arXiv subjects

Ivar Martin

Publications and source records attributed to Ivar Martin.

At least 37 records · Page 2Linked to original sources

arXiv2024

Unconventional gate-induced superconductivity in transition-metal dichalcogenides

Superconductivity in few-layer semiconducting transition metal dichalcogenides (TMDs) can be induced by field-effect doping through ionic-liquid gating. While several experimental observations have been collected over the years, a fully-consistent theoretical picture is still missing. Here we develop a realistic framework that combines the predictive power of first-principles simulations with the versatility and insight of Bardeen-Cooper-Schrieffer gap equations to rationalize such experiments. The multi-valley nature of semiconducting TMDs is taken into account, together with the doping- and momentum-dependent electron-phonon and Coulomb interactions. Consistently with experiments, we find that superconductivity occurs when the electron density is large enough that the Q valleys get occupied, as a result of a large enhancement of electron-phonon interactions. Despite being phonon-driven, the superconducting state is predicted to be sensitive to Coulomb interactions, which can lead to the appearance of a relative sign difference between valleys and thus to a $s_{+-}$ character. We discuss qualitatively how such scenario may account for many of the observed physical phenomena for which no microscopic explanation has been found so far, including in particular the presence of a large subgap density of states, and the sample-dependent dome-shaped dependence of $T_c$ on accumulated electron density. Our results provide a comprehensive analysis of gate-induced superconductivity in semiconducting TMDs, and introduce an approach that will likely be valuable for other multivalley electronic systems, in which superconductivity occurs at relatively low electron density.

cond-mat.supr-con↗

arXiv2024

Tunable Anomalous Hall Effect in a Kagome Ferromagnetic Weyl Semimetal

Emerging from the intricate interplay of topology and magnetism, the giant anomalous Hall effect (AHE) is the most known topological property of the recently discovered kagome ferromagnetic Weyl semimetal Co_3Sn_2S_2 with the magnetic Co atoms arranged on a kagome lattice. Here we report that the AHE in Co_3Sn_2S_2 can be fine-tuned by an applied magnetic field orientated within ~2 degrees of the kagome plane, while beyond this regime, it stays unchanged. Particularly, it can vanish in magnetic fields parallel to the kagome plane and even decrease in magnetic fields collinear with the spin direction. This tunable AHE can be attributed to local spin switching enabled by the geometrical frustration of the magnetic kagome lattice, revealing that spins in a kagome ferromagnet change their switching behavior as the magnetic field approaches the kagome plane. Our results also suggest a versatile way to tune the properties of a kagome magnet.

cond-mat.mtrl-sci↗

arXiv2024

Majorana braiding in superconductors with fixed total number of particles

One-dimensional topological superconductors treated at the mean-field level host zero-energy edge Majorana modes, which encode topological degeneracy of their ground states. Geometric manipulations (braiding) of multiple wires can be used to induce topologically robust transformations within the ground state subspace. The mean-field ground states do not have a definite number of particles and thus cannot describe an isolated system. Projecting such states onto fixed particle number gives a very good approximation to the true ground state of an isolated superconductor. In previous work, we showed that so projecting the prototypical Kitaev wave function of a single wire retains key features of the mean-field description, such as the zero-energy single-particle spectral peaks near the wire edges. Here we consider the case of multiple wires with conserved total charge. Again, using the projected Kitaev wave functions as the template, we identify the many-body counterparts of the mean-field topologically degenerate ground states. We then demonstrate how the quantum gates equivalent to braiding of Majorana zero modes can be implemented, albeit with reduced protection from noise and disorder.

cond-mat.str-el↗

arXiv2024

Superconductivity from domain wall fluctuations in sliding ferroelectrics

Bilayers of two-dimensional van der Waals materials that lack an inversion centre can show a novel form of ferroelectricity, where certain stacking arrangements of the two layers lead to an interlayer polarization. Under an external out-of-plane electric field, a relative sliding between the two layers can occur accompanied by an inter-layer charge transfer and a ferroelectric switching. We show that the domain walls that mediate ferroelectric switching are a locus of strong attractive interactions between electrons. The attraction is mediated by the ferroelectric domain wall fluctuations, effectively driven by the soft interlayer shear phonon. We comment on the possible relevance of this attraction mechanism to the recent observation of an interplay between sliding ferroelectricity and superconductivity in bilayer $\text{T$_d$-MoTe}_2$. We also discuss the possible role of this mechanism in the superconductivity of moiré bilayers.

cond-mat.supr-con↗

arXiv2024

Dynamics and Phases of Nonunitary Floquet Transverse-Field Ising Model

Inspired by current research on measurement-induced quantum phase transitions, we analyze the nonunitary Floquet transverse-field Ising model with complex nearest-neighbor couplings and complex transverse fields. Unlike its unitary counterpart, the model shows a number of steady phases, stable to integrability breaking perturbations. Some phases have robust edge modes and/or spatiotemporal long-range orders in the bulk. The transitions between the phases have extensive entanglement entropy, whose scaling with the system size depends on the number of the real quasiparticle modes in the spectrum at the transition. In particular, the volume law scaling appears on some critical lines, protected by pseudo-Hermiticity. Both the scaling of entanglement entropy in steady states and the evolution after a quench are compatible with the non-Hermitian generalization of the quasiparticle picture of Calabrese and Cardy at least qualitatively.

quant-ph↗

arXiv2023

Current-Induced Spin Accumulation and Magnetoresistance in Chiral Semimetals

Weyl fermions possess the property of spin-momentum locking: the expectation value of the spin is parallel or antiparallel to the momentum at any given point in the Brillouin zone in the vicinity of a Weyl node. This is a direct consequence of the fact that Weyl nodes are monopoles of the Berry curvature, and in this sense an expression of the nontrivial Weyl electronic structure topology. Thanks to this property, an isolated Weyl node produces a large spin accumulation in response to a charge current, $\hbar/2$ per electron, similar to surface states of time-reversal invariant topological insulators. However, in bulk Weyl semimetals, the nodes must occur in pairs of opposite chirality and, when the nodes are at the same energy, the effect cancels out. Here we show that this cancellation is avoided in chiral semimetals, in which Weyl nodes of opposite chirality occur at different energies due to broken mirror symmetry. We find that the spin accumulation is maximized when the Fermi energy coincides with one of the nodes in a pair and reaches the same value as for an isolated node in this case. Moreover, we demonstrate the existence of a distinct magnetoresistance mechanism, closely related to this current-induced spin accumulation.

cond-mat.mes-hall↗

arXiv2023

Physics of the Majorana-superconducting qubit hybrids

Manipulation of decoupled Majorana zero modes (MZMs) could enable topologically-protected quantum computing. However, the practical realization of a large number of perfectly decoupled MZMs needed to perform nontrivial quantum computation has proven to be challenging so far. Fortunately, even a small number of imperfect MZMs can be used to qualitatively extend the behavior of standard superconducting qubits, allowing for new approaches for noise suppression, qubit manipulation and read-out. Such hybrid devices take advantage of interplay of Cooper pair tunneling, coherent single electron tunneling, and Majorana hybridization. Here we provide a qualitative understanding of this system, give analytical results for its ground state energy spanning full parameter range, and describe potential sensing applications enabled by the interplay between Majorana and Cooper pair tunneling.

cond-mat.mes-hall↗

arXiv2023

DFT+DMFT study of the magnetic susceptibility and the correlated electronic structure in transition-metal intercalated NbS$_2$

The Co-intercalated NbS$_2$ (Co$_{1/3}$NbS$_2$) compound exhibits large anomalous Hall conductance, likely due to the non-coplanar magnetic ordering of Co spins. In this work, we study the relation between this novel magnetism and the correlated electronic structure of Co$_{1/3}$NbS$_2$ by adopting dynamical mean field theory (DMFT) to treat the correlation effect of Co $d$ orbitals. We find that the hole doping of Co$_{1/3}$NbS$_2$ can tune the size of the Nb hole pocket at the DMFT Fermi surface, producing features consistent with those observed in angle resolved photoemission spectra [Phys. Rev. B 105, L121102 (2022)]. We also compute the momentum-resolved spin susceptibility, and correlate it with the Fermi surface shape. We find that the magnetic ordering wavevector of Co$_{1/3}$NbS$_2$ obtained from the peak in spin susceptibility agrees with the one observed experimentally by neutron scattering; it is compatible with commensurate non-coplanar $3q$ spin structure. We also discuss how results change if some other than Co transition metal intercalations are used.

cond-mat.str-el↗

arXiv2023

Signatures of Majorana Zero-Modes in an isolated one-dimensional superconductor

We examine properties of the mean-field wave function of the one-dimensional Kitaev model supporting Majorana Zero Modes (MZMs) \emph{when restricted} to a fixed number of particles. Such wave functions can in fact be realized as exact ground states of interacting number-conserving Hamiltonians and amount to a more realistic description of the finite isolated superconductors. Akin to their mean-field parent, the fixed-number wave functions encode a single electron spectral function at zero energy that decays exponentially away from the edges, with a localization length that agrees with the mean-field value. Based purely on the structure of the number-projected ground states, we construct the fixed particle number generalization of the MZM operators. They can be used to compute the edge tunneling conductance; however, notably the value of the zero-bias conductance remains the same as in the mean-field case, quantized to $2e^2/h$. We also compute the topological entanglement entropy for the number-projected wave functions and find that it contains a `robust' $\log(2)$ component as well as a logarithmic correction to the mean field result, which depends on the precise partitioning used to compute it. The presence of the logarithmic term in the entanglement entropy indicates the absence of a spectral gap above the ground state; as one introduces fluctuations in the number of particles, the correction vanishes smoothly.

cond-mat.supr-con↗

arXiv2023

Superconductivity from polar fluctuations in multi-orbital systems

Motivated by the superconductivity near paraelectric (PE) to ferroelectric (FE) quantum critical point (QCP) in polar metals, we study polar fluctuation mediated superconductivity in multi-orbital systems. The PE to FE QCP is approached by softening of a transverse optical (TO) phonon that is odd under inversion ($\mathcal{I}$). We show that the necessary and sufficient condition for the linear coupling between electron-TO phonon is the presence of multiple orbitals on the Fermi-surface, irrespective of the spin-orbital (SO) coupling, multiple electronic bands, or the vicinity to band crossings. We show that the linear coupling to the polar fluctuations (such as TO modes) can generally lead to superconductivity. We also show that irrespective of the strong $\vec{k}$ dependence of the effective electron-electron interaction in the BCS channel, quite generally the even-parity channel leads to the highest critical temperature. In the presence of additional repulsive electron-electron interactions, an odd-parity spin-triplet channel can become the leading BCS instability. Finally, we discuss our results in the context of the superconductivity in $\text{SrTiO}_3$ and $\text{KTaO}_3$ that highlights the importance of the underlying multi-orbital physics if the superconductivity is mediated by the polar fluctuations.

cond-mat.supr-con↗

arXiv2023

Doubling of the superconducting transition temperature in ultra-clean wafer-scale aluminum nanofilms

Superconducting properties of thin films can be vastly different from those of bulk materials. Seminal work has shown the critical temperature Tc of elemental superconductors decreases with decreasing film thickness when the normal-state sheet resistance is lower than the quantum resistance h/(4e2). Sporadic examples on disordered films, however, hinted an enhancement in Tc although, structural and strain characterization was not possible since samples were prepared on a cold substrate in situ. To clarify the role of reduced dimensionality and disorder on the superconducting properties of thin films we employed molecular beam epitaxy to grow wafer-scale high-quality aluminum (Al) nanofilms with normal-state sheet resistance at least 20 times lower than h/(4e2) and investigated their electronic and structural properties ex situ. Defying general expectations, Tc increases with decreasing Al film thickness, reaching 2.4 K for 3.5-nm-thick Al film grown on GaAs: twice that of bulk Al (1.2 K). DFT calculations indicate surface phonon softening impacts superconductivity in pure ultra-thin films, offering a new route for materials engineering in two dimensions.

cond-mat.supr-con↗

arXiv2023

Electromechanical memcapacitive neurons for energy-efficient spiking neural networks

In this article, we introduce a new nanoscale electromechanical device -- a leaky memcapacitor -- and show that it may be useful for the hardware implementation of spiking neurons. The leaky memcapacitor is a movable-plate capacitor that becomes quite conductive when the plates come close to each other. The equivalent circuit of the leaky memcapacitor involves a memcapacitive and memristive system connected in parallel. In the leaky memcapacitor, the resistance and capacitance depend on the same internal state variable, which is the displacement of the movable plate. We have performed a comprehensive analysis showing that several spiking types observed in biological neurons can be implemented with the leaky memcapacitor. Significant attention is paid to the dynamic properties of the model. As in leaky memcapacitors the capacitive and leaking resistive functionalities are implemented naturally within the same device structure, their use will simplify the creation of spiking neural networks.

cs.ET↗

arXiv2022

Integrable nonunitary quantum circuits

We show that the integrable Lindblad superoperators found recently can be used to build integrable nonunitary quantum circuits with two-site gates by demonstrating that the $\check{R}$-matrices are completely positive and trace preserving. Using the bond-site transformation, we obtain the corresponding integrable nonunitary quantum circuits with three-site gates. When restricted to the diagonals of the density matrix, these quantum models reduce to integrable classical cellular automata. This approach may pave the way for a systematic construction of integrable nonunitary quantum circuits.

cond-mat.str-el↗

arXiv2022

Temperature-driven changes in the Fermi surface of graphite

We report on temperature-dependent size and anisotropy of the Fermi pockets in graphite revealed by magnetotransport measurements. The magnetoresistances obtained in fields along the c-axis obey an extended Kohler's rule, with the carrier density following prediction of a temperature-dependent Fermi energy, indicating a change in the Fermi pocket size with temperature. The angle-dependent magnetoresistivities at a given temperature exhibit a scaling behavior. The scaling factor that reflects the anisotropy of the Fermi surface is also found to vary with temperature. Our results demonstrate that temperature-driven changes in Fermi surface can be ubiquitous and need to be considered in understanding the temperature-dependent carrier density and magnetoresistance anisotropy in semimetals.

cond-mat.mtrl-sci↗

arXiv2022

Effect of quasiperiodic and random noise on many-body dynamical decoupling protocols

Symmetries (and their spontaneous rupturing) can be used to protect and engender novel quantum phases and lead to interesting collective phenomena. In Ref. 1, the authors described a general dynamical decoupling (polyfractal) protocol that can be used to engineer multiple discrete symmetries in many-body systems. The present work expands on the former by studying the effect of quasiperiodic and random noise on such a dynamical scheme. We find generally that relaxation of engineered symmetry generators proceeds by i) an initial relaxation on microscopic timescales to a prethermal plateau whose height is independent of noise, ii) a linear relaxation regime with a noise-dependent rate, followed by iii) a slow logarithmic relaxation regime that is only present for quasiperiodic noise. We glean the essential features of these regimes via scaling collapses and show that they can be generally explained by the spectral properties of the various noise waveforms considered. In particular, the quasiperiodic noise is characterised by highly time dependent spectrum with a noise floor that mimics white noise, and peaks that grow sharper with time. We argue that both the noise floor and peaks contribute to the initial linear-in-time relaxation while the logarithmic regime is initiated when the peaks become sufficiently well resolved and cease to contribute to further relaxation. We provide numerical evidence to justify these findings.

quant-ph↗

arXiv2022

Electron spin coherence on a solid neon surface

A single electron floating on the surface of a condensed noble-gas liquid or solid can act as a spin qubit with ultralong coherence time, thanks to the extraordinary purity of such systems. Previous studies suggest that the electron spin coherence time on a superfluid helium (He) surface can exceed 100 s. In this paper, we present theoretical studies of the electron spin coherence on a solid neon (Ne) surface, motivated by our recent experimental realization of single-electron charge qubit on solid Ne. The major spin decoherence mechanisms investigated include the fluctuating Ne diamagnetic susceptibility due to thermal phonons, the fluctuating thermal current in normal metal electrodes, and the quasi-statically fluctuating nuclear spins of the $^{21}$Ne ensemble. We find that at a typical experimental temperature about 10 mK in a fully superconducting device, the electron spin decoherence is dominated by the third mechanism via electron-nuclear spin-spin interaction. For natural Ne with 2700 ppm abundance of $^{21}$Ne, the estimated inhomogeneous dephasing time $T_{2}^{*}$ is around 0.16 ms, already better than most semiconductor quantum-dot spin qubits. For commercially available, isotopically purified Ne with 1 ppm of $^{21}$Ne, $T_{2}^{*}$ can be $0.43$ s. Under the application of Hahn echoes, the coherence time $T_{2}$ can be improved to $30$ ms for natural Ne and $81$ s for purified Ne. Therefore, the single-electron spin qubits on solid Ne can serve as promising new spin qubits.

cond-mat.mes-hall↗

arXiv2022

Topological frequency conversion in Weyl semimetals

We theoretically predict a new working principle for optical amplification, based on Weyl semimetals: when a Weyl semimetal is suitably irradiated at two frequencies, electrons close to the Weyl points convert energy between the frequencies through the mechanism of topological frequency conversion from [Martin et al, PRX 7 041008 (2017)]. Each electron converts energy at a quantized rate given by an integer multiple of Planck's constant multiplied by the product of the two frequencies. In simulations, we show that optimal, but feasible band structures can support topological frequency conversion in the "THz gap" at intensities down to $ 2{\rm W}/{\rm mm^2}$; the gain from the effect can exceed the dissipative loss when the frequencies are larger than the relaxation time of the system. Topological frequency conversion provides a new paradigm for optical amplification, and further extends Weyl semimetals' promise for technological applications.

cond-mat.mes-hall↗

arXiv2022

Tuning between continuous time crystals and many-body scars in long-range XYZ spin chains

Persistent oscillatory dynamics in non-equilibrium many-body systems is a tantalizing manifestation of ergodicity breakdown that continues to attract much attention. Recent works have focused on two classes of such systems: discrete time crystals and quantum many-body scars (QMBS). While both systems host oscillatory dynamics, its origin is expected to be fundamentally different: discrete time crystal is a phase of matter which spontaneously breaks the $\mathbb{Z}_2$ symmetry of the external periodic drive, while QMBS span a subspace of non-thermalizing eigenstates forming an su(2) algebra representation. Here we ask a basic question: is there a physical system that allows to tune between these two dynamical phenomena? In contrast to much previous work, we investigate the possibility of a \emph{continuous} time crystal (CTC) in undriven, energy-conserving systems exhibiting prethermalization. We introduce a long-range XYZ spin model and show that it encompasses both a CTC phase as well as QMBS. We map out the dynamical phase diagram using numerical simulations based on exact diagonalization and time-dependent variational principle in the thermodynamic limit. We identify a regime where QMBS and CTC order co-exist, and we discuss experimental protocols that reveal their similarities as well as key differences.

cond-mat.str-el↗