arXiv subjects

Ivan Jakovac

Publications and source records attributed to Ivan Jakovac.

4 recordsLinked to original sources

arXiv2026

Piezomagnetism in a model cubic noncollinear altermagnet

Altermagnets constitute a distinct class of magnetic materials that combine compensated magnetic order with spin-polarized electronic bands, hence carrying characteristics of both antiferromagnets and ferromagnets. Piezomagnetism - the linear relationship between lattice strain and a net magnetic moment - has emerged as smoking-gun evidence of altermagnetism that distinguishes it from antiferromagnetism. Here, we uncover a large piezomagnetic response in MnTe2, a cubic altermagnet with a noncollinear spin arrangement and weak spin-orbit coupling. We combine dilatometry with nuclear magnetic resonance, a bulk local probe, to observe signatures of both direct and inverse piezomagnetism consistent with symmetry considerations and first-principles calculations. The dilatometry measurements reveal a shear deformation proportional to an applied magnetic field, while magnetic resonance detects a ferromagnetic moment induced by shear strain. The respective results for the piezomagnetic coupling strength are in good agreement, and they are captured by first-principles results. These findings for simple binary MnTe2 position this material as a model altermagnet, demonstrate the utility of nuclear magnetic resonance in investigations of piezomagnetism, and open new avenues for multimodal strain and magnetic-field control in spintronic and memory applications.

cond-mat.mtrl-sci↗

arXiv2024

Properties of an organic model $S=1$ Haldane chain system

We present the properties of a new organic $S=1$ antiferromagnetic chain system $m$-NO$_2$PhBNO (abbreviated BoNO). In this biradical system two unpaired electrons from aminoxyl groups are strongly ferromagnetically coupled ($|J_\text{FM}| /k_B \gtrsim 500$ K) which leads to the formation of an effective $S=1$ state for each molecule. The chains of BoNO biradicals propagate along the crystallographic $a$ axis. Temperature dependence of the $g$ factor and electron paramagnetic resonance (EPR) linewidth are consistent with a low-dimensional system with antiferromagnetic interactions. The EPR data further suggest that BoNO is the first known Haldane system with an almost isotropic $g$ factor ($2.0023 \pm 2 \unicode{x2030}$). The magnetization measurements in magnetic fields up to $40$ T and low-field susceptibility, together with $^1$H nuclear magnetic resonance (NMR) spectra, reveal a dominant intrachain antiferromagnetic exchange coupling of $J_\text{1D}/k_B = (11.3\pm0.1)$ K, and attainable critical magnetic fields of $μ_0 H_\text{c1} \approx 2$ T and $μ_0 H_\text{c2} \approx 33$ T. These measurements therefore suggest that BoNO is a unique Haldane system with extremely small magnetic anisotropy. Present results are crucial for a future in-depth NMR study of the low-temperature Tomonaga-Luttinger liquid (TLL) and magnetic field-induced phases, which can be performed in the entire phase space.

cond-mat.str-el↗

arXiv2023

Uniaxial stress study of spin and charge stripes in La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ by $^{139}$La NMR and $^{63}$Cu NQR

We study the response of spin and charge order in single crystals of La$_{1.875}$Ba$_{0.125}$CuO$_{4}$ to uniaxial stress, through $^{139}$La nuclear magnetic resonance (NMR) and $^{63}$Cu nuclear quadrupole resonance (NQR), respectively. In unstressed La$_{1.875}$Ba$_{0.125}$CuO$_{4}$, the low-temperature tetragonal structure onsets below $T_{\text{LTT}} = 57$K, while the charge order and the spin order transition temperatures are $T_\text{CO} = 54$K and $T_\text{SO} = 37$K, respectively. We find that uniaxial stress along the [110] lattice direction strongly suppresses $T_\text{CO}$ and $T_{\text{SO}}$, but has little effect on $T_\text{LTT}$. In other words, under stress along [110] a large splitting ($\approx 21$K) opens between $T_\text{CO}$ and $T_{\text{LTT}}$, showing that these transitions are not tightly linked. On the other hand, stress along [100] causes a slight suppression of $T_\text{LTT}$ but has essentially no effect on $T_\text{CO}$ and $T_{\text{SO}}$. Magnetic field $H$ along [110] stabilizes the spin order: the suppression of $T_\text{SO}$ under stress along [110] is slower under $H \parallel [110]$ than $H \parallel [001]$. We develop a Landau free energy model and interpret our findings as an interplay of symmetry breaking terms driven by the orientation of spins.

cond-mat.str-el↗

arXiv2020

$^{105}$Pd NMR and NQR study of the cubic heavy fermion system Ce$_3$Pd$_{20}$Si$_6$

We report $^{105}$Pd NMR and NQR measurements on a single crystal of Ce$_3$Pd$_{20}$Si$_6$, where antiferroquadrupolar and antiferromagnetic orders develop at low temperature. From the analysis of NQR and NMR spectra, we have determined the electric field gradient (EFG) tensors and the anisotropic Knight shift ($K$) components for both inequivalent Pd sites - Pd($32f$) and Pd($48h$). The observed EFG values are in excellent agreement with our state-of-the-art DFT calculations. The principal values of the quadrupolar coupling are $(20.37 \pm 0.02)$ MHz and $(5.45 \pm 0.02)$ MHz, for the Pd($32f$) and Pd($48h$) site, respectively, which is large compared to the Larmor frequency defined by the gyromagnetic constant $γ= 1.94838$ MHz/T for $^{105}$Pd. Therefore, the complete knowledge of $K$ and the EFG tensors is crucial to establish the correspondence between NMR spectra and crystallographic sites, which is needed for a complete analysis of the magnetic structure, static spin susceptibility, and the spin-lattice relaxation rate data and a better understanding of the groundstate of Ce$_3$Pd$_{20}$Si$_6$.

cond-mat.str-el↗