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Itamar Kolvin

Publications and source records attributed to Itamar Kolvin.

15 recordsLinked to original sources

Droplet coalescence in fluids obeying Darcy's law

During drop coalescence, a connecting bridge of fluid forms and rapidly expands due to surface tension. For spherical drops, these dynamics are well understood in both the viscous and inertial regimes. However, under strong confinement, fluid motion is fundamentally altered by geometric constraints, leading to dissipation on small lengthscales. We investigate the coalescence of drops confined in a Hele-Shaw cell (two parallel plates separated by a narrow gap). In this geometry, the depth-averaged flow is governed by Darcy's law while surface tension drives the interface motion. We identify two distinct temporal regimes in the evolution of the bridge radius that evolves as a power law ($R_b$). At early times, the bridge grows as $R_b \sim t^{1/2}$, which results from a confinement-dependent meniscus instability that determines the initiation of contact between droplets prior to bridge formation. At later times, the bridge growth slows substantially and follows $R_b \sim t^{1/5}$, consistent with recent theoretical predictions for Darcy-governed coalescence. We show that the transition between these regimes is controlled by several geometric lengthscales. In particular, the onset of the Darcy regime occurs when the interface radius of curvature becomes comparable to the plate spacing, such that the flow becomes fully confined. Using a boundary integral formulation, we find that both scaling laws for $R_b$ are determined by the bridge width. Together, these results identify a new universal regime of drop coalescence in a broad class of fluids obeying Darcy's law.

physics.flu-dyn

A comprehensive study of nonlinear perturbations in the dynamics of planar crack fronts

The interaction of crack fronts with asperities is central to the criteria of fracture in heterogeneous materials and for predicting fracture surface formation. It is known how dynamic crack fronts respond to small, 1st-order, perturbations. However, large and localized disturbances to crack motion induce dynamic and geometric nonlinear effects beyond the existing linear theories. Because the determination of the 3D elastic fields surrounding perturbed crack fronts is a necessary step towards any theoretical study of crack front dynamics, we develop a 2nd-order perturbation theory for the asymptotic fields of planar crack fronts. Based on previous work, we consider two models of fracture. In the so-called scalar elastic model, which is analogous to anti-plane (Mode III) fracture, the stress and displacement fields are obtained through matched asymptotic expansions. A self-consistent expansion is used to resolve the fields near tensile (Mode I) crack fronts. Both methods can be extended to higher perturbation orders. The main results of this work are the explicit 2nd-order expressions of the local dynamic energy-release-rates for perturbations of straight fronts. These general formulae recover the known energy-release-rates of curved quasi-static fronts and of straight dynamic fronts.

cond-mat.soft

Dual Role for Heterogeneity in Dynamic Fracture

We approach the problem of heterogeneous dynamic fracture by considering spatiotemporal perturbations to planar crack fronts. Front propagation is governed by local energy balance between the elastic energy per unit area available to fracture, G, and the dissipation in creating new surfaces. G is known analytically as a perturbation series in the crack front fluctuation. For dissipation that monotonically increases with the crack speed, we derive an equation of motion for crack fronts that is second-order accurate. In the linear order, heterogeneity does not change the net speed of fracture. In the second order, nonlinear interactions of the front and the heterogeneous landscape populate an intermediate-scale fluctuation spectrum. We find that, when dissipation weakly grows with velocity, nonlinearities globally amplify dissipation and reduce the crack speed. Strong velocity dependence, however, mitigates toughening effects and may facilitate fracture.

cond-mat.mtrl-sci

Active assembly and non-reciprocal dynamics of elastic membranes

Equilibrium self-assembly and conventional materials processing techniques fall far short of mimicking dynamic self-actuating processes that are commonplace throughout biology. To bridge the gap between living and synthetic matter, we study adhesive non-thermal fibers immersed in an active fluid. Autonomous chaotic flows power non-equilibrium fiber dynamics, inducing their collisions, generating connections, and weaving a membrane-shaped elastic network. This active assembly generates a hierarchy of shapes, structures, and dynamical processes spanning nanometers to centimeters. Ultimately, it generates an active membrane that exhibits global limit cycles induced by a non-reciprocal coupling between the elastic membrane deformations and the alignment axis of the polar active fluid. Our work merges self-assembly with active matter, demonstrating self-processing materials wherein hierarchical life-like structures and dynamics emerge from an initially structureless suspension.

cond-mat.soft

Traveling waves at the surface of active liquid crystals

Active liquid crystals exert nonequilibrium stresses on their surroundings through constant consumption of energy, giving rise to dynamical steady states not present in equilibrium. The paradigmatic example of an active liquid crystal is a suspension of microtubule bundles powered by kinesin motor proteins, which exhibits self-sustained spatiotemporal chaotic flows. This system has been modelled using continuum theories that couple the microtubule orientation to active flows. Recently the focus has shifted to the interfacial properties of mixtures of active liquid crystals and passive fluids. Active/passive interfaces have been shown to support propagating capillary waves in the absence of inertia and offer a promising route for relating experimental parameters to those of the continuum theory. In this paper we report the derivation of a minimal model that captures the linear dynamics of the interface between an active liquid crystal and a passive fluid. We show that the dynamics of the interface, although powered by active flows throughout the bulk, is qualitatively captured by equations that couple non-reciprocally interface height and nematic director at the interface. This minimal model reproduces the dynamical structure factor evaluated from numerical simulations and the qualitative form of the wave dispersion relation seen in experiments.

cond-mat.soft

Asymmetric fluctuations and self-folding of active interfaces

We study the structure and dynamics of the interface separating a passive fluid from a microtubule-based active fluid. Turbulent-like active flows power giant interfacial fluctuations, which exhibit pronounced asymmetry between regions of positive and negative curvature. Experiments, numerical simulations, and theoretical arguments reveal how the interface breaks up the spatial symmetry of the fundamental bend instability to generate local vortical flows that lead to asymmetric interface fluctuations. The magnitude of interface deformations increases with activity: In the high activity limit, the interface self-folds invaginating passive droplets and generating a foam-like phase, where active fluid is perforated with passive droplets. These results demonstrate how active stresses control the structure, dynamics, and break-up of soft, deformable, and reconfigurable liquid-liquid interfaces.

cond-mat.soft

Dynamics of active liquid interfaces

Controlling interfaces of phase separating fluid mixtures is key to creating diverse functional soft materials. Traditionally, this is accomplished with surface-modifying chemical agents. Using experiment and theory, we study how mechanical activity shapes soft interfaces that separate an active and a passive fluid. Chaotic flows in the active fluid give rise to giant interfacial fluctuations and non-inertial propagating active waves. At high activities, stresses disrupt interface continuity and drive droplet generation, producing an emulsion-like active state comprised of finite-sized droplets. When in contact with a solid boundary, active interfaces exhibit non-equilibrium wetting transitions, wherein the fluid climbs the wall against gravity. These results demonstrate the promise of mechanically driven interfaces for creating a new class of soft active matter.

cond-mat.soft

Topological structure and dynamics of three dimensional active nematics

Point-like motile topological defects control the universal dynamics of diverse two-dimensional active nematics ranging from shaken granular rods to cellular monolayers. A comparable understanding in higher dimensions has yet to emerge. We report the creation of three-dimensional active nematics by dispersing extensile microtubule bundles in a passive colloidal liquid crystal. Light-sheet microscopy reveals the millimeter-scale structure of active nematics with a single bundle resolution and the temporal evolution of the associated nematic director field. The dominant excitations of three-dimensional active nematics are extended charge-neutral disclination loops that undergo complex dynamics and recombination events. These studies introduce a new class of non-equilibrium systems whose turbulent-like dynamics arises from the interplay between internally generated active stresses, the chaotic flows and the topological structure of the constituent defects.

cond-mat.soft

How super-tough gels break

Fracture of highly stretched materials challenges our view of how things break. We directly visualize rupture of tough double-network (DN) gels at >50\% strain. During fracture, crack tip shapes obey a $x\sim y^{1.6}$ power-law, in contrast to the parabolic profile observed in low-strain cracks. A new length-scale $\ell$ emerges from the power-law; we show that $\ell$ scales directly with the stored elastic energy, and diverges when the crack velocity approaches the shear wave speed. Our results show that DN gels undergo brittle fracture, and provide a testing ground for large-strain fracture mechanics.

cond-mat.soft

Nonlinear focusing in dynamic crack fronts and the micro-branching transition

Cracks in brittle materials produce two types of generic surface structures: facets at low velocities and micro-branches at higher ones. Here we observe a transition from faceting to micro-branching in polyacrylamide gels that is characterized by nonlinear dynamic localization of crack fronts. To better understand this process we derive a first-principles nonlinear equation of motion for crack fronts in the context of scalar elasticity. Its solution shows that nonlinear focusing coupled to rate-dependence of dissipation governs the transition to micro-branching.

cond-mat.soft

Topological defects govern crack front motion and facet formation on broken surfaces

Patterns on broken surfaces are well-known from everyday experience, but surprisingly, how and why they form are very much open questions. Well-defined facets are commonly observed1-4 along fracture surfaces which are created by slow tensile cracks. As facets appear in amorphous materials5-7, their formation does not reflect microscopic order. Fracture mechanics, however, predict that slow crack fronts should be straight, creating mirror-like surfaces8-13. In contrast, facet-forming fronts propagate simultaneously within different planes separated by steps. It is therefore unclear why steps are stable, what determines their path and how they couple to crack front dynamics. Here we show, by integrating real-time imaging of propagating crack fronts with surface measurements, that steps are topological defects of crack fronts; crack front separation into discontinuous overlapping segments provides the condition for step stability. Steps drift at a constant angle to the local front propagation direction and the increased local dissipation due to step formation couples to the long-range deformation of the surrounding crack fronts. Slow crack front dynamics are enslaved to changes in step heights and positions. These observations show how 3D topology couples to 2D fracture dynamics to provide a fundamental picture of how patterned surfaces are generated.

cond-mat.soft

Crack front dynamics: the interplay of singular geometry and crack instabilities

When fast cracks become unstable to microscopic branching (micro-branching), fracture no longer occurs in an effective 2D medium. We follow in-plane crack front dynamics via real-time measurements in brittle gels as micro-branching unfolds and progresses. We first show that {\em spatially local} energy balance quantitatively describes crack dynamics, even when translational invariance is badly broken. Furthermore, our results explain micro-branch dynamics; why micro-branches form along spatially localized chains and how finite-time formation of cusps along the crack front leads to their death.

cond-mat.mtrl-sci

A simple nonlinear equation for structural relaxation in glasses

A wide range of glassy and disordered materials exhibit complex, non-exponential, structural relaxation (aging). We propose a simple nonlinear rate equation dδ/dt = a [1-exp (bδ)], where 'δ' is the normalized deviation of a macroscopic variable from its equilibrium value, to describe glassy relaxation. Analysis of extensive experimental data shows that this equation quantitatively captures structural relaxation, where 'a' and 'b' are both temperature-, and more importantly, history-dependent parameters. This analysis explicitly demonstrates that structural relaxation cannot be accurately described by a single non-equilibrium variable. Relaxation rates extracted from the data imply the existence of cooperative rearrangements on a super-molecular scale.

cond-mat.dis-nn

Navier-Stokes hydrodynamics of thermal collapse in a freely cooling granular gas

We employ Navier-Stokes granular hydrodynamics to investigate the long-time behavior of clustering instability in a freely cooling dilute granular gas in two dimensions. We find that, in circular containers, the homogeneous cooling state (HCS) of the gas loses its stability via a sub-critical pitchfork bifurcation. There are no time-independent solutions for the gas density in the supercritical region, and we present analytical and numerical evidence that the gas develops thermal collapse unarrested by heat diffusion. To get more insight, we switch to a simpler geometry of a narrow-sector-shaped container. Here the HCS loses its stability via a transcritical bifurcation. For some initial conditions a time-independent inhomogeneous density profile sets in, qualitatively similar to that previously found in a narrow-channel geometry. For other initial conditions, however, the dilute gas develops thermal collapse unarrested by heat diffusion. We determine the dynamic scalings of the flow close to collapse analytically and verify them in hydrodynamic simulations. The results of this work imply that, in dimension higher than one, Navier-Stokes hydrodynamics of a dilute granular gas is prone to finite-time density blowups. This provides a natural explanation to the formation of densely packed clusters of particles in a variety of initially dilute granular flows.

cond-mat.soft

Experimental Study of Energy Transfer by Inertial Waves During the Build up of Turbulence in a Rotating System

We study the transition from fluid at rest to turbulence in a rotating water cylinder. We show that the energy, injected at a given height, is transported by inertial wave packets through the fluid volume. These waves propagate at velocities consistent with those calculated from linearized theory, even when they possess large amplitudes. A clear "front" in the temporal evolution of the energy power spectrum is detected, defining a time scale for energy transport at the linear wave speed in the system. Nonlinear energy transfer between modes is governed by a different time scale that can be much longer than the linear one. These observations suggest that the energy distribution and statistics in rotating turbulent fields that are driven by intermittent energy sources may be different from those described by the inverse energy cascade in two-dimensional turbulence.

physics.flu-dyn