arXiv subjects

Jürgen König

Publications and source records attributed to Jürgen König.

At least 19 recordsLinked to original sources

arXiv2026

Observation of correlations beyond the single-particle picture in fermionic counting statistics

The analysis of charge fluctuations in a mesoscopic device can shed light on the fundamental question of whether or not a single-particle picture of electron transport is appropriate, even in the presence of Coulomb interaction. It has been shown on general grounds that mapping the interacting system onto a fermionic single-particle description is subject to strict constraints on the charge-transfer statistics. These constraints can be formulated in terms of a sign rule for the factorial cumulants of the full counting statistics. We report here on the experimental observation of a sign-rule violation in a most elementary model system, i.e. a single-level quantum dot, and provide theoretical modeling that can quantitatively reproduce the experimental data. This reveals the presence of correlations introduced by electron-electron interaction.

cond-mat.mes-hall↗

arXiv2026

Coupling-energy driven pumping through quantum dots: Role of coherences

We study the impact of off-resonant tunneling and coherences on the electron pumping through quantum dots. Thereby, we focus on two electron-pump setups where lowest-order tunneling processes are suppressed and the pump is exclusively driven by modulations of the coupling energy. The first setup is driven by switching on and off the couplings between the quantum dot and the leads, while the second setup employs measurements of the dot occupation. We derive exact solutions for arbitrarily strong tunnel couplings in the absence of Coulomb interaction, identify parameter regimes with optimal pumping currents or optimal energy efficiency, and discuss similarities between both pumping mechanisms.

cond-mat.mes-hall↗

arXiv2025

Statistical analysis of electron-induced switching of a spin-crossover complex

Spin-crossover complexes exhibit two stable configurations with distinct spin states. The investigation of these molecules using low-temperature scanning tunneling microscopy has opened new perspectives for understanding the associated switching mechanisms at the single-molecule level. While the role of tunneling electrons in driving the spin-state switching has been clearly evidenced, the underlying microscopic mechanism is not completely understood. In this study, we investigate the electron-induced switching of [Fe(H$_2$B(pz)(pypz))$_2$] (pz = pyrazole, pypz = pyridylpyrazole) adsorbed on Ag(111). The current time traces show transitions between two current levels corresponding to the two spin states. We extract switching rates from these traces by analyzing waiting-time distributions. Their sample-voltage dependence can be explained within a simple model in which the switching is triggered by a transient charging of the molecule. The comparison between experimental data and theoretical modeling provides estimates for the energies of the lowest unoccupied molecular orbitals, which were so far experimentally inaccessible. Overall, our approach offers new insights into the electron-induced switching mechanism and predicts enhanced switching rates upon electronic decoupling of the molecule from the metallic substrate, for example by introducing an ultrathin insulating layer.

cond-mat.mes-hall↗

arXiv2025

Relaxation to persistent currents in a Hubbard trimer coupled to fermionic baths

We consider a ring of fermionic quantum sites, modeled by the Fermi--Hubbard Hamiltonian, in which electrons can move and interact strongly via the Coulomb repulsion. The system is coupled to fermionic cold baths which by the exchange of particles and energy induce relaxation in the system. We eliminate the environment and describe the system effectively by Lindblad master equations in various versions valid for different coupling parameter regimes. The early relaxation phase proceeds in a universal way, irrespective of the relative couplings and approximations. The system settles down to its low--energy sector and is consecutively well approximated by the Heisenberg model. We compare different Lindblad approaches which, in the late relaxation, push the system towards different final states with opposite, extreme spin orders, from ferromagenetic to antiferromagnetic. Due to spin frustration in the trimer (a three site ring), degenerate ground states are formed by spin waves (magnons). The system described by the global coherent version of the Lindblad operators relaxes towards the final states carrying directed persistent spin currents. We numerically confirm these predictions.

cond-mat.str-el↗

arXiv2025

Effective time-dependent temperature for fermionic master equations beyond the Markov and the secular approximations

We consider a fermionic quantum system exchanging particles with an environment at a fixed temperature and study its reduced evolution by means of a Redfield-I equation with time-dependent (non-Markovian) coefficients. We find that the description can be efficiently reduced to a standard-form Redfield-II equation, however, with a time-dependent effective bath temperature obeying a universal law. At early times, after the system and environment start in a product state, the effective temperature appears to be very high, yet eventually it settles down towards the true environment value. In this way, we obtain a time-local master equation, offering high accuracy at all times and preserving the crucial properties of the density matrix. It includes non-Markovian relaxation processes beyond the secular approximation and time-averaging methods and can be further applied to various types of Gorini-Kossakowski-Sudarshan-Lindblad equations. We derive the theory from first principles and discuss its application using a simple example of a single quantum dot.

cond-mat.mes-hall↗

arXiv2024

Quasi-particle propagation across semiconductor-Mott insulator interfaces

As a prototypical example for a heterostructure combining a weakly and a strongly interacting quantum many-body system, we study the interface between a semiconductor and a Mott insulator. Via the hierarchy of correlations, we derive and match the propagating or evanescent (quasi) particle solutions on both sides and assume that the interactions among the electrons in the semiconducting regions can be absorbed by an effective potential. While the propagation is described by a band-like dispersion in both the weakly and the strongly interacting case, the inverse decay length across the interface follows a different dependence on the band gap in the Mott insulator and the semiconductor. As one consequence, tunnelling through a Mott insulating layer behaves quite differently from a semiconducting (or band insulating) layer. For example, we find a strong suppression of tunnelling for energies in the middle between the upper and lower Hubbard band of the Mott insulator.

cond-mat.str-el↗

arXiv2024

Dark versus blocking states in electronic transport: a Lee-Yang zero analysis of full counting statistics

Electronic transport through nanostructures can be suppressed by coherent population trapping, in which quantum coherence leads to a dark state that decouples from the drain electrode. Finite transport, then, relies on decoherence of the dark state. An alternative scenario for reduced transport is weak coupling of a state, referred to as a blocking state, to the drain. This raises the question of whether and how these two scenarios can be distinguished in the transport features. For the example of electron transport through a carbon nanotube, we identify regimes, in which this distinction is possible by analyzing the full counting statistics in terms of Lee-Yang zeros and factorial cumulants.

cond-mat.mes-hall↗

arXiv2023

Independent and coherent transitions between antiferromagnetic states of few-molecule systems

Spin-electronic devices are poised to become part of mainstream microelectronic technology .Downsizing them, however, faces the intrinsic difficulty that as ferromagnets become smaller, it becomes more difficult to stabilize their magnetic moment. Antiferromagnets are much more stable, and thus research on antiferromagnetic spintronics has developed into a fast-growing field. Here, we provide proof of concept data that allows us to expand the area of antiferromagnetic spintronics to the hitherto elusive level of individual molecules. In contrast to all previous work on molecular spintronics, our detection scheme of the molecule's spin state does not rely on a magnetic moment. Instead, we use field-effect transistor devices constituting of an isolated, contacted single-wall carbon nanotube covalently bound to a limited number of molecular antiferromagnets incorporating four Mn(II) or Co(II) ions. Time-dependent quantum transport measurement along the functionalized nanotube show step-like transitions between several distinct current levels, which we attribute to transitions between different antiferromagnetic states of individual molecular complexes grafted on the nanotube. A statistical analysis of the switching events using factorial cumulants indicates that the cobalt complexes switch independently from each other, while a coherent superposition of the antiferromagnetic spin states of the molecules along the nanotube is observed for the manganese complexes. The long coherence time (several seconds at 100 mK) is made possible by the absence of spin and orbital momentum in the relevant states of the manganese complex, while the cobalt complex includes a significant orbital momentum contribution due to the pseudo-octahedral d$^7$ metal centers.

cond-mat.mes-hall↗

arXiv2023

Unraveling spin dynamics from charge fluctuations

The use of single electron spins in quantum dots as qubits requires detailed knowledge about the processes involved in their initialization and operation as well as their relaxation and decoherence. In optical schemes for such spin qubits, spin-flip Raman as well as Auger processes play an important role, in addition to environment-induced spin relaxation. In this paper, we demonstrate how to quantitatively access all the spin-related processes in one go by monitoring the charge fluctuations of the quantum dot. For this, we employ resonance fluorescence and analyze the charge fluctuations in terms of waiting-time distributions and full counting statistics characterized by factorial cumulants.

cond-mat.mes-hall↗

arXiv2023

Full counting statistics in a Majorana single-charge transistor

We study full counting statistics of electron transport through a Majorana single-charge transistor. At low bias voltage, transport is dominated by the so-called Josephson-Majorana cycle, a sequence of normal and anomalous single-charge and Josephson tunneling. Factorial cumulants characterizing the full counting statistics elucidate the correlated nature of the charge transfers in this cycle. Moreover, we predict a topological transition in the full counting statistics from a perfect Poissonian transfer of Cooper pairs to a correlated switching between two distinct fermion parity states with increasing Josephson coupling.

cond-mat.mes-hall↗

arXiv2022

Transfer-matrix summation of path integrals for transport through nanostructures

On the basis of the method of iterative summation of path integrals (ISPI), we develop a numerically exact transfer-matrix method to describe the nonequilibrium properties of interacting quantum-dot systems. For this, we map the ISPI scheme to a transfer-matrix approach, which is more accessible to physical interpretation, allows for a more transparent formulation of the theory, and substantially improves the efficiency. In particular, the stationary limit is directly implemented, without the need of extrapolation. The resulting new method, referred to as "transfer-matrix summation of path integrals" (TraSPI), is then applied to resonant electronic transport through a single-level quantum dot.

cond-mat.mes-hall↗

arXiv2022

Environment-induced decay dynamics of anti-ferromagnetic order in Mott-Hubbard systems

We study the dissipative Fermi-Hubbard model in the limit of weak tunneling and strong repulsive interactions, where each lattice site is tunnel-coupled to a Markovian fermionic bath. For cold baths at intermediate chemical potentials, the Mott insulator property remains stable and we find a fast relaxation of the particle number towards half filling. On longer time scales, we find that the anti-ferromagnetic order of the Mott-Néel ground state on bi-partite lattices decays, even at zero temperature. For zero and non-zero temperatures, we quantify the different relaxation time scales by means of waiting time distributions which can be derived from an effective (non-Hermitian) Hamiltonian and obtain fully analytic expressions for the Fermi-Hubbard model on a tetramer ring.

cond-mat.str-el↗

arXiv2022

Pushing the limits in real-time measurements of quantum dynamics

Time-resolved studies of quantum systems are the key to understand quantum dynamics at its core. The real-time measurement of individual quantum numbers as they switch between certain discrete values, well known as random telegraph signal, is expected to yield maximal physical insight. However, the signal suffers from both systematic errors, such as a limited time resolution and noise from the measurement apparatus, as well as statistical errors due to a limited amount of data. Here we demonstrate that an evaluation scheme based on factorial cumulants can reduce the influence of such errors by orders of magnitude. The error resilience is supported by a general theory for the detection errors as well as experimental data of single-electron tunnelling through a self-assembled quantum dot. Thus, factorial cumulants push the limits in the analysis of random telegraph data which represent a wide class of experiments in physics, chemistry, engineering and life sciences.

cond-mat.mes-hall↗

arXiv2021

Post-processing of real-time quantum event measurements for an optimal bandwidth

Single electron tunneling and its transport statistics have been studied for some time using high precision charge detectors. However, this type of detection requires advanced lithography, optimized material systems and low temperatures (mK). A promising alternative, recently demonstrated, is to exploit an optical transition that is turned on or off when a tunnel event occurs. High bandwidths should be achievable with this approach, although this has not been adequately investigated so far. We have studied low temperature resonance fluorescence from a self-assembled quantum dot embedded in a diode structure. We detect single photons from the dot in real time and evaluate the recorded data only after the experiment, using post-processing to obtain the random telegraph signal of the electron transport. This is a significant difference from commonly used charge detectors and allows us to determine the optimal time resolution for analyzing our data. We show how this post-processing affects both the determination of tunneling rates using waiting-time distributions and statistical analysis using full-counting statistics. We also demonstrate, as an example, that we can analyze our data with bandwidths as high as 350 kHz. Using a simple model, we discuss the limiting factors for achieving the optimal bandwidth and propose how a time resolution of more than 1 MHz could be achieved.

cond-mat.mes-hall↗

arXiv2021

Synchronized coherent charge oscillations in coupled double quantum dots

We study coherent oscillations in double quantum dots tunnel-coupled to metallic leads by means of full counting statistics of electron transport. If two such systems are coupled by Coulomb interaction, there are in total six (instead of only two) oscillation modes of the entangled system with interaction-dependent oscillation frequencies. By tuning the bias voltage, one can engineer decoherence such that only one of the six modes, in which the charge oscillations in both double quantum dots become synchronized in antiphase, is singled out. We suggest to use waiting-time distributions and the $g^{(2)}$-correlation function to detect the common frequency and the phase locking.

cond-mat.mes-hall↗

arXiv2021

Electron Waiting Times in a Strongly Interacting Quantum Dot: Interaction Effects and Higher-Order Tunneling Processes

Distributions of electron waiting times have been measured in several recent experiments and have been shown to provide complementary information compared to what can be learned from the electric current fluctuations. Existing theories, however, are restricted to either weakly coupled nanostructures or phase-coherent transport in mesoscopic conductors. Here, we consider an interacting quantum dot and develop a real-time diagrammatic theory of waiting time distributions that can treat the interesting regime, in which both interaction effects and higher-order tunneling processes are important. Specifically, we find that our quantum-mechanical theory captures higher-order tunneling processes at low temperatures, which are not included in a classical description, and which dramatically affect the waiting times by allowing fast tunneling processes inside the Coulomb blockade region. Our work paves the way for systematic investigations of temporal fluctuations in interacting quantum systems, for example close to a Kondo resonance or in a Luttinger liquid.

cond-mat.mes-hall↗

arXiv2021

Statistical analysis of spin switching in coupled spin-crossover molecules

We study the switching behavior of two spin-crossover molecules residing in a nanojunction device consisting of two closely spaced gold electrodes. The spin states are monitored through a real-time measurement of the resistance of the junction. A statistical analysis of the resistance values, the occupation probabilities, and the lifetimes of the respective spin states shows that the two spin-crossover molecules are coupled to each other. We extract the parameters for a minimal model describing the two coupled spin-crossover molecules. Finally, we use the time dependence of factorial cumulants to demonstrate that the measured data indicates the presence of interactions between the two spin-crossover molecules.

cond-mat.mes-hall↗

arXiv2021

How to get from static to dynamic electromagnetism

We demonstrate how to derive Maxwell's equations, including Faraday's law and Maxwell's correction to Ampère's law, by generalizing the description of static electromagnetism to dynamical situations. Thereby, Faraday's law is introduced as a consequence of the relativity principle rather than an experimental fact, in contrast to the historical course and common textbook presentations. As a by-product, this procedure yields explicit expressions for the infinitesimal Lorentz and, upon integration, the finite Lorentz transformation. The proposed approach helps to elucidate the relation between Galilei and Lorentz transformations and provides an alternative derivation of the Lorentz transformation without explicitly referring to the speed of light.

physics.class-ph↗