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Ivan Iorsh

Publications and source records attributed to Ivan Iorsh.

At least 19 recordsLinked to original sources

Boundary Kerr Signatures of the Interband-Coherence Hall Effect

We identify a Hall response carried by optically induced interband coherence rather than by a non-equilibrium band population. In a weakly doped zinc-blende semiconductor, a longitudinal dc field drives a transverse flux of the conduction--valence coherence created by near-gap light. Angular averaging eliminates the homogeneous coherence density, while a lateral boundary converts the transverse flux into an antisymmetric, edge-localized, helicity-odd polarization. The resulting Kerr signal requires neither spin-orbit coupling nor a spin, valley, or orbital accumulation within an individual band. Within the eight-band Kane model, we derive the boundary kinetic equation and obtain a complex propagation length controlled by optical detuning and interband dephasing. The edge profile is monotonic at optical resonance and develops damped spatial oscillations away from it. The response is enhanced by electron--hole asymmetry and by strong interband mixing, making narrow-gap semiconductors especially favorable to observe the effect. These results establish dc-driven Kerr microscopy as a direct probe of an interband-coherence Hall effect and of multiband quantum kinetics in real space.

cond-mat.dis-nn

Long range spatial correlations in the periodically driven transverse field Ising model

We consider a periodically driven transverse field Ising model and study the long-time behavior of the correlations between the excitations in the spin chain. We show that the longest correlation length is defined by the interference between the topological defects induced by the analog of the Kibble-Zurek mechanism and those induced by the Floquet resonance. We show that although the correlations always have a finite correlation length since the system is integrable, the correlation length can be made arbitrarily large by tuning the drive period.

cond-mat.mes-hall

Quantum Optical Signatures of Band Topology in Solid-State High Harmonics

We develop a general theory of high-harmonic generation (HHG) in solid-state systems, based on a weak-correlation expansion of photonic and matter degrees of freedom. Unlike standard HHG theories, which treat light-matter dynamics through the Schrodinger equation, our approach employs density-matrix evolution, naturally capturing the mixed-state character of both the field and the matter - a critical aspect for describing complex solid-state band structures. We show explicitly that the properties of the emitted fields are governed by the quantum statistics and quantum geometry of the underlying solid. Taking the Su-Schrieffer-Heeger (SSH) model in a one-sided optical cavity as a paradigmatic example and considering the dual regime, we demonstrate that in the topological phase a system exhibits a stronger HHG response and stronger quantum-light signatures than in the trivial phase. Furthermore, we show that cavity-matter interaction gives rise to squeezed high-harmonic quantum light, whose properties are directly imprinted by the current-current fluctuations in the material system. Crucially, the observed squeezing does not rely on a separate quartic Kerr mechanism. In the mesoscopic regime, the genuine quantum Kerr term is higher order in light-matter coupling strength and negligible, while the relevant non-classical effect is governed by current-current fluctuations encoded in the complex susceptibility of the material. This work establishes a direct link between band topology and photon statistics, opening new avenues for topology-sensitive quantum light generation and photon statistics based spectroscopy of solid-state systems.

cond-mat.mes-hall

Polarization Engineering of Second-Harmonic Generation in 3R-MoS$_2$ Waveguides

Chip-scale nonlinear optics enables strong light-matter interactions within compact devices, serving as a fundamental platform for multifunctional integrated photonics from classical optical signal processing to quantum information technologies. Transition metal dichalcogenide (TMDC) waveguides have recently emerged as a highly promising platform owing to their giant material nonlinearity and extended interaction lengths. To date, however, research has predominantly focused on conversion efficiency, leaving the mechanisms governing the polarization state of nonlinear signal largely unexplored. Here, we establish a comprehensive framework for engineering the polarization of second-harmonic generation (SHG) in 3R-MoS$_2$ waveguides. By synergizing polarization-resolved measurements with theoretical modeling, we reveal that the SHG polarization is determined by guided-mode interactions constrained by waveguide geometry and crystal symmetry, and further reshaped during propagation. We demonstrate that thickness-dependent guided-mode confinement and in-plane crystal symmetry provide robust, static control over SHG polarization, while propagation length offers a dynamic tuning knob for continuously tailoring the nonlinear output. Our findings provide a deterministic approach for on-chip polarization engineering, opening opportunities for reconfigurable nonlinear light sources and quantum photonic circuits.

physics.optics

Order-disorder duality of high entropy alloys extends non-linear optics

Order versus disorder in the structure of materials plays a key role in the theoretical prediction of their properties. However, this structural description appears to be ineffective for new families of materials such as high entropy alloys (HEAs), which combine crystallographic order with chemical disorder. Here, we demonstrate for five-element HEAs as pure solid solutions that the chemical disorder of the elements decorating their cubic structure underlies the generation of second optical harmonics, overcoming the theoretical limit imposed on centrosymmetric crystals. Moreover, we discover that this disorder, inherent to HEAs, sets a threshold for non-linear light emission from the 4th to the 26th order. As a consequence of the 0.5 eV broadening of the energy levels of the five elements of the HEA, the emission spectrum covers broad visible (400-650 nm) and infrared (800-1600 nm) ranges. In addition to the challenge of theoretically predicting non-linear effects in unconventional materials, the duality of structural order and chemical disorder in HEAs offers the opportunity to design sustainable alternatives to urgently needed optical materials.

cond-mat.mtrl-sci

Non-Hermitian trapping of Dirac exciton-polariton condensates in a perovskite metasurface

Massless Dirac particles avoid trapping due to their exceptional tunneling properties manifested in the so-called Klein paradox. This conclusion stems from the conservative treatment, but so far, it has not been extended to a non-Hermitian framework. Recently, driven-dissipative bosonic condensation of Dirac exciton-polaritons was demonstrated in metasurface waveguides. Here, we report an experimental observation of spatial binding and energy quantization of Dirac exciton-polaritons in a halide perovskite metasurface. A combination of spatially profiled nonresonant optical excitation and exciton-polariton interaction forms an effective non-Hermitian complex potential responsible for the observed effect. In the case of tightly focused pump spots spanning from 9 to 17~$μ$m, several bound states simultaneously achieve macroscopic occupation, constituting a multi-mode bosonic condensation of exciton-polaritons. Our theoretical analysis based on the driven-dissipative extension of the Dirac equation reveals that the non-Hermitian character of the effective trap allows for confinement even in the case of the gapless Dirac-like photonic dispersion, both above and below the energy of the dispersion crossing.

cond-mat.mes-hall

Intrinsically chiral exciton polaritons in an atomically-thin semiconductor

Photonic bound states in the continuum (BICs) have emerged as a versatile tool for enhancing light-matter interactions by strongly confining light fields. Chiral BICs are photonic resonances with a high degree of circular polarisation, which hold great promise for spin-selective applications in quantum optics and nanophotonics. Here, we demonstrate a novel application of a chiral BIC for inducing strong coupling between the circularly polarised photons and spin-polarised (valley) excitons (bound electron-hole pairs) in atomically-thin transition metal dichalcogenide crystals (TMDCs). By placing monolayer WS$_2$ onto the BIC-hosting metasurface, we observe the formation of intrinsically chiral, valley-selective exciton polaritons, evidenced by circularly polarised photoluminescence (PL) at two distinct energy levels. The PL intensity and degree of circular polarisation of polaritons exceed those of uncoupled excitons in our structure by an order of magnitude. Our microscopic model shows that this enhancement is due to folding of the Brillouin zone creating a direct emission path for high-momenta polaritonic states far outside the light cone, thereby providing a shortcut to thermalisation (energy relaxation) and suppressing depolarisation. Moreover, while the polarisation of the upper polariton is determined by the valley excitons, the lower polariton behaves like an intrinsic chiral emitter with its polarisation fixed by the BIC. Therefore, the spin alignment of the upper and lower polaritons ($\uparrow\downarrow$ and $\uparrow \uparrow$) can be controlled by $σ^+$ and $σ^-$ polarised optical excitation, respectively. Our work introduces a new type of chiral light-matter quasi-particles in atomically-thin semiconductors and provides an insight into their energy relaxation dynamics.

cond-mat.mes-hall

Optical spin precession

Period-averaged electromagnetic spin angular momentum is a well-established quantity for monochromatic fields, governing phenomena such as light-matter interactions with chiral particles and spin-orbit coupling effects. In contrast, the spin angular momentum of non-monochromatic fields remains unexplored. Here, we extend the concept of optical spin to the domain of non-monochromatic electromagnetic fields. Through this formulation, we uncover the precessional dynamics of electromagnetic spin in specific polychromatic configurations, including the superposition of circularly and linearly polarized plane waves propagating orthogonally at different frequencies, as well as fields generated by a precessing magnetic dipole. We discover that the dynamics of the electromagnetic spin in these cases obeys a Landau-Lifshitz-like equation establishing a profound parallel between dynamics of magnetization and photonic spin.

physics.optics

Chiral cavity-induced quantum phase transitions in a quantum ring

We consider a quantum ring placed in a gyrotropic cavity characterized by the energy splitting between the left and right circularly polarized modes. We show that despite the absence of constant magnetic field penetrating through the ring, in the regime of the ultrastrong light matter coupling, the total current in the ground state changes discontinuously with the light matter coupling in the direct analogy with the Aharonov-Bohm ring. We consider the driven-dissipative of the system and show that the discontinuous change of the total angular momentum can be directly probed via the spectral and statical properties of the radiation emitted by the system under weak coherent drive.

cond-mat.mes-hall

Disorder-assisted Spin-Filtering at Metal/Ferromagnet Interfaces: An Alternative Route to Anisotropic Magnetoresistance

We introduce a minimal interface-scattering mechanism that produces a sizable anisotropic magnetoresistance (AMR) in metal/ferromagnet bilayers (e.g., Pt/YIG) without invoking bulk spin or orbital Hall currents. In a $δ$-layer model with interfacial exchange and Rashba spin-orbit coupling, charge transfer at a high-quality interface creates a spin-selective phase condition (interfacial spin filtering) that suppresses backscattering for one spin projection while enhancing momentum relaxation for the other. The resulting resistance anisotropy peaks at an optimal metal thickness of a few nanometers, quantitatively reproducing the thickness and angular dependences typically attributed to spin Hall magnetoresistance (SMR), as well as its characteristic magnitude. Remarkably, the maximal AMR scales linearly with the smaller of the two coupling strengths - exchange or spin-orbit, highlighting a mechanism fundamentally distinct from SMR. Our scattering formulation maps onto Boltzmann boundary conditions and predicts other clear discriminants from SMR, including strong sensitivity to interfacial charge transfer and disorder.

cond-mat.mes-hall

Electron pairing by dispersive phonons in altermagnets: re-entrant superconductivity and continuous transition to finite momentum superconducting state

We consider an altermagnet subject to the electron attractive potential mediated by the dispersive phonons. While altermagnetism suppresses superconductivity, scattering of electrons on the Fermi surface by thermal phonons suppresses altermagnetism. We show that this leads to the re-entrant superconductivity over temperature and to the stabilization of the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) finite momentum superconducting state at low temperatures. The effect is mediated by the retardation effects and no d-wave pairing interaction is required.

cond-mat.supr-con

Linear spectroscopy of collective modes and the gap structure in two-dimensional superconductors

We consider optical response in multi-band, multi-layer two-dimensional superconductors. Within a simple model, we show that linear response to AC gating can detect collective modes of the condensate, such as Leggett and clapping modes. We show how trigonal warping of the superconducting order parameter can help facilitate detection of clapping modes. Taking rhombohedral trilayer graphene as an example, we consider several possible pairing mechanisms and show that all-electronic mechanisms may produce in-gap clapping modes. These modes, if present, should be detectable in the absorption of microwaves applied via the gate electrodes, which are necessary to enable superconductivity in this and many other settings; their detection would constitute strong evidence for unconventional pairing. Last, we show that absorption at frequencies above the superconducting gap $2 |Δ|$ also contains a wealth of information about the gap structure. Our results suggest that linear spectroscopy can be a powerful tool for the characterization of unconventional two-dimensional superconductors.

cond-mat.supr-con

Polaron effect in waveguide quantum optomechanics

We investigate the impact of the quantized mechanical motion of optically trapped atoms, arranged in proximity to a one-dimensional waveguide, on the propagation of polariton modes. Our study identifies a regime of resonant phonon-assisted mixing between lower and upper polaritons, resulting in a pronounced polaron effect. This effect is characterized by the formation of new band gaps and the appearance of weakly dispersive states within the original polariton band gap. The polaron spectrum, which can be directly probed via resonant elastic scattering, provides novel opportunities for quantum optical applications. These findings open avenues for enhanced control in state-of-the-art waveguide quantum electrodynamics experiments with cold atoms.

cond-mat.quant-gas

Exciton-polariton stimulated scattering in hybrid halide perovskites

Halide perovskites, such as methylammonium lead bromide (MAPbBr$_3$), host tightly bound three-dimensional excitons which are robust at room temperature. Excellent optical properties of MAPbBr$_3$ allow for designing of optical single-mode waveguides and cavities in the frequency range close to the excitonic transitions. Taken together, this turns MAPbBr$_3$ into an excellent platform for probing exciton-polariton nonlinear phenomena at room temperature. Here we investigate ultrafast non-equilibrium dynamics of polaritons under pulsed fs non-resonant excitation. We demonstrate the presence of the stimulated acoustic phonon-assisted scattering regime above threshold pump fluence, characterized by the explosive growth of emission intensity, a redshift of the emission spectral maximum, spectral narrowing, and sub-picosecond emission dynamics. Our theoretical findings are well confirmed by the results of experimental measurements.

cond-mat.mtrl-sci

Anomalous Reflection From Hyperbolic Media

Despite the apparent simplicity, the problem of refraction of electromagnetic waves at the planar interface between two media has an incredibly rich spectrum of unusual phenomena. An example is the paradox that occurs when an electromagnetic wave is incident on the interface between a hyperbolic medium and an isotropic dielectric. At certain orientations of the optical axis of the hyperbolic medium relative to the interface, the reflected and transmitted waves are completely absent. In this paper, we formulate the aforementioned paradox and present its resolution by introduction of infinitesimal losses in a hyperbolic medium. We show that the reflected wave exists, but became extremely decaying as the loss parameter tends to zero. As a consequence, all the energy scattered into the reflected channel is absorbed at the interface. We support our reasoning with analytical calculations, numerical simulations, and an experiment with self-complementary metasurfaces in the microwave region. In addition to the great fundamental interest, this paradox resolution discovers a plethora of applications for the reflectors, refractors, absorbers, lenses, antennas, camouflage and holography applications.

physics.optics

Cavity optomechanics in ultrastrong light matter coupling regime: Self-alignment and collective rotation mediated by Casimir torque

We theoretically consider an ensemble of quantum dimers placed inside an optical cavity. We predict two effects: first, an exchange of angular momentum between the dimers mediated by the emission and re-absorption of the cavity photons leads to the alignment of dimers. Furthermore, the optical angular momentum of the vacuum state of the chiral cavity is transferred to the ensemble of dimers which leads to the synchronous rotation of the dimers at certain levels of light-matter coupling strength.

quant-ph

Non-perturbative effects of deep-strong light-matter interaction in a mesoscopic cavity-QED system

We consider a system comprising two groups of quantum dimers placed in a common electromagnetic cavity, and controlled by selectively applying a static external potential to one of the groups. We show that in the regime of deep strong coupling to vacuum electromagnetic fluctuations, the emergent photon-assisted interaction between the dimers leads to a strongly non-linear quantized cross-polarization response of the first, unbiased group of dimers to the potential applied to the second group. The total polarization shows a series of almost ideal steps whose number and position depends on the parity of the numbers of dimers in the groups. This non-perturbative effect is a distinctive feature of mesoscopic systems comprising finite number of dimers and disappears in the thermodynamic limit which is commonly used in the desciption of the generalized Dicke models.

cond-mat.mes-hall

Skyrmion dynamics in moiré magnets

We consider a twisted magnetic bilayer subject to the perpendicular electric field. The interplay of induced Dzyaloshinskii - Moriya interaction and spatially varying moiré exchange potential results in complex non-collinear magnetic phases in these structures. We numerically demonstrate the coexistence of intralayer skyrmions and bound interlayer skyrmion pairs and show that they are characterized by distinct dynamics under the action of external in-plane electric field. Specifically we demonstrate the railing behaviour of skyrmions along the domain walls which could find applications in spintronic devices based on van der Waals magnets.

cond-mat.mes-hall