arXiv subjects

Isabel Guillamón

Publications and source records attributed to Isabel Guillamón.

At least 19 recordsLinked to original sources

arXiv2026

Visualizing impurity-driven scattering phase textures in EuCd2As2

Understanding how disorder modifies electronic states in magnetic semiconductors is important for controlling spin-dependent transport and topological responses. Here we use scanning tunneling microscopy to visualize scattering phase textures in EuCd2As2. By isolating a single surface wavevector we reconstruct spatial phase maps of the local density of states and identify phase dislocations characterized by 2pi winding around impurity sites. These phase singularities emerge systematically within charge puddles generated by Eu interstitials and their positions evolve with bias voltage. We show that their spatial structure is consistent with interference between multiple scattering channels, including contributions from spin-orbit coupling. We provide a model which reproduces phase dislocations and relates the decay of the phase gradient to the relative strength of spin-orbit and scalar scattering. Our results establish a route to access the phase of electronic scattering in real space and study the role of local disorder and spin-orbit interactions in shaping electronic states in quantum materials.

cond-mat.mtrl-sci↗

arXiv2026

Surface charge density wave in UTe2

The spatially uniform electronic density characteristic of a metal can become unstable at low temperatures, leading to the formation of charge density waves (CDWs). These CDWs, observed in dichalcogenides, cuprates and pnictides, arise from the interplay between the crystal lattice and the electronic structure, which can facilitate charge ordering. However, CDWs are rarely observed in the presence of Kondo screening and heavy fermion quasiparticles. The heavy fermion topological superconductor candidate UTe$_2$ presents a notable exception, exhibiting a CDW whose origin remains elusive. Here we report high resolution scanning tunneling microscopy (STM) experiments that reveal the primitive wavevectors of the CDW in UTe$_2$. This allows us to identify hot spots in the electronic band structure that are connected to the CDW. Although the corresponding wavevectors have apparently no specific influence on some bulk properties, for example on antiferromagnetic fluctuations, we find that they lead to a spatial modulation of the heavy fermion hybridization pattern. We propose that surface induced modifications in the U 5f electron valence enable a novel form of purely electron-driven charge ordering.

cond-mat.str-el↗

arXiv2026

Bridging atomic and mesoscopic length scales with Replica Scanning Tunneling Microscopy: Visualizing the atomic lattice of UTe$_2$ and the atomic scale superconducting gap modulations of FeSe close to micron length scales

Scanning Tunneling Microscopy is a cornerstone technique for visualizing the electronic density of states with atomic resolution (typically below 0.1 nm). While the field of view of most STM setups extends up to a few microns, obtaining atomic resolution over these large areas is often impractical and excessively time-consuming. This is due to the need to acquire maps with a point number reaching $10^7$ or more with a full current or conductance vs voltage curve at each point. The standard procedure is to make large scale maps and then select small regions to zoom-in for high-resolution atomic scale analysis. However, this approach fails to address a question which is often critical: Does a specific atomic-scale modulation of the electronic density of states persist over much larger, mesoscopic length scales? Here we present a new method: Replica STM (R-STM), that overcomes this limitation, allowing the study of atomic-scale phenomena up to micron length scales. We obtained new large-area STM tunneling conductance maps in UTe$_2$ and FeSe, spanning areas over 200 nm in size. In these large scale maps we discovered periodic signals with wavelengths significantly exceeding interatomic distances. We show that these large-wavelength periodic signals are replicas of the underlying atomic-scale density of states modulations. R-STM leverages these replica signals to efficiently track atomic-scale features over large areas. We discuss the influence of phase slips, disorder and defects in the replicas. Our results suggest that atomic scale modulations of the superconducting density of states could persist over large length scales in FeSe. R-STM provides a new capability for STM to compare atomic scale with micrometer scale phenomena. The proof of principle of R-STM can be extended to any other scanning probe microscopy experiment where a periodic signal is traced as a function of position.

cond-mat.supr-con↗

arXiv2026

Robust two-dimensional surface superconductivity and vortex lattice in the Weyl semimetal $γ$-PtBi$_2$

The layered compound $γ$-PtBi$_2$ is a topological semimetal with Fermi arcs at the surface joining bulk Weyl points. Recent work has found signatures of surface superconductivity consisting of gap openings compatible with a critical temperature orders of magnitude larger than the bulk value. However, no superconducting vortices have been identified, raising questions about the robustness of the phase coherence. Here we use very low temperature Scanning Tunneling Microscopy (STM) and find robust superconductivity with T$_C=$2.9 K and H$_{C2}\approx$1.8 T linked to the Fermi arcs. We observe quantized superconducting vortices and the Josephson effect, demonstrating two-dimensional macroscopic quantum phase coherence.

cond-mat.supr-con↗

arXiv2026

Scanning tunneling spectroscopy of superconducting nitridized aluminum thin films

Nitride-based superconductors represent a family of superconducting thin film materials displaying higher quality than their corresponding bare superconductor when used in devices for applications such as cosmic radiation sensing. In recent times, Niobium-based and Titanium-based nitrides were used to improve the quality of superconducting devices in quantum technology applications. Recently, nitridized Aluminum (NitrAl) has been found to display higher critical temperatures and enhanced resilience to magnetic fields compared to those of Al, making it a new interesting candidate for superconducting quantum circuit applications. However, the microscopic properties of NitrAl remain highly unexplored. Here we use Scanning Tunneling Microscope (STM) to measure the superconducting density of states of a thin film sample of nitridized-Aluminum (NitrAl), with a room temperature resistivity between pure Al and fully insulating aluminum nitride. We show that the in-gap density of states is zero up to about $\hbarω=250~\mathrm{μeV}$ and that there is a distribution of values of the superconducting gap around $Δ_0=360~\mathrm{μeV}$, close to the BCS expectation $Δ=1.76 k_{\mathrm{B}}T_{\mathrm{c}}$. We also find varying superconducting gap values at the nanometer scale, by approximately 10\%, when probing different regions of the sample. These results suggest a gap which is larger than the one of pure Al, and is spatially more homogeneous than the superconducting gap values often found in thin films. Our work demonstrates that STM is as a powerful tool to screen materials for quantum devices through the measurement of the spatial dependence of the superconducting density of states.

cond-mat.supr-con↗

arXiv2026

Scanning Tunneling Microscopy in high vectorial magnetic fields

The Scanning Tunneling Microscope (STM) is a powerful instrument to study electronic density of states at surfaces down to atomic scale. Many interesting samples require studying variations as a function of the magnetic field, which is most often applied perpendicular to the surface. Conventional STM designs make it challenging to perform measurements when the magnetic field must be applied in other directions. Here we present a new STM setup installed on a rotatable platform. We have designed and built a new STM, which is small enough to allow for full rotation on a space with a diameter of 37 mm, well below the available space within many magnets. We show that the new rotatable STM setup preserves the performance of state-of-the-art STMs in terms of noise and accuracy. Our new approach significantly enhances control over the direction of the applied magnetic field and opens exciting new possibilities to study quantum materials.

cond-mat.supr-con↗

arXiv2026

Conductance of atomic size contacts of Ag and Au at high magnetic fields

Electronic conduction at the atomic scale can be described by Landauer's formalism. In single atom point contacts of noble metals like Au and Ag, there is just one channel open between both electrodes and the conductance is very close to the quantum of conductance $G \approx G_0=\frac{2e^2}{h}$, with the factor of two coming from spin degeneracy. The magnetoconductivity of atomic size contacts has been studied for numerous systems, unveiling local Kondo screening, magnetic order and spin-polarized currents. However, these have been mostly performed in elements with multiple open conduction channels where $G$ differs from $G_0$. The realization of a magnetically active conductor with a single open channel remains difficult to achieve. Here we present measurements of the electronic conductance of single channel Au and Ag atomic-size contacts in magnetic fields up to 20 Tesla. We observe a decrease in $G$ which goes up to about 15% in many Au contacts at 20 T. We perform calculations and find that pure Ag and Au do not present a strong field dependence of $G$, in agreement with previous results at smaller magnetic fields. We also find, however, that residual O$_2$ molecules attached close to the contact produce an an induced spin-polarized current, which leads to a decrease in $G$. We discuss the role of the magnetic response of the electrodes in the jump to contact. Our results suggest that single channel atomic size conductors with a sizeable response to a magnetic field can be built by combining noble metals and magnetically active molecular systems.

cond-mat.mes-hall↗

arXiv2026

Direct observation of vortex liquid droplets in the iron pnictide superconductor CaKAs$_4$Fe$_4$ at $0.5T$_c$

Type-II superconductors under magnetic fields are in a quantum coherent non-dissipative state as long as vortices remain pinned. Dissipation appears when vortices depin, eventually driven by thermal fluctuations. This can be associated to a melting transition between a vortex solid and a vortex liquid. This transition is almost always observed very close to T$_c$ when probed by macroscopic experiments. However, it remains unclear how the vortex solid responds to thermal fluctuations at the scale of individual vortices far from the melting transition. Here we use scanning tunneling microscopy (STM) to visualize vortices in CaKAs$_4$Fe$_4$ (T$_c \approx$ 35 K). We find vortex liquid droplets-localized regions in space where vortices strongly fluctuate due to thermal exctiation-at temperatures as low as 0.5\,T$_c$. Our results show that the onset of dissipation at the local scale occurs at temperatures considerably below T$_c$ in type-II superconductors.

cond-mat.supr-con↗

arXiv2026

Superconducting density of states and vortex lattice of LaRu$_2$P$_2$ observed by Scanning Tunneling Spectroscopy

We provide the superconducting density of states of the iron based superconductor LaRu2P2 (Tc= 4.1 K), measured using millikelvin Scanning Tunneling Microscopy. From the tunneling conductance, we extract a density of states which shows the opening of a s-wave single superconducting gap. The temperature dependence of the gap also follows BCS theory. Under magnetic fields, vortices present Caroli de Gennes Matricon states, although these are strongly broadened by defect scattering. From the vortex core size we obtain a superconducting coherence length of ξ = 50 nm, compatible with the value extracted from macroscopic Hc2 measurements. We discuss the comparison between s-wave LaRu2P2 and pnictide unconventional multiple gap and strongly correlated Fe based superconductors.

cond-mat.supr-con↗

arXiv2025

Electronic band structure from quasiparticle interference and Landau quantization in WTe$_2$

WTe$_2$ stands out as a semimetal presenting Fermi level quantum oscillations in most measured quantities under magnetic fields. However, the electronic band structure above and below the Fermi level has not been explored completely. Here we study the electronic band structure of WTe$_2$ by quasiparticle interference with Scanning Tunneling Microscopy (STM) and observe, with the support of Density Functional Theory (DFT), the electron and hole bands around the Fermi level. We also report on the observation of Landau quantization in atomically resolved measurements and discuss the possible connection with band structure calculations.

cond-mat.mes-hall↗

arXiv2025

Gapless superconductivity from extremely dilute magnetic disorder in 2H-NbSe2-xSx

Most superconducting materials exhibit a vanishing density of states at the Fermi level and Anderson's theorem posits that the superconducting gap is robust against nonmagnetic disorder. Although dilute magnetic impurities lead to localized in-gap states, these states typically have no bearing on the material's bulk superconducting properties. However, numerous experiments reveal a finite density of states at the Fermi level in systems with an apparently negligible number of magnetic impurities. Here, using scanning tunneling microscopy and self-consistent Bogoliubov-de Gennes calculations, we find that gapless superconductivity emerges in 2H-NbSe2-xSx at remarkably low magnetic impurity concentrations. Furthermore, our density functional theory calculations and in-gap quasiparticle interference measurements demonstrate that the Se-S substitution significantly modifies the band structure. This modification favours nesting and dictates the in-gap scattering for x>0, in stark contrast to the dominant charge density wave interactions in pure 2H-NbSe2. Our findings reveal an unusual superconducting response to disorder and highlight the importance of incorporating material-specific band structures in the understanding of a superconductor's response to even very low concentrations of magnetic impurities.

cond-mat.supr-con↗

arXiv2025

Superconducting density of states of PtPb4

PtPb$_4$ is a type II superconductor with a bulk critical temperature $T_{c}\approx 3 $K and an upper critical field of $H_{c2}=0.36 $T. PtPb$_4$ is related to non-superconducting PtSn$_4$, which presents nodal arc states at the surface. Here we measure the superconducting density of states of PtPb$_4$ using millikelvin Scanning Tunneling Microscopy (STM). We observe a fully opened superconducting gap of $Δ=0.48$\ meV similar to expectations from Bardeen Cooper and Schrieffer (BCS) theory ($Δ_0=1.76k_BT_{c}=0.49 $meV). Measurements under magnetic fields applied perpendicular to the surface show a spatially inhomogeneous gap structure, presenting superconducting signatures at fields as high as 1.5 T, significantly above $H_{c2}=0.36 $T. On some locations we find that the superconducting density of states does not vanish above $T_{c}$. We can find signatures of a superconducting gap up to 5K. We discuss possible reasons for the observation of superconducting properties above $T_{c}$ and $H_{c2}$, emphasizing the role played by structural defects.

cond-mat.supr-con↗

arXiv2025

The feedback driven atomic scale Josephson microscope

The ultimate spatial limit to establish a Josephson coupling between two superconducting electrodes is an atomic-scale junction. The Josephson effect in such ultrasmall junctions has been used to unveil new switching dynamics, study coupling close to superconducting bound states or reveal non-reciprocal effects. However, the Josephson coupling is weak and the sensitivity to temperature reduces the Cooper pair current magnitude. Here we show that a feedback element induces a time-dependent bistable regime which consists of spontaneous periodic oscillations between two different Cooper pair tunneling states (corresponding to the DC and AC Josephson regimes respectively). The amplitude of the time-averaged current within the bistable regime is almost independent of temperature. By tracing the periodic oscillations in the new bistable regime as a function of the position in a Scanning Tunneling Microscope, we obtain atomic scale maps of the critical current in 2H-NbSe$_2$ and find spatial modulations due to a pair density wave. Our results fundamentally improve our understanding of atomic size Josephson junctions including a feedback element in the circuit and provide a promising new route to study superconducting materials through atomic scale maps of the Josephson coupling.

cond-mat.supr-con↗

arXiv2024

Diluted Yu-Shiba-Rusinov arrays on the $β$-Bi$_2$Pd anisotropic superconductor

Magnetic adatoms on s-wave superconductors induce bound states inside the superconducting gap, called Yu-Shiba-Rusinov states (YSR). The anisotropy of the Fermi surface determines the spatial extension of bound states in a quasi-two-dimensional superconductor. This is especially important in the diluted impurity limit since the orbital overlap determines the coupling of YSR states of neighboring atoms and the formation of the collective YSR system. Here, we build diluted arrays of Mn atoms with different dimensionalities on the surface of $β$-Bi$_2$Pd, and we measure the evolution of their YSR spectra with the structure. We detect the coupling as a split of YSR peaks in subgap spectra and find that the split size increases with the number of atoms. The orientation of the structures along different directions of the \bipd substrate modulates the split and particle-hole asymmetry of the YSR states due to the anisotropic character of the Fermi surface, captured by the Green function model. With the aid of the model, we found multiple YSR excitations in an extended 2D array of 25 Mn atoms, and we identified that their spatial distribution reflects a chiral LDOS.

cond-mat.supr-con↗

arXiv2024

Anti-hyperuniform diluted vortex matter induced by correlated disorder

Disordered hyperuniform materials are very promising for applications but the successful route for synthesizing them requires to understand the interactions induced by the host media that can switch off this hidden order. With this aim we study the model system of vortices in the $β$-Bi$_2$Pd superconductor where correlated defects seem to play a determinant role for the nucleation of a gel vortex phase at low densities. We directly image vortices in extended fields-of-view and show that the disordered vortex structure in this material is anti-hyperuniform, contrasting with the case of vortex structures nucleated in samples with point-like disorder. Based on numerical simulations, we show that this anti-hyperuniform structure arises both, from the interaction of a diluted vortex structure with a fourfold-symmetric correlated disorder quite likely generated when cleaving the samples and from the out of equilibrium nature of the quenched configuration.

cond-mat.supr-con↗

arXiv2023

Band structure, superconductivity and polytypism in AuSn$_4$

The orthorhombic compound AuSn4 is compositionally similar to the Dirac node arc semimetal PtSn$_4$. AuSn$_4$ is, contrary to PtSn$_4$, superconducting with a critical temperature of T$_c$ = 2.35 K. Recent measurements present indications for quasi two-dimensional superconducting behavior in AuSn$_4$. Here we present measurements of the superconducting density of states and the band structure of AuSn$_4$ through Scanning Tunneling Microscopy (STM) and Angular Resolved Photoemission Spectroscopy (ARPES). The superconducting gap values in different portions of the Fermi surface are spread around Δ0 = 0.4 meV, which is close to but somewhat larger than $Δ=$ 1.76kBT$_c$ expected from BCS theory. We observe superconducting features in the tunneling conductance at the surface up to temperatures about 20% larger than bulk Tc. The band structure calculated with Density Functional Theory (DFT) follows well the results of ARPES. The crystal structure presents two possible stackings of Sn layers, giving two nearly degenerate polytypes. This makes AuSn$_4$ a rather unique case with a three dimensional electronic band structure but properties ressembling those of low dimensional layered compounds.

cond-mat.supr-con↗

arXiv2022

Quantum-well states at the surface of the heavy-fermion superconductor URu$_2$Si$_2$

Electrons can form a two-dimensional electron gas at metal surfaces, where lateral confinement leads to quantum-well states. Such states have been observed for highly itinerant electrons, but it remains an open question whether quantum-well states can be formed from strongly correlated electrons. Here we study atomically flat terraces on surfaces of the heavy-fermion superconductor URu$_2$Si$_2$ using millikelvin scanning tunneling spectroscopy. We observe two-dimensional heavy fermions (2DHF) with an effective mass 17 times the free electron mass that form quantized states separated by a fraction of a meV. Superconductivity at the surface is induced by the bulk into the 2DHF. Our results provide a new route to realize quantum well states in correlated quantum materials.

cond-mat.str-el↗

arXiv2022

Superconducting density of states and bandstructure at the surface of the candidate topological superconductor Au2Pb

The electronic bandstructure of Au$_2$Pb has a Dirac cone which gaps when undergoing a structural transition into a low temperature superconducting phase. This suggests that the superconducting phase ($T_c=1.1$ K) might hold topological properties at the surface. Here we make Scanning Tunneling Microscopy experiments on the surface of superconducting Au$_2$Pb. We measure the superconducting gap and find a sizeable superconducting density of states at the Fermi level. We discuss possible origins for this finding in terms of superconductivity induced into surface states.

cond-mat.supr-con↗