arXiv subjects

Ireneusz Weymann

Publications and source records attributed to Ireneusz Weymann.

At least 55 records · Page 3Linked to original sources

arXiv2017

Spin-resolved dynamical conductance of correlated large-spin magnetic molecules

The finite-frequency transport properties of a large-spin molecule attached to ferromagnetic contacts are studied theoretically in the Kondo regime. The focus is on the behavior of the dynamical conductance in the linear response regime, which is determined by using the numerical renormalization group method. It is shown that the dynamical conductance depends greatly on the magnetic configuration of the device and intrinsic parameters of the molecule. In particular, conductance exhibits characteristic features for frequencies corresponding to the dipolar and quadrupolar exchange fields resulting from the presence of spin-dependent tunneling. Moreover, a dynamical spin accumulation in the molecule, associated with the off-diagonal-in-spin component of the conductance, is predicted. This spin accumulation becomes enhanced with increasing the spin polarization of the leads, and it results in a nonmonotonic dependence of the conductance on frequency, with local maxima occurring for characteristic energy scales.

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arXiv2017

Noise of a chargeless Fermi liquid

We construct a Fermi liquid theory to describe transport in a superconductor-quantum dot- normal metal junction close to the singlet-doublet (parity changing) transition of the dot. Though quasiparticles do not have a definite charge in this chargeless Fermi liquid, in case of particle-hole symmetry, a mapping to the Anderson model unveils a hidden U(1) symmetry and a corresponding pseudo-charge. In contrast to other correlated Fermi-liquids, the back scattering noise reveals an effective charge equal to the charge of Cooper pairs, $e^* = 2e$. In addition,we find a strong suppression of noise when the linear conductance is unitary, even for its non-linear part.

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arXiv2016

Strong spin Seebeck effect in Kondo T-shaped double quantum dots

We theoretically investigate the thermoelectric and spin thermoelectric properties of a T-shaped double quantum dot strongly coupled to two ferromagnetic leads, focusing on transport regime where the system exhibits the two-stage Kondo effect. We study the dependence of the (spin) Seebeck coefficient, the corresponding power factor and the figure of merit on temperature, leads' spin polarization and dot level position. We show that the thermal conductance fulfills a modified Wiedemann-Franz law. We also demonstrate that the spin thermopower is enhanced at temperatures corresponding to the second stage of Kondo screening. Very interestingly, the spin-thermoelectric response of the system is found to be highly sensitive to the spin polarization of the leads. In some cases spin polarization of the order of 1% is sufficient for a strong spin Seebeck effect to occur. This is explained as a consequence of the interplay between the two-stage Kondo effect and the exchange field induced in the double quantum dot. All calculations are performed with the aid of numerical renormalization group technique.

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arXiv2015

Spin-resolved Andreev transport through double-quantum-dot Cooper pair splitters

We investigate the Andreev transport through double-quantum-dot Cooper pair splitters with ferromagnetic leads. The analysis is performed with the aid of the real-time diagrammatic technique in the sequential tunneling regime. We study the dependence of the Andreev current, the differential conductance, and the tunnel magnetoresistance on various parameters of the model in both the linear and nonlinear response regimes. In particular, we analyze the spin-resolved transport in the crossed Andreev reflection regime, where a blockade of the current occurs due to enhanced occupation of the triplet state. We show that in the triplet blockade, finite intradot correlations can lead to considerable leakage current due to direct Andreev reflection processes. Furthermore, we find additional regimes of current suppression resulting from enhanced occupation of singlet states, which decreases the rate of crossed Andreev reflection.We also study how the splitting of Andreev bound states, triggered by either dot level detuning, finite hopping between the dots, or finite magnetic field, affects the Andreev current. While in the first two cases the number of Andreev bound states is doubled, whereas transport properties are qualitatively similar, in the case of finite magnetic field further level splitting occurs, leading to a nontrivial behavior of spin-resolved transport characteristics, and especially that of tunneling magnetoresistance. Finally, we discuss the entanglement fidelity between split Cooper pair electrons and show that by tuning the device parameters, fidelity can reach unity.

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arXiv2014

Transverse anisotropy effects on spin-resolved transport through large-spin molecules

The transport properties of a large-spin molecule strongly coupled to ferromagnetic leads in the presence of transverse magnetic anisotropy are studied theoretically. The relevant spectral functions, linear-response conductance and the tunnel magnetoresistance are calculated by means of the numerical renormalization group method. We study the dependence of transport characteristics on orbital level position, uniaxial and transverse anisotropies, external magnetic field and temperature. It is shown that while uniaxial magnetic anisotropy leads to the suppression of the Kondo effect, finite transverse anisotropy can restore the Kondo resonance. The effect of Kondo peak restoration strongly depends on the magnetic configuration of the device and leads to nontrivial behavior of the tunnel magnetoresistance. We show that the temperature dependence of the conductance at points where the restoration of the Kondo effect occurs is universal and shows a scaling typical for usual spin-one-half Kondo effect.

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arXiv2014

Proximity effect on spin-dependent conductance and thermopower of correlated quantum dots

We study the electric and thermoelectric transport properties of correlated quantum dots coupled to two ferromagnetic leads and one superconducting electrode. Transport through such hybrid devices depends on the interplay of ferromagnetic-contact induced exchange field, superconducting proximity effect and correlations leading to the Kondo effect. We consider the limit of large superconducting gap. The system can be then modeled by an effective Hamiltonian with a particle-non-conserving term describing the creation and annihilation of Cooper pairs. By means of the full density-matrix numerical renormalization group method, we analyze the behavior of electrical and thermal conductances, as well as the Seebeck coefficient as a function of temperature, dot level position and the strength of the coupling to the superconductor. We show that the exchange field may be considerably affected by the superconducting proximity effect and is generally a function of Andreev bound state energies. Increasing the coupling to the superconductor may raise the Kondo temperature and partially restore the exchange-field-split Kondo resonance. The competition between ferromagnetic and superconducting proximity effects is reflected in the corresponding temperature and dot level dependence of both the linear conductance and the (spin) thermopower.

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arXiv2013

Probing the Rashba effect via the induced magnetization around a Kondo impurity

When a single magnetic adatom is deposited on a surface of a metal, it affects the charge and spin texture of the electron gas surrounding it. The screening of the local moment by conduction electrons gives rise to the Kondo effect. Here we investigate the effect of the Rashba spin orbit coupling on the local magnetization density of states (LMDOS) around a Cobalt impurity on a Au(111) surface in a magnetic field. We show that the in-plane component of the LMDOS is exclusively associated with the Rashba spin orbit interaction. This observation can be experimentally exploited to confirm the presence of the Rashba effect on surfaces, such as Au(111), by performing spin-polarized STM measurements around the Kondo impurity.

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arXiv2013

Temperature dependence of electronic transport through molecular magnets in the Kondo regime

The effects of finite temperature in transport through nanoscopic systems exhibiting uniaxial magnetic anisotropy D, such as molecular magnets, adatoms, or quantum dots side-coupled to a large spin are analyzed in the Kondo regime. The linear-response conductance is calculated by means of the full density-matrix numerical renormalization group method as a function of temperature T, magnetic anisotropy D, and exchange coupling J between the molecule's core spin and the orbital level. It is shown that such system displays a two-stage Kondo effect as a function of temperature and a quantum phase transition as a function of the exchange coupling J. Moreover, additional peaks are found in the linear conductance for temperatures of the order of T\sim|J| and T\simD. It is also shown that the conductance variation with T remarkably depends on the sign of the exchange coupling J.

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arXiv2013

Underscreened Kondo effect in S=1 magnetic quantum dots: Exchange, anisotropy and temperature effects

We present a theoretical analysis of the effects of uniaxial magnetic anisotropy and contact-induced exchange field on the underscreened Kondo effect in S=1 magnetic quantum dots coupled to ferromagnetic leads. First, by using the second-order perturbation theory we show that the coupling to spin-polarized electrode results in an effective exchange field $B_{\rm eff}$ and an effective magnetic anisotropy $D_{\rm eff}$. Second, we confirm these findings by using the numerical renormalization group method, which is employed to study the dependence of the quantum dot spectral functions, as well as quantum dot spin, on various parameters of the system. We show that the underscreened Kondo effect is generally suppressed due to the presence of effective exchange field and can be restored by tuning the anisotropy constant, when $|D_{\rm eff}| = |B_{\rm eff}|$. The Kondo effect can also be restored by sweeping an external magnetic field, and the restoration occurs twice in a single sweep. From the distance between the restored Kondo resonances one can extract the information about both the exchange field and the effective anisotropy. Finally, we calculate the temperature dependence of linear conductance for the parameters where the Kondo effect is restored and show that the restored Kondo resonances display a universal scaling of $S=1/2$ Kondo effect.

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arXiv2012

The Influence of Magnetic Anisotropy on the Kondo Effect and Spin-Polarized Transport through Magnetic Molecules, Adatoms and Quantum Dots

Transport properties in the Kondo regime of a nanosystem displaying uniaxial magnetic anisotropy (such as a magnetic molecule, magnetic adatom or quantum dot coupled to a localized magnetic moment) are analyzed theoretically. In particular, the influence of spin-polarized transport through a local orbital of the system and exchange coupling of conduction electrons to the system's magnetic core on the Kondo effect is discussed. The numerical renormalization group method is applied to calculate the spectral functions and linear conductance in the case of the parallel and antiparallel configurations of the electrodes' magnetic moments. It is shown that both the magnetic anisotropy as well as the exchange coupling between electrons tunneling through the conducting orbital and magnetic core play an important role in formation of the Kondo resonance, leading generally to its suppression. Specific transport properties of such a system appear also as a nontrivial behavior of tunnel magnetoresistance. It is also shown that the Kondo effect can be restored by an external magnetic field in both the parallel and antiparallel magnetic configurations.

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arXiv2012

Electrically controlled quantum dot based spin current injector

We present a proposal for a fully electrically controllable quantum dot based spin current injector. The device consists of a quantum dot that is strongly coupled to a ferromagnetic electrode on one side and weakly coupled to a nonmagnetic electrode on the other side. The presence of ferromagnetic electrode results in an exchange field that splits the dot level. We show that this exchange-induced splitting can lead to almost full spin polarization of the current flowing through the device. Moreover, we also demonstrate that the sign of the polarization can be changed by the gate or the bias voltage within a switching time in the nanosecond range. Thus the proposed device can operate as an electrically controlled, fast switchable spin current source, which can be realized in various state-of-the-art nanostructures.

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arXiv2011

Interplay of the Kondo Effect and Spin-Polarized Transport in Magnetic Molecules, Adatoms and Quantum Dots

We study the interplay of the Kondo effect and spin-polarized tunneling in a class of systems exhibiting uniaxial magnetic anisotropy, such as magnetic molecules, magnetic adatoms, or quantum dots coupled to a single localized magnetic moment. Using the numerical renormalization group method we calculate the spectral functions and linear conductance in the Kondo regime. We show that the exchange coupling between conducting electrons and localized magnetic core generally leads to suppression of the Kondo effect. We also predict a nontrivial dependence of the tunnel magnetoresistance on the strength of exchange coupling and on the anisotropy constant.

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arXiv2010

Spin effects in transport through single-molecule magnets in the sequential and cotunneling regimes

We analyze the stationary spin-dependent transport through a single-molecule magnet weakly coupled to external ferromagnetic leads. Using the real-time diagrammatic technique, we calculate the sequential and cotunneling contributions to current, tunnel magnetoresistance and Fano factor in both linear and nonlinear response regimes. We show that the effects of cotunneling are predominantly visible in the blockade regime and lead to enhancement of tunnel magnetoresistance (TMR) above the Julliere value, which is accompanied with super-Poissonian shot noise due to bunching of inelastic cotunneling processes through different virtual spin states of the molecule. The effects of external magnetic field and the role of type and strength of exchange interaction between the LUMO level and the molecule's spin are also considered. When the exchange coupling is ferromagnetic, we find an enhanced TMR, while in the case of antiferromagnetic coupling we predict a large negative TMR effect.

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arXiv2010

Kondo effect in a quantum dot coupled to ferromagnetic leads and side-coupled to a nonmagnetic reservoir

Equilibrium transport properties of a single-level quantum dot tunnel-coupled to ferromagnetic leads and exchange-coupled to a side nonmagnetic reservoir are analyzed theoretically in the Kondo regime. The equilibrium spectral functions and conductance through the dot are calculated using the numerical renormalization group (NRG) method. It is shown that in the antiparallel magnetic configuration, the system undergoes a quantum phase transition with increasing exchange coupling $J$, where the conductance drops from its maximum value to zero. In the parallel configuration, on the other hand, the conductance is generally suppressed due to an effective spin splitting of the dot level caused by the presence of ferromagnetic leads, irrespective of the strength of exchange constant. However, for $J$ ranging from J=0 up to the corresponding critical value, the Kondo effect and quantum critical behavior can be restored by applying properly tuned compensating magnetic field.

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arXiv2010

Underscreened Kondo effect in quantum dots coupled to ferromagnetic leads

We analyze the equilibrium transport properties of underscreened Kondo effect in the case of a two-level quantum dot coupled to ferromagnetic leads. Using the numerical renormalization group (NRG) method, we have determined the gate voltage dependence of the dot's spin and level-resolved spectral functions. We have shown that the polarization of the dot is very susceptible to spin imbalance in the leads and changes sign in the middle of the S=1 Coulomb valley. Furthermore, we have also found that by fine-tuning an external magnetic field one can compensate for the presence of ferromagnetic leads and restore the Kondo effect in the case of $S=1/2$ Coulomb valley. However, the underscreened Kondo effect cannot be fully recovered due to its extreme sensitivity with respect to the magnetic field.

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arXiv2009

The tunnel magnetoresistance in chains of quantum dots weakly coupled to external leads

We analyze numerically the spin-dependent transport through coherent chains of three coupled quantum dots weakly connected to external magnetic leads. In particular, using the diagrammatic technique on the Keldysh contour, we calculate the conductance, shot noise and tunnel magnetoresistance (TMR) in the sequential and cotunneling regimes. We show that transport characteristics greatly depend on the strength of the interdot Coulomb correlations, which determines the spacial distribution of electron wave function in the chain. When the correlations are relatively strong, depending on the transport regime, we find both negative TMR as well as TMR enhanced above the Julliere value, accompanied with negative differential conductance (NDC) and super-Poissonian shot noise. This nontrivial behavior of tunnel magnetoresistance is associated with selection rules that govern tunneling processes and various high-spin states of the chain that are relevant for transport. For weak interdot correlations, on the other hand, the TMR is always positive and not larger than the Julliere TMR, although super-Poissonian shot noise and NDC can still be observed.

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arXiv2009

Negative tunnel magnetoresistance and differential conductance in transport through double quantum dots

Spin-dependent transport through two coupled single-level quantum dots weakly connected to ferromagnetic leads with collinear magnetizations is considered theoretically. Transport characteristics, including the current, linear and nonlinear conductance, and tunnel magnetoresistance are calculated using the real-time diagrammatic technique in the parallel, serial, and intermediate geometries. The effects due to virtual tunneling processes between the two dots via the leads, associated with off-diagonal coupling matrix elements, are also considered. Negative differential conductance and negative tunnel magnetoresistance have been found in the case of serial and intermediate geometries, while no such behavior has been observed for double quantum dots coupled in parallel. It is also shown that transport characteristics strongly depend on the magnitude of the off-diagonal coupling matrix elements.

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arXiv2007

Transport through two-level quantum dots weakly coupled to ferromagnetic leads

Spin-dependent transport through a two-level quantum dot in the sequential tunneling regime is analyzed theoretically by means of a real-time diagrammatic technique. It is shown that the current, tunnel magnetoresistance, and shot noise (Fano factor) strongly depend on the transport regime, providing a detailed information on the electronic structure of quantum dots and their coupling to external leads. When the dot is asymmetrically coupled to the leads, a negative differential conductance may occur in certain bias regions, which is associated with a super-Poissonian shot noise. In the case of a quantum dot coupled to one half-metallic and one nonmagnetic lead, one finds characteristic Pauli spin blockade effects. Transport may be also suppressed when the dot levels are coupled to the leads with different coupling strengths. The influence of an external magnetic field on transport properties is also discussed.

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