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Irfan H. Abidi

Publications and source records attributed to Irfan H. Abidi.

6 recordsLinked to original sources

AI based design of 2D material integrated optical polarizers

On-chip integration of highly anisotropic two-dimensional (2D) materials offers new opportunities for realizing high performance polarization selective devices. Obtaining optimized designs for such devices requires extensively sweeping large parameter spaces, which in conventional approaches relies on massive mode simulations that demand considerable computational resources. Here, we address this limitation by developing a machine learning (ML) model based on fully connected neural networks (FCNNs). Trained by using mode simulation results for low resolution structural parameters, the FCNN model can accurately predict polarizer figures of merits (FOMs) for high resolution parameters and rapidly map the global variation trend across the entire parameter space. We test the performance of the FCNN model using two types of polarizers with 2D graphene oxide (GO) and molybdenum disulfide (MoS2). Results show that, compared to conventional mode simulation approach, our approach can not only reduce the overall computing time by about 4 orders of magnitude, but also achieve highly accurate FOM predictions with an average deviation of less than 0.04. In addition, the measured FOM values for the fabricated devices show good agreement with the predicted ones, with discrepancies remaining below 0.2. These results validate artificial intelligence (AI) as an effective approach for designing and optimizing 2D-material based optical polarizers with high efficiency.

physics.optics↗

Enhanced selfphase modulation in silicon nitride waveguides with integrated 2D MoS2 films

On-chip integration of 2D materials provides a promising route towards next-generation integrated optical devices with performance beyond existing limits. Here, significantly enhanced spectral broadening induced by self-phase modulation (SPM) is experimentally demonstrated in silicon nitride (Si3N4) waveguides integrated with 2D monolayer molybdenum disulfide (MoS2) films. Monolayer MoS2 films with ultrahigh optical nonlinearity are synthesized via low-pressure chemical vapor deposition (LPCVD) and subsequently transferred onto Si3N4 waveguides, with precise control of the film coating length and placement achieved by selectively opening windows on the chip silica upper cladding. Detailed SPM measurements at telecom wavelengths are performed using fabricated waveguides with various MoS2 film coating lengths. Compared to devices without MoS2, increased spectral broadening of sub-picosecond optical pulses is observed for the hybrid devices, achieving a broadening factor of up to ~ 2.4 for a device with a 1.4-mm-long MoS2 film. Theoretical fitting of the experimental results further reveals an increase of up to ~27 fold in the nonlinear parameter (γ) for the hybrid MoS2 / Si3N4 waveguides and an equivalent Kerr coefficient (n2) of MoS2 nearly 5 orders of magnitude higher than Si3N4. These results confirm the effectiveness of on-chip integration of 2D MoS2 films to enhance the nonlinear optical performance of integrated photonic devices.

physics.optics↗

Silicon Integrated Photonic Waveguide Polarizers with 2D MoS2 Films

Polarization control is of fundamental importance for modern optical systems, and optical polarizers serve as critical components for enabling this functionality. Here, we experimentally demonstrate optical polarizers by integrating 2D molybdenum disulfide (MoS2) films onto silicon photonic waveguides. High-quality monolayer MoS2 films with highly anisotropic light absorption are synthesized via a low-pressure chemical vapor deposition (LPCVD) method and subsequently transferred onto silicon-on-insulator (SOI) nanowire waveguides to fabricate integrated optical polarizers. Detailed measurements are carried out for the fabricated devices with various MoS2 film coating lengths and silicon waveguide geometry. The results show that a maximum polarization-dependent loss of ~21 dB is achieved, together with a high figure of merit of ~4.2. In addition, the hybrid waveguide polarizers exhibit broad operation bandwidth exceeding ~100 nm and excellent power durability. These results highlight the strong potential for on-chip integration of 2D MoS2 films to implement high-performance polarization selective devices.

physics.optics↗

Intrinsic defect engineering of CVD grown monolayer MoS$_2$ for tuneable functional nanodevices

Defects in atomically thin materials can drive new functionalities and expand applications to multifunctional systems that are monolithically integrated. An ability to control formation of defects during the synthesis process is an important capability to create practical deployment opportunities. Molybdenum disulfide (MoS$_2$), a two-dimensional (2D) semiconducting material harbors intrinsic defects that can be harnessed to achieve tuneable electronic, optoelectronic, and electrochemical devices. However, achieving precise control over defect formation within monolayer MoS$_2$, while maintaining the structural integrity of the crystals remains a notable challenge. Here, we present a one-step, in-situ defect engineering approach for monolayer MoS$_2$ using a pressure dependent chemical vapour deposition (CVD) process. Monolayer MoS$_2$ grown in low-pressure CVD conditions (LP-MoS$_2$) produces sulfur vacancy (Vs) induced defect rich crystals primarily attributed to the kinetics of the growth conditions. Conversely, atmospheric pressure CVD grown MoS$_2$ (AP-MoS$_2$) passivates these Vs defects with oxygen. This disparity in defect profiles profoundly impacts crucial functional properties and device performance. AP-MoS$_2$ shows a drastically enhanced photoluminescence, which is significantly quenched in LP-MoS$_2$ attributed to in-gap electron donor states induced by the Vs defects. However, the n-doping induced by the Vs defects in LP-MoS$_2$ generates enhanced photoresponsivity and detectivity in our fabricated photodetectors compared to the AP-MoS$_2$ based devices. Defect-rich LP-MoS$_2$ outperforms AP-MoS$_2$ as channel layers of field-effect transistors (FETs), as well as electrocatalytic material for hydrogen evolution reaction (HER). This work presents a single-step CVD approach for in-situ defect engineering in monolayer MoS$_2$ and presents a pathway to control defects in other monolayer material systems.

physics.app-ph↗

Quantum emitter formation in carbon-doped monolayer hexagonal boron nitride

Single photon emitters (SPEs) in hexagonal boron nitride (hBN) are promising candidates for quantum light generation. Despite this, techniques to control the formation of hBN SPEs down to the monolayer limit are yet to be demonstrated. Recent experimental and theoretical investigations have suggested that the visible wavelength single photon emitters in hBN originate from carbon-related defects. Here we demonstrate a simple strategy for controlling SPE creation during the chemical vapor deposition growth of monolayer hBN via regulating surface carbon concentration. By increasing surface carbon concentration during hBN growth, we observe increases in carbon doping levels by 2.4 fold for B-C bonds and 1.6 fold for N-C bonds. For the same samples we observe an increase in SPE density from 0.13 to 0.30 emitters/um2. Our simple method enables the reliable creation of hBN SPEs in monolayer samples for the first time, opening the door to advanced 2D quantum state engineering.

cond-mat.mtrl-sci↗

Selective Defect Formation in Hexagonal Boron Nitride

Luminescent defect-centers in hexagonal boron nitride (hBN) have emerged as a promising 2D-source of single photon emitters (SPEs) due to their high brightness and robust operation at room temperature. The ability to create such emitters with well-defined optical properties is a cornerstone towards their integration into on-chip photonic architectures. Here, we report an effective approach to fabricate hBN single photon emitters (SPEs) with desired emission properties in two isolated spectral regions via the manipulation of boron diffusion through copper during atmospheric pressure chemical vapor deposition (APCVD)--a process we term gettering. Using the gettering technique we deterministically place the resulting zero-phonon line (ZPL) between the regions 550-600 nm or from 600-650 nm, paving the way for hBN SPEs with tailored emission properties across a broad spectral range. Our ability to control defect formation during hBN growth provides a simple and cost-effective means to improve the crystallinity of CVD hBN films, and lower defect density making it applicable to hBN growth for a wide range of applications. Our results are important to understand defect formation of quantum emitters in hBN and deploy them for scalable photonic technologies.

physics.app-ph↗