arXiv subjects

Ivan V. Pechenezhskiy

Publications and source records attributed to Ivan V. Pechenezhskiy.

12 recordsLinked to original sources

arXiv2026

Evidence for a low-gap component in compressively stressed niobium thin films

We investigate the microwave response of sputtered Nb films as a function of biaxial film stress. Although transport measurements show nearly identical superconducting transition temperatures ($9.0\pm 0.2$K) and residual resistance ratios across the stress series, microwave resonators fabricated from highly compressive films exhibit enhanced temperature-dependent loss and larger frequency shifts. A conventional single-phase Mattis--Bardeen description yields an effective critical temperature of $2.4\pm0.2$K, approximately a factor of four below the value obtained from transport measurements. We show that the data are instead consistent with the presence of an additional low-gap component whose contribution increases with compressive stress. These results show that conventional transport measurements can overlook stress-dependent low-energy excitations that strongly influence microwave performance.

quant-ph↗

arXiv2026

Quasiparticle-induced transitions in a fluxonium qubit

Quasiparticles are a prominent decoherence source in superconducting qubits, but their effects are notoriously difficult to isolate in fluxonium. Unlike the transmon, fluxonium is insensitive to offset charge, precluding charge-parity detection of quasiparticle tunneling. We address this challenge by measuring the excitation and de-excitation rates in a fluxonium qubit under controlled on-chip quasiparticle injection and isolating the quasiparticle-induced contribution by subtracting the background transition rates. We show that to accurately model the external magnetic flux dependence of the quasiparticle-induced transition rates, it is necessary to account for the superconducting gap asymmetry across the Josephson junctions. A comparison between theory and experiment constrains the relative quasiparticle densities in the small junction and the junction array and helps explain previously reported discrepancies between the bounds on the quasiparticle densities inferred for these two circuit elements.

quant-ph↗

arXiv2026

Low-loss Nb on Si superconducting resonators from a dual-use spintronics deposition chamber and with acid-free post-processing

Magnetic impurities are known to degrade superconductivity. For this reason, physical vapor deposition chambers that have previously been used for magnetic materials have generally been avoided for making high-quality superconducting resonator devices. In this article, we show by example that such chambers can be used for this purpose; with Nb films sputtered in a chamber that continues to be used for magnetic materials, we demonstrate compact (\SI{3}{\micro\meter} gap) coplanar waveguide resonators with low-power internal quality factors near one million. We achieve this using a resist strip bath with no post-fabrication acid treatment, which results in performance comparable to previous strip baths with acid treatments. We also find evidence that this improved resist strip bath provides a better surface chemical template for post-fabrication hydrogen fluoride processing. These results are consistent across three Si substrate preparation methods, including a \SI{700}{\celsius} anneal. These results will inform nanofabrication for other superconducting materials and the integration of magnetic materials for hybrid systems.

quant-ph↗

arXiv2024

Measurement-induced state transitions in dispersive qubit readout schemes

The dispersive-readout scheme enables quantum nondemolition measurement of superconducting qubits. An increased readout power can shorten the readout time and reduce the state discrimination error but can promote qubit transitions into higher noncomputational states. The ability to predict the onset of these measurement-induced state transitions can aid the optimization of qubit circuits and provide means for comparing the readout performance of different qubit types. Building upon the concept of dressed coherent states, we consider two straightforward metrics for determining the maximum number of photons that can be used for dispersive readout without causing state transitions. We focus on the fluxonium readout to demonstrate the independence of the metrics from any qubit-type-specific approximations. The dispersive readout of transmons and other superconducting qubits can be treated universally in the same fashion.

quant-ph↗

arXiv2024

Modeling phonon-mediated quasiparticle poisoning in superconducting qubit arrays

Correlated errors caused by ionizing radiation impacting superconducting qubit chips are problematic for quantum error correction. Such impacts generate quasiparticle (QP) excitations in the qubit electrodes, which temporarily reduce qubit coherence significantly. The many energetic phonons produced by a particle impact travel efficiently throughout the device substrate and generate quasiparticles with high probability, thus causing errors on a large fraction of the qubits in an array simultaneously. We describe a comprehensive strategy for the numerical simulation of the phonon and quasiparticle dynamics in the aftermath of an impact. We compare the simulations with experimental measurements of phonon-mediated QP poisoning and demonstrate that our modeling captures the spatial and temporal footprint of the QP poisoning for various configurations of phonon downconversion structures. We thus present a path forward for the operation of superconducting quantum processors in the presence of ionizing radiation.

quant-ph↗

arXiv2021

The superconducting quasicharge qubit

The non-dissipative non-linearity of a Josephson junction converts macroscopic superconducting circuits into artificial atoms, enabling some of the best controlled quantum bits (qubits) today. Three fundamental types of superconducting qubits are known, each reflecting a distinct behavior of quantum fluctuations in a Cooper pair condensate: single charge tunneling (charge qubit), single flux tunneling (flux qubit), and phase oscillations (phase qubit). Yet, the dual nature of charge and flux suggests that circuit atoms must come in pairs. Here we introduce the missing one, named "blochnium". It exploits a coherent insulating response of a single Josephson junction that emerges from the extension of phase fluctuations beyond the $2π$-interval. Evidence for such effect was found in an out-of-equilibrium dc-transport through junctions connected to high-impedance leads, although a full consensus is absent to date. We shunt a weak junction with an exceptionally high-value inductance -- the key technological innovation behind our experiment -- and measure the rf-excitation spectrum as a function of external magnetic flux through the resulting loop. The junction's insulating character manifests by the vanishing flux-sensitivity of the qubit transition between the ground and the first excited states, which nevertheless rapidly recovers for transitions to higher energy states. The spectrum agrees with a duality mapping of blochnium onto transmon, which replaces the external flux by the offset charge and introduces a new collective quasicharge variable in place of the superconducting phase. Our result unlocks the door to an unexplored regime of macroscopic quantum dynamics in ultrahigh-impedance circuits, which may have applications to quantum computing and quantum metrology of direct current.

cond-mat.supr-con↗

arXiv2020

Counting statistics of microwave photons in circuit QED

In superconducting circuit architectures for quantum computing, microwave resonators are often used both to isolate qubits from the electromagnetic environment and to facilitate qubit state readout. We analyze the full counting statistics of photons emitted from such driven readout resonators both in and beyond the dispersive approximation. We calculate the overlap between emitted-photon distributions for the two qubit states and explore strategies for its minimization with the purpose of increasing fidelity of intensity-sensitive readout techniques. In the dispersive approximation and at negligible qubit relaxation, both distributions are Poissonian, and the overlap between them can be easily made arbitrarily small. Nondispersive terms of the Hamiltonian generate squeezing and the Purcell decay with the latter effect giving the dominant contribution to the overlap between two distributions.

quant-ph↗

arXiv2018

Microwave-Activated Controlled-Z Gate for Fixed-Frequency Fluxonium Qubits

The superconducting fluxonium circuit is an artificial atom with a strongly anharmonic spectrum: when biased at a half flux quantum, the lowest qubit transition is an order of magnitude smaller in frequency than those to higher levels. Similar to conventional atomic systems, such a frequency separation between the computational and noncomputational subspaces allows independent optimizations of the qubit coherence and two-qubit interactions. Here we describe a controlled-Z gate for two fluxoniums connected either capacitively or inductively, with qubit transitions fixed near 500 MHz. The gate is activated by a microwave drive at a resonance involving the second excited state. We estimate intrinsic gate fidelities over 99.9% with gate times below 100 ns.

quant-ph↗

arXiv2018

Digital coherent control of a superconducting qubit

High-fidelity gate operations are essential to the realization of a fault-tolerant quantum computer. In addition, the physical resources required to implement gates must scale efficiently with system size. A longstanding goal of the superconducting qubit community is the tight integration of a superconducting quantum circuit with a proximal classical cryogenic control system. Here we implement coherent control of a superconducting transmon qubit using a Single Flux Quantum (SFQ) pulse driver cofabricated on the qubit chip. The pulse driver delivers trains of quantized flux pulses to the qubit through a weak capacitive coupling; coherent rotations of the qubit state are realized when the pulse-to-pulse timing is matched to a multiple of the qubit oscillation period. We measure the fidelity of SFQ-based gates to be ~95% using interleaved randomized benchmarking. Gate fidelities are limited by quasiparticle generation in the dissipative SFQ driver. We characterize the dissipative and dispersive contributions of the quasiparticle admittance and discuss mitigation strategies to suppress quasiparticle poisoning. These results open the door to integration of large-scale superconducting qubit arrays with SFQ control elements for low-latency feedback and stabilization.

quant-ph↗

arXiv2017

Imaging structural transitions in organometallic molecules on Ag(100) for solar thermal energy storage

The use of opto-thermal molecular energy storage at the nanoscale creates new opportunities for powering future microdevices with flexible synthetic tailorability. Practical application of these molecular materials, however, requires a deeper microscopic understanding of how their behavior is altered by the presence of different types of substrates. Here we present single-molecule resolved scanning tunneling microscopy imaging of thermally- and optically-induced structural transitions in (fulvalene)tetracarbonyldiruthenium molecules adsorbed onto a Ag(100) surface as a prototype system. Both the parent complex and the photoisomer display distinct thermally-driven phase transformations when they are in contact with a Ag(100) surface. This behavior is consistent with the loss of carbonyl ligands due to strong molecule-surface coupling. Ultraviolet radiation induces marked structural changes only in the intact parent complex, thus indicating a photoisomerization reaction. These results demonstrate how stimuli-induced structural transitions in this class of molecule depend on the nature of the underlying substrate.

cond-mat.mtrl-sci↗

arXiv2016

Phonon-Mediated Quasiparticle Poisoning of Superconducting Microwave Resonators

Nonequilibrium quasiparticles represent a significant source of decoherence in superconducting quantum circuits. Here we investigate the mechanism of quasiparticle poisoning in devices subjected to local quasiparticle injection. We find that quasiparticle poisoning is dominated by the propagation of pair-breaking phonons across the chip. We characterize the energy dependence of the timescale for quasiparticle poisoning. Finally, we observe that incorporation of extensive normal metal quasiparticle traps leads to a more than order of magnitude reduction in quasiparticle loss for a given injected quasiparticle power.

cond-mat.supr-con↗

arXiv2013

Intermolecular interactions and substrate effects for an adamantane monolayer on the Au(111) surface

We study theoretically and experimentally the infrared (IR) spectrum of an adamantane monolayer on a Au(111) surface. Using a new STM-based IR spectroscopy technique (IRSTM) we are able to measure both the nanoscale structure of an adamantane monolayer on Au(111) as well as its infrared spectrum, while DFT-based ab initio calculations allow us to interpret the microscopic vibrational dynamics revealed by our measurements. We find that the IR spectrum of an adamantane monolayer on Au(111) is substantially modified with respect to the gas-phase IR spectrum. The first modification is caused by the adamantane--adamantane interaction due to monolayer packing and it reduces the IR intensity of the 2912 cm$^{-1}$ peak (gas phase) by a factor of 3.5. The second modification originates from the adamantane--gold interaction and it increases the IR intensity of the 2938 cm$^{-1}$ peak (gas phase) by a factor of 2.6, and reduces its frequency by 276 cm$^{-1}$. We expect that the techniques described here can be used for an independent estimate of substrate effects and intermolecular interactions in other diamondoid molecules, and for other metallic substrates.

cond-mat.mes-hall↗