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Itamar Procaccia

Publications and source records attributed to Itamar Procaccia.

At least 91 records · Page 5Linked to original sources

Stochastic Approach to Plasticity and Yield in Amorphous Solids

We focus on the probability distribution function (pdf) $P(Δγ; γ)$ where $Δγ$ are the {\em measured} strain intervals between plastic events in an athermal strained amorphous solids, and $γ$ measures the accumulated strain. The tail of this distribution as $Δγ\to 0$ (in the thermodynamic limit) scales like $Δγ^η$. The exponent $η$ is related via scaling relations to the tail of the pdf of the eigenvalues of the {\em plastic modes} of the Hessian matrix $P(λ)$ which scales like $λ^θ$, $η=(θ-1)/2$. The numerical values of $η$ or $θ$ can be determined easily in the unstrained material and in the yielded state of plastic flow. Special care is called for in the determination of these exponents between these states as $γ$ increases. Determining the $γ$ dependence of the pdf $P(Δγ; γ)$ can shed important light on plasticity and yield. We conclude that the pdf's of both $Δγ$ and $λ$ are not continuous functions of $γ$. In slowly quenched amorphous solids they undergo two discontinuous transitions, first at $γ=0^+$ and then at the yield point $γ=γ_{_{\rm Y}}$ to plastic flow. In quickly quenched amorphous solids the second transition is smeared out due to the non existing stress peak before yield. The nature of these transitions and scaling relations with the system size dependence of $\langle Δγ\rangle$ are discussed.

cond-mat.soft↗

The Static Lengthscale Characterizing the Glass Transition at Lower Temperatures

The existence of a static lengthscale that grows in accordance with the dramatic slowing down observed at the glass transition is a subject of intense interest. A recent publication compared two proposals for this length scale, one based on the point-to-set correlation technique and the other on the scale where the lowest eigenvalue of the Hessian matrix becomes sensitive to disorder. The conclusion was that both approaches lead to the same lengthscale, but the former is easier to measure at higher temperatures and the latter at lower temperatures. But even after using both methods together, the range of increase in the observed lengthscales was limited by the relaxation times reachable by standard molecular dynamics techniques (i.e. about 4-5 orders of magnitude). In this paper we therefore attempt to explore the typical scale at even lower temperatures, testing for this purpose two approaches, one based on the idea of vapor deposition and the other on a swap Monte Carlo technique. We conclude that the first approach does not help in getting to lower temperatures, but the second one does so quite effectively. We can reach a typical lengthscale that grows in accordance with at least $15$ orders of magnitude increase in the relaxation time, competing with the best experimental conditions. We conclude by discussing the relationship between the observed lengthscale and various models of the relaxation time.

cond-mat.stat-mech↗

Consequences of Disorder on the Stability of Amorphous Solids

Highly acurate numerical simulations are employed to highlight the subtle but important differences in the mechanical stability of perfect crystalline solids versus amorphous solids. We stress the difference between strain values at which the shear modulus vanishes and strain values at which a plastic instability insues. The temperature dependence of the yield strain is computed for the two types of solids, showing different scaling laws: $γ_{_{Y}}\simeq γ_{_{Y}}^{0}-C_1 T^{1/3}$ for crystals versus $γ_{_{Y}}\simeq γ_{_{Y}}^{0}- C_2 T^{2/3}$ for amorphous solids.

cond-mat.dis-nn↗

Modeling Barkhausen Noise in Magnetic Glasses with Dipole-Dipole Interactions

Long-ranged dipole-dipole interactions in magnetic glasses give rise to magnetic domains having labyrinthine patterns. Barkhausen Noise is then expected to result from the movement of domain boundaries which is supposed to be modeled by the motion of elastic membranes with random pinning. We propose an atomistic model of such magnetic glasses in which we measure the Barkhausen Noise which indeed results from the movement of domain boundaries. Nevertheless the statistics of the Barkhausen Noise is found in striking disagreement with the expectations in the literature. In fact we find exponential statistics without any power law, stressing the fact that Barkhausen Noise can belong to very different universality classes. In this glassy system the essence of the phenomenon is the ability of spin-carrying particles to move and minimize the energy without any spin flip. A theory is offered in excellent agreement with the measured data without any free parameter.

cond-mat.soft↗

The yield of Amorphous Solids Under Stress Control at Low Temperatures

The yield of amorphous solids like metallic glasses under external stress was discussed asserting that it is related to the glass transition by increasing temperature, or that it can be understood using statistical theories of various sorts. Here we study the approach to stress-controlled yield and argue that neither assertions can be supported, at least at low temperatures. The yield of amorphous solids at low temperatures is a highly structured phenomenon, characterized by a specific series of mechanical instabilities, and having no similarity at all to fluidization by increased temperature, real or fictive. The series of instabilities followed by stress controlled yield at low but finite temperature protocols can be predicted by analyzing athermal quasi-static strain controlled protocols, making the latter highly relevant for the deep understanding of the mechanical properties of amorphous solids.

cond-mat.soft↗

Energy and Vorticity Spectra in Turbulent Superfluid $^4$He from $T=0$ to $T_λ$

We discuss the energy and vorticity spectra of turbulent superfluid $^4$He in all the temperature range from $T=0$ up to the phase transition "$λ$ point", $T_λ\simeq 2.17\,$K. Contrary to classical developed turbulence in which there are only two typical scales, i.e. the energy injection $L$ and the dissipation scales $η$, here the quantization of vorticity introduces two additional scales, i.e the vortex core radius $a_0$ and the mean vortex spacing $\ell$. We present these spectra for the super- and normal-fluid components in the entire range of scales from $L$ to $a_0$ including the cross-over scale $\ell$ where the hydrodynamic eddy-cascade is replaced by the cascade of Kelvin waves on individual vortices. At this scale a bottleneck accumulation of the energy was found earlier at $T=0$. We show that even very small mutual friction dramatically suppresses the bottleneck effect due to the dissipation of the Kelvin waves. Using our results for the spectra we estimate the Vinen "effective viscosity" $ν'$ in the entire temperature range and show agreement with numerous experimental observation for $ν'(T)$.

cond-mat.other↗

The Anatomy of Plastic Events in Magnetic Amorphous Solids

Plastic events in amorphous solids can be much more than just "shear transformation zones" when the positional degrees of freedom are coupled non-trivially to other degrees of freedom. Here we consider magnetic amorphous solids where mechanical and magnetic degrees of freedom interact, leading to rather complex plastic events whose nature must be disentangled. In this paper we uncover the anatomy of the various contributions to some typical plastic events. These plastic events are seen as Barkhausen Noise or other "serrated noises". Using theoretical considerations we explain the observed statistics of the various contributions to the considered plastic events. The richness of contributions and their different characteristics imply that in general the statistics of these "serrated noises" cannot be universal, but rather highly dependent on the state of the system and on its microscopic interactions.

cond-mat.soft↗

Shear Transformation Zones: State Determined or Protocol Dependent?

The concept of a Shear Transformation Zone (STZ) refers to a region in an amorphous solid that undergoes a plastic event when the material is put under an external mechanical load. An important question that had accompanied the development of the theory of plasticity in amorphous solids for many years now is whether an STZ is a {\em region} existing in the material (which can be predicted by analyzing the unloaded material), or is it an {\em event} that depends on the loading protocol (i.e., the event cannot be predicted without following the protocol itself). In this Letter we present strong evidence that the latter is the case. Infinitesimal changes of protocol result in macroscopically big jumps in the positions of plastic events, meaning that these can never be predicted from considering the unloaded material.

cond-mat.soft↗

Elasticity and Plasticity in Stiff and Flexible Oligomeric Glasses

In this paper we focus on the mechanical properties of oligomeric glasses (waxes), employing a microscopic model that provides, via numerical simulations, information about the shear modulus of such materials, the failure mechanism via plastic instabilities and about the geometric responses of the oligomers themselves to a mechanical load. We present a microscopic theory that explains the numerically observed phenomena, including an exact theory of the shear modulus and of the plastic instabilities, both local and system spanning. In addition we present a model to explain the geometric changes in the oligomeric chains under increasing strains.

cond-mat.soft↗

The Glass Transition in Fluids with Magnetic Interactions

We study the glass transition in fluids where particles are endowed with spins, such that magnetic and positional degrees of freedom are coupled. Novel results for slowing down in the spin time-correlation functions are described, and the effects of magnetic fields on the glass transition are studied. Aging effects in such systems and the corresponding data collapse are presented and discussed.

cond-mat.soft↗

Mechanical Properties and Plasticity of a Model Glass Loaded Under Stress Control

Much of the progress achieved in understanding plasticity and failure in amorphous solids had been achieved using experiments and simulations in which the materials were loaded using strain control. There is paucity of results under stress control. Here we present a new method that was carefully geared to allow loading under stress control either at $T=0$ or at any other temperature, using Monte-Carlo techniques. The method is applied to a model perfect crystalline solid, to a crystalline solid contaminated with topological defects, and to a generic glass. The highest yield stress belongs to the crystal, the lowest to the crystal with a few defects, with the glass in between. Although the glass is more disordered than the crystal with a few defects, it yields stress is much higher than that of the latter. We explain this fact by considering the actual microscopic interactions that are typical to glass forming materials, pointing out the reasons for the higher cohesive nature of the glass. The main conclusion of this paper is that the instabilities encountered in stress-control condition are the identical saddle-node bifurcation seen in strain-control. Accordingly one can use the latter condition to infer about the former. Finally we discuss temperature effects and comment on the time needed to see a stress controlled material failure.

cond-mat.stat-mech↗

Evolution of Neutron-Initiated Micro-Big-Bang in superfluid He 3B

A nuclear capture reaction of a single neutron by ultra-cold superfluid $^3$He results in a rapid overheating followed by the expansion and subsequent cooling of the hot subregion, in a certain analogy with the Big Bang of the early Universe. It was shown in a Grenoble experiment that a significant part of the energy released during the nuclear reaction was not converted into heat even after several seconds. It was thought that the missing energy was stored in a tangle of quantized vortex lines. This explanation, however, contradicts the expected lifetime of a bulk vortex tangle, $10^{-5}-10^{-4}\,$s, which is much shorter than the observed time delay of seconds. In this Letter we propose a scenario that resolves the contradiction: the vortex tangle, created by the hot spot, emits isolated vortex loops that take with them a significant part of the tangle's energy. These loops quickly reach the container walls. The dilute ensemble of vortex loops attached to the walls can survive for a long time, while the remaining bulk vortex tangle decays quickly.

cond-mat.other↗

Statistical Physics of Pure Barkhausen Noise

We discuss a model metallic glass in which Barkhausen Noise can be studied in exquisite detail, free of thermal effects and of the rate of ramping of the magnetic field. The mechanism of the jumps in magnetic moment that cause the Barkhausen Noise can be fully understood as consecutive instabilities where an eigenvalue of the Hessian matrix hits zero, leading to a magnetization jump $Δm$ which is simultaneous with a stress and energy changes $Δσ$ and $ΔU$ respectively. Contrary to common belief we find no "movements of magnetic domain boundaries" across pinning sites, no fractal domains, no self-organized criticality and no exact scaling behaviour. We present a careful numerical analysis of the statistical properties of the phenomenon, and show that with every care taken this analysis is tricky, and easily misleading. Without a guiding theory it is almost impossible to get the right answer for the statistics of Barkhausen Noise. We therefore present an analytic theory, showing that the probability distribution function (pdf) of Barkhausen Noise is not a power law times an exponential cutoff.

cond-mat.stat-mech↗

Percolating Plastic Failure as a Mechanism for Shear Softening in Amorphous Solids

``Shear softening" refers to the observed reduction in shear modulus when the stress on an amorphous solid is increased beyond the initial linear region. Careful numerical quasi-static simulations reveal an intimate relation between plastic failure and shear softening. The attaintment of the steady-state value of the shear modulus associated with plastic flow is identified with a percolation of the regions that underwent a plastic event. We present an elementary ``two-state" model that interpolates between failed and virgin regions and provides a simple and effective characterization of the shear softening.

cond-mat.soft↗

Atomistic Simulations of Magnetic Amorphous Solids: Magnetostriction, Barkhausen noise and novel singularities

We present results of atomistic simulations of a new model of a magnetic amorphous solid subjected to external mechanical strains and magnetic fields. The model employed offers new perspectives on important effects like Barkhausen noise and magnetostriction. It is shown that the plastic response in such systems exhibit singularities characterized by unexpected exponents requiring careful theoretical reasoning. The spatial structure of the plastic events requires a new coarse grained elasto-magnetic theory which is provided here.

cond-mat.soft↗

Plasticity-Induced Magnetization in Amorphous Magnetic Solids

Amorphous magnetic solids, like metallic glasses, exhibit a novel effect: the growth of magnetic order as a function of mechanical strain under athermal conditions in the presence of a magnetic field. The magnetic moment increases in steps whenever there is a plastic event. Thus plasticity induces the magnetic ordering, acting as the effective noise driving the system towards equilibrium. We present results of atomistic simulations of this effect in a model of a magnetic amorphous solid subjected to pure shear and a magnetic field. To elucidate the dependence on external strain and magnetic field we offer a mean-field theory that provides an adequate qualitative understanding of the observed phenomenon.

cond-mat.soft↗

On the Effect of Micro-alloying on the Mechanical Properties of Metallic Glasses

"Micro-alloying", referring to the addition of small concentration of a foreign metal to a given metallic glass, was used extensively in recent years to attempt to improve the mechanical properties of the latter. The results are haphazard and nonsystematic. In this paper we provide a microscopic theory of the effect of micro-alloying, exposing the delicate consequences of this procedure and the large parameter space which needs to be controlled. In particular we consider two very similar models which exhibit opposite trends for the change of the shear modulus, and explain the origins of the difference as displayed in the different microscopic structure and properties.

cond-mat.mtrl-sci↗

Analytic solution of the dynamics of quantum vortex reconnection

Experimental and simulational studies of the dynamics of vortex reconnections in quantum fluids showedthat the distance $d$ between the reconnecting vortices is close to a universal time dependence $d=D[κ|t_0-t|]^α$ with $α$ fluctuating around 1/2 and $κ=h/m$ is the quantum of circulation. Dimensional analysis, based on the assumption that the quantum of circulation $κ=h/m$ is the only relevant parameter in the problem, predicts $α=1/2$. The theoretical calculation of the dimensionless coefficient $D$ in this formula remained an open problem. In this Letter we present an analytic calculation of $D$ in terms of the given geometry of the reconnecting vortices. We start from the numerically observed generic geometry on the way to vortex reconnection and demonstrate that the dynamics is well described by a self-similar analytic solution which provides the wanted information.

cond-mat.other↗