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Ivan Curlik

Publications and source records attributed to Ivan Curlik.

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II. Exploring the role of the Crystal Electric Field in the vicinity of a Quantum Critical Point

Very low temperature thermodynamic properties of the Yb$M_{5-x}X_x$ (with $M$= Ni, Cu, and $X$= Cd, Mg, Au, Zn, Ag) cubic compounds are analyzed covering a broad range of behavior between magnetic and Fermi-liquid ground states GS using the {\it chemical doping}: $\zeta$ as control parameter. This allows to gain insight into the evolution of the GS behavior including a quantum critical point QCP. Doniach-Lavagna phase diagram limitations are improved by taking into account crystal electric field CEF splittings. Three regions are recognized as a function of $\zeta$: i) a magnetic one with long range magnetic order and $T_{ord}\propto T_N \approx 1$\,K, that weakens the interactions between $0.8\,K \geq T_m\geq 0.4$\,K, exhibiting very low Kondo temperature $T_K^{GS}$ in respective doublets GS. Then, for $T_Q\leq 0.4$\,K, quantum fluctuations start to dominate the scenario with the specific heat $C_{4f}/T(T\geq T_Q)$ showing $T$ power law dependencies, and a very heavy-fermion {\it plateau} below $T_Q$. ii) beyond the QCP the typical Non-Fermi-Liquid logarithmic $T$ dependence: $C_{4f}/T \propto \ln(T/T_0)$, with traces of magnetic order. At the non-magnetic limit: iii) the alloys behave as valence-fluctuation systems with growing $T_K$ that overcomes the CEF splitting. With this experimental information, a realistic phase diagram can be drawn around the QCP where the scenario is dominated by low lying quantum fluctuations, without $C_{4f}/T|_{Lim T\to 0}$ divergences but a clear drop entering into the non-magnetic phase.

cond-mat.str-el

Quantum Fluctuations in Magnetically Frustrated Gd2GaSbO7 and Gd2InSbO7 Pyrochlores

Gd2GaSbO7 and Gd2InSbO7 pyrochlore compounds exhibit quantum fluctuations in a spin ice-like state. These compounds have not been adequately studied based on the concept of magnetic frustration. Here, we have synthesised and characterised Gd2GaSbO7 and Gd2InSbO7 to investigate their ground-state magnetic properties. We confirmed the cubic pyrochlore structure via X-ray powder diffraction. Magnetic and heat capacity measurements show an absence of magnetic order down to 400 mK. Interestingly, the low-temperature magnetic heat capacity of Gd2GaSbO7 and Gd2InSbO7 exhibits a broad maximum around T_{\text{max}} = 0.9 K and T_{\text{max}} = 1 K, respectively. The low-temperature Cmag data fit with the power-law C_{\text{mag}} \approx T^{\frac{d}{n}} with dependencies of T^{1.71} for Gd2GaSbO7 and T^{1.49} for Gd2InSbO7, suggesting spin fluctuations caused by the disorder of magnetic moments at low temperatures. Both compounds retain residual entropy akin to water ice, resembling the spin ice state. Additionally, we analysed the ratio between nearest-neighbour exchange and dipolar interaction for all reported Gd-based pyrochlores, finding that Gd2InSbO7 has the lowest and weakest exchange interaction among them. This indicates that chemical pressure affects exchange interaction due to the different pathways of mediators between magnetic ions. This study reveals robust quantum fluctuations in the ground state in GGSO and GISO, similar to quantum spin ice compounds such as Pr2Zr2O7, Pr2Sn2O7, and Yb2GaSbO7. Other Gd-pyrochlore compounds exhibit long-range magnetic order, which is in stark contrast to this.

cond-mat.str-el

The magnetic field induced ferromagnetism in EuPd$_2$Sn$_4$ novel compound

We report on crystal structure, magnetic and thermal physical properties of EuPd$_2$Sn$_4$ stannide. From the magnetic susceptibility measurements a divalent state of Eu rare earth element was determined together with an antiferromagnetic (AFM) order at 11 K. By applying magnetic field, the magnetic behavior variation reveals a complex magnetic structure. Above a critical field Bc a ferromagnetic (FM)-like character starts to prevail. AFM and FM regimes are separated by a metamagnetic region. Heat capacity measurements confirm this behavior.

cond-mat.str-el

Competing magnetic interactions in the orthorhombic GdNiAl3

Magnetization and heat capacity measurements of ternary rare earth intermetallic compound GdNiAl3 demonstrate para to ferromagnetic transition at Tc=165.5K. In addition multiple short range magnetic transitions observed below Tc are suggestive of competing interactions in this compound. As a result of this a weak Griffiths phase type behaviour is observed in the paramagnetic region. This complex behaviour is rather supported by the random orientation of Ni centered tricapped trigonal prisms with additional Al atoms in the structure. Heat capacity and resistivity data display an interesting peak at 72 K, which is highly unaffected by magnetic fields up to 90KOe.

cond-mat.str-el