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Jürgen Volz

Publications and source records attributed to Jürgen Volz.

35 records · Page 2Linked to original sources

Beyond the Tavis-Cummings model: revisiting cavity QED with atomic ensembles

The interaction of an ensemble of $N$ two-level atoms with a single mode electromagnetic field is described by the Tavis-Cummings model. There, the collectively enhanced light-matter coupling strength is given by $g_N = \sqrt{N} \bar{g}_1$, where $\bar{g}_1$ is the ensemble-averaged single-atom coupling strength. Formerly, this model has been employed to describe and to analyze numerous cavity-based experiments. Here, we show that this is only justified if the effective scattering rate into non-cavity modes is negligible compared to the cavity's free-spectral range. In terms of experimental parameters, this requires that the optical depth of the ensemble is low, a condition that is violated in several state-of-the-art experiments. We give quantitative conditions for the validity of the Tavis-Cummings model and derive a more general Hamiltonian description that takes into account the cascaded interaction of the photons with all consecutive atoms. We show that the predictions of our model can differ quantitatively and even qualitatively from those obtained with the Tavis-Cummings model. Finally, we present experimental data, for which the deviation from the predictions of the Tavis-Cummings model is apparent. Our findings are relevant for all experiments in which optically dense ensembles of quantum emitters are coupled to an optical resonator.

quant-ph↗

High-Q Lithium Niobate Microcavities and Their Applications

Lithium niobate (LN) is an excellent nonlinear optical and electro-optic material that has found many applications in classical nonlinear optics, optical fiber communications and quantum photonics. Here we review the recent development of thin-film LN technology that has allowed the miniaturization of LN photonic devices and microcavities with ultrahigh quality factors. We discuss the design principle of LN devices that makes use of the largest nonlinear coefficients, various device fabrication approaches and resulting device performances, and the current and potential applications of LN microcavities.

physics.app-ph↗

Coupling a single trapped atom to a whispering-gallery-mode microresonator

We demonstrate trapping of a single 85Rb atom at a distance of 200 nm from the surface of a whispering-gallery-mode bottle microresonator. The atom is trapped in an optical potential, which is created by retroreflecting a red-detuned focused laser beam from the resonator surface. We counteract the trap-induced light shift of the atomic transition frequency by superposing a second laser beam with suitably chosen power and detuning. This allows us to observe a vacuum Rabi-splitting in the excitation spectrum of the coupled atom-resonator system. This first demonstration of stable and controlled interaction of a single atom with a whispering-gallery-mode in the strong coupling regime opens up the route towards the implementation of quantum protocols and applications that harvest the chiral atom-light coupling present in this class of resonators.

quant-ph↗

Slow light-enhanced optical imaging of microfiber radius variations with sub-Angström precision

Optical fibers play a key role in many different fields of science and technology. In particular, fibers with a diameter of several micrometers are intensively used in photonics. For these applications, it is often important to precisely know and control the fiber radius. Here, we demonstrate a novel technique to determine the local radius variation of a 30-micrometer diameter silica fiber with sub-Ångström precision with axial resolution of several tens of micrometers over a fiber length of more than half a millimeter. Our method relies on taking an image of the fiber's whispering-gallery modes (WGMs). In these WGMs, the speed of light propagating along the fiber axis is strongly reduced. This enables us to determine the fiber radius with a significantly enhanced precision, far beyond the diffraction limit. By exciting different axial modes, we verify the precision and reproducibility of our method and demonstrate that we can achieve a precision better than 0.3 Å. The method can be generalized to other experimental situations where slow light occurs and, thus, has a large range of potential applications in the realm of precision metrology and optical sensing.

physics.optics↗

Correlating photons using the collective nonlinear response of atoms weakly coupled to an optical mode

Photons in a nonlinear medium can repel or attract each other, resulting in a strongly correlated quantum many-body system. Typically, such strongly correlated states of light arise from the extreme nonlinearity granted by quantum emitters that are strongly coupled to a photonic mode. However, in these approaches, unavoidable dissipation, like photon loss, blurs nonlinear quantum effects. Here, we generate strongly correlated photon states using only weak coupling and taking advantage of dissipation. We launch light through an ensemble of non-interacting waveguide-coupled atoms, which induce correlations between simultaneously arriving photons through collectively enhanced nonlinear interactions. These correlated photons then experience less dissipation than the uncorrelated ones. Depending on the number of atoms, we experimentally observe strong photon bunching or anti-bunching of the transmitted light. This realization of a collectively enhanced nonlinearity may turn out transformational for quantum information science and opens new avenues for generating nonclassical light, covering frequencies from the microwave to the X-ray regime.

quant-ph↗

Wavelength-scale errors in optical localization due to spin-orbit coupling of light

The precise determination of the position of point-like emitters and scatterers using far-field optical imaging techniques is of utmost importance for a wide range of applications in medicine, biology, astronomy, and physics. Although the optical wavelength sets a fundamental limit to the image resolution of unknown objects, the position of an individual emitter can in principle be estimated from the image with arbitrary precision. This is used, e.g., in stars' position determination and in optical super-resolution microscopy. Furthermore, precise position determination is an experimental prerequisite for the manipulation and measurement of individual quantum systems, such as atoms, ions, and solid state-based quantum emitters. Here we demonstrate that spin-orbit coupling of light in the emission of elliptically polarized emitters can lead to systematic, wavelength-scale errors in the estimate of the emitter's position. Imaging a single trapped atom as well as a single sub-wavelength-diameter gold nanoparticle, we demonstrate a shift between the emitters' measured and actual positions which is comparable to the optical wavelength. Remarkably, for certain settings, the expected shift can become arbitrarily large. Beyond their relevance for optical imaging techniques, our findings apply to the localization of objects using any type of wave that carries orbital angular momentum relative to the emitter's position with a component orthogonal to the direction of observation.

quant-ph↗

Observation of Multimode Strong Coupling of Cold Atoms to a 30-m Long Optical Resonator

We report on the observation of multimode strong coupling of a small ensemble of atoms interacting with the field of a 30-m long fiber resonator containing a nanofiber section. The collective light--matter coupling strength exceeds the free spectral range and the atoms couple to consecutive longitudinal resonator modes. The measured transmission spectra of the coupled atom-resonator system provide evidence of this regime, realized with a few hundred atoms with an intrinsic single-atom cooperativity of 0.26. These results are the starting point for studies in a new setting of light-matter interaction, with strong quantum non-linearities and a new type of dynamics.

quant-ph↗

Fiber ring resonator with nanofiber section for chiral cavity quantum electrodynamics and multimode strong coupling

We experimentally realize an optical fiber ring resonator that includes a tapered section with subwavelength-diameter waist. In this section, the guided light exhibits a significant evanescent field which allows for efficient interfacing with optical emitters. A commercial tunable fiber beam splitter provides simple and robust coupling to the resonator. Key parameters of the resonator such as its out-coupling rate, free spectral range, and birefringence can be adjusted. Thanks to the low taper- and coupling-losses, the resonator exhibits an unloaded finesse of F=75+/-1, sufficient for reaching the regime of strong coupling for emitters placed in the evanescent field. The system is ideally suited for trapping ensembles of laser-cooled atoms along the nanofiber section. Based on measured parameters, we estimate that the system can serve as a platform for optical multimode strong coupling experiments. Finally, we discuss the possibilities of using the resonator for applications based on chiral quantum optics.

quant-ph↗

Quantum optical circulator controlled by a single chirally coupled atom

We demonstrate a fiber-integrated quantum optical circulator that is operated by a single atom and that relies on the chiral interaction between emitters and transversally confined light. Like its counterparts in classical optics, our circulator exhibits an inherent asymmetry between light propagation in the forward and the backward direction. However, rather than a magnetic field or a temporal modulation, it is the internal quantum state of the atom that controls the operation direction of the circulator. This working principle is compatible with preparing the circulator in a coherent superposition of its operational states. Such a quantum circulator may thus become a key element for routing and processing quantum information in scalable integrated optical circuits. Moreover, it features a strongly nonlinear response at the single-photon level, thereby enabling, e.g., photon number-dependent routing and novel quantum simulation protocols.

quant-ph↗

Chiral Quantum Optics

At the most fundamental level, the interaction between light and matter is manifested by the emission and absorption of single photons by single quantum emitters. Controlling light--matter interaction is the basis for diverse applications ranging from light technology to quantum--information processing. Many of these applications are nowadays based on photonic nanostructures strongly benefitting from their scalability and integrability. The confinement of light in such nanostructures imposes an inherent link between the local polarization and propagation direction of light. This leads to {\em chiral light--matter interaction}, i.e., the emission and absorption of photons depend on the propagation direction and local polarization of light as well as the polarization of the emitter transition. The burgeoning research field of {\em chiral quantum optics} offers fundamentally new functionalities and applications both for single emitters and ensembles thereof. For instance, a chiral light--matter interface enables the realization of integrated non--reciprocal single--photon devices and deterministic spin--photon interfaces. Moreover, engineering directional photonic reservoirs opens new avenues for constructing complex quantum circuits and networks, which may be applied to simulate a new class of quantum many--body systems.

quant-ph↗

Chiral nanophotonic waveguide interface based on spin-orbit coupling of light

Controlling the flow of light by means of nanophotonic waveguides has the potential of transforming integrated information processing much in the same way that conventional glass fibers have revolutionized global communication. Owing to the strong transverse confinement of the light, such waveguides give rise to a coupling between the internal spin of the guided photons and their orbital angular momentum. Here, we employ this spin-orbit coupling of light to break the mirror symmetry of the scattering of light by a single gold nanoparticle on the surface of a nanophotonic waveguide. We thereby realize a chiral waveguide coupler in which the handedness of the incident light determines the direction of propagation in the waveguide. Using this effect, we control the directionality of the scattering process and direct up to 94% of the incoupled light into a given direction. This enables novel ways for controlling and manipulating light in optical waveguides and nanophotonic structures as well as for the design of integrated optical sensors.

quant-ph↗

Nonlinear pi phase shift for single fiber-guided photons interacting with a single atom

Realizing a strong interaction between individual optical photons is an important objective of research in quantum science and technology. Since photons do not interact directly, this goal requires, e.g., an optical medium in which the light experiences a phase shift that depends nonlinearly on the photon number. Once the additional phase shift for two photons reaches pi, such an ultra-strong nonlinearity could even enable the direct implementation of high-fidelity quantum logic operations. However, the nonlinear response of standard optical media is many orders of magnitude too weak for this task. Here, we demonstrate the realization of an optical fiber-based nonlinearity that leads to an additional two-photon phase shift close to the ideal value of pi. Our scheme employs a whispering-gallery-mode resonator, interfaced by an optical nanofiber, where the presence of a single rubidium atom in the resonator results in a strongly nonlinear response. We experimentally show that this results in entanglement of initially independent incident photons. The demonstration of this ultra-strong nonlinearity in a fiber-integrated system is a decisive step towards scalable quantum logics with optical photons.

quant-ph↗

Fiber-optical switch controlled by a single atom

We demonstrate highly efficient switching of optical signals between two optical fibers controlled by a single atom. The key element of our experiment is a whispering-gallery mode bottle microresonator, which is coupled to a single atom and interfaced by two tapered fiber couplers. Even in the presence of the coupling fibers, the atom--resonator system reaches the strong coupling regime of cavity quantum electrodynamics (CQED), leading to a vacuum Rabi splitting in the excitation spectrum. We systematically investigate the switching efficiency of our system, i.e., the probability that the CQED fiber-optical switch redirects the light into the desired output. We obtain a large redirection efficiency reaching a raw fidelity of more than 60% without post-selection.

quant-ph↗

Strong coupling between single atoms and non-transversal photons

We investigate the interaction between single quantum emitters and non-transversally polarised photons for which the electric field vector amplitude has a significant component in the direction of propagation. Even though this situation seems to be at odds with the description of light as a transverse wave, it regularly occurs when interfacing or manipulating emitters with non-paraxial, guided, or evanescent light. Here, we couple single rubidium atoms to single photons which are confined in an optical microresonator by continuous total internal reflection. We experimentally show that the non-transversal polarisation decisively alters the physics of strong light--matter interaction. This effect has far-reaching and highly advantageous implications, which, e.g., significantly advance the field of cavity quantum electrodynamics with whispering-gallery-mode resonators. In particular, our finding allows us to experimentally realise a paradigmatic quantum system, which is ideally suited for basic studies and technological applications.

quant-ph↗

Coherence of a qubit stored in Zeeman levels of a single optically trapped atom

We experimentally investigate the coherence properties of a qubit stored in the Zeeman substates of the 5S1/2, F=1 hyperfine ground level of a single optically trapped Rb-87 atom. Larmor precession of a single atomic spin-1 system is observed by preparing the atom in a defined initial spin-state and then measuring the resulting state after a programmable period of free evolution. Additionally, by performing quantum state tomography, maximum knowledge about the spin coherence is gathered. By using an active magnetic field stabilization and without application of a magnetic guiding field we achieve transverse and longitudinal dephasing times of T2*=75..150 \mus and T1>0.5 ms respectively. We derive the light-shift distribution of a single atom in the approximately harmonic potential of a dipole trap and show that the measured atomic spin coherence is limited mainly by residual position- and state-dependent effects in the optical trapping potential. The improved understanding enables longer coherence times, an important prerequisite for future applications in long-distance quantum communication and computation with atoms in optical lattices or for a loophole-free test of Bell's inequality.

quant-ph↗

Measuring the internal state of a single atom without energy exchange

Real quantum measurements almost always cause a much stronger back action than required by the laws of quantum mechanics. In particular, free-space optical detection methods for single atoms and ions such as the shelving technique, though being among the most sensitive detection methods in quantum physics, inevitably require spontaneous scattering, even in the dispersive regime. This causes heating, a limitation for atom-based quantum information processing where it obviates straightforward reuse of the qubit. No such energy exchange is required by quantum mechanics. Here we experimentally demonstrate optical detection of an atomic qubit with significantly less than one spontaneous scattering event. We measure transmission and reflection of an optical cavity containing the atom. In addition to the qubit detection itself, we quantitatively measure how much spontaneous scattering has occurred. This allows us to relate the information gained to the amount of spontaneous emission, and we obtain a detection error below 10% while scattering less than 0.2 photons on average. Furthermore, we perform a quantum Zeno type experiment to quantify the measurement back action and find that every incident photon leads to an almost complete state collapse. Together, these results constitute a full experimental characterization of a quantum measurement in the "energy exchange-free" regime below a single spontaneous emission event. Besides its fundamental interest, this means significant simplification for proposed neutral-atom quantum computation schemes and may enable sensitive detection of molecules and atoms lacking closed transitions.

quant-ph↗

Cavity-based single atom preparation and high-fidelity hyperfine state readout

We prepare and detect the hyperfine state of a single 87Rb atom coupled to a fiber-based high finesse cavity on an atom chip. The atom is extracted from a Bose-Einstein condensate and trapped at the maximum of the cavity field, resulting in a reproducibly strong atom-cavity coupling. We use the cavity reflection and transmission signal to infer the atomic hyperfine state with a fidelity exceeding 99.92% in a read-out time of 100 microseconds. The atom is still trapped after detection.

quant-ph↗