arXiv subjects

Ingrid Stolt

Publications and source records attributed to Ingrid Stolt.

3 recordsLinked to original sources

arXiv2021

RKKY coupled local moment magnetism in NaFe$_{1-x}$Cu$_{x}$As

A central question in a large class of strongly correlated electron systems, including heavy fermion compounds and iron pnictides, is the identification of different phases and their origins. It has been shown that the antiferromagnetic (AFM) phase in some heavy fermion compounds is induced by Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction between localized moments, and that the competition between this interaction and Kondo effect is responsible for quantum criticality. However, conclusive experimental evidence of the RKKY interaction in pnictides is lacking. Here, using high resolution $^{23}$Na NMR measurements on lightly Cu-doped metallic single crystals of NaFe$_{1-x}$Cu$_{x}$As ~($x \approx 0.01$) and numerical simulation, we show direct evidence of the RKKY interaction in this pnictide system. Aided by computer simulation, we identify the $^{23}$Na NMR satellite resonances with the RKKY oscillations of spin polarization at Fe sites. Our $^{23}$Na spin-lattice and spin-spin relaxation data exhibits signature of an itinerant and inhomogeneous AFM phase in this system, accompanied by a simulation of Cu-induced perturbation to the ordered moments on the Fe sites. Our NMR results indicate coexistence of local and itinerant magnetism in lightly Cu-doped NaFe$_{1-x}$Cu$_{x}$As.

cond-mat.str-el↗

arXiv2020

Stripe Antiferromagnetism and Disorder in the Mott Insulator NaFe$_{1-x}$Cu$_{x}$As ($x \lesssim 0.5$)

Neutron scattering measurements have demonstrated that the heavily Cu-doped NaFe$_{1-x}$Cu$_{x}$As compound behaves like a Mott insulator exhibiting both real space Fe-Cu stripes, as well as antiferromagnetism below a Néel temperature for $x\lesssim 0.5$. We have investigated evolution of structural and magnetic ordering using $^{23}$Na and $^{75}$As NMR for single crystals ($x$ = 0.39 and 0.48), confirming antiferromagnetism in the form of magnetic stripes. We show that end-chain defects in these stripes are the principal source of magnetic disorder and are responsible for cluster spin-glass transitions in both compounds, in the latter case coexistent with antiferromagnetism. Aided by our numerical simulation of the $^{75}$As spectra, we show that a staggered magnetization at the Fe sites is induced by non-magnetic Cu dopants.

cond-mat.str-el↗

arXiv2019

Toward the Mott state with Magnetic Cluster Formation in Heavily Cu-Doped NaFe$_{1-x}$Cu$_{x}$As

Recent neutron scattering measurements indicate that NaFe$_{1-x}$Cu$_{x}$As forms an antiferromagnetic stripe phase near $x\approx 0.5$ in a Mott insulating state. This copper concentration is well in excess of that required for superconductivity, $x < 0.04$. We have investigated the development of magnetism in this compound using $^{23}$Na nuclear magnetic resonance (NMR) spectra and spin-lattice relaxation measurements performed on single crystals ($x$ = 0.13, 0.18, 0.24, and 0.39). We find multiple inequivalent Na sites, each of which is associated with a different number of nearest neighbor Fe sites occupied by a Cu dopant. We show that the distribution of Cu substituted for Fe is random in-plane for low concentrations ($x = 0.13$ and 0.18), but deviates from this with increasing Cu doping. As is characteristic of many pnictide compounds, there is a spin pseudo gap that increases in magnitude with dopant concentration. This is correlated with a corresponding increase in orbital NMR frequency shift indicating a change in valence from Cu$^{2+}$ to a Cu$^{1+}$ state as $x$ exceeds 0.18, concomitant with the change of Fe$^{2+}$ to Fe$^{3+}$ resulting in the formation of magnetic clusters. However, for $x\leq 0.39$ there is no evidence of long-range static magnetic order.

cond-mat.str-el↗