arXiv subjects

Ish Dhand

Publications and source records attributed to Ish Dhand.

26 records · Page 2Linked to original sources

arXiv2018

Pulsed polarisation for robust DNP

Dynamical nuclear polarisation (DNP) is an important technique that uses polarisation transfer from electron to nuclear spins to achieve nuclear hyperpolarisation. As the electron spin of the nitrogen vacancy (NV) centres in diamond can be optically initialised nearly perfectly even at room temperature and ambient conditions, new opportunities become possible by the combination of efficient DNP with optically polarised NV centres. Among such applications are nanoscale nuclear magnetic resonance spectroscopy of liquids, hyperpolarised nanodiamonds as MRI contrast agents as well as the initialisation of nuclear spin based diamond quantum simulators. Current realisations of DNP perform the polarisation transfer by achieving energetic resonance between electrons and nuclei via carefully tuned microwave fields or by using quasi-adiabatic sweep-based schemes across resonance points. The former limits robustness against control errors while the latter limits polarisation rates, making the realisation of the applications extremely challenging. Here we introduce the concept of Hamiltonian engineering by pulse sequences and use it for the systematic design of polarisation sequences that are simultaneously robust and fast. We derive sequences theoretically and demonstrate experimentally that they are capable of efficient polarisation transfer from an optically polarised nitrogen-vacancy centre in diamond to the surrounding $^{13}$C nuclear spin bath even in the presence of control errors, making it an ideal tool for the realisation of the above NV centre based applications.

quant-ph↗

arXiv2017

Robust techniques for polarization and detection of nuclear spin ensembles

Highly sensitive nuclear spin detection is crucial in many scientific areas including nuclear magnetic resonance spectroscopy (NMR), imaging (MRI) and quantum computing. The tiny thermal nuclear spin polarization represents a major obstacle towards this goal which may be overcome by Dynamic Nuclear Spin Polarization (DNP) methods. The latter often rely on the transfer of the thermally polarized electron spins to nearby nuclear spins, which is limited by the Boltzmann distribution of the former. Here we demonstrate the polarization and read out of a nuclear spin bath consisting of $^{13}$C nuclear spins in diamond by using a single nitrogen-vacancy (NV) center. Our method utilizes microwave dressed states to transfer the NV's high ($>$~92~\%) non-equilibrium electron spin polarization induced by short laser pulses to the surrounding carbon nuclear spins, where the NV is repeatedly repolarized optically, thus providing an effectively infinite polarization reservoir. A saturation of the polarization in the nuclear "frozen core" is achieved, which is confirmed by the decay of the polarization transfer signal and shows an excellent agreement with theoretical simulations. Hereby we introduce the Polarization Read Out by Polarization Inversion (PROPI) method as a quantitative magnetization measure of the nuclear spin bath. Moreover, we show that using the integrated solid effect both for single and double quantum transitions a nuclear spin polarization can be achieved even when the static magnetic field is not aligned along the NV's crystal axis. This opens a path for the application of our DNP technique to spins in and outside of nanodiamonds, enabling their application as MRI tracers.

quant-ph↗

arXiv2016

Multi-Photon Multi-Channel Interferometry for Quantum Information Processing

This thesis reports advances in the theory of design, characterization and simulation of multi-photon multi-channel interferometers. I advance the design of interferometers through an algorithm to realize an arbitrary discrete unitary transformation on the combined spatial and internal degrees of freedom of light. This procedure effects an arbitrary $n_{s}n_{p}\times n_{s}n_{p}$ unitary matrix on the state of light in $n_{s}$ spatial and $n_{p}$ internal modes. I devise an accurate and precise procedure for characterizing any multi-port linear optical interferometer using one- and two-photon interference. Accuracy is achieved by estimating and correcting systematic errors that arise due to spatiotemporal and polarization mode mismatch. Enhanced accuracy and precision are attained by fitting experimental coincidence data to a curve simulated using measured source spectra. The efficacy of our characterization procedure is verified by numerical simulations. I develop group-theoretic methods for the analysis and simulation of linear interferometers. I devise a graph-theoretic algorithm to construct the boson realizations of the canonical SU$(n)$ basis states, which reduce the canonical subgroup chain, for arbitrary $n$. The boson realizations are employed to construct $\mathcal{D}$-functions, which are the matrix elements of arbitrary irreducible representations, of SU$(n)$ in the canonical basis. I show that immanants of principal submatrices of a unitary matrix $T$ are a sum of the diagonal $\mathcal{D}(Ω)$-functions of group element $Ω$ over $t$ determined by the choice of submatrix and over the irrep $(λ)$ determined by the immanant under consideration. The algorithm for $\mathrm{SU}(n)$ $\mathcal{D}$-function computation and the results connecting these functions with immanants open the possibility of group-theoretic analysis and simulation of linear optics.

quant-ph↗

arXiv2016

Accurate and precise characterization of linear optical interferometers

We combine single- and two-photon interference procedures for characterizing any multi-port linear optical interferometer accurately and precisely. Accuracy is achieved by estimating and correcting systematic errors that arise due to spatiotemporal and polarization mode mismatch. Enhanced accuracy and precision are attained by fitting experimental coincidence data to curve simulated using measured source spectra. We employ bootstrapping statistics to quantify the resultant degree of precision. A scattershot approach is devised to effect a reduction in the experimental time required to characterize the interferometer. The efficacy of our characterization procedure is verified by numerical simulations.

quant-ph↗

arXiv2016

D-functions and immanants of unitary matrices and submatrices

Motivated by recent results in multiphoton interferometry, we expand a result of Kostant on immanants of an arbitrary $m\times m$ unitary matrix $T\in$ su$(m)$ to the submatrices of $T$. Specifically, we show that immanants of principal submatrices of a unitary matrix $T$ are a sum $\sum_{t} D^{(λ)}_{tt}(Ω)$ of the diagonal $D$-functions of group element $Ω$, with $t$ determined {by} the choice of submatrix, and the irrep $(λ)$ determined by the immanant under consideration. We also provide evidence that this result extends to some submatrices that are not principal diagonal, and we discuss how this result can be extended to cases where $T$ carries an su$(m)$ representation that is different from the defining representation.

math-ph↗

arXiv2015

Algorithms for SU(n) boson realizations and D-functions

Boson realizations map operators and states of groups to transformations and states of bosonic systems. We devise a graph-theoretic algorithm to construct the boson realizations of the canonical SU$(n)$ basis states, which reduce the canonical subgroup chain, for arbitrary $n$. The boson realizations are employed to construct $\mathcal{D}$-functions, which are the matrix elements of arbitrary irreducible representations, of SU$(n)$ in the canonical basis. We demonstrate that our $\mathcal{D}$-function algorithm offers significant advantage over the two competing procedures, namely factorization and exponentiation.

quant-ph↗

arXiv2015

Realization of arbitrary discrete unitary transformations using spatial and internal modes of light

Any lossless transformation on $n_{s}$ spatial and $n_{p}$ internal modes of light can be described by an $n_{s}n_{p}\times n_{s}n_{p}$ unitary matrix, but there is no known procedure to effect an arbitrary $n_{s}n_{p}\times n_{s}n_{p}$ unitary matrix on light in $n_{s}$ spatial and $n_{p}$ internal modes. We devise an algorithm to realize an arbitrary discrete unitary transformation on the combined spatial and internal degrees of freedom of light. Our realization uses beamsplitters and operations on internal modes to effect arbitrary linear transformations. The number of beamsplitters required to realize a unitary transformation is reduced as compared to existing realization by a factor $n_{p}^2/2$ at the cost of increasing the number of internal optical elements by a factor of two. Our algorithm thus enables the optical implementation of higher dimensional unitary transformations.

quant-ph↗

arXiv2014

Stability of the Trotter-Suzuki decomposition

The Trotter-Suzuki decomposition is an important tool for the simulation and control of physical systems. We provide evidence for the stability of the Trotter-Suzuki decomposition. We model the error in the decomposition and determine sufficiency conditions that guarantee the stability of this decomposition under this model. We relate these sufficiency conditions to precision limitations of computing and control in both classical and quantum cases. Furthermore we show that bounded-error Trotter-Suzuki decomposition can be achieved by a suitable choice of machine precision.

math-ph↗