arXiv subjects

Ioan M. Pop

Publications and source records attributed to Ioan M. Pop.

At least 37 records · Page 2Linked to original sources

arXiv2024

Pure kinetic inductance coupling for cQED with flux qubits

We demonstrate a qubit-readout architecture where the dispersive coupling is entirely mediated by a kinetic inductance. This allows us to engineer the dispersive shift of the readout resonator independent of the qubit and resonator capacitances. We validate the pure kinetic coupling concept and demonstrate various generalized flux qubit regimes from plasmon to fluxon, with dispersive shifts ranging from 60 kHz to 2 MHz at the half-flux quantum sweet spot. We achieve readout performances comparable to conventional architectures with quantum state preparation fidelities of 99.7 % and 92.7 % for the ground and excited states, respectively, and below 0.1 % leakage to non-computational states.

quant-ph↗

arXiv2024

Strong Charge-Photon Coupling in Planar Germanium Enabled by Granular Aluminium Superinductors

High kinetic inductance superconductors are gaining increasing interest for the realisation of qubits, amplifiers and detectors. Moreover, thanks to their high impedance, quantum buses made of such materials enable large zero-point fluctuations of the voltage, boosting the coupling rates to spin and charge qubits. However, fully exploiting the potential of disordered or granular superconductors is challenging, as their inductance and, therefore, impedance at high values are difficult to control. Here we have integrated a granular aluminium resonator, having a characteristic impedance exceeding the resistance quantum, with a germanium double quantum dot and demonstrate strong charge-photon coupling with a rate of $g_\text{c}/2π= (566 \pm 2)$ MHz. This was achieved due to the realisation of a wireless ohmmeter, which allows \emph{in situ} measurements during film deposition and, therefore, control of the kinetic inductance of granular aluminium films. Reproducible fabrication of circuits with impedances (inductances) exceeding 13 k$Ω$ (1 nH per square) is now possible. This broadly applicable method opens the path for novel qubits and high-fidelity, long-distance two-qubit gates.

cond-mat.mes-hall↗

arXiv2024

Solomon equations for qubit and two-level systems: Insights into non-Poissonian quantum jumps

We measure and model the combined relaxation of a qubit coupled to a discrete two-level system~(TLS) environment, also known as the central spin model. If the TLSs are much longer-lived than the qubit, non-exponential relaxation and non-Poissonian quantum jumps can be observed. In the limit of large numbers of TLSs, the relaxation is likely to follow a power law, which we confirm with measurements on a superconducting fluxonium qubit. Moreover, the observed relaxation and quantum jump statistics are described by the Solomon equations, for which we present a derivation starting from the general Lindblad equation for an arbitrary number of TLSs. We also show how to reproduce the non-Poissonian quantum jump statistics using a diffusive stochastic Schrödinger equation. The fact that the measured quantum jump statistics can be reproduced by the Solomon equations, which ignore the quantum measurement backaction, hints at a quantum-to-classical transition.

quant-ph↗

arXiv2024

Two-level system hyperpolarization using a quantum Szilard engine

The innate complexity of solid state physics exposes superconducting quantum circuits to interactions with uncontrolled degrees of freedom degrading their coherence. By using a simple stabilization sequence we show that a superconducting fluxonium qubit is coupled to a two-level system (TLS) environment of unknown origin, with a relatively long energy relaxation time exceeding $50\,\text{ms}$. Implementing a quantum Szilard engine with an active feedback control loop allows us to decide whether the qubit heats or cools its TLS environment. The TLSs can be cooled down resulting in a four times lower qubit population, or they can be heated to manifest themselves as a negative temperature environment corresponding to a qubit population of $\sim 80\,\%$. We show that the TLSs and the qubit are each other's dominant loss mechanism and that the qubit relaxation is independent of the TLS populations. Understanding and mitigating TLS environments is therefore not only crucial to improve qubit lifetimes but also to avoid non-Markovian qubit dynamics.

quant-ph↗

arXiv2024

Hydrogen crystals reduce dissipation in superconducting resonators

We show that the internal quality factors of high impedance superconducting resonators made of granular aluminum can be improved by coating them with micrometric films of solid para-hydrogen molecular crystals. We attribute the average measured $\approx 8\%$ reduction in dissipation to absorption of stray terahertz radiation at the crystal-resonator interface and the subsequent dissipation of its energy in the form of phonons below the pair-breaking gap. Our results prove that, contrary to expectations, replacing the vacuum dielectric atop a superconducting resonator can be beneficial, thanks to the added protection against Cooper pair-braking terahertz radiation. Moreover, at the level of internal quality factors in the $10^5$ range, the hydrogen crystal does not introduce additional losses, which is promising for embedding impurities to couple to superconducting thin-film devices in hybrid quantum architectures.

cond-mat.supr-con↗

arXiv2023

Non-degenerate parametric amplifiers based on dispersion engineered Josephson junction arrays

Determining the state of a qubit on a timescale much shorter than its relaxation time is an essential requirement for quantum information processing. With the aid of a new type of non-degenerate parametric amplifier, we demonstrate the continuous detection of quantum jumps of a transmon qubit with 90% fidelity in state discrimination. Entirely fabricated with standard two-step optical lithography techniques, this type of parametric amplifier consists of a dispersion engineered Josephson junction (JJ) array. By using long arrays, containing $10^3$ JJs, we can obtain amplification at multiple eigenmodes with frequencies below $10~\mathrm{GHz}$, which is the typical range for qubit readout. Moreover, by introducing a moderate flux tunability of each mode, employing superconducting quantum interference device (SQUID) junctions, a single amplifier device could potentially cover the entire frequency band between 1 and $10~\mathrm{GHz}$.

quant-ph↗

arXiv2023

Implementation of a transmon qubit using superconducting granular aluminum

The high kinetic inductance offered by granular aluminum (grAl) has recently been employed for linear inductors in superconducting high-impedance qubits and kinetic inductance detectors. Due to its large critical current density compared to typical Josephson junctions, its resilience to external magnetic fields, and its low dissipation, grAl may also provide a robust source of non-linearity for strongly driven quantum circuits, topological superconductivity, and hybrid systems. Having said that, can the grAl non-linearity be sufficient to build a qubit? Here we show that a small grAl volume ($10 \times 200 \times 500 \,\mathrm{nm^3}$) shunted by a thin film aluminum capacitor results in a microwave oscillator with anharmonicity $α$ two orders of magnitude larger than its spectral linewidth $Γ_{01}$, effectively forming a transmon qubit. With increasing drive power, we observe several multi-photon transitions starting from the ground state, from which we extract $α= 2 π\times 4.48\,\mathrm{MHz}$. Resonance fluorescence measurements of the $|0> \rightarrow |1>$ transition yield an intrinsic qubit linewidth $γ= 2 π\times 10\,\mathrm{kHz}$, corresponding to a lifetime of $16\,\mathrm{μs}$. This linewidth remains below $2 π\times 150\,\mathrm{kHz}$ for in-plane magnetic fields up to $\sim70\,\mathrm{mT}$.

quant-ph↗

arXiv2022

Operating in a deep underground facility improves the locking of gradiometric fluxonium qubits at the sweet spots

We demonstrate flux-bias locking and operation of a gradiometric fluxonium artificial atom using two symmetric granular aluminum (grAl) loops to implement the superinductor. The gradiometric fluxonium shows two orders of magnitude suppression of sensitivity to homogeneous magnetic fields, which can be an asset for hybrid quantum systems requiring strong magnetic field biasing. By cooling down the device in an external magnetic field while crossing the metal-to-superconductor transition, the gradiometric fluxonium can be locked either at $0$ or $Φ_0/2$ effective flux bias, corresponding to an even or odd number of trapped fluxons, respectively. At mK temperatures, the fluxon parity prepared during initialization survives to magnetic field bias exceeding $100 \,Φ_0$. However, even for states biased in the vicinity of $1 \,Φ_0$, we observe unexpectedly short fluxon lifetimes of a few hours, which cannot be explained by thermal or quantum phase slips. When operating in a deep-underground cryostat of the Gran Sasso laboratory, the fluxon lifetimes increase to days, indicating that ionizing events activate phase slips in the grAl superinductor.

quant-ph↗

arXiv2022

Materials and devices for fundamental quantum science and quantum technologies

Technologies operating on the basis of quantum mechanical laws and resources such as phase coherence and entanglement are expected to revolutionize our future. Quantum technologies are often divided into four main pillars: computing, simulation, communication, and sensing & metrology. Moreover, a great deal of interest is currently also nucleating around energy-related quantum technologies. In this Perspective, we focus on advanced superconducting materials, van der Waals materials, and moiré quantum matter, summarizing recent exciting developments and highlighting a wealth of potential applications, ranging from high-energy experimental and theoretical physics to quantum materials science and energy storage.

quant-ph↗

arXiv2021

Energy-participation quantization of Josephson circuits

Superconducting microwave circuits incorporating nonlinear devices, such as Josephson junctions, are one of the leading platforms for emerging quantum technologies. Increasing circuit complexity further requires efficient methods for the calculation and optimization of the spectrum, nonlinear interactions, and dissipation in multi-mode distributed quantum circuits. Here, we present a method based on the energy-participation ratio (EPR) of a dissipative or nonlinear element in an electromagnetic mode. The EPR, a number between zero and one, quantifies how much of the energy of a mode is stored in each element. It obeys universal constraints--valid regardless of the circuit topology and nature of the nonlinear elements. The EPR of the elements are calculated from a unique, efficient electromagnetic eigenmode simulation of the linearized circuit, including lossy elements. Their set is the key input to the determination of the quantum Hamiltonian of the system. The method provides an intuitive and simple-to-use tool to quantize multi-junction circuits. It is especially well-suited for finding the Hamiltonian and dissipative parameters of weakly anharmonic systems, such as transmon qubits coupled to resonators, or Josephson transmission lines. We experimentally tested this method on a variety of Josephson circuits, and demonstrated agreement within several percents for nonlinear couplings and modal Hamiltonian parameters, spanning five-orders of magnitude in energy, across a dozen samples.

quant-ph↗

arXiv2021

Superconducting microwave magnetometer for absolute flux detection

Superconducting quantum interference devices (SQUIDs) are among the most sensitive detectors for out-of-plane magnetic field components. However, due to their periodic response with short modulation period $M = 1 Φ_0$, determined by the magnetic flux quantum $Φ_0 \approx 2.068\times 10^{-15}\,\mathrm{Wb}$, it is difficult to infer the value of the magnetic flux unambiguously, especially in case the magnetic flux enclosed in the SQUID loop changes by many flux quanta. Here, we demonstrate that by introducing a second degree of freedom in the form of a second SQUID, we substantially enhance the modulation period $M$ of our device without sacrificing sensitivity. As a proof of concept, we implement our idea by embedding two asymmetric direct current SQUIDs into a common tank circuit. By measuring the reflection coefficient of the device, we extract the two lowest energy eigenfrequencies as a function of the external magnetic flux created by a superconducting field coil, from which we experimentally deduce a modulation period $M \geq 15 Φ_0$, as well as the magnetic offset-field $B_0 = 22\,\mathrm{nT}$ present in our experiment.

quant-ph↗

arXiv2020

Quantum non-demolition dispersive readout of a superconducting artificial atom using large photon numbers

Reading out the state of superconducting artificial atoms typically relies on dispersive coupling to a readout resonator. For a given system noise temperature, increasing the circulating photon number $\bar{n}$ in the resonator enables a shorter measurement time and is therefore expected to reduce readout errors caused by spontaneous atom transitions. However, increasing $\bar{n}$ is generally observed to also increase these transition rates. Here we present a fluxonium artificial atom in which we measure an overall flat dependence of the transition rates between its first two states as a function of $\bar{n}$, up to $\bar{n}\approx200$. Despite the fact that we observe the expected decrease of the dispersive shift with increasing readout power, the signal-to-noise ratio continuously improves with increasing $\bar{n}$. Even without the use of a parametric amplifier, at $\bar{n}=74$, we measure fidelities of 99% and 93% for feedback-assisted ground and excited state preparation, respectively.

quant-ph↗

arXiv2020

Minimizing the discrimination time for quantum states of an artificial atom

Fast discrimination between quantum states of superconducting artificial atoms is an important ingredient for quantum information processing. In circuit quantum electrodynamics, increasing the signal field amplitude in the readout resonator, dispersively coupled to the artificial atom, improves the signal-to-noise ratio and increases the measurement strength. Here we employ this effect over two orders of magnitude in readout power, made possible by the unique combination of a dimer Josephson junction array amplifier with a large dynamic range, and the fact that the readout of our granular aluminum fluxonium artificial atom remained quantum-non-demolition (QND) at relatively large photon numbers in the readout resonator, up to $\overline{n} = 110$. Using Bayesian inference, this allows us to detect quantum jumps faster than the readout resonator response time $2/κ$, where $κ$ is the bandwidth of the readout resonator.

quant-ph↗

arXiv2020

Reducing the impact of radioactivity on quantum circuits in a deep-underground facility

As quantum coherence times of superconducting circuits have increased from nanoseconds to hundreds of microseconds, they are currently one of the leading platforms for quantum information processing. However, coherence needs to further improve by orders of magnitude to reduce the prohibitive hardware overhead of current error correction schemes. Reaching this goal hinges on reducing the density of broken Cooper pairs, so-called quasiparticles. Here, we show that environmental radioactivity is a significant source of nonequilibrium quasiparticles. Moreover, ionizing radiation introduces time-correlated quasiparticle bursts in resonators on the same chip, further complicating quantum error correction. Operating in a deep-underground lead-shielded cryostat decreases the quasiparticle burst rate by a factor fifty and reduces dissipation up to a factor four, showcasing the importance of radiation abatement in future solid-state quantum hardware.

cond-mat.supr-con↗

arXiv2020

Quantum versus classical switching dynamics of driven-dissipative Kerr resonators

We report a first-principles study of the driven dissipative dynamics for Kerr oscillators in the mesoscopic regime. This regime is characterized by large Kerr nonlinearity, realized here using the nonlinear kinetic inductance of a large array of Josephson junctions. The experimentally measured nonlinear resonance lineshapes of the junction array modes show significant deviations from steady-state numerical predictions, and necessitate time-dependent numerical simulations indicative of strong measurement-induced dephasing in the system arising from the large cross-Kerr effect between array modes. Analytical and numerical calculations of switching rate corroborate this by showing the emergence of a slow time scale, which is much longer than the linear decay rate and is set by fluctuation-induced switching times in the bistable regime. Furthermore, our analysis shows that the usual quantum-activated escape treatment is inadequate for prediction of the switching rates at large frequency shifts caused by strong nonlinearities, necessitating a quantum treatment that utilizes the full system Liouvillian. Based on our analysis, we identify a universal crossover parameter that delineates the regimes of validity of semiclassical and quantum descriptions, respectively. Our work shows how dynamical switching effects in strongly nonlinear systems provide a platform to study quantum-to-classical transitions.

quant-ph↗

arXiv2019

State preparation of a fluxonium qubit with feedback from a custom FPGA-based platform

We developed a versatile integrated control and readout instrument for experiments with superconducting quantum bits (qubits), based on a field-programmable gate array (FPGA) platform. Using this platform, we perform measurement-based, closed-loop feedback operations with $428 \, \mathrm{ns}$ platform latency. The feedback capability is instrumental in realizing active reset initialization of the qubit into the ground state in a time much shorter than its energy relaxation time $T_1$. We show experimental results demonstrating reset of a fluxonium qubit with $99.4\,\%$ fidelity, using a readout-and-drive pulse sequence approximately $1.5 \, \mathrm{μs}$ long. Compared to passive ground state initialization through thermalization, with the time constant given by $T_1 = ~ 80 \, \mathrm{μs}$, the use of the FPGA-based platform allows us to improve both the fidelity and the time of the qubit initialization by an order of magnitude.

quant-ph↗

arXiv2019

Microscopic charging and in-gap states in superconducting granular aluminum

Following the emergence of superconducting granular aluminum (grAl) as a material for high-impedance quantum circuits, future development hinges on a microscopic understanding of its phase diagram, and whether the superconductor-to-insulator transition (SIT) is driven by disorder or charging effects. Beyond fundamental relevance, these mechanisms govern noise and dissipation in microwave circuits. Although the enhancement of the critical temperature, and the SIT in granular superconductors have been studied for more than fifty years, experimental studies have so far provided incomplete information on the microscopic phenomena. Here we present scanning tunneling microscope measurements of the local electronic structure of superconducting grAl. We confirm an increased superconducting gap in individual grains both near and above the Mott resistivity $ρ_\mathrm{M} \approx 400\ μΩcm$. Above $ρ_\mathrm{M}$ we find Coulomb charging effects, a first indication for decoupling, and in-gap states on individual grains, which could contribute to flux noise and dielectric loss in quantum devices. We also observe multiple low-energy states outside the gap, which may indicate bosonic excitations of the superconducting order parameter.

cond-mat.supr-con↗

arXiv2019

Onset of phase diffusion in high kinetic inductance granular aluminum micro-SQUIDs

Superconducting granular aluminum is attracting increasing interest due to its high kinetic inductance and low dissipation, favoring its use in kinetic inductance particle detectors, superconducting resonators or quantum bits. We perform switching current measurements on DC-SQUIDs, obtained by introducing two identical geometric constrictions in granular aluminum rings of various normal-state resistivities in the range from $ρ_\mathrm{n} = 250\,μΩ\mathrm{cm}$ to $5550\,μΩ\mathrm{cm}$. The relative high kinetic inductance of the SQUID loop, in the range of tens of nH, leads to a suppression of the modulation in the measured switching current versus magnetic flux, accompanied by a distortion towards a triangular shape. We observe a change in the temperature dependence of the switching current histograms with increasing normal-state film resistivity. This behavior suggests the onset of a diffusive motion of the superconducting phase across the constrictions in the two-dimensional washboard potential of the SQUIDs, which could be caused by a change of the local electromagnetic environment of films with increasing normal-state resistivities.

cond-mat.supr-con↗