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J. Äystö

Publications and source records attributed to J. Äystö.

31 records · Page 2Linked to original sources

Characterization of a cylindrical plastic β-detector with Monte Carlo simulations of optical photons

In this work we report on the Monte Carlo study performed to understand and reproduce experimental measurements of a new plastic \b{eta}-detector with cylindrical geometry. Since energy deposition simulations differ from the experimental measurements for such a geometry, we show how the simulation of production and transport of optical photons does allow one to obtain the shapes of the experimental spectra. Moreover, taking into account the computational effort associated with this kind of simulation, we develop a method to convert the simulations of energy deposited into light collected, depending only on the interaction point in the detector. This method represents a useful solution when extensive simulations have to be done, as in the case of the calculation of the response function of the spectrometer in a total absorption γ-ray spectroscopy analysis.

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Mass of astrophysically relevant $^{31}$Cl and the breakdown of the isobaric multiplet mass equation

The mass of $^{31}$Cl has been measured with the JYFLTRAP double Penning trap mass spectrometer at the Ion-Guide Isotope Separator On-Line (IGISOL) facility. The determined mass-excess value, -7034.7(34) keV, is 15 times more precise than in the Atomic Mass Evaluation 2012. The quadratic form of the isobaric multiplet mass equation for the T=3/2 quartet at A=31 fails ($χ^2_n$=11.6) and a non-zero cubic term, d=-3.5(11) keV, is obtained when the new mass value is adopted. $^{31}$Cl has been found to be less proton-bound with a proton separation energy of $S_p$=265(4) keV. Energies for the excited states in $^{31}$Cl and the photodisintegration rate on $^{31}$Cl have been determined with significantly improved precision using the new $S_p$ value. The improved photodisintegration rate helps to constrain astrophysical conditions where $^{30}$S can act as a waiting point in the rapid proton capture process in type I x-ray bursts.

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Total Absorption Spectroscopy Study of $^{92}$Rb Decay: A Major Contributor to Reactor Antineutrino Spectrum Shape

The antineutrino spectra measured in recent experiments at reactors are inconsistent with calculations based on the conversion of integral beta spectra recorded at the ILL reactor. $^{92}$Rb makes the dominant contribution to the reactor spectrum in the 5-8 MeV range but its decay properties are in question. We have studied $^{92}$Rb decay with total absorption spectroscopy. Previously unobserved beta feeding was seen in the 4.5-5.5 region and the GS to GS feeding was found to be 87.5(25)%. The impact on the reactor antineutrino spectra calculated with the summation method is shown and discussed.

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Coulomb displacement energies as a probe for nucleon pairing in the $f_{7/2}$ shell

Coulomb displacement energies of $T=1/2$ mirror nuclei have been studied via a series of high-precision $Q_\mathrm{EC}$-value measurements with the double Penning trap mass spectrometer JYFLTRAP. Most recently, the $Q_\mathrm{EC}$ values of the $f_{7/2}$-shell mirror nuclei $^{45}$V ($Q_\mathrm{EC}=7123.82(22)$ keV) and $^{49}$Mn ($Q_\mathrm{EC}=7712.42(24)$ keV) have been measured with an unprecedented precision. The data reveal a 16-keV ($1.6σ$) offset in the adopted Atomic Mass Evaluation 2012 value of $^{49}$Mn suggesting the need for further measurements to verify the breakdown of the quadratic form of the isobaric multiplet mass equation. Precisely measured $Q_\mathrm{EC}$ values confirm that the pairing effect in the Coulomb energies is quenched when entering the $f_{7/2}$ shell and reaches a minimum in the midshell.

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Isomeric states close to doubly magic $^{132}$Sn studied with JYFLTRAP

The double Penning trap mass spectrometer JYFLTRAP has been employed to measure masses and excitation energies for $11/2^-$ isomers in $^{121}$Cd, $^{123}$Cd, $^{125}$Cd and $^{133}$Te, for $1/2^-$ isomers in $^{129}$In and $^{131}$In, and for $7^-$ isomers in $^{130}$Sn and $^{134}$Sb. These first direct mass measurements of the Cd and In isomers reveal deviations to the excitation energies based on results from beta-decay experiments and yield new information on neutron- and proton-hole states close to $^{132}$Sn. A new excitation energy of 144(4) keV has been determined for $^{123}$Cd$^m$. A good agreement with the precisely known excitation energies of $^{121}$Cd$^m$, $^{130}$Sn$^m$, and $^{134}$Sb$^m$ has been found.

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Precision Mass Measurements beyond $^{132}$Sn: Anomalous behaviour of odd-even staggering of binding energies

Atomic masses of the neutron-rich isotopes $^{121-128}$Cd, $^{129,131}$In, $^{130-135}$Sn, $^{131-136}$Sb, and $^{132-140}$Te have been measured with high precision (10 ppb) using the Penning trap mass spectrometer JYFLTRAP. Among these, the masses of four r-process nuclei $^{135}$Sn, $^{136}$Sb, and $^{139,140}$Te were measured for the first time. The data reveals a strong $N$=82 shell gap at $Z$=50 but indicates the importance of correlations for $Z>50$. An empirical neutron pairing gap expressed as the odd-even staggering of isotopic masses shows a strong quenching across $N$=82 for Sn, with the $Z$-dependence that is unexplainable by the current theoretical models.

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Mass measurements in the vicinity of the doubly-magic waiting point 56Ni

Masses of 56,57Fe, 53Co^m, 53,56Co, 55,56,57Ni, 57,58Cu, and 59,60Zn have been determined with the JYFLTRAP Penning trap mass spectrometer at IGISOL with a precision of dm/m \le 3 x 10^{-8}. The QEC values for 53Co, 55Ni, 56Ni, 57Cu, 58Cu, and 59Zn have been measured directly with a typical precision of better than 0.7 keV and Coulomb displacement energies have been determined. The Q values for proton captures on 55Co, 56Ni, 58Cu, and 59Cu have been measured directly. The precision of the proton-capture Q value for 56Ni(p,gamma)57Cu, Q(p,gamma) = 689.69(51) keV, crucial for astrophysical rp-process calculations, has been improved by a factor of 37. The excitation energy of the proton emitting spin-gap isomer 53Co^m has been measured precisely, Ex = 3174.3(10) keV, and a Coulomb energy difference of 133.9(10) keV for the 19/2- state has been obtained. Except for 53Co, the mass values have been adjusted within a network of 17 frequency ratio measurements between 13 nuclides which allowed also a determination of the reference masses 55Co, 58Ni, and 59Cu.

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A Hot Cavity Laser Ion Source at IGISOL

A development program is underway at the IGISOL (Ion Guide Isotope Separator On-Line) facility, University of Jyvaskyla, to efficiently and selectively produce low-energy radioactive ion beams of silver isotopes and isomers, with a particular interest in N=Z 94Ag. A hot cavity ion source has been installed, based on the FEBIAD (Forced Electron Beam Induced Arc Discharge) technique, combined with a titanium:sapphire laser system for selective laser ionization. The silver recoils produced via the heavy-ion fusion-evaporation reaction, 40Ca(58Ni, p3n)94Ag, are stopped in a graphite catcher, diffused, extracted and subsequently ionized using a three-step laser ionization scheme. The performance of the different components of the hot cavity laser ion source is discussed and initial results using stable 107,109Ag are presented.

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Mass Measurements and Implications for the Energy of the High-Spin Isomer in 94Ag

Nuclides in the vicinity of 94Ag have been studied with the Penning trap mass spectrometer JYFLTRAP at the Ion-Guide Separator On-Line. The masses of the two-proton-decay daughter 92Rh and the beta-decay daughter 94Pd of the high-spin isomer in 94Ag have been measured, and the masses of 93Pd and 94Ag have been deduced. When combined with the data from the one-proton or two-proton-decay experiments, the results lead to contradictory mass excess values for the high-spin isomer in 94Ag, -46370(170) or -44970(100) keV, corresponding to excitation energies of 6960(400) or 8360(370) keV, respectively.

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Mass measurements in the vicinity of the rp-process and the nu p-process paths with JYFLTRAP and SHIPTRAP

The masses of very neutron-deficient nuclides close to the astrophysical rp- and nu p-process paths have been determined with the Penning trap facilities JYFLTRAP at JYFL/Jyväskylä and SHIPTRAP at GSI/Darmstadt. Isotopes from yttrium (Z = 39) to palladium (Z = 46) have been produced in heavy-ion fusion-evaporation reactions. In total 21 nuclides were studied and almost half of the mass values were experimentally determined for the first time: 88Tc, 90-92Ru, 92-94Rh, and 94,95Pd. For the 95Pdm, (21/2^+) high-spin state, a first direct mass determination was performed. Relative mass uncertainties of typically $δm / m = 5 \times 10^{-8}$ were obtained. The impact of the new mass values has been studied in nu p-process nucleosynthesis calculations. The resulting reaction flow and the final abundances are compared to those obtained with the data of the Atomic Mass Evaluation 2003.

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Evolution of the N=50 shell gap energy towards $^{78}$Ni

Atomic masses of the neutron-rich isotopes $^{76-80}$Zn, $^{78-83}$Ga, $^{80-85}Ge, $^{81-87}$As and $^{84-89}$Se have been measured with high precision using the Penning trap mass spectrometer JYFLTRAP at the IGISOL facility. The masses of $^{82,83}$Ga, $^{83-85}$Ge, $^{84-87}$As and $^{89}$Se were measured for the first time. These new data represent a major improvement in the knowledge of the masses in this neutron-rich region. Two-neutron separation energies provide evidence for the reduction of the N=50 shell gap energy towards germanium Z=32 and a subsequent increase at gallium (Z=31). The data are compared with a number of theoretical models. An indication of the persistent rigidity of the shell gap towards nickel (Z=28) is obtained.

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A sextupole ion beam guide to improve the efficiency and beam quality at IGISOL

The laser ion source project at the IGISOL facility, Jyvaskyla, has motivated the development and construction of an rf sextupole ion beam guide (SPIG) to replace the original skimmer electrode. The SPIG has been tested both off-line and on-line in proton-induced fission, light-ion and heavy-ion induced fusion-evaporation reactions and, in each case, has been directly compared to the skimmer system. For both fission and light-ion induced fusion, the SPIG has improved the mass-separated ion yields by a factor of typically 4 to 8. Correspondingly, the transmission efficiency of both systems has been studied in simulations with and without space charge effects. The transport capacity of the SPIG has been experimentally determined to be 10^12 ions/s before space charge effects start to take effect. A direct comparison with the simulation has been made using data obtained via light-ion fusion evaporation. Both experiment and simulation show an encouraging agreement as a function of current extracted from the ion guide.

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Q value of the 100Mo Double-Beta Decay

Penning trap measurements using mixed beams of 100Mo - 100Ru and 76Ge - 76Se have been utilized to determine the double-beta decay Q-values of 100Mo and 76Ge with uncertainties less than 200 eV. The value for 76Ge, 2039.04(16) keV is in agreement with the published SMILETRAP value. The new value for 100Mo, 3034.40(17) keV is 30 times more precise than the previous literature value, sufficient for the ongoing neutrinoless double-beta decay searches in 100Mo. Moreover, the precise Q-value is used to calculate the phase-space integrals and the experimental nuclear matrix element of double-beta decay.

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