Isaac M. Pope | Searcharxiv

arXiv2026

A thermoelastic limit on the focal intensity in Fabry-P\'erot cavities

Light in the mode of a Fabry-P\'erot cavity heats the mirror surfaces via optical absorption, causing thermoelastic deformation of the mirror substrates, which in turn dictates the shape of the mode. We develop an analytical model which predicts that this effect limits the maximum focal intensity of the mode. Using two near-concentric Fabry-P\'erot cavities -- one with 4.5-fold higher mirror absorption than the other -- we measure the thermoelastic properties of the cavity mirrors and demonstrate that it is possible to achieve at least 70% of this predicted limit (in the high-absorption cavity), and that the predicted limit is 2.9 TW/cm^2 (in the low-absorption cavity).

physics.optics↗

arXiv2023

Probing the limits of optical cycling in a predissociative diatomic molecule

Molecular predissociation is the spontaneous, nonradiative bond breaking process that can occur upon excitation. In the context of laser cooling, predissociation is an unwanted consequence of molecular structure that limits the ability to scatter a large number of photons required to reach the ultracold regime. Unlike rovibrational branching, predissociation is irreversible since the fragments fly apart with high kinetic energy. Of particular interest is the simple diatomic molecule, CaH, for which the two lowest electronically excited states used in laser cooling lie above the dissociation threshold of the ground potential. In this work, we present measurements and calculations that quantify the predissociation probabilities affecting the cooling cycle. The results allow us to design a laser cooling scheme that will enable the creation of an ultracold and optically trapped cloud of CaH molecules. In addition, we use the results to propose a two-photon pathway to controlled dissociation of the molecules, in order to gain access to their ultracold fragments, including hydrogen.

physics.atom-ph↗