phonon, since we identify several mechanisms that do not involve squeezing and yet which produce similar oscillations. We show that a reliable detection requires a time and frequency resolved measurement of the phonon spectral function.

cond-mat.str-el

Interplay between nematicity and Bardasis-Schrieffer modes in the short-time dynamics of unconventional superconductors

Motivated by the recent experiments suggesting the importance of nematicity in the phase diagrams of ironbased and cuprate high-Tc superconductors, we study the influence of nematicity on the collective modes inside the superconducting state in a non-equilibrium. In particular, we consider the signatures of collective modes in short-time dynamics of a system with competing nematic and s- and d-wave superconducting orders. In the rotationally symmetric state, we show that the Bardasis-Schrieffer mode, corresponding to the subdominant pairing, hybridizes with the nematic collective mode and merges into a single in-gap mode, with the mixing vanishing only close to the phase boundaries. For the d-wave ground state, we find that nematic interaction suppresses the damping of the collective oscillations in the short-time dynamics. Additionally, we find that even inside the nematic s+d-wave superconducting state, a Bardasis-Schrieffer-like mode leads to order parameter oscillations that strongly depend on the competition between the two pairing symmetries. We discuss the connection of our results to the recent pump-probe experiments on high-Tc superconductors.

cond-mat.supr-con

Variation of shear moduli across superconducting phase transitions

We study how shear moduli of a correlated metal change across superconducting phase transitions. Using a microscopic theory we explain why for most classes of superconductors this change is small. The Fe-based and the A15 systems are notable exceptions where the change is boosted by five orders of magnitude. We show that this boost is a consequence of enhanced nematic correlation. The theory explains the unusual temperature dependence of the orthorhombic shear and the back-bending of the nematic transition line in the superconducting phase of the Fe-based systems.

cond-mat.supr-con

Collective modes in pumped unconventional superconductors with competing ground states

Motivated by the recent development of terahertz pump-probe experiments, we investigate the short-time dynamics in superconductors with multiple attractive pairing channels. Studying a single-band square lattice model with spin-spin interaction as an example, we find the signatures of collective excitations of the pairing symmetries (known as Bardasis-Schrieffer modes) as well as the order parameter amplitude (Higgs mode) in the short-time dynamics of the spectral gap and quasiparticle distribution after an excitation by a pump pulse. We show that the polarization and intensity of the pulse can be used to control the symmetry of the non-equilibrium state as well as frequencies and relative intensities of the contributions of different collective modes. We find particularly strong signatures of the Bardasis-Schrieffer mode in the dynamics of the quasiparticle distribution function. Our work shows the potential of modern ultrafast experiments to address the collective excitations in unconventional superconductors and highlights the importance of sub-dominant interactions for the non-equilibrium dynamics in these systems.

cond-mat.supr-con

Disorder-Induced Electronic Nematicity

We expose the theoretical mechanisms underlying disorder-induced nematicity in systems exhibiting strong fluctuations or ordering in the nematic channel. Our analysis consists of a symmetry-based Ginzburg-Landau approach and associated microscopic calculations. We show that a single featureless point-like impurity induces nematicity locally, already above the critical nematic transition temperature. The persistence of fourfold rotational symmetry constrains the resulting disorder-induced nematicity to be inhomogeneous and spatially average to zero. Going beyond the single impurity case, we discuss the effects of finite disorder concentrations on the appearance of nematicity. We identify the conditions that allow disorder to enhance the nematic transition temperature, and we provide a concrete example. The presented theoretical results can explain a large series of recent experimental discoveries of disorder-induced nematic order in iron-based superconductors.

cond-mat.supr-con

Charge Nematicity and Electronic Raman Scattering in Iron-based Superconductors

We review the recent developments in electronic Raman scattering measurements of charge nematic fluctuations in iron-based superconductors. A simple theoretical framework of a $d$-wave Pomeranchuk transition is proposed in order to capture the salient features of the spectra. We discuss the available Raman data in the normal state of 122 iron-based systems, particularly Co doped BaFe$_2$As$_2$, and we show that the low energy quasi-elastic peak, the extracted nematic susceptibility and the scattering rates are consistent with an electronic driven structural phase transition. In the superconducting state with a full gap the quasi-elastic peak transforms into a finite frequency nematic resonance, evidences for which are particularly strong in the electron doped systems. A crucial feature of the analysis is the fact that the electronic Raman signal is unaffected by the acoustic phonons. This makes Raman spectroscopy a unique probe of electronic nematicity.

cond-mat.supr-con

Quantum critical elasticity

We discuss elastic instabilities of the atomic crystal lattice at zero temperature. Due to long-range shear forces of the solid, at such transitions the phonon velocities vanish, if at all, only along certain crystallographic directions, and, consequently, the critical phonon fluctuations are suppressed to a lower dimensional manifold and governed by a Gaussian fixed-point. In case of symmetry-breaking elastic transitions, a characteristic critical phonon thermodynamics arises that is found, e.g., to violate Debye's $T^3$-law for the specific heat. We point out that quantum critical elasticity is triggered whenever a critical soft mode couples linearly to the strain tensor. In particular, this is relevant for the electronic Ising-nematic quantum phase transition in a tetragonal crystal as discussed in the context of certain cuprates, ruthenates and iron-based superconductors.

cond-mat.str-el

Manifestation of nematic degrees of freedom in the Raman response function of iron pnictides

We establish a relation between the Raman response function in the $B_{1g}$ channel and the electronic contribution to the nematic susceptibility within the spin-driven approach to electron nematicity of the iron based superconductors. The spin-driven nematic phase, characterized by the broken $C_4$ symmetry, but unbroken $O(3$) spin-rotational symmetry, is generated by the presence of magnetic fluctuations associated with the striped phase. It occurs as a separate phase between $T_N$ and $T_s$ in systems where the structural and magnetic phase transitions are separated. Detecting the presence of nematic degrees of freedom in iron-based superconductors is a difficult task, since it involves measuring higher order spin correlation functions. We show that the nematic degrees of freedom manifest themselves in the experimentally measurable Raman response function. We calculate the Raman response function in tetragonal phase in the large $N$ limit by considering Aslamazov-Larkin type of diagrams that contain a series of inserted fermionic boxes that resemble the nematic coupling constant of the theory. These diagrams effectively account for collisions between spin fluctuations. By summing an infinite number of such higher order diagrams, we demonstrate that the electronic Raman response function shows a clear maximum at the structural phase transition in the $B_{1g}$ channel. Hence, the Raman response function can be used to probe nematic degrees of freedom.

cond-mat.str-el

Effects of Lifshitz Transition on Charge Transport in Magnetic Phases of Fe-Based Superconductors

The unusual temperature dependence of the resistivity and its in-plane anisotropy observed in the Fe-based superconducting materials, particularly Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, has been a longstanding puzzle. Here we consider the effect of impurity scattering on the temperature dependence of the average resistivity within a simple two-band model of a dirty spin density wave metal. The sharp drop in resistivity below the Néel temperature $T_N$ in the parent compound can only be understood in terms of a Lifshitz transition following Fermi surface reconstruction upon magnetic ordering. We show that the observed resistivity anisotropy in this phase, arising from nematic defect structures, is affected by the Lifshitz transition as well.

cond-mat.supr-con

Structural Transition of Wigner Crystal on Liquid Substrate

The physics of an electron solid, held on a cryogenic liquid surface by a pressing electric field, is examined in a low-density regime that has not been explored before. We consider the effect of the pressing field in distorting the surface at the position of each electron and hence inducing an attractive force between the electrons. The system behavior is described in terms of an interplay between the repulsive Coulomb interaction and the attractive surface-induced interaction between individual electrons. For small densities and large enough pressing fields, we find a parameter regime where a square lattice is more favorable than the usual triangular lattice; we map out the first-order transition curve separating the two lattice geometries at zero temperature. In addition, our description allows an alternate static perspective on the charge-density wave instability of the system, corresponding to the formation of multi-electron dimples.

cond-mat.mes-hall