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J. -P. Ebran

Publications and source records attributed to J. -P. Ebran.

At least 19 recordsLinked to original sources

Nuclear structure within a relativistic mean field approach including chiral symmetry and confinement-inspired nucleon response

The relativistic mean field approach, within a theoretical framework known as the chiral confining model incorporating chiral symmetry breaking and confinement-inspired nucleon response, is applied for the first time to finite nuclei. Model parameters are calibrated through a Bayesian approach using nuclear empirical properties and doubly magic nuclei. The model provides a satisfactory description of binding energies and charge radii for medium and heavy nuclei, while larger discrepancies are observed in light nuclei. This behavior is linked to the constrained form of the chiral potential, which reduces flexibility away from saturation density. Charge radii are reproduced with very good accuracy, although density profiles remain slightly more diffuse than experimental ones. The extension to open-shell nuclei with a separable Gogny pairing interaction reveals enhanced pairing correlations associated with the large Dirac and non-relativistic effective masses, reduced spin-orbit splittings, and increased single-particle level density around the Fermi surface. Finally, departures from the linear sigma model potential motivated by the Nambu-Jona-Lasinio framework are explored. Allowing additional flexibility in the chiral potential improves the description of light nuclei and reduces the effective masses, which in turn suppresses the anomalous pairing. These results highlight the sensitivity of finite nuclei properties to the structure of the chiral potential and the associated single-particle spectrum.

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A unified mechanism for the origin and evolution of nuclear magicity

A simple pattern of organization, the nuclear shell structure, emerges from the complex interactions between nucleons in nuclei and determines, to some significant degree, nuclear structure properties. Recent experimental investigations of exotic nuclei revealed a shortfall in our current understanding of nuclear shell evolution and nuclear magicity. We introduce a novel perspective in the Energy Density Functional framework, where the Dirac mass kinetic term, which stems from the singular participation of a spin-0 boson in the nuclear strong force, plays a pivotal role in generating the nuclear shell structure. Namely, the combination of the Dirac mass kinetic term with the spin-orbit term redefines magic numbers both in stable and exotic nuclei. The identification of this mechanism allows to provide a broad understanding of the origin and evolution of nuclear magic numbers.

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The $α$-particle condensation in diluted $^{16}\text{O}$ at finite temperature

We investigate the effect of temperature on $α$-particle clustering in the diluted nucleus $^{16}\text{O}$ using the multi-constrained finite-temperature relativistic Hartree-Bogoliubov model with the DD-ME2 interaction. At a critical density the nucleus undergoes a Mott-like transition from a homogeneous to a localised configuration characterised by $α$-particle clustering and the emergence of a finite non-axial octupole deformation. We study the interplay between the onset of localisation under nuclear dilution and the suppression of deformation and $α$-particle clustering due to increasing temperature. Investigating the temperature-density plane, our findings indicate that temperature delays the formation of non-axial octupole deformation and $α$-particle clustering in dilute environments. Following the transition from homogeneous to clustered configurations, the non-axial octupole deformation continues to increase with further dilution of the system and becomes nearly independent of temperature. We found that $α$-particle clusters appear at temperatures up to $T = 4.10$ MeV and at a corresponding normalised density $ρ_{\text{Mott}}/ρ_0 \approx 0.09$.

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Refined topology of the N = 20 island of inversion with high precision mass measurements of $^{31-33}$Na and $^{31-35}$Mg

Mass measurements of $^{31-33}$Na and $^{31-35}$Mg using the TITAN MR-TOF-MS at TRIUMF's ISAC facility are presented, with the uncertainty of the $^{33}$Na mass reduced by over two orders of magnitude. The excellent performance of the MR-TOF-MS has also allowed the discovery of a millisecond isomer in $^{32}$Na. The precision obtained shows that the binding energy of the normally closed N = 20 neutron shell reaches a minimum for $^{32}$Mg but increases significantly for $^{31}$Na, hinting at the possibility of enhanced shell strength toward the unbound $^{28}$O. We compare the results with new ab initio predictions that raise intriguing questions of nuclear structure beyond the dripline.

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Large quadrupole deformation in $^{20}$Ne challenges rotor model and modern theory: urging for $α$ clusters in nuclei

The spectroscopic quadrupole moment of the first excited state, $Q_{_S}(2^{+}_{1})$, at 1.634 MeV in $^{20}$Ne was determined from sensitive reorientation-effect Coulomb-excitation measurements using a heavy target and safe energies well below the Coulomb barrier. Particle-$γ$ coincidence measurements were collected at iThemba LABS with a digital data-acquisition system using the {\sc AFRODITE} array coupled to an annular, doubled-sided silicon detector. A precise value of $Q_{_S}(2^{+}_{1})=-0.22(2)$ eb was determined at backward angles in agreement with the only safe-energy measurement prior to this work, $Q_{_S}(2^{+}_{1})=-0.23(8)$ eb. This result adopts 1$\hbarω$ shell-model calculations of the nuclear dipole polarizability of the 2$^+_1$ state that contributes to the effective quadrupole interaction and determination of $Q_{_S}(2^{+}_{1})$. It disagrees, however, with the ideal rotor model for axially-symmetric nuclei by almost $3σ$. Larger discrepancies are computed by modern state-of-the-art calculations performed in this and prior work, including {\it ab initio} shell model with chiral effective interactions and the multi-reference relativistic energy density functional ({\sc MR-EDF}) model. The intrinsic nucleon density of the 2$^+_1$ state in $^{20}$Ne calculated with the {\sc MR-EDF} model illustrates the presence of $α$ clustering, which explains the largest discrepancy with the rotor model found in the nuclear chart and motivates the explicit inclusion of $α$ clustering for full convergence of $E2$ collective properties.

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Use of quantality in nuclei and many-body systems

The use of quantality is discussed in the case of nuclei and other many-body systems such as atomic electrons. This dimensionless quantity is known to indicate when a many-body system behaves like a crystal or a quantum liquid. Its role is further analyzed by showing its relation to the scattering length. The emergence of a fundamental lengthscale, the limit radius, is also shown. It corresponds to the hard-core of the nucleon-nucleon interaction in the case of nucleons, and to a value close to the Bohr radius in the case of atomic electrons. The occurrence of a cluster phase in nuclei is analyzed using the quantality through its relation to the localization parameter, allowing for the identification of both the number of nucleons and the density as control parameters for the occurrence of this phase. The relation of the quantality to the magnitude of the interaction also exhibits a third dimensionless parameter, monitoring the magnitude of the spin-orbit effect in finite systems, through the realization of the pseudo-spin symmetry. The impact of quantality on the spin-orbit effect is compared in various many-body systems. The role of quantality in the relative effect of the binding energy and the shell one is also analyzed in nuclei. Finally, additional dimensionless quantities are proposed from the generalization of the quantality. Nuclei are found to be exceptional systems because all their dimensionless quantities are close to the order of unity, at variance with other many-body systems.

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Microscopic description of $α$, $2α$, and cluster decays of $^{216-220}$Rn and $^{220-224}$Ra

Alpha and cluster decays are analyzed for heavy nuclei located above $^{208}$Pb on the chart of nuclides: $^{216-220}$Rn and $^{220-224}$Ra, that are also candidates for observing the $2 α$ decay mode. A microscopic theoretical approach based on relativistic Energy Density Functionals (EDF), is used to compute axially-symmetric deformation energy surfaces as functions of quadrupole, octupole and hexadecupole collective coordinates. Dynamical least-action paths for specific decay modes are calculated on the corresponding potential energy surfaces. The effective collective inertia is determined using the perturbative cranking approximation, and zero-point and rotational energy corrections are included in the model. The predicted half-lives for $α$-decay are within one order of magnitude of the experimental values. In the case of single $α$ emission, the nuclei considered in the present study exhibit least-action paths that differ significantly up to the scission point. The differences in alpha-decay lifetimes are not only driven by Q values, but also by variances of the least-action paths prior to scission. In contrast, the $2 α$ decay mode presents very similar paths from equilibrium to scission, and the differences in lifetimes are mainly driven by the corresponding Q values. The predicted $^{14}$C cluster decay half-lives are within three orders of magnitudes of the empirical values, and point to a much more complex pattern compared to the alpha-decay mode.

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Alpha-particle formation and clustering in nuclei

The nucleonic localization function has been used for a decade to study the formation of alpha-particles in nuclei, by providing a measure of having nucleons of a given spin in a single place. However, differences in interpretation remain, compared to the nucleonic density of the nucleus. In order to better understand the respective role of the nucleonic localization function and the densities in the alpha-particle formation in cluster states or in alpha-decay mechanism, both an analytic approximation and microscopic calculations, using energy density functionals, are undertaken. The nucleonic localization function is shown to measure the anti-centrifugal effect, and is not sensitive to the level of compactness of the alpha-particle itself. It probes the purity of the spatial overlap of four nucleons in the four possible (spin, isospin) states. The density provides, in addition, information on the compactness of an alpha-particle cluster. The respective roles of the nucleonic localization function and the density are also analyzed in the case of alpha-particle emission. More generally, criteria to assess the prediction of alpha-cluster in nuclear states are provided.

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Covariant energy density functionals with and without tensor couplings at the Hartree-Bogoliubov level

Background: The study of additional terms in functionals is relevant to better describe nuclear structure phenomenology. Among these terms, the tensor one is known to impact nuclear structure properties, especially in neutron-rich nuclei. However, its effect has not been studied on the whole nuclear chart yet. Purpose: The impact of terms corresponding to the tensor at the Hartree level, is studied for infinite nuclear matter as well as deformed nuclei, by developing new density-dependent functionals including these terms. In particular, we study in details the improvement such a term can bring to the description of specific nuclear observables. Methods: The framework of covariant energy density functional is used at the Hartree-Bogoliubov level. The free parameters of covariant functionals are optimized by combining Markov-Chain-Monte-Carlo and simplex algorithms. Results: An improvement of the RMS binding energies, spin-orbit splittings and gaps is obtained over the nuclear chart, including axially deformed ones, when including tensors terms. Small modifications of the potential energy surface and densities are also found. In infinite matter, the Dirac mass is shifted to a larger value, in better agreement with experiments. Conclusions: Taking into account additional terms corresponding to the tensor terms in the vector-isoscalar channel at the Hartree level, improves the description of nuclear properties, both in nuclei and in nuclear matter.

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Rooting the EDF method into the ab initio framework. PGCM-PT formalism based on MR-IMSRG pre-processed Hamiltonians

Recently, ab initio techniques have been successfully connected to the traditional valence-space shell model. In doing so, they can either explicitly provide ab initio shell-model effective Hamiltonians or constrain the construction of empirical ones. In the present work, the possibility to follow a similar path for the nuclear energy density functional (EDF) method is analyzed. For this connection to be actualized, two theoretical techniques are instrumental: the recently proposed ab initio PGCM-PT many-body formalism and the MR-IMSRG pre-processing of the nuclear Hamiltonian. Based on both formal arguments and numerical results, possible new lines of research are briefly discussed, namely to compute ab initio EDF effective Hamiltonians at low computational cost, to constrain empirical ones or to produce them directly via an effective field theory that remains to be invented.

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Zero- and finite-temperature electromagnetic strength distributions in closed- and open-shell nuclei from first principles

Ab initio approaches to the nuclear many-body problem have seen their reach considerably extended over the past decade. However, collective excitations have been scarcely addressed so far due to the prohibitive cost of solving the corresponding equations of motion. Here, a numerically efficient method to compute electromagnetic response functions at zero- and finite-temperature in superfluid and deformed nuclei from an ab initio standpoint is presented and applied to $^{16}$O, $^{28}$Si, $^{46}$Ti and $^{56}$Fe. This work opens the path to systematic ab initio calculations of nuclear responses to electroweak probes across a significant portion of the nuclear chart.

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Low-energy monopole strength in spherical and deformed nuclei : cluster and soft modes

Background : Several recent experiments report significant low-energy isoscalar monopole strength, below the giant resonance, in various nuclei. In light $α$-conjugate nuclei, these low-energy resonances were recently interpreted as cluster vibration modes. However, the nature of these excitations in neutron-rich nuclei remain elusive. Purpose : The present work provides a systematic analysis of the low-energy monopole strength in isotopic chains, from Neon to Germanium, in order to monitor and understand its nature and conditions of emergence. Methods : We perform covariant quasiparticle random phase approximation (QRPA) calculations, formulated within the finite amplitude method (FAM), on top of constrained relativistic Hartree-Bogoliubov (RHB) reference states. Results : Neutron excess leads to the appearance of low-energy excitations according to a systematic pattern reflecting the single-particle features of the underlying RHB reference state. With the onset of deformation, these low-energy resonances get split and give rise to more complex patterns, with possible mixing with the giant resonance. At lower energy, cluster-like excitations found in $N=Z$ systems survive in neutron-rich nuclei, with valence neutrons arranging in molecular-like orbitals. Finally, at very low energy, pair excitations are also found in superfluid nuclei, but remain negligible in most of the cases. Conclusions : The low-energy part of the monopole strength exhibits various modes, from cluster vibrations ($\sim$ 5-10 MeV) to components of the giant resonance downshifted by the onset of deformation, including soft modes ($\sim$ 10-15 MeV) as well as pair excitation ($<$ 5 MeV), with possible mixing, depending on neutron-excess, deformation, and pairing energy.

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Localisation and alpha radioactivity

Relativistic energy density functional approaches are known to well describe nuclear states which involve alpha clusters. Here, alpha emitting nuclei are analysed through the behavior of the spatial localisation of nucleonic states, calculated with an axially deformed RHB approach over the nuclear chart. The systematic occurrence of more localised valence states, having a n = 1 radial quantum number, allows to pinpoint nuclei in agreement with experimentally known alpha-emitters. The cases of 212Po and 104Te are investigated, showing the concomitant contributions of the pseudospin symmetry and the presence of n = 1 states, on the alpha preformation probability. The impact of the localisation of valence states, on alpha preformation probability, is then analysed. It allows to study shell effects on this probability, over isotopic and isotonic chains. Finally, a phenomenological law is also provided, relating this probability to the radial quantum number of the valence states.

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Low-energy cluster vibrations in N = Z nuclei

Significant transition strength in light $α$-conjugate nuclei at low energy, typically below 10 MeV, has been observed in many experiments. In this work the isoscalar low-energy response of N=Z nuclei is explored using the Finite Amplitude Method (FAM) based on the microscopic framework of nuclear energy density functionals. Depending on the multipolarity of the excitation and the equilibrium deformation of a particular isotope, the low-energy strength functions display prominent peaks that can be attributed to vibration of cluster structures: $α$+$^{12}$C+$α$ and $α$+$^{16}$O in $^{20}$Ne, $^{12}$C+$^{12}$C in $^{24}$Mg, 4$α$+$^{12}$C in $^{28}$Si, etc. Such cluster excitations are favored in light nuclei with large deformation.

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Microscopic description of the self-conjugate $^{108}$Xe and $^{104}$Te $α$-decay chain

A microscopic calculation of half-lives for the recently observed $^{108}$Xe $\to$ $^{104}$Te $\to$ $^{100}$Sn $α$-decay chain is performed using a self-consistent framework based on energy density functionals. The relativistic density functional DD-PC1 and a separable pairing interaction of finite range are used to compute axially-symmetric deformation energy surfaces of $^{104}$Te and $^{108}$Xe as functions of quadrupole, octupole and hexadecupole collective coordinates. Dynamic least-action paths are determined that trace the $α$-particle emission from the equilibrium deformation to the point of scission. The calculated half-lives: 197 ns for $^{104}$Te and 50 $μ$s for $^{108}$Xe, are compared to recent experimental values of the half-lives of superallowed $α$-decay of $^{104}$Te: $< 18$ ns, and $^{108}$Xe: 58$^{+106}_{-23}$ $μ$s.

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Taming nuclear complexity with a committee of multilayer neural networks

We demonstrate that a committee of deep neural networks is capable of predicting the ground-state and excited energies of more than 1800 atomic nuclei with an accuracy akin to the one achieved by state-of-the-art nuclear energy density functionals (EDFs) and a major speed-up. An active learning strategy is proposed to train this algorithm with a minimal set of 210 nuclei. This approach enables future fast studies of the influence of EDFs parametrizations on structure properties over the whole nuclear chart and suggests that for the first time an artificial intelligence successfully encoded the laws of nuclear deformation.

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Alpha-particle condensation: a nuclear quantum phase transition

When the density of a nuclear system is decreased, homogeneous states undergo the so-called Mott transition towards clusterised states, e.g. alpha clustering, both in nuclei and in nuclear matter. Here we investigate such a quantum phase transition (QPT) by using microscopic energy density functional (EDF) calculations both with the relativistic and the Gogny approaches on the diluted $^{16}$O nucleus. The evolution of the corresponding single-particle spectrum under dilution is studied, and a Mott-like transition is predicted at about 1/3 of the saturation density. Complementary approaches are used in order to understand this QPT. A study of spatial localisation properties as a function of the density allows to derive a value of the Mott density in agreement with the one obtained by fully microscopic calculations in $^{16}$O and in nuclear matter. Moreover a study of the spontaneous symmetry breaking of the rotational group in $^{16}$O, down to the discrete tetrahedral one, provides further insight on the features displayed by the single-particle spectrum obtained within the EDF approach.The content of the tetrahedrally deformed A-nucleon product state in terms of spherical particle-hole configurations is investigated. Finally a study of quartet condensation and the corresponding macroscopic QPT is undertaken in infinite matter.

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Single-particle spatial dispersion and clusters in nuclei

The spatial dispersion of the single-nucleon wave functions is analyzed using the self-consistent mean-field framework based on nuclear energy density functionals, and with the harmonic oscillator approximation for the nuclear potential. It is shown that the dispersion depends on the radial quantum number n, but displays only a very weak dependence on the orbital angular momentum. An analytic expression is derived for the localization parameter that explicitly takes into account the radial quantum number of occupied single-nucleon states. The conditions for single-nucleon localization and formation of cluster structures are fulfilled in relatively light nuclei with $A \leq 30$ and $n=1$ states occupied. Heavier nuclei exhibit the quantum liquid phase of nucleonic matter because occupied levels that originate from $n > 1$ spherical states are largely delocalized. Nevertheless, individual $α$-like clusters can be formed from valence nucleons filling single-particle levels originating from $n=1$ spherical mean-field states.

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